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Crystallization management of CsPbI2Br perovskites by PbAc2-incorporated twice spin-coating process for efficient and stable CsPbI2Br perovskite solar cells

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Journal of energy Chemistry 2024年第10期97卷 419-428页

作者： Yu Liu Kun Lang Huifang Han Huijing Liu Yao Fu Pengchen Zou Yinhui Lyu Jia Xu Jianxi Yao State Key Laboratory of Alternate Electrical power System with Renewable energy Sources Beijing Key Laboratory of Energy Safety and Clean Utilization North China Electric Power University

CsPbI2Br perovskite solar cell has been extensively studied due to its exceptional thermal stability and relatively stable perovskite phase ***,the presence of bromine leads to a rapid crystallization rate of CsPbI2Br films,resulting in small grain size and high defect ***,CsPbI2Br demonstrates poor light absorption due to its wide ***,it is crucial to control the crystallization rate and increase the film thickness to reduce defect density,enhance light absorption,and improve photovoltaic *** this study,we utilized a PbAc2-incorporated twice spincoating（PTS） process to address these ***,PbAc2was added to the CsPbI2Br precursor solution to form a CsPbI2Br film,which was then coated with the CsPbI2Br precursor solution to produce the PTS film,Ac-can delay the perovskite crystallization,leading to the formation of thicker and denser CsPbI2Br ***,lone-pair electrons of the oxygen atom provided by Ac-formed coordination bonds with under-coordinated Pb2+ions to fill halogen ion vacancies,thereby reducing the defect ***,the PTS CsPbI2Br device achieved a peak power conversion efficiency（PCE） of 16.19% and maintained 96.7% of its initial PCE over 1500 h at room temperature under 25% relative humidity without any encapsulation.

关键词： Crystallization management CsPbI2Br PbAc2 Perovskite solar cells Twice spin-coating process

Enhanced properties of stone coal-based composite phase change materials for thermal energy storage

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International Journal of Minerals,Metallurgy and Materials 2024年第1期31卷 206-215页

作者： Baoshan Xie Huan Ma Chuanchang Li Jian Chen Key Laboratory of Renewable energy Electric-Technology of Hunan Province School of Energy and Power EngineeringChangsha University of Science and TechnologyChangsha 410114China State Key Laboratory of Disaster Prevention and Reduction for power Grid Changsha University of Science and TechnologyChangsha 410114China

Phase change materials (PCMs) can be incorporated with low-cost minerals to synthesize composites for thermal energy storage in building *** coal (SC) after vanadium extraction treatment shows potential for secondary utilization in composite *** prepared SC-based composite PCMs with SC as a matrix,stearic acid (SA) as a PCM,and expanded graphite (EG) as an *** combined roasting and acid leaching treatment of raw SC was conducted to understand the effect of vanadium extraction on promoting loading *** showed that the combined treatment of roasting at 900℃ and leaching increased the SC loading of the composite by 6.2%by improving the specific surface *** loading capacity and thermal conductivity of the composite obviously increased by 127%and 48.19%,respectively,due to the contribution of 3wt% *** data were supported by the high load of 66.69%and thermal conductivity of 0.59 W·m^(-1)·K-1of the designed *** obtained composite exhibited a phase change temperature of 52.17℃,melting latent heat of 121.5 J·g^(-1),and good chemical *** SC-based composite has prospects in building applications exploiting the secondary utilization of minerals.

关键词： thermal energy storage phase change material stone coal vanadium extraction secondary utilization

Thermal comfort in a building with Trombe wall integrated with phase change materials in hot summer and cold winter region without air conditioning

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Energy and Built Environment

energy and Built Environment 2024年第1期5卷 58-69页

作者： Jie Li Yuan Zhang Ziyang Zhu Jiangtian Zhu Jing Luo Fen Peng Xiaoqin Sun school of energy and power Engineering Changsha University of Science and TechnologyChangshaHunan 410114PR China

Trombe wall and phase change materials(PCMs)are two effective ways to regulate indoor thermal ***,Trombe wall surfers from overheating in summer and PCMs suffer from low heat transfer rate caused by the limited thermal *** compensate the shortcomings of the two methods,this paper proposed a Trombe wall system integrated with *** on a light-weight building envelope in Changsha,China,the thermal comfort of 10 kinds of Trombe wall systems with PCMs with a melting temperature of 18-28℃ were *** the integrated indoor discomfort duration(I_(D)),integrated indoor discomfort degree-hour(I_(DH)),indoor air temperature(T_(in)),PCM liquid fraction(γ)and heat flux across wall(q)as evaluation indexes,the indoor thermal comfort was assessed in hot summer and cold winter *** show that the Trombe wall helped PCMs complete the phase change process *** wall with PCM25 next to the wall inner surface possessed the lowest annual I_(D) and I_(DH),as 2877 h and 12,974℃·h,*** with the values in a traditional building,the I_(D) and I_(DH) were reduced by 7.01% and 14.14%.In order to give full play to the heat storage and heat release of the Trombe wall with PCMs,PCMs with phase change temperature 7℃ lower than the peak ambient temperature in summer or 8℃ higher than the winter night temperature was recommended according to regional climate conditions.

关键词： Trombe wall Phase change materials Integrated indoor discomfort duration Integrated discomfort degree-hour Liquid fraction

Numerical study on the cavity dynamics for vertical water entries of twin spheres

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Defence Technology（防务技术） 2024年第2期32卷 459-472页

作者： Xu Wang Xujian Lyu Ruisheng Sun Dongdong Tang school of energy and power Engineering Nanjing University of Science and TechnologyNanjing210094China Shanghai Institute of Spacecraft Equipment Shanghai200240China

In this study, a three dimensional(3D) numerical model of six-degrees-of-freedom(6DOF) is applied to simulate the water entries of twin spheres side-by-side at different lateral distances and time *** turbulence structure is described using the shear-stress transport k-ω(SST k-ω) model, and the volume of fluid(VOF) method is used to track the complex air-liquid interface. The motion of spheres during water entry is simulated using an independent overset grid. The numerical model is verified by comparing the cavity evolution results from simulations and experiments. Numerical results reveal that the time interval between the twin water entries evidently affects cavity expansion and contraction behaviors in the radial direction. However, this influence is significantly weakened by increasing the lateral distance between the two spheres. In synchronous water entries, pressure is reduced on the midline of two cavities during surface closure, which is directly related to the cavity volume. The evolution of vortexes inside the two cavities is analyzed using a velocity vector field, which is affected by the lateral distance and time interval of water entries.

关键词： Twin water entries Side-by-side Cavity Numerical simulation

A Methodology for Assessing Axial Compressor Stability with Inlet Temperature Ramp Distortion

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Journal of Thermal Science 2024年第3期33卷 856-871页

作者： SUN Dakun GU Benhao NING Fangfei FANG Yibo DONG Xu XU Dengke SUN Xiaofeng school of energy and power Engineering Beihang UniversityBeijing102206China Research Institute of Aero-engine Beihang UniversityBeijing102206China

Based on a small perturbation stability model for periodic flow,the effects of inlet total temperature ramp distortion on the axial compressor are investigated and the compressor stability is quantitatively *** the beginning,a small perturbation stability model for the periodic flow in compressors is proposed,referring to the governing equations of the Harmonic Balance *** stability model is validated on a single-stage low-speed compressor TA36 with uniform inlet ***,the unsteady flow of TA36 with different inlet total temperature ramps and constant back pressure is simulated based on the Harmonic Balance *** on these simulations,the compressor stability is analyzed using the proposed small perturbation ***,the Dynamic Mode Decomposition method is employed to accurately extract pressure *** two parameters of the temperature ramp,ramp rate and Strouhal number,are discussed in this *** results indicate the occurrence and extension of hysteresis loops in the rows,and a decrease in compressor stability with increasing ramp *** performance is divided into two phases,stable and limit,based on the ramp ***,the model predictions suggest that a decrease in period length and an increase in Strouhal number lead to improved compressor *** DMD results imply that for compressors with inlet temperature ramp distortion,the increase of high-order modes and oscillations at the rotor tip is always the signal of decreasing stability.

关键词： axial compressor stability small perturbation model inlet temperature ramp distortion harmonic balance method dynamic mode decomposition method

Improvement of Film Cooling Design for Turbine Vane Leading Edge Considering Combustor Outflow

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Journal of Thermal Science 2024年第1期33卷 311-327页

作者： WANG Xinyu LIU Cunliang FU Zhongyi LI Yang ZHU Huiren school of power and energy Northwestern Polytechnical UniversityXi'an 710072China AECC Hunan Aviation powerplant Research Institute Zhuzhou 412002China

As the interaction between the combustor and the turbine in the aero-engine continues to increase,the film cooling design considering the combustor swirling outflow has become the research *** swirling inflow and high-temperature gas first affect the vane leading edge(LE).However,no practical improved solution for the LE cooling design has been proposed considering the combustor swirling *** this paper,the improved scheme of showerhead cooling is carried out around the two ways of adopting the laid-back-fan-shaped hole and reducing the coolant outflow *** film cooling effectiveness(η) and the coolant flow state are obtained by PSP(pressure-sensitive-paint) and numerical simulation methods,*** research results show that the swirling inflow increases the film distribution inhomogeneity by imposing the radial pressure gradient on the vane to make the film excessively gather in some *** showerhead film cooling adopts the laid-back-fan-shaped hole to reduce the momentum when the coolant flows *** this cooling scheme improves the film attachment and increases the surface-averaged film cooling effectiveness(η_(sur)) by as much as15.4%,the film distribution inhomogeneity *** reducing the coolant outlet angle,the wall-tangential velocity of the coolant increases,and the wall-normal velocity *** the swirl intake condition,both ηand the film distribution uniformity are significantly increased,and the growth of η_(sur) is up to 16.5%.This paper investigates two improved schemes to improve the showerhead cooling under the swirl intake condition to provide a reference for the vane cooling design.

关键词： turbine vane showerhead cooling swirling inflow laid-back-fan-shaped hole film hole inclination

Design of highly active and durable oxygen evolution catalyst with intrinsic chlorine inhibition property for seawater electrolysis

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Nano Materials Science 2024年第4期6卷 413-418页

作者： Jieli Chen Xiaodong Shi Suyang Feng Jing Li Xiaohong Gao Xiao Wu Ke Li Anyuan Qi Chenghang You Xinlong Tian school of Marine Science and Engineering School of Chemical Engineering and Technology Hainan University National energy Group Ledong power Generation Co. Ltd

High-efficiency seawater electrolysis is impeded by the low activity and low durability of oxygen evolution catalysts due to the complex composition and competitive side reactions in ***,a heterogeneousstructured catalyst is constructed by depositing NiFe-layered double hydroxides （NiFe-LDH） on the substrate of MXene （V2CTx） modified Ni foam （NF）,and abbreviated as NiFe-LDH/V2CTx/*** demonstrated,owing to the intrinsic negative charge characteristic of V2CTx,chlorine ions are denied entry to the interface between NiFeLDH and V2CTx/NF substrate,thus endowing NiFe-LDH/V2CTx/NF catalyst with high corrosion resistance and durable stability for 110 h at 500 mA ***,the two-dimensional structure and high electrical conductivity of V2CTxcan respectively enlarge the electrochemical active surface area and guarantee fast charge transfer,thereby synergistically promoting the catalytic performance of NiFe-LDH/V2CTx/NF in both deionized water electrolyte (261 m V at 100 m A cm-2) and simulated seawater electrolyte (241 mV at 100 mA cm-2).This work can guide the preparation of oxygen evolution catalysts and accelerate the industrialization of seawater electrolysis.

关键词： NiFe-LDH/V 2 CT x /NF catalyst Oxygen evolution reaction Seawater electrolysis Chlorine inhibition

Strong hetero-interface interaction in 2D/2D WSe2/ZnIn2S4 heterostructures for highly-efficient photocatalytic hydrogen generation

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Journal of energy Chemistry 2024年第10期97卷 379-387页

作者： Xu Guo Xing Liu Jing Shan Zhuo Xu Zhiming Fang Lu Wang Shengzhong Liu school of energy Power and Mechanical Engineering North China Electric Power University Shaanxi Key Laboratory for Advanced energy Devices School of Materials Science and Engineering Shaanxi Normal University Qinghai Advanced energy Storage Laboratory SPIC Qinghai Photovoltaic Industry Innovation Center Co. Ltd.State Power Investment Corporation Key Laboratory of Photoelectric Conversion and Utilization of Solar energy Dalian Institute of Chemical Physics Chinese Academy of Sciences Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences

Green hydrogen is urgently required for sustainable development of human beings and rational construction of heterostructures holds great promising for photocatalytic hydrogen ***,2D/2D WSe2/ZnIn2S4heterostructures with strong hetero-interface interaction and abundant contact were constructed via an impregnation-annealing *** charge transfer from ZnIn2S4to WSe2was evidenced by transient absorption spectroscopy in crafted heterostructures owing to the tight and2D face-to-face *** a result,the prepared WSe2/ZnIn2S4heterostructures exhibited boosted photocatalytic performance and a highest hydrogen evolution rate of 3.377 mmol/（g h） was achieved with an apparent quantum yield of 45.7% at 420 *** work not only provides new strategies to achieve efficient 2D/2D heterostructures but also paves the way for the development of green hydrogen in the future.

关键词： Indium compounds

High-stability temperature control and frequency-domain analysis of sandwich-like insulation design based on phase change materials for satellite thermal management

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Science China(Technological Sciences) 2024年第8期67卷 2387-2404页

作者： WANG ZiHan HE ChenBo HU Yang TANG GuiHua Key Laboratory of Thermo-Fluid Science and Engineering Ministry of EducationSchool of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049China

High-stability thermal management is critical for the measurements of high sensitivity for temperature, but also challenging because any small thermal disturbances could lead to unacceptable temperature fluctuations. The present work delivers a design for passive temperature control, customized for a component in the satellites for gravitational wave detection. A novel sandwichlike structure is proposed with the configurations of proper materials, consisting of a layer of insulation material and two layers of nanocomposite phase change materials, bringing an integration of heat insulation and absorption/storage. Its performance is examined using an improved thermal network model and the revised transfer function method(TFM). The basic results of the two methods are validated by present COMSOL simulations and available numerical and experimental data in the literature. An effective reduction of temperature fluctuation is achieved to the scale of 0.1 K, even under two thermal disturbances from different directions: a radiative heat flux of 20 W m~(-2)(inside) and a temperature fluctuation of about 20 K(outside). Moreover,the TFM is employed to analyze the effects of the frequency of thermal disturbance: excellent damping performance is obtained for over 3.2 mHz and the underlying mechanism is discussed. Overall, the present design is expected to be combined with active temperature control to explore more possible ways for temperature control with higher stability.

关键词： temperature control sandwich insulation structure phase change material thermal network model transfer function method

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