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A review on Bi_(2)WO_(6)-based photocatalysts synthesis, modification, and applications in environmental remediation, life medical, and clean energy

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Frontiers of environmental Science & Engineering 2024年第7期18卷 87-108页

作者： Wei Mao Xuewu Shen Lixun Zhang Yang Liu Zehao Liu Yuntao Guan Guangdong Provincial Engineering Technology Research center for Urban Water Cycle and Water environment Safety Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China State environmental Protection Key Laboratory of Microorganism application and Risk Control School of EnvironmentTsinghua UniversityBeijing 100084China

Photocatalysis has emerged a promising strategy to remedy the current energy and environmental crisis due to its ability to directiy convert clean solar energy into chemical *** tungstate(Bi_(2)WO_(6))has been shown to be an excellent visible light response,a well-defined perovskite crystal structure,and an abundance of oxygen atoms(providing efficient channels for photogenerated carrier transfer)due to their suitable band gap,effective electron migration and separation,making them ideal *** has been extensively applied as photocatalyst in aspects including pollutant removal,carbon dioxide reduction,solar hydrogen production,ammonia synthesis by nitrogen photocatalytic reduction,and cancer *** this review,the fabrication and application of Bi_(2)WO_(6) in photocatalysis were comprehensively *** photocatalytic properties of BizwO-based materials were significantly enhanced by carbon modification,the construction of heterojunctions,and the atom doping to improve the photogenerated carrier migration rate,the number of surface active sites,and the photoexcitation ability of the *** addition,the potential development directions and the existing challenges to improve the photocatalytic performance of Bi_(2)WO_(6)-based materials were discussed.

关键词： Bismuth tungstate Synthesis and modification Photocatalytic application environmental remediation Clean energy Medical science

An empirical method for joint inversion of wave and wind parameters based on SAR and wave spectrometer data

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Acta Oceanologica Sinica 2024年第5期43卷 133-144页

作者： Yong Wan Xiaona Zhang Shuyan Lang Ennan Ma Yongshou Dai College of Oceanography and Space Informatics China University of PetroleumQingdao 266580China National satellite Marine application center Beijing 100081China Key Laboratory of Space Ocean Remote Sensing and application Ministry of Natural ResourcesBeijing 100081China College of Control Science and Engineering China University of PetroleumQingdao 266580China

Synthetic aperture radar(SAR)and wave spectrometers,crucial in microwave remote sensing,play an essential role in monitoring sea surface wind and wave ***,they face inherent limitations in observing sea surface *** systems,for instance,are hindered by an azimuth cut-off phenomenon in sea surface wind field *** spectrometers,while unaffected by the azimuth cutoff phenomenon,struggle with low azimuth resolution,impacting the capture of detailed wave and wind field *** study utilizes SAR and surface wave investigation and monitoring(SWIM)data to initially extract key feature parameters,which are then prioritized using the extreme gradient boosting(XGBoost)*** research further addresses feature collinearity through a combined analysis of feature importance and correlation,leading to the development of an inversion model for wave and wind parameters based on XGBoost.A comparative analysis of this model with ERA5 reanalysis and buoy data for of significant wave height,mean wave period,wind direction,and wind speed reveals root mean square errors of 0.212 m,0.525 s,27.446°,and 1.092 m/s,compared to 0.314 m,0.888 s,27.698°,and 1.315 m/s from buoy data,*** results demonstrate the model’s effective retrieval of wave and wind ***,the model,incorporating altimeter and scatterometer data,is evaluated against SAR/SWIM single and dual payload inversion methods across different wind *** comparison highlights the model’s superior inversion accuracy over other methods.

关键词： synthetic aperture radar(SAR) wave spectrometer extreme gradient boosting(XGBoost) joint inversion method wave and wind parameters

Long-term Variation of the Solar Polar Magnetic Fields at Different Latitudes

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Research in Astronomy and Astrophysics 2024年第7期24卷 193-200页

作者： Shuhong Yang Jie Jiang Zifan Wang Yijun Hou Chunlan Jin Qiao Song Yukun Luo Ting Li Jun Zhang Yuzong Zhang Guiping Zhou Yuanyong Deng Jingxiu Wang National Astronomical Observatories Chinese Academy of Sciences School of Astronomy and Space Science University of Chinese Academy of Sciences State Key Laboratory of Solar Activity and Space Weather National Space Science CenterChinese Academy of Sciences School of Space and environment Beihang University Key Laboratory of Space Weather National Satellite Meteorological Center (National Center for Space Weather) Innovation center for FengYun Meteorological satellite (FYSIC) School of Physics and Materials Science Anhui University

The polar magnetic fields of the Sun play an important role in governing solar activity and powering fast solar wind. However, because our view of the Sun is limited in the ecliptic plane, the polar regions remain largely uncharted. Using the high spatial resolution and polarimetric precision vector magnetograms observed by Hinode from 2012 to 2021, we investigate the long-term variation of the magnetic fields in polar caps at different *** Hinode magnetic measurements show that the polarity reversal processes in the north and south polar caps are non-simultaneous. The variation of the averaged radial magnetic flux density reveals that, in each polar cap, the polarity reversal is completed successively from the 70° latitude to the pole, reflecting a poleward magnetic flux migration therein. These results clarify the polar magnetic polarity reversal process at different latitudes.

关键词： dynamo Sun: magnetic fields Sun: photosphere

Humic acid-mediated transport of a typical soil passivation remediation product(chloropyromorphite)in saturated porous media

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Journal of environmental Sciences 2024年第7期141卷 51-62页

作者： Xinying Li Mengjia Zhang Siyuan Li Wei Wei School of environment Jiangsu Engineering Lab of Water and Soil Eco-remediationJiangsu Province Engineering Research Center of Environmental Risk Prevention and Emergency Response TechnologyNanjing Normal UniversityNanjing 210023China Jiangsu center for Collaborative Innovation in Geographical Information Resource Development and application Nanjing 210023China

Conversion of labile Pb species into chloropyromorphite(CPY)using phosphorus-bearing amendments was considered to be an ideal strategy in soil passivation ***,the fate and transport of CPY in the soil are poorly *** study aims to fill the knowledge gap by evaluating the fate and transport of CPY under environmentally relevant conditions of humic acid(HA),pH,electrolyte concentration,and species through the saturated sandy *** showed that bare CPY colloids are basically immobile in sandy porous media while the co-existence of HA made the transport of CPY improved by30%-93.5%.Facilitated transport of CPY was attributed to the increased stability of CPY and the repulsive interaction between CPY particles and sands due to HA *** mobility of CPY was also increased with increasing pH from 5.0 to *** the pH was 9 with a10 mmol/L NaCl background solution,the stronger energy barrier between CPY and sand led to enhanced transport *** divalent Ca^(2+)had a more dramatic effect than monovalent Na^(+)on the aggregation and sedimentation of CPY colloids due to its effectivescreening of the surface charge of CPY and bridging interaction with CPY ***-LandauVerwey-Overbeek theory and attachment efficiency calculation indicated that high energy barriers were responsible for the high mobility of CPY colloids,while the retention of CPY in sands was mainly caused by secondary energy minimum and physically *** findings of this work can help to evaluate the fate of soil passivation remediation products in natural water and soil.

关键词： Chloropyromorphite DLVO theory Stability Saturated porous medium Transport

Challenges and prospects for room temperature solid-state sodiumsulfur batteries

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Nano Research 2024年第3期17卷 1402-1426页

作者： Yashuang Qiu Jing Xu Research center of Grid Energy Storage and Battery application School of Electrical and Information EngineeringZhengzhou UniversityZhengzhou 450001China

Room temperature sodium-sulfur(Na-S)batteries,known for their high energy density and low cost,are one of the most promising next-generation energy storage ***,the polysulfide shuttling and uncontrollable Na dendrite growth as well as safety issues caused by the use of organic liquid electrolytes in Na-S cells,have severely hindered their ***-state electrolytes instead of liquid electrolytes are considered to be the most direct and effective solution to solve the above ***,its practical application is still greatly challenged due to the poor interfacial compatibility between the all-solid-state electrolytes and the anode/cathode,ionic conductivity,and the shuttle effect caused by the presence of liquid phase in the quasi-solid-state *** paper presents a comprehensive review of solid-state Na-S batteries from the perspective of regulating interfacial compatibility and improving ionic conductivity as well as suppressing polysulfide *** to different components,solid-state electrolytes were divided into five categories:solid inorganic electrolytes,solid polymer electrolytes,polymer/inorganic solid hybrid electrolytes,gel polymer electrolytes,and liquid–solid inorganic hybrid ***,the prospect of developing high performance solid-state electrolytes to improve the cycling stability of room temperature Na-S cells is envisaged.

关键词： sodium-sulfur batteries solid-state electrolytes ionic conductivity polysulfide shuttling interfacial compatibility

Fusion SST from Infrared and Microwave Measurement of FY-3D Meteorological satellite

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Journal of Tropical Meteorology 2024年第1期30卷 89-96页

作者：张淼徐娜陈林 National satellite Meteorological center/National center for Space Weather Beijing 100081 China Innovation center for Fengyun Meteorological satellite(FYSIC) Beijing 100081 China Key Laboratory of Radiometric Calibration and Validation for environmental satellites China Meteorological AdministrationBeijing 100081 China

Sea surface temperature(SST)is one of the important parameters of global ocean and climate research,which can be retrieved by satellite infrared and passive microwave remote sensing *** satellite infrared SST offers high spatial resolution,it is limited by cloud *** the other hand,passive microwave SST provides all-weather observation but suffers from poor spatial resolution and susceptibility to environmental factors such as rainfall,coastal effects,and high wind *** achieve high-precision,comprehensive,and high-resolution SST data,it is essential to fuse infrared and microwave SST *** this study,data from the Fengyun-3D(FY-3D)medium resolution spectral imager II(MERSI-II)SST and microwave imager(MWRI)SST were ***,the accuracy of both MERSIII SST and MWRI SST was verified,and the latter was bilinearly interpolated to match the 5km resolution grid of MERSI *** pretreatment and quality control of MERSI SST and MWRI SST,a Piece-Wise Regression method was employed to correct biases in MWRI ***,SST data were selected based on spatial resolution and accuracy within a 3-day window of the analysis ***,an optimal interpolation method was applied to fuse the FY-3D MERSI-II SST and MWRI *** results demonstrated a significant improvement in spatial coverage compared to MERSI-II SST and MWRI ***,the fusion SST retained true spatial distribution details and exhibited an accuracy of–0.12±0.74℃compared to OSTIA *** study has improved the accuracy of FY satellite fusion SST products in China.

关键词： SST data fusion FY3 infrared microwave

Morphological characteristics and evolution model of slope units along loess gully cross section

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Frontiers of Earth Science 2024年第1期18卷 17-29页

作者： Lulu LIU Fayuan LI Xue YANG Jianhua CHENG School of Geography Nanjing Normal UniversityNanjing 210023China Jiangsu center for Collaborative Innovation in Geographical Information Resource Development and application Nanjing 210023China Key Laboratory of Virtual Geographic environment(Ministry of Education) Nanjing Normal UniversityNanjing 210023China

Gully morphology is an important part of loess landform *** with gully development,the variation of its cross section is the most significant,and it can intuitively reflect the characteristics of the lateral widening of the gully ***,in-depth research of the variation of the cross-sectional morphology of the gully is helpful to understanding the development process of the loess *** on the DEMs(Digital Elevation Model)of nine periods of an indoor simulated loess small watershed,this paper studies the evolution model of a complete branch ditch in the watershed using the digital terrain analysis theory and *** show that with the development of the gully,the average gradient of the gully slope continuously decreases,and the slope morphology is mostly a concave slope along the slope *** degree of downward concave first increases and then gradually tends to be *** gully erosion mode is gradually transformed from downward cutting erosion to lateral *** more mature the gully development,the lower the depth of gully bottom cutting is compared with the width of gully ***,the surface cutting depth tends to be stable and the slope is ***,the transformation law of the slope morphology of the gully cross section with the development of the gully is studied,and the prediction model of the transformation of the slope morphology of the gully cross section is established by using the Markov *** Markov model can better reflect the dynamic change of the slope morphology of the gully cross section,which is of great significance to revealing the external performance and internal mechanism of the gully morphology.

关键词： gully cross section slope morphology Markov chain digital elevation model

Geomorphology-oriented theoretical framework and construction method for value-added DEM

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Journal of Geographical Sciences 2024年第1期34卷 165-184页

作者： ZHANG Haiping TANG Guoan XIONG Liyang YANG Xin LI Fayuan Key Laboratory of Virtual Geographic environment Ministry of EducationNanjing Normal UniversityNanjing 210023China School of Geography Nanjing Normal UniversityNanjing 210023China Jiangsu center for Collaborative Innovation in Geographical Information Resource Development and application Nanjing 210023China

Digital elevation model(DEM)plays a fundamental role in the study of the earth system by expressing surface configuration,understanding surface process,and revealing surface *** is widely used in analysis and modeling in the field of ***,traditional DEM has the defect of single attribute,which is difficult to support the research in earth system science oriented to geoscience process and mechanism ***,realizing the value-added data model on the basis of traditional DEM is necessary to serve digital elevation modeling and terrain analysis under the background of a new geomorphology research paradigm and earth observation technology.A theoretical framework for value-added DEM that mainly includes concept,connotation,content,and categories,is constructed in this *** relationship between different types of value-added DEMs as well as the research significance and application category of this theoretical framework are also *** following are different methods of value-added DEMs:(1)value-added methods of DEM space and time dimensions that emphasize the integration of the ground and underground as well as coupling of time and space,(2)attribute-based value-added methods composed of material(including underground,surface,and ground)and morphological properties,and(3)value-added methods of features and physical elements that consider geographical objects and landform features formed by natural processes and artificial *** digital terrace,slope,and watershed models are used as examples to illustrate application scenarios of the three kinds of value-added *** study aims to improve expression methods of DEMs under the background of new surveying and mapping technologies by adding value to the DEM at three levels of dimensions,attributes,and elements as well as support knowledge-driven digital geomorphological analysis in the era of big data.

关键词： spatial data model value-added DEM digital terrain analysis geomorphological ontology geomorphology

Electric-controlled pressure relief valve for enhanced safety in liquid-cooled lithium-ion battery packs

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Journal of Energy Chemistry 2024年第3期90卷 98-109,I0004页

作者： Yuhang Song Jidong Hou Nawei Lyu Xinyuan Luo Jingxuan Ma Shuwen Chen Peihao Wu Xin Jiang Yang Jin Research center of Grid Energy Storage and Battery application School of Electrical and Information EngineeringZhengzhou UniversityZhengzhou 450001HenanChina

The liquid-cooled battery energy sto rage system(LCBESS) has gained significant attention due to its superior thermal management ***,liquid-cooled battery pack(LCBP) usually has a high sealing level above IP65,which can trap flammable and explosive gases from battery thermal runaway and cause *** poses serious safety risks and challenges for *** this study,we tested overcharged battery inside a commercial LCBP and found that the conventionally mechanical pressure relief valve(PRV) on the LCBP had a delayed response and low-pressure relief efficiency.A realistic 20-foot model of an energy storage cabin was constructed using the Flacs finite element simulation *** studies were conducted to evaluate the pressure relief efficiency and the influence on neighboring battery packs in case of internal explosions,considering different sizes and installation positions of the ***,a newly developed electric-controlled PRV integrated with battery fault detection is introduced,capable of starting within 50 ms of the battery safety valve ***,the PRV was integrated with the battery management system and changed the battery charging and discharging strategy after the PRV was *** tests confirmed the efficacy of this method in preventing *** paper addresses the safety concerns associated with LCBPs and proposes an effective solution for explosion relief.

关键词： Pressure relief valve Liquid-cooled battery pack Explosion Flacs