Abstract: Zeolite HZSM-5 calcined at different temperatures were studied by29Si MAS NMR and EPR method. It was concluded that in certain temperature range, dealumination did not necessarily occur simultaneously with f...
Abstract: Zeolite HZSM-5 calcined at different temperatures were studied by29Si MAS NMR and EPR method. It was concluded that in certain temperature range, dealumination did not necessarily occur simultaneously with framework dehydroxylation and thus framework Lewis acidic sites emerged. Two processes may be operative with one of them being predominant at different temperatures.
The potential predictability of seasonal extreme precipitation accumulation(sepa) across China’s mainland is evaluated, based on daily precipitation observations during 1960-2013 at 675 stations. The potential pred...
The potential predictability of seasonal extreme precipitation accumulation(sepa) across China’s mainland is evaluated, based on daily precipitation observations during 1960-2013 at 675 stations. The potential predictability value(PPV) of sepa is calculated for each station by decomposing the observed sepa variance into a part associated with stochastic daily rainfall variability and another part associated with longer timescale climate processes. We construct a Markov Chain model for each station and apply a Monte Carlo simulation to estimate the stochastic part of the variance. The results suggest that there are more potentially predictable regions for summer than for the other seasons, especially over the Yangtze River valley, North China Plain and northwestern China. There are also regions of large PPVs in southern China for autumn and winter and northwestern China for spring. The sepa series for the regions of large PPVs are deemed non-stochastic, either with long-term trends(e.g., increasing trends in inland northwestern China) or significant correlation with well-known large-scale climate processes(e.g., East Asian Winter Monsoon for southern China in winter, El Ni?o for the Yangtze River valley in summer). This fact not only verifies our claim that the regions have potential predictability but also facilitates predictive studies of the regional extreme precipitation and the mechanisms associated with large-scale climate processes.
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