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Steam reforming of acetic acid over Ni/biochar of low metal-loading:involvement of biochar in tailoring reaction intermediates renders superior catalytic performance

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Chinese Journal of Chemical Engineering 2024年第4期68卷 241-252页

作者： Yunyu Guo Yiran Wang Shu Zhang Yi Wang Song Hu Jun Xiang Walid Nabgan Xun Hu School of Material Science and Engineering University of JinanJinan 250022China Joint international Research Laboratory of Biomass Energy and Materials College of Materials Science and EngineeringNanjing Forestry UniversityNanjing 210037China State Key Laboratory of Coal Combustion Huazhong University of Science and TechnologyWuhan 430074China Departament d'Enginyeria Química Universitat Rovira i VirgiliTarragona 43007Spain

Biochar is a reactive carrier as it may be partially gasified with steam in steam reforming,which could influence the formation of reaction intermediates and modify catalytic ***,the Ni/biochar as well as two comparative catalysts,Ni/Al_(2)O_(3) and Ni/SiO_(2),with low nickel loading(2%(mass))was conducted to probe involvement of the varied carriers in the steam *** results indicated that the Ni/biochar performed excellent catalytic activity than Ni/SiO_(2) and Ni/Al_(2)O_(3),as the biochar carrier facilitated quick conversion of the -OH from dissociation of steam to gasify the oxygen-rich carbonaceous intermediates like C=O and C-O-C,resulting in low coverage while high exposure of nickel species for maintaining the superior catalytic *** converse,strong adsorption of aliphatic intermediates over Ni/Al_(2)O_(3) and Ni/SiO_(2) induced serious coking with polymeric coke as the main type(21.5%and 32.1%,respectively),which was significantly higher than that over Ni/biochar(3.9%).The coke over Ni/biochar was mainly aromatic or catalytic type with nanotube morphology and high *** high resistivity of Ni/biochar towards coking was due to the balance between formation of coke and gasification of coke and partially biochar with steam,which created developed mesopores in spent Ni/biochar while the coke blocked pores in Ni/Al_(2)O_(3) and Ni/SiO_(2) catalysts.

关键词： Steam reforming Acetic acid Ni/biochar catalyst Property of coke Reaction intermediates

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Solution of the Center Problem for a Class of Polynomial Differential Systems

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Acta Mathematica Sinica,English Series 2024年第7期40卷 1685-1696页

作者： Chang Jian Liu Jaume Llibre Rafael Ramírez Valentín Ramírez School of Mathematics(Zhuhai) Sun Yat-sen UniversityZhuhai519086P.R.China Departament de Matemàtiques Universitat Autònoma de Barcelona08193BellaterraBarcelonaCataloniaSpain Departament d’Enginyeria informàtica i Matemàtiques Universitat Rovira i VirgiliAvinguda dels Paiïsos Catalans 2643007TarragonaCataloniaSpain

Consider the polynomial differential system of degree m of the form x=-y(1+μ(a_(2)x-a_(1)y))+x(v(a_(1)x+a_(2)y)+Ω_(m-1)(x,y)),y=x(1+μ(a_(2)x-a_(1)y))+y(v(a_(1)x+a_(2)y)+Ω_(m-1)(x,y)),whereμandνare real numbers such that(μ^(2)+v^(2))(μ+v(m-2))(a_(1)^(2)+a_(2)^(2))≠m>2 andΩ_(m−1)(x,y)is a homogenous polynomial of degree m−1.A conjecture,stated in *** Equations 2019,suggests that whenν=1,this differential system has a weak center at the origin if and only if after a convenient linear change of variable(x,y)→(X,Y)the system is invariant under the transformation(X,Y,t)→(−X,Y,−t).For every degree m we prove the extension of this conjecture to any value ofνexcept for a finite set of values ofμ.

关键词： Center problem polynomial differential system

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Umami taste components in chicken-spices blends and potential effect of aroma on umami taste intensity

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Food Science and Human Wellness 2024年第3期13卷 1220-1230页

作者： Rani Andaleeb Yiwen Zhu Ninglong Zhang Danni Zhang Muzahir Hussain Yin Zhang Yingshuang Lu Yuan Liu Department of Food Science&Technology School of Agriculture&BiologyShanghai Jiao Tong UniversityShanghai 200240China Tianjin Key Laboratory of Food Science and Health School of MedicineNankai UniversityTianjin 300071China MoBioFood Research Group Department of Biochemistry and BiotechnologyUniversitat Rovirai VirgiliTarragona 43007Spain Animal Nutrition Institut de Recercai Tecnologia Agroalimentàries(IRTA)Centre Mas BovéConstantí43120Spain Key Laboratory of Meat Processing of Sichuan Chengdu UniversityChengdu 610106China

in this study,umami taste intensity(UTi)and umami taste components in chicken breast(CB)and chickenspices blends were characterized using sensory and instrumental *** main objective was to assess the aroma-umami taste interactions in different food matrices and reconcile the aroma-taste perception to assist future product *** impact of key aroma,including vegetable-note"2-pentylfuran",meaty"methional",green"hexanal",and spicy-note-estragole and caryophyllene"on UTi was evaluated in monosodium glutamate and chicken *** found that spices significantly decreased UTi and umami taste components in ***,the perceptually similar odorants and tastants exhibited the potential to enhance UTi in food *** was able to increase the UTi,whereas spicy and green-note components could reduce the UTi *** information would be valuable to food engineers and formulators in aroma selection to control the UTi perceived by consumers,thus,improving the quality and acceptability of the chicken products.

关键词： Chicken-spices blends Umami taste components Aroma-taste interactions Perceptual similarity Umami taste intensity

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Multi-gigahertz mode-locked femtosecond Yb:KLuW waveguide lasers

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Photonics Research 2022年第11期10卷 2584-2589页

作者： Ji EUN BAE XAViER MATEOS MAGDALENA AGUiLÓ FRANCESC DÍAZ JAViER GARCÍA AJATES CAROLiNA ROMERO JAViER RODRÍGUEZ VÁZQUEZ DE ALDANA FABiAN ROTERMUND Department of Physics Korea Advanced Institute of Science and Technology(KAIST)34141 DaejeonRepublic of Korea Universitat rovira i virgili(URV) Fı´sica i Cristal·lografia de Materials i Nanomaterials(FiCMA)43007 TarragonaSpain Grupo de investigación en Aplicaciones del Láser y Fotónica University of Salamanca37008 SalamancaSpain

We demonstrate multi-gigahertz continuous-wave mode-locking of a Yb:KLuW waveguide laser. A femtosecondlaser-inscribed Yb:KLuW channel waveguide in an extended laser cavity delivers a fundamentally mode-locked laser near 1030 nm. A tunable few-centimeter-long cavity containing a single-walled carbon nanotube saturable absorber as mode-locker generates self-starting femtosecond pulses with average output powers exceeding210 mW at repetition rates of 2.27, 2.69, and 3.55 GHz. The laser cavity, which includes a wedged waveguide,is extended by using a lens pair that controls the laser fluence on the saturable absorber for reliable mode-locked operation without instability. The presented laser performance, mode-locked up to 3.55 GHz, highly suggests the potential of crystalline Yb:KLuW waveguides for realizing high-power ultrafast lasers with higher GHz repetition rates in a quasi-monolithic cavity.

关键词： waveguide femtosecond mode

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Microwave-Assisted Hydrolysis of Hemicellulose over Sulfonated Catalysts

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Advances in Materials Physics and Chemistry 2022年第11期12卷 306-322页

作者： itidel Belkadhi Mohamed Achraf Bouabdellah Lassâad Ben Hammouda Zouhaier Ksibi Francesco Medina university Tunis-El Manar Tunisia rovira i virgili university Tarragona Spain

Sulfonated catalysts based on zirconia (SO3H-ZrO2), silica (SO3H-SBA-15) and zeolite (SO3H-ZSM-5) were studied in the catalytic hydrolysis reaction of hemicellulose in a microwave reactor. The prepared catalysts were characterized by various techniques (XRD, N2 physisorption at 77 K, SEM, TEM and NH3-TPD). The obtained results reveal that despite the differences in their structural and textural properties, the ZrO2, Al-SBA-15 and H-ZSM-5 supports show similar conversions. Doping supports with sulfonate species created hydrogen bonds between SO3H groups and increased the amount of weak acid sites, which enhanced the hydrolysis of hemicellulose. SO3H- ZSM-5 showed the highest catalytic activity followed by SO3H-SBA-15 while SO3H-ZrO2 exhibited a poor conversion. Furthermore, the catalytic hydrolysis of the hemicellulose leads to several interesting products, such as formic acid, acetic acid, lactic acid and xylan. The correlation between the catalytic performances and the acidic properties of the different samples indicates that the best catalytic performances were obtained with the least acidic solids and especially when the density of strong acid sites decreases.

关键词： ZrO2 Al-SBA-15 H-ZSM-5 SO3H Hemicellulose Microwave

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“Professional Corpora”:Teaching Strategies for Work with Online Documentation,Translation Memories and Content Management

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中国翻译 2008年第2期29卷 41-45页

作者： Anthony Pym rovira i virgili university TarragonaSpain

The expansion of electronic memory capacity is having fundamental long-term effects on the way texts are produced and used,and thus on the way they are *** are increasingly working on data bases in non-linear ways,separated from awareness of any active communicative *** enhances productivity and consistency but challenges more humanistic values like understanding,cooperation, and job *** order to address these changes,teaching practices should 1)make students aware of the communicative functions of texts, particularly the ways in which particular parts of texts become high-risk in particular situations,2)teach students how to use electronic tech- nologies within such a frame,and how to teach themselves about the technologies,and 3)train students for a range of professional communica- tion jobs,incorporating both the technical sides and the various revision and editing techniques now required by the technologies.

关键词：翻译文本教学策略内容管理记忆

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The Limit Case of a Domination Property

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Acta Mathematica Sinica,English Series 2012年第3期28卷 463-468页

作者： Magdalena LEMANSKA Juan A. RODRíGUEZ-VELZQUEZ ismael G. YERO Department of Technical Physics and Applied Mathematics Gdańsk University of Technology Departament d’Enginyeria informàtica i Matemàtiques Universitat Rovira i Virgili Departament d'Enginyeria informàtica i Matemàtiques Universitat Rovira i Virgili

The domination number γ,（G） of a connected graph G of order n is bounded below by

关键词： Dominating set domination number

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Measurement of serum paraoxonase-1 activity in the evaluation of liver function

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World Journal of Gastroenterology 2009年第16期15卷 1929-1933页

作者： Jordi Camps Judit Marsillach Jorge Joven Centre of Biomedical Research University Hospital Sant JoanInstitute of Health Research Pere VirgiliUniversity Rovira i Virgili

Paraoxonase-1 (PON1) is an esterase and lactonase synthesized by the liver and found in the circulation associated with high-density lipoproteins. The physiological function of PON1 seems to be to degrade specific oxidized cholesteryl esters and oxidized phospholipids in lipoproteins and cell membranes. PON1 is, therefore, an antioxidant enzyme. Alterations in circulating PON1 levels have been reported in a variety of diseases involving oxidative stress including chronic liver diseases. Measurement of serum PON1 activity has been proposed as a potential test for the evaluation of liver function. However, this measurement is still restricted to research and has not been extensively applied in routine clinical chemistry laboratories. The reason for this restriction is due to the problem that the substrate commonly used for PON1 measurement, paraoxon, is toxic and unstable. The recent development of new assays with non-toxic substrates makes this proposal closer to a practical development. The present editorial summarizes PON1 biochemistry and function, its involvement with chronic liver impairment, and some aspects related to the measurement of PON1 activity in circulation.

关键词：肝功能活性酯酶血清检测临床化学实验室 PON1 高密度脂蛋白

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A Feature Selection Strategy to Optimize Retinal Vasculature Segmentation

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Computers, Materials & Continua 2022年第2期70卷 2971-2989页

作者： Jose Escorcia-Gutierrez Jordina Torrents-Barrena Margarita Gamarra Natasha Madera Pedro Romero-Aroca Aida Valls Domenec Puig Electronic and Telecommunications Engineering Program Universidad Autónoma del CaribeBarranquilla080001Colombia Department of Computational Science and Electronic Universidad de la CostaCUCBarranquilla080001Colombia Ophthalmology Service Universitari Hospital Sant JoanInstitut de Investigacio Sanitaria Pere VirgiliReus43201Spain Departament d’Enginyeria informàtica i Matemàtiques Escola Tècnica Superior d’EnginyeriaUniversitat Rovira i VirgiliTarragona43007Spain

Diabetic retinopathy (DR) is a complication of diabetesmellitus thatappears in the retina. Clinitians use retina images to detect DR pathologicalsigns related to the occlusion of tiny blood vessels. Such occlusion brings adegenerative cycle between the breaking off and the new generation of thinnerand weaker blood vessels. This research aims to develop a suitable retinalvasculature segmentation method for improving retinal screening proceduresby means of computer-aided diagnosis systems. The blood vessel segmentationmethodology relies on an effective feature selection based on SequentialForward Selection, using the error rate of a decision tree classifier in theevaluation function. Subsequently, the classification process is performed bythree alternative approaches: artificial neural networks, decision trees andsupport vector machines. The proposed methodology is validated on threepublicly accessible datasets and a private one provided by Hospital Sant Joanof Reus. in all cases we obtain an average accuracy above 96% with a sensitivityof 72% in the blood vessel segmentation process. Compared with the state-ofthe-art, our approach achieves the same performance as other methods thatneed more computational *** method significantly reduces the numberof features used in the segmentation process from 20 to 5 dimensions. Theimplementation of the three classifiers confirmed that the five selected featureshave a good effectiveness, independently of the classification algorithm.

关键词： Diabetic retinopathy artificial neural networks decision trees support vector machines feature selection retinal vasculature segmentation

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ScY@C_(3v)(8)-C_(82):Metal-Metalσ^(2)Bond in Mixed Rare-Earth Di-metallofullerenes

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Chinese Journal of Chemistry 2023年第15期41卷 1809-1814页

作者： Lihao Zheng Yannick Roselló Yingjing Yan Yang-Rong Yao Xiaolin Fan Josep M.Poblet Antonio Rodríguez-Fortea Ning Chen College of Chemistry Chemical Engineering and Materials Scienceand State Key Laboratory of Radiation Medicine and ProtectionSoochow UniversitySuzhouJiangsu 215123China Departament de Quimica Fisica i inorganica Universitat Rovira i VirgiliMarcelli Domingo 143007 TarragonaSpain Department of Materials Science and Engineering CAS Key Laboratory of Materials for Energy ConversionAnhui Laboratory of Advanced Photon Science and TechnologyUniversity of Science and Technology of ChinaHefeiAnhui 230026China

Comprehensive Summary The experimental investigation of rare-earth metal-metal bonds remains a challenge in the study of chemical ***,we report the synthesis and characterization of a novel heteronuclear di-metallofullerene,ScY@C_(3v)(8)-C_(82),which contains a mixed rare-earth metal-metal ***@C_(3v)(8)-C_(82)was successfully synthesized by arc-discharging method and characterized by mass spectrometry,UV-vis-NiR spectroscopy and single-crystal X-ray diffraction crystallography,which unambiguously determined its molecular *** calculations were also performed to study the optimized positions of Sc-Y metallic dimer and the electronic *** combined experimental and theoretical results confirmed that both Sc and Y atoms transfer two electrons to the C_(3v)(8)-C_(82)cage,i.e.,(ScY)4+@(C_(3v)(8)-C_(82))4-.in particular,a covalent Sc-Yσ2 bond,which has never been reported before,is proven to be formed inside C_(3v)(8)-C_(82)fullerene *** work presents a novel di-metallofullerene containing mixed rare-earth metal-metal bond and expands the understanding of metal-metal bonding of rare earth elements.

关键词： Fullerenes Endohedral fullerenes Rare earths Densityfunctional calculations Metal-metal bond

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