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Covalent organic framework/carbon black/molecularly imprinted polydopamine composites for the selective recognition and electrochemical detection of ciprofloxacin

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Food Science and Human Wellness 2024年

作者： Yufeng Sun Yongfeng Chen Xiaomin Pang Geoffrey I.N.waterhouse Xuguang Qiao Zhixiang Xu Key laboratory of Food Processing Technology and quality Control in Shandong Province， College of Food Science and Engineering， Shandong Agricultural University School of Chemical Sciences， The University of Auckland

In this work， a novel electrochemical sensor based on covalent organic framework@carbon black@molecularly imprinted polydopamine （COF@CB@MPDA） was developed for selective recognition and determination of ciprofloxacin （CF）. COF@CB@MPDA possessed good water dispersibility and was synthesized by the self-polymerization of dopamine under alkaline conditions in the presence of the COF， CB and CF. The high surface area COF enhanced the adsorption of CF， whilst CB gave the composites high electrical conductivity to improve the sensitivity of the proposed COF@CB@MPDA/GCE sensor. The specific recognition of CF by COF@CB@MPDA involved hydrogen bonding and van der Waals interactions. Under optimized conditions， the sensor showed a good linear relationship with CF concentration over the range 5.0 × 10-7mol/L and 1.0 × 10-4mol/L， with a limit of detection （LOD） of 9.53 × 10-8mol/L. Further， the developed sensor exhibited high selectivity， repeatability and stability for CF detection in milk and milk powders. The method used to fabricate the COF@CB@MPDA/GCE sensor could be easily adapted for the selective recognition and detection of other antibacterial agents and organic pollutants in the environment.

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Pursuing the goal of carbon neutrality in China:path for realization of carbon sequestration in planted forests

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Frontiers of Agricultural Science and Engineering 2024年第3期11卷 355-366页

作者： Lei DENG Haitao HU Jiwei LI Xue LI Chunbo HUANG Zhijing YU Hailong ZHANG Qing QU Xiaozhen WANG Lingbo DONG Zhouping SHANGGUAN State Key laboratory of Soil Erosion and Dryland Farming on the Loess Plateau Northwest A&F UniversityYangling 712100China College of Soil and water Conservation Science and Engineering(Institute of Soil and water Conservation) Northwest A&F UniversityYangling 712100China Shaanxi Forestry Survey and Planning Institute Xi’an 710000China College of Landscape Architecture Northeast Forestry UniversityHarbin 150040China Institute of Soil and water Conservation Chinese Academy of Sciences and Ministry of Water ResourcesYangling 712100China Key laboratory of Regional Ecology and Environmental Change School of Geography and Information EngineeringChina University of GeosciencesWuhan 430074China

Tree plantations are an important forest resource that substantively contributes to climate change mitigation and carbon *** the area and standing volume of tree plantations in China have increased,issues such as unreasonable structure,low productivity,limited ecological functionality and diminishing ecological stability have occurred,which hinder the ability of tree plantations to enhance carbon *** study outlined the trajectory of carbon sequestration and its associated benefits in tree plantations by examining the current state of tree plantation establishment and growth,elucidated the strategies for advantages of carbon sequestration and climate change mitigation in planted forests,and summarized the existing problems with tree *** paper underscores the pressing need for concerted efforts to boost carbon sequestration within planted forests and proposes management and development strategies for Chinese tree *** the future,it will be necessary to apply scientific theories to practice and develop multi-objective management optimization models for the high-quality development of tree *** will involve establishing a cohesive national carbon trading market,improving the prediction of carbon sequestration,and identifying priority zones for afforestation and reforestation,to better serve China’s national strategy for achieving peak carbon and carbon neutrality.

关键词： Planted forest carbon stock carbon sequestration carbon management climate change promotion path

Chemical modification of barite for improving the performance of weighting materials for water-based drilling fluids

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Petroleum Science 2024年第1期21卷 551-566页

作者： Li-Li Yang Ze-Yu Liu Shi-bo Wang Xian-Bo He Guan-Cheng Jiang Jie Zhang MOE Key laboratory of Petroleum Engineering State Key Laboratory of Petroleum Resources and ProspectingChina University of Petroleum(Beijing)Changping DistrictBeijing102249China MOE Key CNPC Drilling research Institute Changping DistrictBeijing102206China

With increasing drilling depth and large dosage of weighting materials,drilling fluids with high solid content are characterized by poor stability,high viscosity,large water loss,and thick mud cake,easier leading to reservoir damage and wellbore *** this paper,micronized barite(MB)was modified(mMB)by grafting with hydrophilic polymer onto the surface through the free radical polymerization to displace conventional API barite *** suspension stability of water-based drilling fluids(WBDFs)weighted with API barite:mMB=2:1 in 600 g was significantly enhanced compared with that with API barite/WBDFs,exhibiting the static sag factor within 0.54 and the whole stability index of *** viscosity and yield point reached the minimum,with a reduction of more than 40%compared with API barite only at the same *** multi-stage filling and dense accumulation of weighting materials and clays,filtration loss was decreased,mud cake quality was improved,and simultaneously it had great reservoir protection performance,and the permeability recovery rate reached 87%.In addition,it also effectively improved the lubricity of *** sticking coefficient of mud cake was reduced by 53.4%,and the friction coefficient was ***,mMB can serve as a versatile additive to control the density,rheology,filtration,and stability of WBDFs weighted with API barite,thus regulating comprehensive performance and achieving reservoir protection *** work opened up a new path for the productive drilling of extremely deep and intricate wells by providing an efficient method for managing the performance of high-density WBDFs.

关键词： Drilling fluids Weighting materials Filtration control Reservoir protection Stability property

Health risk assessment of municipal solid waste incineration emissions based on regression analysis

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Eco-Environment & Health 2024年第3期3卷 338-346页

作者： Zhuoshi Huang Jicui Cui Abdoulaye Boré Wenchao Ma Ziyi Zhang Zhi Qiao Ziyang Lou Johann Fellner School of Environmental Science and Engineering Tianjin UniversityTianjin 300072China Key laboratory of Agro-Forestry Environmental Processes and Ecological Regulation of Hainan Province College of Ecology and EnvironmentHainan UniversityHaikou 570228China Offshore Environmental Technology&Services Limited Beijing 100027China Shanghai Engineering research Center of Solid Waste Treatment and Resource Recovery School of Environmental Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China Christian Doppler laboratory for Anthropogenic Resource Institute for Water Quality and Resource ManagementTU WienKarlsplatz 13/2261040 ViennaAustria

This study examined the potential health risks posed by the operation of 96 waste-to-energy(WtE)plants in 30 cities in the Bohai Rim of *** a sophisticated simulation approach,the Weather research and Forecasting(WRF)model coupled with the California Puff(CALPUFF)model,we obtained the spatial distribution of pollutants emitted by WtE plants in the *** indices(HI)and cancer risks(CR)were calculated for each plant using the United States Environmental Protection Agency's recommended *** results indicated that both HIs and CRs were generally low,with values below the accepted threshold of 1.0 and 1.0×10^(-6),***,the average HI and CR values for the entire study area were 2.95×10^(-3)and 3.43×10^(-7),***,some variability in these values was observed depending on the location and type of WtE plant.A thorough analysis of various parameters,such as waste composition,moisture content,and operating conditions,was conducted to identify the factors that influence the health risks associated with *** findings suggest that proper waste sorting and categorization,increased cost of construction,and elevated height of chimneys are effective strategies for reducing the health risks associated with ***,this study provides valuable insights into the potential health risks associated with WtE plants in the Bohai Rim region of *** findings can serve as useful guidelines for law enforcement wings and industry professionals seeking to minimize the risks associated with municipal solid waste(MSW)management and promote sustainable development.

关键词： Incineration WRF/CALPUFF Health risk assessment Ridge regression model MSW classification

Multivariate statistical and bioinformatic analyses for the seasonal variations of actinobacterial community structures in a drinking water reservoir

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Journal of Environmental Sciences 2024年第3期137卷 1-17页

作者： Haihan Zhang Sixuan Pan BenMa Tinglin Huang Dmitry B.Kosolapov Manli Ma Xiang Liu Huan Liu Xiaoyan Liu Shaanxi Key laboratory of Environmental Engineering Key Laboratory of Northwest Water ResourceEnvironment and EcologyMOEXi’an University of Architecture and TechnologyXi’an 710055China School of Environmental and Municipal Engineering Xi’an University of Architecture and TechnologyXi’an 710055China Papanin Institute for Biology of Inland waters of Russian Academy of Sciences(IBIW RAS) 109BorokNekouzYaroslavl152742Russia

Actinobacterial community is a conspicuous part of aquatic ecosystems and displays an important role in the case of biogeochemical cycle,but little is known about the seasonal variation of actinobacterial community in reservoir ecological *** this study,the high-throughput techniques were used to investigate the structure of the aquatic actinobacterial community and its inducing water quality parameters in different *** results showed that the highest diversity and abundance of actinobacterial community occurred in winter,with Sporichthya(45.42%)being the most abundant genus and Rhodococcus sp.(29.32%)being the most abundant *** analysis and correlation analysis suggested that in autumn the dynamics of actinobacterial community were infuenced by more factors and Nocardioides ***2R5S2 was the potential keystone species which was negatively correlated with temperature(R=-0.72,Pwater qualities,while the physiochemical parameters(path coefficient=1.571,Pwater reservoirs and provide scientific guidance for further water quality management and protection in water sources.

关键词： Source water reservoir High-throughput sequencing Correlation analysis Network analysis Partial least squares path modeling

Geographical features and development models of estuarine cities

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Journal of Geographical Sciences 2024年第1期34卷 25-40页

作者： CHEN Mingxing XIAN Yue HUANG Yaohuan SUN Zhigang WU Chengbin Key laboratory of Regional Sustainable Development Modeling Institute of Geographic Sciences and Natural Resources ResearchCASBeijing 100101China College of Resource and Environment University of Chinese Academy of SciencesBejing 100049China State Key laboratory of Resources and Environmental Information System Institute of Geographic Sciences and Natural Resources ResearchCASBeijing 100101China Key laboratory of Ecosystem Network Observation and Modeling Institute of Geographic Sciences and Natural Resources ResearchCASBeijing 100101China Zhongke Shandong Dongying Institute of Geography Dongying 257509ShandongChina CAs Engineering laboratory for Yellow River Delta Modern Agriculture Institute of Geographic Sciences and Natural Resources ResearchCASBeijing 100101China

Cities are the key areas for human beings to achieve sustainable development goals in the *** cities are a special type of coastal city in urgent need of a clear *** paper proposed that estuarine cities are cities developed on the coast where rivers and oceans meet and defined four connotations,including the intersection of rivers and marine water systems,the coordinated development of land and oceans,the location advantages of connecting rivers and seas,and the important fragility of the ecological *** used Hydro SHEDS,OSM,GPW,and urban socioeconomic statistics and selected 50 estuarine cities with large rivers as representatives to summarize the main geographical basis and socioeconomic *** are primarily found in low-altitude,flat regions with average annual temperatures that mainly vary from 10℃to 25℃,relatively abundant precipitation,and extensive biological *** are substantial variations in the socioeconomic features of estuarine *** proposed eight development patterns,including open and inclusive city spirit,high-quality livable cities,high-quality development driven by innovation,integration of internal and external communication with ports and cities,construction of an international financial center,ecological environment protection and restoration,active promotion of cultural tourism,and positive international exchanges.

关键词： estuarine cities great rivers development models sustainability physical geography socioeconomy

考虑生态系统服务价值基于混合双主体代理和元胞自动机建模的高密度人口流域土地利用/土地覆盖动态模拟方法研究（英文）

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Engineering 2024年第6期 182-195页

作者：李雨桐蔡宴朋付强张晓东万航杨志峰 Guangdong Provincial Key laboratory of water quality Improvement and Ecological Restoration for watersheds Institute of Environmental and Ecological Engineering Guangdong University of Technology School of water Conservancy and Civil Engineering Northeast Agricultural University School of Environmental Science and Engineering Shandong University

Land use/land cover represents the interactive and comprehensive influences between human activities and natural conditions, leading to potential conflicts among natural and human-related issues as well as among stakeholders. This study introduced economic standards for farmers. A hybrid approach(CA-ABM)of cellular automaton(CA) and an agent-based model(ABM) was developed to effectively deal with social and land-use synergic issues to examine human–environment interactions and projections of land-use conversions for a humid basin in south China. Natural attributes and socioeconomic data were used to analyze land use/land cover and its drivers of change. The major modules of the CA-ABM are initialization, migration, assets, land suitability, and land-use change decisions. Empirical estimates of the factors influencing the urban land-use conversion probability were captured using parameters based on a spatial logistic regression(SLR) model. Simultaneously, multicriteria evaluation(MCE) and Markov models were introduced to obtain empirical estimates of the factors affecting the probability of ecological land conversion. An agent-based CA-SLR-MCE-Markov(ABCSMM) land-use conversion model was proposed to explore the impacts of policies on land-use conversion. This model can reproduce observed land-use patterns and provide links for forest transition and urban expansion to land-use decisions and ecosystem services. The results demonstrated land-use simulations under multi-policy scenarios, revealing the usefulness of the model for normative research on land-use management.

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Inkjet-Printing Controlled Phase Evolution Boosts the Efficiency of Hole Transport Material Free and Carbon-Based CsPbBr_(3) Perovskite Solar Cells Exceeding 9%

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Energy & Environmental Materials 2024年第2期7卷 209-220页

作者： Lihua Zhang Shi Chen Jie Zeng Zhengyan Jiang Qian Ai Xianfu Zhang Bihua Hu Xingzhu Wang Shihe Yang Baomin Xu Department of Materials Science and Engineering and Shenzhen Engineering research and Development Center for Flexible Solar Cells Southern University of Science and TechnologyShenzhen 518055China Department of Chemistry The Hong Kong University of Science and TechnologyClear Water BayHong KongChina Henan Key laboratory of Photovoltaic Materials Henan UniversityKaifeng 475004China Guangdong Key Lab of Nano-Micro Material research School of Chemical Biology and BiotechnologyShenzhen Graduate SchoolPeking UniversityShenzhen 518055China Key University laboratory of Highly Efficient Utilization of Solar Energy and Sustainable Development of Guangdong Southern University of Science and TechnologyShenzhen 518055China Guangdong-Hong Kong-Macao Joint laboratory for Photonic-Thermal-Electrical Energy Materials and Devices Southern University of Science and TechnologyShenzhen 518055China

Hole transport material free carbon-based all-inorganic CsPbBr_(3)perovskite solar cells(PSCs)are promising for commercialization due to its low-cost,high open-circuit voltage(V_(oc))and superior *** to the different solubility of PbBr_(2)and CsBr in conventional solvents,CsPbBr_(3)films are mainly obtained by multi-step spin-coating through the phase evolution from PbBr_(2)to CsPb_(2)Br_(5)and then to CsPbBr_(3).The scalable fabrication of high-quality CsPbBr_(3)films has been rarely ***,an inkjet-printing method is developed to prepare high-quality CsPbBr_(3)*** formation of long-range crystalline CsPb_(2)Br_(5)phase can effectively improve phase purity and promote regular crystal stacking of CsPbBr_(3).Consequently,the inkjet-printed CsPbBr_(3)C-PSCs realized PCEs up to 9.09%,8.59%and 7.81%with active areas of 0.09,0.25,and 1 cm^(2),respectively,demonstrating the upscaling potential of our fabrication method and *** high performance is mainly ascribed to the high purity,strong crystal orientation,reduced surface roughness and lower trap states density of the as-printed CsPbBr_(3)*** work provides insights into the relationship between the phase evolution mechanisms and crystal growth dynamics of cesium lead bromide halide films.

关键词： all-inorganic perovskite solar cells CsPbBr_(3) inkjet-printing phase evolution

A novel electro-Fenton hybrid system for enhancing the interception of volatile organic compounds in membrane distillation desalination

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Journal of Environmental Sciences 2024年第4期138卷 189-199页

作者： Hongxin Liu Kuiling Li Kunpeng Wang Zhiyong Wang Zimou Liu Sichao Zhu Dan Qu Yu Zhang Jun Wang State Key laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China State Key laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua UniversityBeijing 100084China School of Chemical and Environmental Engineering Beijing CampusChina University of Mining and TechnologyBeijing 100083China Beijing Key Lab for Source Control Technology of water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China

Membrane distillation(MD)is a promising alternative desalination technology,but the hydrophobic membrane cannot intercept volatile organic compounds(VOCs),resulting in aggravation in the quality of *** term of this,electro-Fenton(EF)was coupled with sweeping gas membrane distillation(SGMD)in a more efficient way to construct an advanced oxidation barrier at the gas-liquid interface,so that the VOCs could be trapped in this layer to guarantee the water quality of the *** the so-called EF-MD process,an interfacial interception barrier containing hydroxyl radical formed on the hydrophobic membrane *** contributed to the high phenol rejection of 90.2% with the permeate phenol concentration lower than 1.50 mg/*** interceptions can be achieved in a wide temperature range,even though the permeate flux of phenol was also *** EF-MD system was robust to high salinity and could electrochemically regenerate ferrous ions,which endowed the long-term stability of the *** novel EF-MD configuration proposed a valuable strategy to intercept VOCs in MD and will broaden the application of MD in hypersaline wastewater treatment.

关键词： Membrane distillation VOC interception Interfacial oxidation Electro-Fenton Hypersaline wastewater