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Thermal management by manipulating electromagnetic parameters

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Chinese Physics B 2024年第5期33卷 21-27页

作者：王云梁迪飞韩天成邓龙江 National Engineering research center of Electromagnetic Radiation Control materials University of Electronic Science and Technology of ChinaChengdu 611731China Key Laboratory of Multi-spectral Absorbing materials and structures of Ministry of Education University of Electronic Science and Technology of ChinaChengdu 611731China

Electromagnetic absorbing materials may convert electromagnetic energy into heat energy and dissipate ***,in a high-power electromagnetic radiation environment,the temperature of the absorbing material rises significantly and even *** becomes critical to ensure electromagnetic absorption performance while minimizing temperature ***,we systematically study the coupling mechanism between the electromagnetic field and the temperature field when the absorbing material is irradiated by electromagnetic *** find out the influence of the constitutive parameters of the absorbing materials(including uniform and non-uniform)on the temperature ***,through a smart design,we achieve better absorption and lower temperature *** accuracy of the model is affirmed as simulation results aligned with theoretical *** work provides a new avenue to control the temperature distribution of absorbing materials.

关键词： multi-physics field electromagnetic-thermal coupling microwave absorption high power application

Ultra-high-temperature application of MXene: Stabilization of 2D Ti_(3)C_(2)T_(x) for cross-scale strengthening and toughening of 3D TiC

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Journal of Advanced Ceramics 2024年第1期13卷 1-10页

作者： Lu Liu Guobing Ying Quanguo Jiang Dong Wen Peng Wang Meng Wu Ziying Ji Yongting Zheng Xiang Wang Department of materials Science and Engineering College of Mechanics and MaterialsHohai UniversityNanjing 211100China Key Laboratory of Superlight materials&Surface Technology Ministry of EducationHarbin Engineering UniversityHarbin 150001China Shenzhen Key Laboratory for Advanced materials School of Materials Science and EngineeringHarbin Institute of Technology(Shenzhen)Shenzhen 518055China center for Composite materials and structures Harbin Institute of TechnologyHarbin 150001China

Transition metal carbide/nitride cores within MXenes make them considerably useful for ultra-high-temperature ***,extensive research on Ti_(3)C_(2)T_(x) MXene has revealed its tendency to undergo a phase transition to TiCy at temperatures above 800℃due to high activity of a superficial Ti atomic ***,spark plasma sintering of Ti_(3)C_(2)T_(x) and TiC is performed to prevent the Ti_(3)C_(2)T_(x) phase transition at temperatures up to 1900℃through the fabrication of composites at a pressure of 50 *** a focused ion beam scanning electron microscope to separate layered substances in the composites and examining selected area diffraction spots in a transmission electron microscope enabled identification of non-phase-transitioned ***-principles calculations based on density functional theory indicated the formation of strong chemical bonding interfaces between Ti_(3)C_(2)T_(x) and TiC,which imposed a stability constraint on the Ti atomic layer at the Ti_(3)C_(2)T_(x) *** performance tests,such as three-point bending and fracture toughness analysis,demonstrated that the addition of Ti_(3)C_(2)T_(x) can effectively improve the cross-scale strengthening and toughening of the TiC matrix,providing a new path for designing and developing two-dimensional(2D)carbides cross-scale-enhanced three-dimensional(3D)carbides with the same elements relying on a wide variety of MXenes.

关键词： MXene ultra-high-temperature phase stability interface bonding cross-scale strengthening and toughening structural ceramic composites

Gate Tunable Labyrinth Domain structures in a van der Waals Itinerant Ferromagnet Cr_(7)Te_(8)

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Chinese Physics Letters 2024年第9期41卷 122-132页

作者： Kui Meng Zeya Li Yicheng Shen Xiangyu Bi Junhao Rao Yuting Qian Zhansheng Gao Peng Chen Caiyu Qiu Feng Qin Jinxiong Wu Feng Luo Junwei Huang Hongtao Yuan National Laboratory of Solid State Microstructures Jiangsu Key Laboratory of Artificial Functional MaterialsCollege of Engineering and Applied Sciencesand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210000China center for the Physics of Low-Dimensional materials Henan Joint International Research Laboratory of New Energy Materials and DevicesSchool of Physics and ElectronicsHenan UniversityKaifeng 475004China Tianjin Key Lab for Rare Earth materials and Applications Center for Rare Earth and Inorganic Functional MaterialsSmart Sensor Interdisciplinary Science CenterSchool of Materials Science and EngineeringNankai UniversityTianjin 300350China

Manipulating magnetic domain structure plays a key role in advanced spintronics *** rationale is that the labyrinthine domain structure,normally appearing in ferromagnetic thin films with strong magnetic anisotropy,shows a great potential to increase data storage density for designing magnetic nonvolatile memory and logic ***,an electrical control of labyrinthine domain structure remains ***,we demonstrate the gate-driven evolution of labyrinthine domain structures in an itinerant ferromagnet Cr_(7)Te_(8).By combining electric transport measurements and micromagnetic finite difference simulations,we find that the hysteresis loop of anomalous Hall effect in Cr_(7)Te_(8)samples shows distinct features corresponding to the generation of labyrinthine domain *** labyrinthine domain structures are found to be electrically tunable via Li-electrolyte gating,and such gate-driven evolution in Cr_(7)Te_(8)originates from the reduction of the magnetic anisotropic energy with gating,revealed by our micromagnetic *** results on the gate control of anomalous Hall effect in an itinerant magnetic material provide an opportunity to understand the formation and evolution of labyrinthine domain structures,paving a new route towards electric-field driven spintronics.

关键词： rational electrolyte ferromagnetic

Electroluminescence from pure resonant states in hBN-based vertical tunneling junctions

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Light(Science & Applications) 2024年第8期13卷 1557-1564页

作者： Magdalena Grzeszczyk Kristina Vaklinova Kenji Watanabe Takashi Taniguchi Konstantin SNovoselov Maciej Koperski Institute for Functional Intelligent materials National University of SingaporeSingapore 117544Singapore research center for Functional materials National Institute for Materials ScienceTsukuba 305-0044Japan International center for materials Nanoarchitectonics National Institute for Materials ScienceTsukuba 305-0044Japan Department of materials Science and Engineering National University of SingaporeSingapore 117575Singapore

Defect centers in wide-band-gap crystals have garnered interest for their potential in applications among optoelectronic and sensor ***,defects embedded in highly insulating crystals,like diamond,silicon carbide,or aluminum oxide,have been notoriously difficult to excite electrically due to their large internal *** address this challenge,we realized a new paradigm of exciting defects in vertical tunneling junctions based on carbon centers in hexagonal boron nitride(hBN).The rational design of the devices via van der Waals technology enabled us to raise and control optical processes related to defect-to-band and intradefect *** fundamental understanding of the tunneling events was based on the transfer of the electronic wave function amplitude between resonant defect states in hBN to the metallic state in graphene,which leads to dramatic changes in the characteristics of electrons due to different band structures of constituent *** our devices,the decay of electrons via tunneling pathways competed with radiative recombination,resulting in an unprecedented degree of tuneability of carrier dynamics due to the significant sensitivity of the characteristic tunneling times on the thickness and structure of the *** enabled us to achieve a high-efficiency electrical excitation of intradefect transitions,exceeding by several orders of magnitude the efficiency of optical excitation in the sub-band-gap *** work represents a significant advancement towards a universal and scalable platform for electrically driven devices utilizing defect centers in wide-band-gap crystals with properties modulated via activation of different tunneling mechanisms at a level of device engineering.

关键词： carbide tunneling defect

Inclusion of CoTiO_(3) to ameliorate the re/dehydrogenation properties of the Mg–Na–Al system

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Journal of Magnesium and Alloys 2024年第3期12卷 1215-1226页

作者： N.A.Ali N.Y.Yusnizam N.A.Sazelee Sami-ullah Rather Haizhen Liu M.Ismail Energy Storage research Group Faculty of Ocean Engineering TechnologyUniversiti Malaysia Terengganu21030 Kuala NerusTerengganuMalaysia Department of Chemical and materials Engineering King Abdulaziz UniversityP.O.Box80204Jeddah 21589Saudi Arabia Guangxi Novel Battery materials research center of Engineering Technology School of Physical Science and TechnologyGuangxi UniversityNanning 530004China State Key Laboratory of Featured Metal materials and Life-Cycle Safety for Composite structures Nanning 530004China

For the first time,the MgH_(2)–NaAlH_(4)(ratio 4:1)destabilized system with CoTiO_(3) addition has been *** CoTiO_(3)-doped MgH_(2)–NaAlH_(4) sample begins to dehydrogenate at 130℃,which is declined by 40℃ compared to the undoped MgH_(2)–NaAlH_(4).Moreover,the de/rehydrogenation kinetics characteristics of the CoTiO_(3)-doped MgH_(2)–NaAlH_(4) were greatly *** the inclusion of CoTiO_(3),the MgH_(2)–NaAlH_(4) composite absorbed 5.2 wt.%H_(2),higher than undoped MgH_(2)–NaAlH_(4).In the context of dehydrogenation,the CoTiO_(3)-doped MgH_(2)–NaAlH_(4) sample desorbed 2.6 wt.%H_(2),almost doubled compared to the amount of hydrogen desorbed from the undoped MgH_(2)–NaAlH_(4) *** activation energy obtained by the Kissinger analysis for MgH_(2) decomposition was significantly lower by 35.9 kJ/mol than the undoped MgH_(2)–NaAlH_(4) *** reaction mechanism demonstrated that new phases of MgCo and AlTi_(3) were generated in situ during the heating process and are likely to play a substantial catalytic function and be useful in ameliorating the de/rehydrogenation properties of the destabilized MgH_(2)–NaAlH_(4) system with the inclusion of CoTiO_(3).

关键词： Destabilize system Magnesium hydride Sodium alanate Hydrogen storage Additive.

Quantum confinement of carriers in the type-I quantum wells structure

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Chinese Physics B 2024年第9期33卷 553-558页

作者： Xinxin Li Zhen Deng Yang Jiang Chunhua Du Haiqiang Jia Wenxin Wang Hong Chen Key Laboratory for Renewable Energy Beijing Key Laboratory for New Energy Materials andDevicesBeijing National Laboratory for Condensed Matter PhysicsInstitute of PhysicsChineseAcademy of SciencesBeijing 100190China center of materials and Optoelectronics Engineering University of Chinese Academy ofSciencesBeijing 100049China The Yangtze River Delta Physics research center Liyang 213000China Songshan Lake materials Laboratory Dongguan 523808China

Quantum confinement is recognized to be an inherent property in low-dimensional ***,it is believed that the carriers trapped within the well cannot escape due to the discrete energy ***,our previous research has revealed efficient carrier escape in low-dimensional structures,contradicting this conventional *** this study,we review the energy band structure of quantum wells along the growth direction considering it as a superposition of the bulk material dispersion and quantization energy dispersion resulting from the quantum confinement across the whole Brillouin *** accounting for all wave vectors,we obtain a certain distribution of carrier energy at each quantized energy level,giving rise to the energy *** results enable carriers to escape from the well under the influence of an electric ***,we have compiled a comprehensive summary of various energy band scenarios in quantum well structures relevant to carrier *** a new interpretation holds significant value in deepening our comprehension of low-dimensional energy bands,discovering new physical phenomena,and designing novel devices with superior performance.

关键词： energy band quantum confinement type-I quantum wells low-dimensional structures

SnIP-type atomic-scale inorganic double-helix semiconductors: Synthesis, properties, and applications

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Nano research 2024年第3期17卷 2111-2128页

作者： Mudussar Ali Bowen Zhang Muhammad Khurram Qingfeng Yan Engineering research center of Advanced Rare Earth materials(Ministry of Education) Department of ChemistryTsinghua UniversityBeijing 100084China

Flexible inorganic double helical semiconductors similar to DNA have fueled the demand for efficient materials with innovative structures and excellent *** recent discovery of tin phosphide iodide(SnIP),the first carbon-free double helical semiconductor at an atomic level,has opened new avenues of research for semiconducting devices such as thermoelectric and sensor devices,solar cells,and *** has drawn significant academic attention due to its high structural flexibility,band gap in the visible spectrum range,and non-toxic ***,the recent progress in developing SnIP,including its prestigious structure,versatile and intriguing properties,and synthesis,is *** analogues of SnIP and SnIP-based hybrid materials and their applications in photocatalysis are also ***,the review concludes with a critical summary and future aspects of this new inorganic semiconductor.

关键词： tin phosphide iodide(SnIP) inorganic semiconductor inorganic double helix SnIP-based hybrids photocatalysis flexible material

Highly uniform Co-Cu bimetallic sulfides for rechargeable alkaline aqueous zinc batteries

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Chinese Chemical Letters 2024年第2期35卷 521-526页

作者： Xiaofang Bai Yuwei Zhao Mangwei Cui Tianshuo Guo Zijie Tang Chuan Li Heng Gao Shuo Yang Lingzhi Zhao Chunyi Zhi Hongfei Li Department of materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Songshan Lake materials Laboratory Dongguan 523808China Department of materials Science and Engineering City University of Hong KongHong KongChina International Centre for Quantum and Molecular structures Department of PhysicsShanghai UniversityShanghai 200444China Guangdong Provincial Engineering Technology research center for Low Carbon and Advanced Energy materials Institute of Semiconductor Science and TechnologySouth China Normal UniversityGuangzhou 510631China

Rechargeable alkaline aqueous zinc batteries(RAZBs)have attracted increasing ***,most RAZBs are hindered by the limited availability of cathode *** practical electrochemical performance of most cathode materials is lower than the theoretical value due to their poor electrical conductivity and low utilization *** this work,we develop a facile hydrothermal procedure to prepare highly uniform bimetallic sulfides as novel cathode materials for ***-cobalt binary metallic oxides materials possess higher conductivity and larger capacity compared with their mono-metal oxides compounds due to bimetallic synergistic effects and multiple oxidation ***,bimetallic sulfide compounds have smaller bond energy and longer bond length than their oxides,leading to less structural damage,faster kinetics of electrochemical reactions,and better *** as-prepared Co-Cu bimetallic sulfides show enhanced electrochemical performance due to various valences of Co and Cu as well as the existence of *** a result,aqueous Zn/CuCo_(2)S_(4) battery shows a high specific capacity of 117.4 mAh/g at 4 A/g and a good cycle life of over 8000 *** on PANa hydrogel electrolytes,a flexible Zn/CuCo_(2)S_(4) battery demonstrates excellent cycling *** battery can also meet the requirements of electronic devices with different shapes and performs well in extreme environments,such as freezing,drilling,and *** work opens new avenues to obtain high-rate and long-life cathode materials for RAZBs by utilizing the synergistic effects of bimetallic sulfides and provides a new platform for flexible energy storage devices.

关键词： Aqueous zinc batteries Bimetallic sulfides Cathode materials Rate performance Cycling stability

Properties and Characteristics of Regolith-Based materials for Extraterrestrial Construction

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Engineering 2024年第6期37卷 159-181页

作者： Cheng Zhou Yuyue Gao Yan Zhou Wei She Yusheng Shi Lieyun Ding Changwen Miao National center of Technology Innovation for Digital Construction Huazhong University of Science and TechnologyWuhan 430074China School of Civil and hydraulic Engineering Huazhong University of Science and TechnologyWuhan 430074China School of materials Science and Engineering Southeast UniversityNanjing 214135China State Key Laboratory of materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

The construction of extraterrestrial bases has become a new goal in the active exploration of deep *** the construction techniques,in situ resource-based construction is one of the most promising because of its good sustainability and acceptable economic cost,triggering the development of various types of extraterrestrial construction materials.A comprehensive survey and comparison of materials from the perspective of performance was conducted to provide suggestions for material selection and *** types of typical construction materials are discussed in terms of their reliability and applicability in extreme extraterrestrial ***,thermal and optical,and radiation-shielding properties are *** influencing factors and optimization methods for these properties are *** the perspective of material properties,the existing challenges lie in the comprehensive,long-term,and real characterization of regolith-based construction ***,the suggested future directions include the application of high-throughput characterization methods,accelerated durability tests,and conducting extraterrestrial experiments.

关键词： Extraterrestrial construction Characterization Mechanical property Thermal property Optical property Radiation-shielding