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Memristive switching in the surface of a charge-density-wave topological semimetal

Science Bulletin 2024年第13期69卷 2042-2049页

作者： Jianwen Ma Xianghao Meng Binhua Zhang Yuxiang Wang Yicheng Mou Wenting Lin Yannan Dai Luqiu Chen Haonan Wang Haoqi Wu Jiaming Gu Jiayu Wang Yuhan Du Chunsen Liu Wu Shi Zhenzhong Yang Bobo Tian Lin Miao Peng Zhou Chun-Gang Duan Changsong Xu Xiang Yuan Cheng Zhang State Key Laboratory of Surface Physics and Institute for Nanoelectronic devices and Quantum Computing Fudan UniversityShanghai 200433China State Key Laboratory of Precision Spectroscopy East China Normal UniversityShanghai 200241China Key Laboratory of Computational Physical Sciences(Ministry of Education) Institute of Computational Physical SciencesState Key Laboratory of Surface PhysicsDepartment of PhysicsFudan UniversityShanghai 200433China Shanghai Qi Zhi Institute Shanghai 200030China School of Physics Southeast UniversityNanjing 211189China Key Laboratory of Polar Materials and devices(Ministry of Education) Department of ElectronicsEast China Normal UniversityShanghai 200241China Shanghai center of Brain–inspired intelligent Materials and devices East China Normal UniversityShanghai 200241China State Key Laboratory of ASIC and System School of MicroelectronicsFudan UniversityShanghai 200433China Frontier Institute of Chip and System Fudan UniversityShanghai 200433China Zhangjiang Fudan International Innovation center Fudan UniversityShanghai 201210China School of Physics and Electronic Science East China Normal UniversityShanghai 200241China

Owing to the outstanding properties provided by nontrivial band topology,topological phases of matter are considered as a promising platform towards low-dissipation electronics,efficient spin-charge conversion,and topological quantum *** ferroelectricity in topological materials enables the non-volatile control of the quantum states,which could greatly facilitate topological electronic ***,ferroelectricity is generally incompatible with systems featuring metallicity due to the screening effect of free *** this study,we report the observation of memristive switching based on the ferroelectric surface state of a topological semimetal(TaSe_(4))*** find that the surface state of(TaSe_(4))2I presents out-of-plane ferroelectric polarization due to surface *** the combination of ferroelectric surface and charge-density-wave-gapped bulk states,an electric-switchable barrier height can be achieved in(TaSe_(4))2I-metal *** employing a multi-terminal-grounding design,we manage to construct a prototype ferroelectric memristor based on(TaSe_(4))2I with on/off ratio up to 103,endurance over 103 cycles,and good retention *** origin of the ferroelectric surface state is further investigated by first-principles calculations,which reveal an interplay between ferroelectricity and band *** emergence of ferroelectricity in(TaSe_(4))2I not only demonstrates it as a rare but essential case of ferroelectric topological materials,but also opens new routes towards the implementation of topological materials in functional electronic devices.

关键词： Topological semimetal Schottky barrier Surface ferroelectricity Memristor

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Autonomous aeroamphibious invisibility cloak with stochastic-evolution learning

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Advanced Photonics 2024年第1期6卷 64-72页

作者： Chao Qian Yuetian Jia Zhedong Wang Jieting Chen Pujing Lin Xiaoyue Zhu Erping Li Hongsheng Chen Zhejiang University ZJU-UIUC InstituteInterdisciplinary Center for Quantum InformationState Key Laboratory of Extreme Photonics and InstrumentationHangzhouChina Zhejiang University ZJU-Hangzhou Global Science and Technology Innovation CenterKey Laboratory of Advanced Micro/Nano Electronic Devices and Smart Systems of ZhejiangHangzhouChina Zhejiang University Jinhua Institute of Zhejiang UniversityJinhuaChina

Being invisible ad libitum has long captivated the popular imagination,particularly in terms of safeguarding modern high-end instruments from potential *** ago,the advent of metamaterials and transformation optics sparked considerable interest in invisibility cloaks,which have been mainly demonstrated in ground and waveguide ***,an omnidirectional flying cloak has not been achieved,primarily due to the challenges associated with dynamic synthesis of metasurface *** demonstrate an autonomous aeroamphibious invisibility cloak that incorporates a suite of perception,decision,and execution modules,capable of maintaining invisibility amidst kaleidoscopic backgrounds and neutralizing external *** physical breakthrough lies in the spatiotemporal modulation imparted on tunable metasurfaces to sculpt the scattering field in both space and frequency *** intelligently control the spatiotemporal metasurfaces,we introduce a stochastic-evolution learning that automatically aligns with the optimal solution through maximum probabilistic *** a fully self-driving experiment,we implement this concept on an unmanned drone and showcase adaptive invisibility in three canonical landscapes-sea,land,and air-with a similarity rate of up to 95%.Our work extends the family of invisibility cloaks to flying modality and inspires other research on material discoveries and homeostatic meta-devices.

关键词： intelligent metasurfaces optical materials and structures deep learning

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Diphylleia Grayi-Inspired intelligent Temperature-Responsive Transparent Nanofiber Membranes

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Nano-Micro Letters 2024年第4期16卷 67-78页

作者： Cengceng Zhao Gaohui Liu Yanyan Lin Xueqin Li Na Meng Xianfeng Wang Shaoju Fu Jianyong Yu Bin Ding Shanghai Frontier Science research center of Advanced Textiles College of TextilesDonghua UniversityShanghai 201620People’s Republic of China

Nanofiber membranes(NFMs) have become attractive candidates for next-generation flexible transparent materials due to their exceptional flexibility and breathability. However, improving the transmittance of NFMs is a great challenge due to the enormous reflection and incredibly poor transmission generated by the nanofiber-air interface. In this research, we report a general strategy for the preparation of flexible temperature-responsive transparent(TRT) membranes,which achieves a rapid transformation of NFMs from opaque to highly transparent under a narrow temperature window. In this process, the phase change material eicosane is coated on the surface of the polyurethane nanofibers by electrospray technology. When the temperature rises to 37 ℃, eicosane rapidly completes the phase transition and establishes the light transmission path between the nanofibers, preventing light loss from reflection at the nanofiber-air interface. The resulting TRT membrane exhibits high transmittance(> 90%), and fast response(5 s). This study achieves the first TRT transition of NFMs, offering a general strategy for building highly transparent nanofiber materials, shaping the future of next-generation intelligent temperature monitoring, anti-counterfeiting measures, and other high-performance devices.

关键词： Biomimetic Transparent Nanofibrous membrane Temperature response Phase change materials

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A near-zero quiescent power breeze wake-up anemometer based on a rolling-bearing triboelectric nanogenerator

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Microsystems & Nanoengineering 2024年第2期10卷 241-249页

作者： Xianpeng Fu Zhichao Jiang Jie Cao Zefang Dong Guoxu Liu Meiling Zhu Chi Zhang CAS center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and SensorBeijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing101400China School of Nanoscience and Engineering University of Chinese Academy of SciencesBeijing100049China center on Nanoenergy research Guangxi Colleges and Universities Key Laboratory of Blue Energy and Systems IntegrationSchool of Physical Science&TechnologyGuangxi UniversityNanning530004China Institute of intelligent Flexible Mechatronics Jiangsu UniversityZhenjiang212013China College of Engineering Mathematics and Physical ScienceUniversity of ExeterExeterEX44QFUK

Wind sensors have always played an irreplaceable role in environmental information monitoring and are expected to operate with lower power consumption to extend service ***,we propose a breeze wake-up anemometer(B-WA)based on a rolling-bearing triboelectric nanogenerator(RB-TENG)with extremely low static *** B-WA consists of two RB-TENGs,a self-waking-up module(SWM),a signal processing module(SPM),and a wireless transmission *** two RB-TENGs are employed for system activation and wind-speed *** the ambient wind-speed exceeds 2 m/s,the wake TENG(W-TENG)and the SWM can wake up the system within 0.96 *** the same time,the SPM starts to calculate the signal frequency from the measured TENG(M-TENG)to monitor the wind speed with a sensitivity of 9.45 Hz/(m/s).After the wind stops,the SWM can switch off the B-WA within 0.52 s to decrease the system energy *** quiescent on-duty mode,the operating power of the B-WA is less than 30 nW,which can greatly extend the service lifetime of the *** integrating triboelectric devices and rolling bearings,this work has realized an ultralow quiescent power and self-waked-up wireless wind-speed monitoring system,which has foreseeable applications in remote weather monitoring,IoT nodes,and so on.

关键词： generator power service

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Nanoindentation behavior and creep-induced cracking of long-term crept austenitic steel at 650℃

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Journal of Iron and Steel research(International) 2024年第2期31卷 464-474页

作者： Zhen Zhang Yu-hang Duan Shuai Wang Jin-shan Chen An-zhe Wang Xiang-yang Mao Yuan-ji Shi Jie Zhang Ming Liu Zheng-fei Hu School of Materials Science and Engineering Nanjing Institute of TechnologyNanjing211167JiangsuChina Jiangsu Key Laboratory of Advanced Structural Materials and Application Technology Nanjing211167JiangsuChina Jiangsu Wind Power Engineering Technology center Nanjing210023JiangsuChina Nanjing Vocational University of Industry Technology Nanjing210023JiangsuChina Baoshan Iron&Steel Co. Ltd.Shanghai201900China Fujian Provincial Key Laboratory of Terahertz Functional devices and intelligent Sensing School of Mechanical Engineering and AutomationFuzhou UniversityFuzhou350116FujianChina School of Materials Science and Engineering Tongji UniversityShanghai201804China

The grain boundary(GB)damage of long-term crept HR3C(25Cr–20Ni–Nb–N)austenitic steel with solid solution state was investigated by nanoindentation test accompanied with in-situ electron back-scattered *** corresponding microstructure was characterized by scanning electron microscopy and transmission electron *** show that the increase in nanoindentation hardness at the GBs and triple grain junctions may be related to the dislocation accumulation and carbide growth during the *** M23C6 and dislocations piling-up at the GB accelerate the nucleation and coalescence of creep cavity along the *** nanoindentation hardness in grains varies with orientation of the stress *** orientation difference of neighbor grains may induce local high geometrically necessary dislocation densities and strain gradients near the GB,consequently causing stress concentration and subsequent crack growth at specific GBs.

关键词： Austenitic steel Creep Nanoindentation Grain orientation Creep-induced cracking

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Advances in neuromorphic computing:Expanding horizons for AI development through novel artificial neurons and in-sensor computing

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Chinese Physics B 2024年第3期33卷 1-23页

作者：杨玉波赵吉哲刘胤洁华夏扬王天睿郑纪元郝智彪熊兵孙长征韩彦军王健李洪涛汪莱罗毅 Department of Electronic Engineering Tsinghua UniversityBeijing 100084China Beijing National research center for Information Science and Technology Tsinghua UniversityBeijing 100084China

AI development has brought great success to upgrading the information *** the same time,the large-scale artificial neural network for building AI systems is thirsty for computing power,which is barely satisfied by the conventional computing *** the post-Moore era,the increase in computing power brought about by the size reduction of CMOS in very large-scale integrated circuits(VLSIC)is challenging to meet the growing demand for AI computing *** address the issue,technical approaches like neuromorphic computing attract great attention because of their feature of breaking Von-Neumann architecture,and dealing with AI algorithms much more parallelly and energy *** by the human neural network architecture,neuromorphic computing hardware is brought to life based on novel artificial neurons constructed by new materials or *** it is relatively difficult to deploy a training process in the neuromorphic architecture like spiking neural network(SNN),the development in this field has incubated promising technologies like in-sensor computing,which brings new opportunities for multidisciplinary research,including the field of optoelectronic materials and devices,artificial neural networks,and microelectronics integration *** vision chips based on the architectures could reduce unnecessary data transfer and realize fast and energy-efficient visual cognitive *** paper reviews firstly the architectures and algorithms of SNN,and artificial neuron devices supporting neuromorphic computing,then the recent progress of in-sensor computing vision chips,which all will promote the development of AI.

关键词： neuromorphic computing spiking neural network(SNN) in-sensor computing artificial intelligence

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基于电荷密度波半金属材料的表面忆阻转变（英文）

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Science Bulletin 2024年第13期 2042-2049页

作者：马健文孟祥浩张宾花王宇祥牟毅成林文亭代艳南陈璐秋王浩南吴昊奇顾嘉明王嘉宇杜宇涵刘春森石武杨振中田博博苗霖周鹏段纯刚徐长松袁翔张成 State Key Laboratory of Surface Physics and Institute for Nanoelectronic devices and Quantum Computing Fudan University State Key Laboratory of Precision Spectroscopy East China Normal University Key Laboratory of Computational Physical Sciences (Ministry of Education) Institute of Computational Physical Sciences State Key Laboratory of Surface PhysicsDepartment of Physics Fudan University Shanghai Qi Zhi Institute School of Physics Southeast University Key Laboratory of Polar Materials and devices (Ministry of Education) Department of Electronics East China Normal University Shanghai center of Brain-inspired intelligent Materials and devices East China Normal University State Key Laboratory of ASIC and System School of Microelectronics Fudan University Frontier Institute of Chip and System Fudan University Zhangjiang Fudan International Innovation center Fudan University School of Physics and Electronic Scienc5 East China Normal University

Owing to the outstanding properties provided by nontrivial band topology, topological phases of matter are considered as a promising platform towards low-dissipation electronics, efficient spin-charge conversion, and topological quantum computation. Achieving ferroelectricity in topological materials enables the non-volatile control of the quantum states, which could greatly facilitate topological electronic research. However, ferroelectricity is generally incompatible with systems featuring metallicity due to the screening effect of free carriers. In this study, we report the observation of memristive switching based on the ferroelectric surface state of a topological semimetal（TaSe4）2I. We find that the surface state of（TaSe4）2I presents out-of-plane ferroelectric polarization due to surface reconstruction. With the combination of ferroelectric surface and charge-density-wave-gapped bulk states, an electric-switchable barrier height can be achieved in（TaSe4）2I-metal contact. By employing a multi-terminal-grounding design,we manage to construct a prototype ferroelectric memristor based on（TaSe4）2I with on/off ratio up to10～3, endurance over 10～3cycles, and good retention characteristics. The origin of the ferroelectric surface state is further investigated by first-principles calculations, which reveal an interplay between ferroelectricity and band topology. The emergence of ferroelectricity in（TaSe4）2I not only demonstrates it as a rare but essential case of ferroelectric topological materials, but also opens new routes towards the implementation of topological materials in functional electronic devices.

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intelligent ion gels: Design, performance, and applications

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SmartMat 2024年第1期5卷 38-58页

作者： Naiwei Gao Caofeng Pan Beijing Key Laboratory of Micro‐nano Energy and Sensor CAS Center for Excellence in NanoscienceBeijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijingChina Key Laboratory of Optoelectronic devices and Systems of Ministry of Education Center for Stretchable Electronics and Nano SensorsCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhenChina School of Nanoscience and Engineering University of Chinese Academy of SciencesBeijingChina

intelligent ion gels,which possess highly tunable mechanical,electrical,and stimulus‐responsive properties,have emerged as powerful candidates in the field of artificial intelligence,telemedicine,and health *** enrich the functionality of ion gels,it is critical to explore the link between the structure and function of ion *** this review,we provide an overview of the synthesis path and functional derivatives of ion *** conformational relationships of ion gels have been discussed,such as the effect of structure on electrical conductivity as well as sensing *** the perspective of stimulus response,the role of ion gels in areas such as bionic haptics,neural devices,artificial muscles,and intelligent displays has also been *** is possible that smart ion gels will open up a new horizon in the upcoming smart era,especially after the current challenges are resolved.

关键词： chemical structure intelligent electronics ion gels stimulus‐responsive

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Reconfigurable memlogic long wave infrared sensing with superconductors

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Light(Science & Applications) 2024年第5期13卷 908-920页

作者： Bingxin Chen Huanyi Xue Hong Pan Liping Zhu Xiaomi Yan Jingzhe Wang Yanru Song Zhenghua An State Key Laboratory of Surface Physics and Institute for Nanoelectronic devices and Quantum Computing Department of PhysicsFudan UniversityShanghai 200438China. ShanghaiTech Quantum Device Lab ShanghaiTech UniversityShanghai 201210China. Shanghai Qi Zhi Institute 41th FloorAI TowerNo.701 Yunjin RoadXuhui DistrictShanghai 200232China. Yiwu research Institute of Fudan University Chengbei RoadYiwu City 322000 ZhejiangChina. Zhangjiang Fudan International Innovation center Fudan UniversityShanghai 201210China

Optical sensors with in-cell logic and memory capabilities offer new horizons in realizing machine vision beyond von Neumann architectures and have been attempted with two-dimensional materials,memristive oxides,phasechanging materials *** the unparalleled performance of superconductors with both quantum-limited optical sensitivities and ultra-wide spectrum coverage,here we report a superconducting memlogic long-wave infrared sensor based on the bistability in hysteretic superconductor-normal phase *** cooperatively by electrical and optical pulses,the device offers deterministic in-sensor switching between resistive and superconducting(hence dissipationless)states with persistence>105 *** results in a resilient reconfigurable memlogic system applicable for,e.g.,encrypted ***,a high infrared sensitivity at 12.2μm is achieved through its in-situ metamaterial perfect absorber *** work opens the avenue to realize all-in-one superconducting memlogic sensors,surpassing biological retina capabilities in both sensitivity and wavelength,and presents a groundbreaking opportunity to integrate visional perception capabilities into superconductor-based intelligent quantum machines.

关键词： wave superconductor quantum

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A Generic Strategy to Create Mechanically Interlocked Nanocomposite/Hydrogel Hybrid Electrodes for Epidermal Electronics

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Nano-Micro Letters 2024年第5期16卷 120-133页

作者： Qian Wang Yanyan Li Yong Lin Yuping Sun Chong Bai Haorun Guo Ting Fang Gaohua Hu Yanqing Lu Desheng Kong College of Engineering and Applied Sciences National Laboratory of Solid State Microstructureand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210023People’s Republic of China State Key Laboratory of Analytical Chemistry for Life Science and Jiangsu Key Laboratory of Artificial Functional MaterialsNanjing UniversityNanjing 210023People’s Republic of China College of Chemical Engineering and Technology Engineering Research Center of Seawater Utilization Technology of Ministry of EducationState Key Laboratory of Reliability and Intelligence of Electrical EquipmentHebei University of TechnologyTianjin 300130People’s Republic of China Key Laboratory of intelligent Optical Sensing and Manipulation Nanjing UniversityNanjing 210093People’s Republic of China

Stretchable electronics are crucial enablers for next-generation wearables intimately integrated into the human *** the primary compliant conductors used in these devices,metallic nanostructure/elastomer composites often struggle to form conformal contact with the textured *** electrodes have been consequently developed based on conductive nanocomposite and soft hydrogels to establish seamless skin-device ***,chemical modifications are typically needed for reliable bonding,which can alter their original *** overcome this limitation,this study presents a facile fabrication approach for mechanically interlocked nanocomposite/hydrogel hybrid *** this physical process,soft microfoams are thermally laminated on silver nanowire nanocomposites as a porous interface,which forms an interpenetrating network with the *** microfoam-enabled bonding strategy is generally compatible with various *** resulting interlocked hybrids have a 28-fold improved interfacial toughness compared to directly stacked *** electrodes achieve firm attachment to the skin and low contact impedance using tissue-adhesive *** have been successfully integrated into an epidermal sleeve to distinguish hand gestures by sensing mus-cle *** nanocomposite/hydrogel hybrids reported here offer a promising platform to combine the benefits of both materials for epidermal devices and systems.

关键词： Stretchable electronics Epidermal electronics Silver nanowire Conductive nanocomposites Hydrogel

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