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High-energy-density lithium manganese iron phosphate for lithium-ion batteries: Progresses, challenges, and prospects

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Journal of Energy Chemistry 2025年第1期100卷 1-17页

作者： Bokun Zhang Xiaoyun Wang Shuai Wang Yan Li Libo Chen Handong Jiao Zhijing Yu Jiguo Tu State Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing Research institute for Intelligent Wearable Systems The Hong Kong Polytechnic University institute of Advanced Structure Technology Beijing Institute of Technology

The soaring demand for smart portable electronics and electric vehicles is propelling the advancements in high-energy–density lithium-ion *** manganese iron phosphate (LiMnxFe1-xPO4) has garnered significant attention as a promising positive electrode material for lithium-ion batteries due to its advantages of low cost,high safety,long cycle life,high voltage,good high-temperature performance,and high energy *** LiMnxFe1-xPO4has made significant breakthroughs in the past few decades,there are still facing great challenges in poor electronic conductivity and Li-ion diffusion,manganese dissolution affecting battery cycling performance,as well as low tap *** review systematically summarizes the reaction mechanisms,various synthesis methods,and electrochemical properties of LiMnxFe1-xPO4to analyze reaction processes accurately and guide material ***,the main challenges currently faced are concluded,and the corresponding various modification strategies are discussed to enhance the reaction kinetics and electrochemical performance of LiMnxFe1-xPO4,including multi-scale particle regulation,heteroatom doping,surface coating,as well as microscopic morphology ***,in view of the current research challenges faced by intrinsic reaction processes,kinetics,and energy storage applications,the promising research directions are *** importantly,it is expected to provide key insights into the development of high-performance and stable LiMnxFe1-xPO4materials,to achieve practical energy storage requirements.

关键词： Lithium manganese iron phosphate High energy density Lithium-ion batteries Reaction mechanism Tap density

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Comments on “Prediction on CO_(2) uptake of recycled aggregate concrete”, Frontiers of Structural and Civil Engineering, 14, 746−759 (2020)

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Frontiers of Structural and Civil Engineering 2021年第6期15卷 1504-1506页

作者： Rui NEVES Barreiro Technology School Polytechnic Institute of SetúbalBarreiro 2910761Portugal

A methodology to compute the CO_(2) uptake of recycled aggregate concrete is proposed in the commented *** some typos in several formulas,it is found that the approach to estimate the specific surface area of the recycled aggregates is not *** issue has some impact in the conclusions of the commented ***,aiming to improve the understanding,accuracy and findings of the commented paper,an alternative approach to estimate the specific surface area of the recycled aggregates,as well as an erratum of the formulas and revised conclusions are suggested.

关键词： concrete aggregate revised

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Spherical f-Tilings by Two Noncongruent Classes of Isosceles Triangles-Ⅱ

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Acta Mathematica Sinica,English Series 2014年第8期30卷 1435-1464页

作者： Ana BREDA Robert DAWSON Patrícia RIBEIRO Department of Mathematics University of Aveiro Department of Mathematics and Computing Science Saint Mary’s University Halifax Department of Mathematics EST SetbalPolytechnic Institute of Setbal

In this work,we give a complete classification of spherical dihedral f-tilings when the prototiles are two noncongruent isosceles triangles with certain adjacency *** it will be shown,this class is composed by two dis... 详细信息

关键词： Spherical tilings dihedral triangulations f-tilings spherical trigonometry

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Catalyst–Support Interaction in Polyaniline‑Supported Ni_(3)Fe Oxide to Boost Oxygen Evolution Activities for Rechargeable Zn‑Air Batteries

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Nano-Micro Letters 2025年第1期17卷 176-190页

作者： Xiaohong Zou Qian Lu Mingcong Tang Jie Wu Kouer Zhang Wenzhi Li Yunxia Hu Xiaomin Xu Xiao Zhang Zongping Shao Liang An Department of Mechanical Engineering The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and TechnologyNanjing University of Information Science and TechnologyNanjing 210044People’s Republic of China Department of Chemistry The Chinese University of Hong KongMa Lin BuildingShatinHong Kong SAR 999077People’s Republic of China WA School of Mines:Minerals Energy and Chemical Engineering(WASM‑MECE)Curtin UniversityPerthWA 6102Australia Research institute for Advanced Manufacturing The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Research institute for Smart Energy The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China

Catalyst–support interaction plays a crucial role in improving the catalytic activity of oxygen evolution reaction(OER).Here we modulate the catalyst–support interaction in polyaniline-supported Ni_(3)Fe oxide(Ni_(3)Fe oxide/PANI)with a robust hetero-interface,which significantly improves oxygen evolution activities with an overpotential of 270 mV at 10 mA cm^(-2)and specific activity of 2.08 mA cm_(ECSA)^(-2)at overpotential of 300 mV,3.84-fold that of Ni_(3)Fe *** is revealed that the catalyst–support interaction between Ni_(3)Fe oxide and PANI support enhances the Ni–O covalency via the interfacial Ni–N bond,thus promoting the charge and mass transfer on Ni_(3)Fe *** the excellent activity and stability,rechargeable Zn-air batteries with optimum Ni_(3)Fe oxide/PANI are assembled,delivering a low charge voltage of 1.95 V to cycle for 400 h at 10 mA cm^(-2).The regulation of the effect of catalyst–support interaction on catalytic activity provides new possibilities for the future design of highly efficient OER catalysts.

关键词： Catalyst-support interaction Supported catalysts Heterointerface Oxygen evolution reaction Zn-air batteries

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MULTISCALE ISSUES IN DNS OF MULTIPHASE FLOWS

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Acta Mathematica Scientia 2010年第2期30卷 551-562页

作者： G.Tryggvason S.Thomas B.Aboulhasanzadeh Worcester polytechnic institute

Direct numerical simulations （DNS） have now become a well established tool to examine complex multiphase flows. Such flows typically exhibit a large range of scales and it is generally necessary to use different descriptions of the flow depending on the scale that we are examining. Here we discuss multiphase flows from a multiscale perspective. Those include both how DNS are providing insight and understanding for modeling of scales much larger than the ＂dominant scale＂（defined where surface tension, viscous forces or inertia are important）, as well as how DNS are often limited by the need to resolve processes taking place on much smaller scales. Both problems can be cast into a language introduced for general classes of multiscale problems and reveal that while the classification may be new, the issues are not.

关键词： direct numerical simulations multiphase flow multiscale problems

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PARALLEL ADAPTIVE SIMULATION OF A PLUNGING LIQUID JET

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Acta Mathematica Scientia 2010年第2期30卷 522-538页

作者： Azat Yu.Galimov Onkar Sahni Richard T.Lahey Jr. Mark S.Shephard Donald A.Drew Kenneth E.Jansen Rensselaer polytechnic institute

This paper is concerned with three-dimensional numerical simulation of a plunging liquid jet. The transient processes of forming an air cavity around the jet, capturing an initially large air bubble, and the break-up of this large toroidal-shaped bubble into smaller bubbles were analyzed. A stabilized finite element method （FEM） was employed under parallel numerical simulations based on adaptive, unstructured grid and coupled with a level-set method to track the interface between air and liquid. These simulations show that the inertia of the liquid jet initially depresses the pool＇s surface, forming an annular air cavity which surrounds the liquid jet. A toroidal liquid eddy which is subse- quently formed in the liquid pool results in air cavity collapse, and in turn entrains air into the liquid pool from the unstable annular air gap region around the liquid jet.

关键词： plunging liquid jet air entrainment two-phase flows level set method parallel adaptive simulation

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The kinesin-like proteins, KAC1/2, regulate actin dynamics underlying chloroplast light-avoidance in Physcomitrella patens

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Journal of Integrative Plant Biology 2015年第1期57卷 106-119页

作者： Zhiyuan Shen Yen-Chen Liu Jeffrey P.Bibeau Kyle P.Lemoi Erkan Tüzel Luis Vidali Department of Biology and Biotechnology Worcester Polytechnic Institute Department of Physics Worcester Polytechnic Institute

In plants, light determines chloroplast position; these organelles show avoidance and accumulation re- sponses in high and low fluence-rate light, respectively. Chloroplast motility in response to light is driven by cytoskeletal elements. The actin cytoskeleton mediates chloroplast photorelocation responses in Arabidopsis thali- ana. In contrast, in the moss Physcomitrella patens, both, actin filaments and microtubules can transport chloroplasts. Because of the surprising evidence that two kinesin-like proteins （called KACs） are important for actin-dependent chloroplast photorelocation in vascular plants, we wanted to determine the cytoskeletal system responsible for the function of these proteins in moss. We performed gene- specific silencing using RNA interference in P. patens. We confirmed existing reports using gene knockouts, that PpKAC1 and PpKAC2 are required for chloroplast dispersion under uniform white light conditions, and that the two proteins are functionally equivalent. To address the specificcytoskeletal elements responsible for motility, this loss-of- function approach was combined with cytoskeleton-targeted drug studies. We found that, in P. patens, these KACs mediate the chloroplast light-avoidance response in an actin filament- dependent, rather than a microtubule-dependent manner. Using correlation-decay analysis of cytoskeletal dynamics, we found that PpKAC stabilizes cortical actin filaments, but has no effect on microtubule dynamics.

关键词： Actin filaments cytoskeleton intracellular transport kinesin-14 light-avoidance response microtubule moss RNAi

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Schedule optimization to improve trunk-local bus transfer efficiency in small conurbations: A case study of New York's capital region

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Journal of Central South University 2016年第7期23卷 1817-1822页

作者：张大鹏王晓坤 Department of Civil Engineering Rensselaer Polytechnic Institute

Fostering the use of transit has been broadly accepted as an effective way to improve social equity and reduce the externalities caused by transportation. In the great body of transit literature, many have focused on the improvement of transfer efficiency. However, investigation on transit transfer efficiency is still lacking for medium sized cities or suburban areas that have sprawled from city centers. The special features associated with such an urban form lead to unique travel patterns and bus operations. This work develops a process to improve bus transfer efficiency for small conurbations considering their special characteristics. A case study of New York's Capital District is used to illustrate the proposed method. Results show that the transfer waiting time can be remarkably shortened. The proposed method can be widely adapted to other transit systems in small conurbations.

关键词： transfer efficiency small conurbation rural transit

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Effect of scanning speeds on electrochemical corrosion resistance of laser cladding TC4 alloy

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Chinese Physics B 2019年第2期28卷 383-390页

作者： Xiaotian Feng Jianbo Lei Hong Gu Shengfeng Zhou Laser Technology institute Tianjin Polytechnic University

In order to study the effect of scanning speed on the electrochemical corrosion resistance of laser cladding TC4 alloy in artificial seawater, the x-ray diffraction analysis, microstructure of cross-section, microhardness variation, and impedance spectrum have been studied in comparison with the TC4 titanium alloy. The results show that the main phase of cladding coating is α-Ti, and the change of scanning speed has no obvious effect on it; therefore, the supersaturated α-Ti solid solution is formed, and the acicular α martensite is obtained. As the scanning speed increases, the microstructure of cladding coating is orthogonal basket-weave, the crystal surface spacing decreases, and the average microhardness of laser cladding TC4 alloy slightly increases. When the scanning speed increases to 10 mm/s, the microhardness is about 14.71%higher than that of the substrate, and the electrochemical corrosion resistance of laser cladding TC4 alloy is also improved,which is about 2.48 times more than the substrate. Grain refinement has a great effect on enhancing the anti-electrochemical corrosion.

关键词： laser cladding TC4 alloy grain refinement electrochemical corrosion

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Variational solutions for Hermite-Gaussian solitons in nonlocal nonlinear media

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Chinese Physics B 2009年第7期18卷 2853-2857页

作者：白东峰黄长春贺军峰王毅 Department of Mechanical Engineering Henan Polytechnic Institute

The physical features exhibited by Hermite-Gaussian （HC） beams propagating in nonlocal nonlinear media with Gaussian-shaped response are discussed with an approximate variational *** direct numerical simulations,we find that the beam properties in the normalized system are different with the change of the degree of *** is shown that initial HG profiles break up into several individual beams with propagation when the degree of nonlocality α is *** beams can propagate stably when a is large enough.

关键词： nonlocal nonlinear media variational approach Hermite-Gaussian solitons

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