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B-N covalent bond-involved π-extension of multiple resonance emitters enables high-performance narrowband electroluminescence

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National science Review 2024年第06期11卷 243-253页

作者： Xingyu Huang Jiahui Liu Yulin Xu Guohao Chen Manli Huang Mingxin Yu Xialei Lv Xiaojun Yin Yang Zou Jingsheng Miao Xiaosong Cao Chuluo Yang Shenzhen Key Laboratory of New information Display and Storage Materials College of Materials Science and EngineeringShenzhen University college of physics and Optoelectronic engineering Shenzhen University

Multi-boron-embedded multiple resonance thermally activated delayed fluorescence（MR-TADF） emitters show promise for achieving both high color-purity emission and high exciton utilization ***, their development is often impeded by a limited synthetic scope and excessive molecular weights,which challenge material acquisition and organic light-emitting diode（OLED） fabrication by vacuum deposition. Herein, we put forward a B–N covalent bond-involved π-extension strategy via post-functionalization of MR frameworks, leading to the generation of high-order B/N-based motifs. The structurally and electronically extended π-system not only enhances molecular rigidity to narrow emission linewidth but also promotes reverse intersystem crossing to mitigate efficiency roll-off. As illustrated examples, ultra-narrowband sky-blue emitters（full-width at half-maximum as small as 8 nm in n-hexane）have been developed with multi-dimensional improvement in photophysical properties compared to their precursor emitters, which enables narrowband OLEDs with external quantum efficiencies(EQEmax) of up to 42.6%, in company with alleviated efficiency decline at high brightness, representing the best efficiency reported for single-host OLEDs. The success of these emitters highlights the effectiveness of our molecular design strategy for advanced MR-TADF emitters and confirms their extensive potential in high-performance optoelectronic devices.

关键词： narrowband electroluminescence thermally activated delayed fluorescence (TADF) multiple resonance emitters ultra-high external quantum efficiency

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Tunable hexagonal boron nitride topological optical delay line in the visible region

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Chinese Optics Letters 2024年第5期22卷 124-130页

作者：费宏明武敏林瀚杨毅彪肖连团 college of physics Taiyuan University of TechnologyTaiyuan 030024China college of information engineering Shanxi Vocational University of Engineering Science and TechnologyJinzhong 030619China college of science RMIT UniversityMelbourneVictoria 3000Australia college of Electronic information and Optical engineering Taiyuan University of TechnologyTaiyuan 030024China

Tunability,ultracompact design,high group index,low loss,and broad bandwidth are desired properties for integrated optical delay lines(ODLs).However,those properties are challenging to achieve simultaneously in the visible *** paper proposes a tunable hexagonal boron nitride topological optical delay line(ODL)in the visible region based on valley photonic *** topological edge state from the beard-type boundary allows the achievement of an ultralow group velocity close to zero,which results in a large group index of 629 at 645 ***,we demonstrate tuning of the slow-light wavelength and optical delay times with electrically tunable liquid crystals by applying external *** device has an ultracompact size of 5μm×2.7μm with an optical delay distance of 25a(a is the lattice constant)and a delay time of 12 *** design can provide a new possibility for designing ODLs working in the visible region for optical communication and quantum computing systems.

关键词： valley photonic crystal topological edge states optical delay lines

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Two simple memristive maps with adaptive energy regulation and digital signal process verification

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Journal of Zhejiang University-science A(Applied physics & engineering) 2024年第5期25卷 382-394页

作者： Feifei YANG Lujie REN Jun MA Zhigang ZHU college of Electrical and information engineering Lanzhou University of TechnologyLanzhou 730050China department of physics Lanzhou University of TechnologyLanzhou 730050China School of information science and engineering Dalian Polytechnic UniversityDalian 116034China

Mathematical models can produce desired dynamics and statistical properties with the insertion of suitable nonlinear terms,while energy characteristics are crucial for practical application because any hardware realizations of nonlinear systems are relative to energy *** involvement of memristive terms relative to memristors enables multistability and initial-dependent property in memristive *** this study,two kinds of memristors are used to couple a capacitor or an inductor,along with a nonlinear resistor,to build different neural *** corresponding circuit equations are derived to develop two different types of memristive oscillators,which are further converted into two kinds of memristive maps after linear *** Hamilton energy function for memristive oscillators is obtained by applying the Helmholz theorem or by mapping from the field energy of the memristive *** Hamilton energy functions for both memristive maps are obtained by replacing the gains and discrete variables for the memristive oscillator with the corresponding parameters and *** two memristive maps have rich dynamic behaviors including coherence resonance under noisy excitation,and an adaptive growth law for parameters is presented to express the self-adaptive property of the memristive maps.A digital signal process(DSP)platform is used to verify these *** scheme will provide a theoretical basis and experimental guidance for oscillator-to-map transformation and discrete map-energy calculation.

关键词： Hamilton energy Discrete memristor Self-adaptive regulation Digital signal process(DSP)implementation

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Fe3O4/Fe/FeS Tri-Heterojunction Node Spawning N-Carbon Nanotube Scaffold Structure for High-Performance Sodium-Ion Battery

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Energy & Environmental Materials 2024年第4期7卷 143-152页

作者： Yuan Liu Qing Lin Xiaocui Chen Xufeng Meng Baoxiu Hou Haiyan Liu Shuaihua Zhang Ningzhao Shang Zheng Wang Chaoyue Zhang Jianjun Song Xiaoxian Zhao department of Chemistry College of Science Hebei Agricultural University college of Chemistry and Chemical engineering Qingdao University college of physics Qingdao University

The Fe-based anode of sodium-ion batteries attracts much attention due to the abundant source,low-cost,and high specific ***,the low electron and ion transfer rate,poor structural stability,and shuttle effect of NaS2intermediate restrain its further ***,the Fe3O4/Fe/FeS tri-heterojunction node spawned N-carbon nanotube scaffold structure（FHNCS） was designed using the modified MIL-88B（Fe） as a template followed by catalytic growth and sulfidation process.

关键词： anode core-shell heterojunction hollow structure sodium ion batteries

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Thermogalvanic hydrogel-based e-skin for self-powered on-body dual-modal temperature and strain sensing

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Microsystems & Nanoengineering 2024年第2期10卷 293-302页

作者： Zhaosu Wang Ning Li Xinru Yang Zhiyi Zhang Hulin Zhang Xiaojing Cui college of Electronic information and Optical engineering Taiyuan University of TechnologyTaiyuan030024China college of Materials science and engineering Taiyuan University of TechnologyTaiyuan030024China School of physics and information engineering Shanxi Normal UniversityTaiyuan030031China

Sensing of both temperature and strain is crucial for various diagnostic and therapeutic ***,we present a novel hydrogel-based electronic skin(e-skin)capable of dual-mode sensing of temperature and *** thermocouple ion selected for this study is the iodine/triiodide(I−/I3−)redox couple,which is a common component in everyday *** leveraging the thermoelectric conversion in conjunction with the inherent piezoresistive effect of a gel electrolyte,self-powered sensing is achieved by utilizing the temperature difference between the human body and the external *** composite hydrogels synthesized from polyvinyl alcohol(PVA)monomers using a simple freeze‒thaw method exhibit remarkable flexibility,extensibility,and adaptability to human *** incorporation of zwitterions further augments the resistance of the hydrogel to dehydration and low temperatures,allowing maintenance of more than 90%of its weight after 48 h in the *** its robust thermal current response,the hydrogel was encapsulated and then integrated onto various areas of the human body,including the cheeks,fingers,and ***,the detection of the head-down state and the monitoring of foot movements demonstrate the promising application of the hydrogel in supervising the neck posture of sedentary office workers and the activity *** successful demonstration of self-powered on-body temperature and strain sensing opens up new possibilities for wearable intelligent electronics and robotics.

关键词： hydrogel modal utilizing

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Optimizing electronic structure of Mo_(2)TiC_(2)T_(x) MXene through Nb doping for enhanced electrochemical performance

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Nano Research 2024年第8期17卷 7174-7181页

作者： Jingyuan Zhao Wenzheng Yan Zhaoxi Liu Xiaobin Liu Yapeng Tian Xinwei Cui Henan Institute of Advanced Technology College of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450003China college of physics and Electronic information engineering Guilin University of TechnologyGuilin 514004China

MXene is a promising electrode material for both high volumetric capacitance and high-rate performance in ***,the current study has mainly focused on the monometallic element Ti_(3)C_(2)T_(x) MXene until now,while the bimetallic and multimetallic MXene have received comparatively less *** this work,we demonstrate that the electronic structure of the Mo_(2)TiC_(2)T_(x) MXene could be regulated by fine-tuning the content of doped Nb *** enhanced electron cloud density of surface–O termination and the electron spin of the Mo atoms in the Mo_(2)TiC_(2)T_(x) MXene,leads to the boost of electric double-layer capacitor(EDLC)and improvement of *** a consequence,the electrochemical performance of Nb-doped Mo_(2)TiC_(2)T_(x) MXene(Nb-0.3-MXene)demonstrates a capacitance of 398 F·cm^(−3),roughly doubling that of the pristine Mo_(2)TiC_(2)T_(x) MXene electrode at 197 F·cm^(−3) in the 3 M H_(2)SO_(4) *** the same time,the Nb-0.3-MXene could even maintain a capacitance of 82.75% at 200 mV·s−1,with high cyclic stability for 19,000 cycles at 10 A·g−***,Nb-0.3-MXene-based hybrid supercapacitors deliver a remarkable volumetric energy density of 48.1 W·h·L^(−1)at 230.7 W·L^(−1),and 34.4 W·h·L^(−1)at a high power density of 82.6 kW·L^(−1).There exists a balance between the volumetric capacitance and rate performance with different ratios of Nb atoms in the Nb-doped MXene due to the strong interaction between the Nb-doped MXene and the intercalated ***,optimizing the electronic structure of MXene through heteroatom doping is of great potential for enhanced supercapacitor performance.

关键词： niobium doping electronic structure Mo_(2)TiC_(2)T_(x)MXene electron spin rate performance volumetric capacitance

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WebFLex:A Framework for Web Browsers-Based Peer-to-Peer Federated Learning Systems Using WebRTC

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Computers, Materials & Continua 2024年第3期78卷 4177-4204页

作者： Mai Alzamel Hamza Ali Rizvi Najwa Altwaijry Isra Al-Turaiki department of Computer science College of Computer and Information SciencesKing Saud UniversityRiyadhKingdom of Saudi Arabia department of Computer science and engineering Punjab Engineering CollegeChandigarhIndia

Scalability and information personal privacy are vital for training and deploying large-scale deep learning *** learning trains models on exclusive information by aggregating weights from various devices and taking advantage of the device-agnostic environment of web ***,relying on a main central server for internet browser-based federated systems can prohibit scalability and interfere with the training process as a result of growing client ***,information relating to the training dataset can possibly be extracted from the distributed weights,potentially reducing the privacy of the local data used for *** this research paper,we aim to investigate the challenges of scalability and data privacy to increase the efficiency of distributed training *** a result,we propose a web-federated learning exchange(WebFLex)framework,which intends to improve the decentralization of the federated learning *** is additionally developed to secure distributed and scalable federated learning systems that operate in web browsers across heterogeneous ***,WebFLex utilizes peer-to-peer interactions and secure weight exchanges utilizing browser-to-browser web real-time communication(WebRTC),efficiently preventing the need for a main central *** has actually been measured in various setups using the MNIST *** results show WebFLex’s ability to improve the scalability of federated learning systems,allowing a smooth increase in the number of participating devices without central data *** addition,WebFLex can maintain a durable federated learning procedure even when faced with device disconnections and network ***,it improves data privacy by utilizing artificial noise,which accomplishes an appropriate balance between accuracy and privacy preservation.

关键词： Federated learning web browser privacy deep learning

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Quantum circuit-based proxy blind signatures:A novel approach and experimental evaluation on the IBM quantum cloud platform

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Chinese physics B 2024年第5期33卷 247-253页

作者：娄小平昝慧茹徐雪娇 college of information science and engineering Hunan Normal UniversityChangsha 410081China

This paper presents a novel approach to proxy blind signatures in the realm of quantum circuits,aiming to enhance security while safeguarding sensitive *** main objective of this research is to introduce a quantum proxy blind signature(QPBS)protocol that utilizes quantum logical gates and quantum measurement *** QPBS protocol is constructed by the initial phase,proximal blinding message phase,remote authorization and signature phase,remote validation,and de-blinding *** innovative design ensures a secure mechanism for signing documents without revealing the content to the proxy signer,providing practical security authentication in a quantum environment under the assumption that the CNOT gates are securely *** existing approaches,our proposed QPBS protocol eliminates the need for quantum entanglement preparation,thus simplifying the implementation *** assess the effectiveness and robustness of the QPBS protocol,we conduct comprehensive simulation studies in both ideal and noisy quantum environments on the IBM quantum cloud *** results demonstrate the superior performance of the QPBS algorithm,highlighting its resilience against repudiation and forgeability,which are key security concerns in the realm of proxy blind ***,we have established authentic security thresholds(82.102%)in the presence of real noise,thereby emphasizing the practicality of our proposed solution.

关键词： proxy blind signature quantum circuits quantum computation IBM quantum cloud platform

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Ground state of Rydberg-dressed Bose gas confined in a toroidal trap

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Communications in Theoretical physics 2024年第1期76卷 29-35页

作者： Lin-Xue Wang Hong-Li Yang Hui Liu Si-Lin Chen Ya-Jun Wang Xiao-Fei Zhang department of physics School of Physics and Information ScienceShaanxi University of Science and TechnologyXi'an 710021China department of Basic sciences Air Force Engineering UniversityXi'an 710051China

The experimental realization of Rydberg dressing technology in ultracold atomic systems provides another superior platform for studying novel states of matter and macroscopic quantum *** this work,based on the mean-field theory,we have investigated the ground-state phases of a two-component Bose–Einstein condensate with Rydberg interaction and confined in a toroidal *** effects of the Rydberg interaction and external potential,especially the Rydberg blockade radius,on the ground-state structure of such a system have been investigated in full parameter *** results show that the Rydberg blockade radius,which can be regarded as another controllable parameter,can be used to obtain a variety of ground-state *** interestingly,it is found that for weak Rydberg interactions,the Rydberg blockade radius breaks the spontaneous rotational symmetry of the system,leading to the formation of a discrete unit cell *** strongly interacting cases,it can be used to realize different orders of discrete rotational symmetry breaking.

关键词： Bose-Einstein condensate Rydberg dressing toroidal trap

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Deep learning-assisted common temperature measurement based on visible light imaging

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Chinese physics B 2024年第8期33卷 230-236页

作者：朱佳仪何志民黄成曾峻林惠川陈福昌余超群李燕张永涛陈焕庭蒲继雄 college of physics and information engineering Minnan Normal UniversityZhangzhou 363000China Fujian Provincial Key Laboratory of Light Propagation and Transformation College of Information Science&EngineeringHuaqiao UniversityXiamen 361021China

Real-time,contact-free temperature monitoring of low to medium range(30℃-150℃)has been extensively used in industry and agriculture,which is usually realized by costly infrared temperature detection *** paper proposes an alternative approach of extracting temperature information in real time from the visible light images of the monitoring target using a convolutional neural network(CNN).A mean-square error ofinformation from the images which were collected under different illuminance and were not used for *** to the conventional machine learning algorithms mentioned in the recent literatures,this real-time,contact-free temperature measurement approach that does not require any further image processing operations facilitates temperature monitoring applications in the industrial and civil fields.

关键词： convolutional neural network visible light image temperature measurement low-to-medium-range temperatures

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