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Nanofluidic memristor based on the elastic deformation of nanopores with nanoparticle adsorption

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National Science Review 2024年第4期11卷 46-54页

作者： Xi Zhou Yuanyuan Zong Yongchang Wang Miao Sun Deli Shi Wei Wang Guanghua Du Yanbo Xie department of Chemistry and Chemical Engineering Northwestern Polytechnical University School of physical Science and Technology Northwestern Polytechnical University School of Aeronautics and Institute of Extreme Mechanics Northwestern Polytechnical University Institute of Modern Physics Chinese Academy of Sciences

The memristor is the building block of neuromorphic computing. We report a new type of nanofluidic memristor based on the principle of elastic strain on polymer nanopores. With nanoparticles absorbed at the wall of a single conical polymer nanopore, we find a pinched hysteresis of the current within a scanning frequency range of 0.01–0.1 Hz, switching to a diode below 0.01 Hz and a resistor above 0.1 Hz. We attribute the current hysteresis to the elastic strain at the tip side of the nanopore, caused by electrical force on the particles adsorbed at the inner wall surface. Our simulation and analytical equations match well with experimental results, with a phase diagram for predicting the system transitions. We demonstrate the plasticity of our nanofluidic memristor to be similar to a biological synapse. Our findings pave a new way for ionic neuromorphic computing using nanofluidic memristors.

关键词： nanofluidics memristor neurocomputing elastic deformation

A critical review on solid-state welding of high entropy alloys-processing,microstructural characteristics and mechanical properties of joints

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Defence Technology（防务技术） 2024年第4期34卷 78-133页

作者： Tushar Sonar Mikhail Ivanov Evgeny Trofimov Aleksandr Tingaev Ilsiya Suleymanova department of Welding Engineering Institution of Engineering and TechnologySouth Ural State University(National Research University)Chelyabinsk454080Russia department of Materials Science Physical and Chemical Properties of MaterialsInstitution of Engineering and TechnologySouth Ural State University(National Research University)Chelyabinsk454080Russia

The high entropy alloys(HEAs)are the newly developed high-performance materials that have gained significant importance in defence,nuclear and aerospace sector due to their superior mechanical properties,heat resistance,high temperature strength and corrosion *** alloys are manufactured by the equal mixing or larger proportions of five or more alloying *** exhibit superior mechanical performance compared to traditional engineering alloys because of the extensive alloying composition and higher entropy of *** state welding(SSW)techniques such as friction stir welding(FSW),rotary friction welding(RFW),diffusion bonding(DB)and explosive welding(EW)have been efficiently deployed for improving the microstructural integrity and mechanical properties of welded HEA *** HEA interlayers revealed greater potential in supressing the formation of deleterious intermetallic phases and maximizing the mechanical properties of HEAs *** similar and dissimilar joining of HEAs has been manifested to be viable for HEA systems which further expands their industrial ***,the main objective of this review paper is to present a critical review of current state of research,challenges and opportunities and main directions in SSW of HEAs mainly CoCrFeNiMn and Al_xCoCrFeNi *** state of the art of problems,progress and future outlook in SSW of HEAs are critically reviewed by considering the formation of phases,microstructural evolution and mechanical properties of HEAs joints.

关键词： High entropy alloys Solid state welding Microstructure Mechanical properties

Elastic wave insulation and propagation control based on the programmable curved-beam periodic structure

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Applied Mathematics and Mechanics(English Edition) 2024年第10期45卷 1791-1806页

作者： Jiajia MAO Hong CHENG Tianxue MA Beijing Key Laboratory of Nonlinear Vibrations and Strength of Mechanical Structures Department of MechanicsSchool of MathematicsStatistics and MechanicsBeijing University of TechnologyBeijing 100124China department of Mechanics School of Physical Science and EngineeringBeijing Jiaotong UniversityBeijing 100044China

Curved-beams can be used to design modular multistable metamaterials(MMMs)with reprogrammable material properties,i.e.,programmable curved-beam periodic structure(PCBPS),which is promising for controlling the elastic wave *** PCBPS is theoretically equivalent to a spring-oscillator system to investigate the mechanism of bandgap,analyze the wave propagation mechanisms,and further form its geometrical and physical criteria for tuning the elastic wave *** the equivalent model,we calculate the analytical solutions of the dispersion relations to demonstrate its adjustability,and investigate the wave propagation characteristics through the *** validate the equivalent system,the finite element method(FEM)is *** is revealed that the bandgaps of the PCBPS can be turned on-and-off and shifted by varying its physical and geometrical *** findings are highly promising for advancing the practical application of periodic structures in wave insulation and propagation control.

关键词： curved-beam based periodic structure equivalent stiffness spring-oscillator system dispersion relation wave propagation

Anchoring heterometallic cluster on P-doped carbon nitride for efficient photocatalytic nitrogen fixation in water and air ambient

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Chinese Chemical Letters 2024年第4期35卷 176-180页

作者： Chao-Long Chen Rong Chen La-Sheng Long Lan-Sun Zheng Xiang-Jian Kong Collaborative Innovation Center of Chemistry for Energy Materials State Key Laboratory of Physical Chemistry of Solid Surfaces and Department of ChemistryCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China

Light-driven nitrogen fixation to produce ammonia is a green and economical technology of nitrogen reduction but is still quite challenging, especially in an air atmosphere without any sacrificial ***, we demonstrate efficient photocatalytic nitrogen fixation using water and air directly by loading lanthanide–transition metal(4f–3d) cluster NdCo_(3) on two-dimensional P-doped graphitic carbon nitrides(PCN) material surface. Benefiting from the increase in the number of nitrogen vacancies(NVs) and highly matched band gap structure and excellent hole trapping ability of clusters, the NdCo_(3)/PCN photocatalyst exhibits efficient nitrogen reduction activity with 371(in air) and 825 μmol h^(-1)g^(-1)(in pure nitrogen)without any sacrificial reagents. The introduction of potassium sulfate inhibits hydrogen production and promotes nitrogen reduction activation. This work suggests that anchoring precisely structured clusters on 2D materials may enhance photocatalytic nitrogen reduction under normal temperature and pressure.

关键词： Photocatalytic Nitrogen fixation 4f-3d Cluster Air atmosphere

Using satellite-derived land surface temperatures to clarify the spatiotemporal warming trends of the Alborz Mountains in northern Iran

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Journal of Mountain Science 2024年第2期21卷 449-469页

作者： ROSHAN Gholamreza SARLI Reza GHANGHERMEH Abdolazim TAHERIZADEH Mehrnoosh NIKNAM Arman department of Geography Golestan UniversityGorgan 49138-15759Iran department of Forest Resources Management Faculty of ForestryUniversity of Agriculture in KrakowAL.29 Listopada 4631-425 KrakówPoland department of Geoinformatics Physical and Environmental GeographyUniversity of SzegedSzeged 6722Hungary

The Alborz Mountains are some of the highest in Iran,and they play an important role in controlling the climate of the country’s northern *** land surface temperature(LST)is an important variable that affects the ecosystem of this *** study investigated the spatiotemporal changes and trends of the nighttime LST in the western region of the Central Alborz Mountains at elevations of 1500-4000 m above sea *** data were extracted for the period of 2000-2021,and the Mann-Kendall nonparametric test was applied to evaluating the changes in the *** results indicated a significant increasing trend for the monthly average LST in May-August along the southern *** the northern and southern aspects showed decreasing trends for the monthly average LST in October,November,and March and an increasing trend in other *** all elevations,the average decadal change in the monthly average LST was more severe along the southern aspect(0.60°C)than along the northern aspect(0.37°C).The LST difference between the northern and southern aspects decreased in the cold months but increased in the hot *** the same elevation,the difference in the lapse rate between the northern and southern aspects was greater in the hot months than in the cold *** increasing elevation,the lapse rate between the northern and southern aspects *** change was concluded to greatly decrease the difference in LST at different elevations for April-July.

关键词： Global warming Mountainous areas Lapse rate Surface air temperatures Alborz

Active and passive modulation of solar light transmittance in a uniquely multifunctional dual-band single molecule for smart window applications

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Journal of Energy Chemistry 2024年第1期88卷 293-305,I0007页

作者： Pooja V.Chavan Pramod V.Rathod Joohyung Lee Sergei V.Kostjuk Hern Kim department of Energy Science and Technology Environmental Waste Recycle InstituteMyongji UniversityYonginGyeonggi-do 17058Republic of Korea department of Chemical Engineering Myongji UniversityYonginGyeonggi-do 17058Republic of Korea Research Institute for physical Chemical Problems of the Belarusian State University MinskBelarus

Functional materials may change color by heat and electricity separately or simultaneously in smart *** materials have not only demonstrated remarkable potential in the modulation of solar radiation but are also leading to the development of indoor environments that are more comfortable and conducive to improving individuals'quality of ***,dual-responsive materials have not received ample research attention due to economic and technological *** a consequence,the broader utilization of smart windows faces *** address this new generational multistimulus responsive chromic materials,our group has adopted a developmental strategy to create a poly(NIPAM)n-HV as a switchable material by anchoring active viologen(HV)onto a phase-changing poly(NIPAM)n-based smart material for better utility and *** constructed smart windows facilitate individualistic reversible switching,from a highly transparent state to an opaque state(thermochromic)and a red state(electrochromic),as well as facilitate a simultaneous dual-stimuli response reversible switching from a clear transparent state to a fully opaque(thermochromic)and orange(electrochromic)*** privacy can be attained in smart windows designed for exclusive settings by achieving zero *** unique chromic mode operates independently and modulates visible and near-infrared(NIR)light in a distinct ***,these smart windows with thermal and electric dual-stimuli responsiveness demonstrate remarkable heat regulation capabilities,rendering them highly attractive for applications in building facades,energy harvesting,privacy protection,and color display.

关键词： Smart windows Thermochromism Electrochromism Energy saving Dual-responsive material

Current progress in glass-based nanochannels

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International Journal of Smart and Nano Materials 2024年第1期15卷 222-237页

作者： Yixin Ling Xuelian Yang Lei Zhou Zhenkang Lei Yaqi Hou Xu Hou state Key Laboratory of physical Chemistry of Solid Surfaces and Department of ChemistryCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamenChina Institute of Flexible Electronics(IFE Future Technologies)Xiamen UniversityXiamenChina Institute of Artificial Intelligence Xiamen UniversityXiamenChina department of Physics Research Institute for Biomimetics and Soft MatterFujian Provincial Key Laboratory for Soft Materials ResearchJiujiang Research InstituteCollege of Physical Science and TechnologyXiamen UniversityXiamenChina

Glass-based nanochannels have become powerful tools for chemi-cal and biological sensing due to their advantages of easy prepara-tion,flexible modification,and high ***,research on ion transport behaviors in glass-based nanochannels and their applications in nanofluidic iontronics has gradually become a focus,including various ion transport behaviors such as resistive-pulse,ion rectification,ionic current memory,*** this review,we summarize the progress of manufacturing methods for glass-based nanochannels and discuss several typical ion transport behaviors of glass-based nanochannels,as well as the main application scenarios of glass-based nanochannels in terms of biosensing,detection,and neuromorphic *** enormous assistance of artificial intel-ligence in the standardized manufacturing process of glass-based nanochannels was anticipated,and the potential development of glass-based nanochannels in achieving neuromorphic functions was expected.

关键词： Glass-based nanochannels biosensing ionic rectification ionic memristive effect nanofluidic neuromorphic functions

Structure,electronic,and nonlinear optical properties of superalkaline M_(3)O(M=Li,Na)doped cyclo[18]carbon

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Chinese Physics B 2024年第2期33卷 311-317页

作者：刘晓东卢其亮罗其全 School of Physics and Material Science Anhui UniversityHefei 230601China Institute of physical Science and Information Technology Anhui UniversityHefei 230601China department of Chemical Physics University of Science and Technology of ChinaHefei 230026China

Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic *** have low ionization *** a superalkali in cyclo[18]carbon is an effective method to improve the optical properties of the system because considerable electron transfer *** this paper,the geometry,bonding properties,electronic structure,absorption spectrum,and nonlinear optical(NLO)properties of superalkaline M_(3)O(M=Li,Na)-doped cyclo[18]carbon were studied by using density functional theory.M_(3)O and the C_(18) rings are not *** C_(18) ring still exhibits alternating long and short *** charge transfer between M_(3)O and C_(18) forms stable[M_(3)O]+[C_(18)]-ionic complexes.C_(18)M_(3)O(M=Li,Na)shows striking optical nonlinearity,i.e.,their first-and second-order hyperpolarizability(βvec andγ||)increase considerably atλ=1907 nm and 1460 nm.

关键词： superalkaline doped cyclocarbon structure and electronic properties nonlinear optical properties density functional theory(DFT)

Earth's core-mantle boundary shaped by the crystallization of a hydrous terrestrial magma ocean

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National Science Review 2024年第7期11卷 73-75页

作者： Qingyang Hu Jie Deng Yukai Zhuang Zhenzhong Yang Rong Huang Center for High Pressure Science and Technology Advanced Research(HPSTAR) Shanghai Advanced Research in physical Sciences(SHARPS) department of Geosciences Princeton University Institute of Atomic and Molecular Physics Sichuan University Key Laboratory of Polar Materials and Devices Department of Electronics East China Normal University

A water-rich global magma ocean(MO)likely existed in the early Hadean eon and subsequently cooled and *** water is an oxidant and is known to fundamentally affect liquid crystallization, the role of primordial water d... 详细信息

关键词： CROSSOVER MELT