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Heteroatom tuning in agarose derived carbon aerogel for enhanced potassium ion multiple energy storage

Carbon Energy 2024年第3期6卷 239-254页

作者： Kaijun Xie Xin Liu Haolin Li Long Fang Kai Xia Dongjiang Yang Yihui Zou Xiaodong Zhang State Key laboratory of Bio-fibers and Eco-textiles Shandong Collaborative Innovation Center of Marine Biobased Fibers and Ecological TextilesInstitute of Marine Biobased MaterialsCollege of Chemistry and Chemical EngineeringCollege of Environmental Science and EngineeringQingdao UniversityQingdaoChina

The incorporation of heteroatoms into carbon aerogels(CAs)can lead to structural distortions and changes in active sites due to their smaller size and electronegativity compared to pure carbon.However,the evolution of the electronic structure from single-atom doping to heteroatom codoping in CAs has not yet been thoroughly investigated,and the impact of codoping on potassium ion(K+)storage and diffusion pathways as electrode material remains unclear.In this study,experimental and theoretical simulations were conducted to demonstrate that heteroatom codoping,composed of multiple heteroatoms(O/N/B)with different properties,has the potential to improve the electrical properties and stability of CAs compared to single-atom doping.Electronic states near the Fermi level have revealed that doping with O/N/B generates a greater number of active centers on adjacent carbon atoms than doping with O and O/N atoms.As a result of synergy with enhanced wetting ability(contact angle of 9.26°)derived from amino groups and hierarchical porous structure,ON-CA has the most optimized adsorption capacity(−1.62 eV)and diffusion barrier(0.12 eV)of K^(+).The optimal pathway of K^(+)in ON-CA is along the carbon ring with N or O doping.As K^(+)storage material for supercapacitors and ion batteries,it shows an outstanding specific capacity and capacitance,electrochemical stability,and rate performance.Especially,the assembled symmetrical K^(+)supercapacitor demonstrates an energy density of 51.8 Wh kg^(−1),an ultrahigh power density of 443Wkg^(−1),and outstanding cycling stability(maintaining 83.3%after 10,000 cycles in 1M KPF6 organic electrolyte).This research provides valuable insights into the design of highperformance potassium ion storage materials.

关键词： agarose carbon aerogels O/N/B codoping potassium-ion battery potassium-ion supercapacitor

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Analysis of quality-related proteins in golden pompano(Trachinotus ovatus)fillets with modified atmosphere packaging under superchilling storage

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Food science and Human Wellness 2024年第4期13卷 2253-2265页

作者： Chuang Pan Xiaofan Zhang Shengjun Chen Yong Xue Yanyan Wu Yueqi Wang Di Wang South China Sea Fisheries Research Institute Chinese Academy of Fishery SciencesKey Laboratory of Aquatic Product ProcessingMinistry of Agriculture and Rural AffairsNational R&D Centre for Aquatic Product ProcessingGuangzhou 510300China Co-innovation center of Jiangsu marine Bio-industry technology Jiangsu Ocean UniversityLianyungang 222005China collaborative innovation center of Seafood Deep Processing Dalian Polytechnic UniversityDalian 116034China Key laboratory of Efficient Utilization and Processing of marine Fishery Resources of Hainan Province Sanya Tropical Fisheries Research InstituteSanya 572018China College of Food science and Engineering Ocean University of ChinaQingdao 266003China

Here,we aimed to study the changes in proteome of golden pompano fillets during post-mortem storage.Tandem mass tags(TMT)-labeled quantitative proteomic strategy was applied to investigate the relationships between protein changes and quality characteristics of modified atmosphere packaging(MAP)fillets during superchilling(-3°C)storage.Scanning electron microscopy was used to show that the muscle histology microstructure of fillets was damaged to varying degrees,and low-field nuclear magnetic resonance was used to find that the immobilized water and free water in the muscle of fillets changed significantly.Total sulfhydryl content,TCA-soluble peptides and Ca2+-ATPase activity also showed that the fillet protein had a deterioration by oxidation and denaturation.The Fresh(FS),MAP,and air packaging(AP)groups were set.Total of 150 proteins were identified as differential abundant proteins(DAPs)in MAP/FS,while 209 DAPs were in AP/FS group.The KEGG pathway analysis indicated that most DAPs were involved in binding proteins and protein turnover.Correlation analysis found that 52 DAPs were correlated with quality traits.Among them,8 highly correlated DAPs are expected to be used as potential quality markers for protein oxidation and water-holding capacity.These results provide a further understanding of the muscle deterioration mechanism of packaging golden pompano fillets during superchilling.

关键词： Tandem mass tags(TMT)proteomics Trachinotus ovatus Modified atmosphere packaging Superchilling storage Low-field nuclear magnetic resonance Protein deterioration

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基于聚吡咯/蛭石/海藻纤维复合半导体材料的瞬态压阻传感器

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science China Materials 2024年第2期67卷 580-587页

作者：王鹏真梁俊轩田维亮张克伟夏延致 State Key laboratory of Bio-Fibers and Eco-Textiles Collaborative Innovation Center for Marine Biomass FibersMaterials and Textiles of Shandong ProvinceCollege of Materials Science and EngineeringInstitute of Marine Biobased MaterialsQingdao UniversityQingdao 266071China Key laboratory of Chemical Engineering in South Xinjiang College of Chemistry and Chemical EngineeringTarim UniversityAlaer 843300China

电子皮肤、人机交互和健康监测等领域推动了柔性压力传感器的快速发展.然而,同时满足耐用和瞬态的需求对柔性压力传感器是一个巨大的挑战.本文开发了一种用于柔性瞬态压阻传感器的安全、耐受的聚吡咯/蛭石/海藻酸盐半导体框架.将带负电... 详细信息

电子皮肤、人机交互和健康监测等领域推动了柔性压力传感器的快速发展.然而,同时满足耐用和瞬态的需求对柔性压力传感器是一个巨大的挑战.本文开发了一种用于柔性瞬态压阻传感器的安全、耐受的聚吡咯/蛭石/海藻酸盐半导体框架.将带负电荷的蛭石纳米片插层到可生物降解的海藻酸盐织物中,进一步用高灵敏度的导电聚吡咯修饰.由此产生的多维框架实现了柔性传感器的稳定性,并且在使用寿命结束后可以在不留下电子垃圾的情况下逐渐降解.所获得的瞬态压阻传感器显示出了快速的响应时间(81/99 ms)和出色的抗疲劳性能.此外,我们开发了一种有效的机器学习模型用于人体动作识别和预测,准确率为100%.本工作为柔性瞬态电子学中有机-无机界面的设计提供了一种有前景的策略,并在基于舒适生物纤维的柔性平台中展现了广阔的应用前景.

关键词： piezoresistive sensors transient electronics machine learning tolerable hybrids

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Impacts of major volcanic eruptions over the past two millennia on both global and Chinese climates:A review

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science China Earth sciences 2024年第1期67卷 61-78页

作者： Weiyi SUN Deliang CHEN Guonian LÜ Liang NING Chaochao GAO Renhe ZHANG Bin WANG Jian LIU Key laboratory for Virtual Geographic Environment Ministry of EducationState Key Laboratory Cultivation Base of Geographical Environment Evolution of Jiangsu ProvinceJiangsu Center for Collaborative Innovation in Geographical Information Resource Development and ApplicationSchool of Geography ScienceNanjing Normal UniversityNanjing 210023China Regional Climate Group Department of Earth SciencesUniversity of GothenburgGothenburg 40530Sweden College of Environmental and Resource science Zhejiang UniversityHangzhou 310058China Department of Atmospheric and Oceanic sciences&Institute of Atmospheric sciences Fudan UniversityShanghai 200437China Department of Atmospheric sciences and Atmosphere-Ocean Research center University of Hawaii at ManoaHonoluluHI 96825USA Jiangsu Provincial Key laboratory for Numerical Simulation of Large Scale Complex Systems School of Mathematical ScienceNanjing Normal UniversityNanjing 210023China Open Studio for the Simulation of Ocean-Climate-Isotope Qingdao National Laboratory for Marine Science and TechnologyQingdao 266237China

Major volcanic eruptions(MVEs)have attracted increasing attention from the scientific community.Previous studies have explored the climatic impact of MVEs over the past two millennia.However,proxy-based reconstructions and climate model simulations indicate divergent responses of global and China’s regional climates to MVEs.Here,we used multiple data from observations,reconstructions,simulations,and assimilations to summarize the historical facts of MVEs,the characteristics and mechanisms of their climatic impact,and directions for future research.We reviewed volcanic datasets and determined intensive MVE periods;these periods corresponded to the years 530–700,1200‒1460,and 1600‒1840 CE.After tropical MVEs,a substantial cooling effect is observed throughout the globe and China on the interannual-interdecadal time scales but an inconsistent cooling magnitude is detected between reconstructions and simulations.In the first summer after tropical MVEs,a decrease in global and monsoonal precipitation is observed.In reconstructions and simulations,an increased precipitation is seen for the Yangtze River Basin,while large uncertainties in precipitation changes are present for other regions of China.Decadal drought can be induced by frequent eruptions and volcanism superimposed on low solar irradiation and internal variability.MVEs affect climate directly through the radiative effect and indirectly by modulating internal variability,such as the El Niño‒Southern Oscillation(ENSO)and Atlantic Multidecadal Oscillation(AMO).However,changes in the phase,amplitude,and periodicity of ENSO and AMO after MVEs and the associated mechanisms remain controversial,which could account for model-reconstruction disagreements.Moreover,other internal variability,uncertainties in reconstruction methods and aerosol‒climate models,and climate background may also induce model-reconstruction disagreements.Knowledge gaps and directions for future research are also discussed.

关键词： Major volcanic eruption Climate variability Mechanism Past two millennia Internal variability

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Ecology and risks of the global plastisphere as a newly expanding microbial habitat

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The innovation 2024年第1期5卷 49-58页

作者： Changchao Li Michael RGillings Chao Zhang Qinglin Chen Dong Zhu Jie Wang Kankan Zhao Qicheng Xu Polly Hangmei Leung Xiangdong Li Jian Liu Ling Jin Department of Civil and Environmental Engineering The Hong Kong Polytechnic UniversityKowloonHong KongChina Environment Research Institute Shandong UniversityQingdao 266237China State Key laboratory of marine Pollution City University of Hong KongKowloon TongHong KongChina ARC Centre of Excellence in Synthetic Biology Faculty of Science and EngineeringMacquarie UniversitySydneyNSW 2109Australia Key laboratory of Urban Environment and Health Ningbo Urban Environment Observation and Research StationInstitute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Beijing Key laboratory of Farmland Soil Pollution Prevention and Remediation College of Resources and Environmental SciencesChina Agricultural UniversityBeijing 100193China Institute of Soil and Water Resources and Environmental science College of Environmental and Resource SciencesZhejiang UniversityHangzhou 310058China Jiangsu collaborative innovation center for Solid Organic Waste Resource Utilization Nanjing Agricultural UniversityNanjing 210095China Department of Health technology and Informatics and Research Institute for Future Food The Hong Kong Polytechnic UniversityKowloonHong KongChina Southern marine science and Engineering Guangdong laboratory(Guangzhou) Guangzhou 511458China

Plastic offers a new niche for microorganisms,the plastisphere.The everincreasing emission of plastic waste makes it critical to understand the microbial ecology of the plastisphere and associated effects.Here,we present a global fingerprint of the plastisphere,analyzing samples collected from freshwater,seawater,and terrestrial ecosystems.The plastisphere assembles a distinct microbial community that has a clearly higher heterogeneity and a more deterministically dominated assembly compared to natural habitats.New coexistence patterns—loose and fragile networks with mostly specialist linkages among microorganisms that are rarely found in natural habitats—are seen in the plastisphere.Plastisphere microbiomes generally have a great potential to metabolize organic compounds,which could accelerate carbon turnover.Microorganisms involved in the nitrogen cycle are also altered in the plastisphere,especially in freshwater plastispheres,where a high abundance of denitrifiers may increase the release of nitrite(aquatic toxicant)and nitrous oxide(greenhouse gas).Enrichment of animal,plant,and human pathogens means that the plastisphere could become an increasingly mobile reservoir of harmful microorganisms.Our findings highlight that if the trajectory of plastic emissions is not reversed,the expanding plastisphere could pose critical planetary health challenges.

关键词： reservoir mostly habitat

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CAS-ESM2.0 Successfully Reproduces Historical Atmospheric CO_(2) in a Coupled Carbon−Climate Simulation

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Advances in Atmospheric sciences 2024年第4期41卷 572-580页

作者： Jiawen ZHU Juanxiong HE Duoying JI Yangchun LI He ZHANG Minghua ZHANG Xiaodong ZENG Kece FEI Jiangbo JIN International center for Climate and Environment sciences Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China collaborative innovation center on Forecast and Evaluation of Meteorological Disasters(CIC-FEMD) Nanjing University of Information Science&TechnologyNanjing 210044China College of Global Change and Earth System science Beijing Normal UniversityBeijing 100875China State Key laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric Physics Chinese Academy of SciencesBeijing 100029China School of marine and Atmospheric sciences Stony Brook UniversityNY 11790USA University of Chinese Academy of sciences Beijing 100049China

The atmospheric carbon dioxide(CO_(2))concentration has been increasing rapidly since the Industrial Revolution,which has led to unequivocal global warming and crucial environmental change.It is extremely important to investigate the interactions among atmospheric CO_(2),the physical climate system,and the carbon cycle of the underlying surface for a better understanding of the Earth system.Earth system models are widely used to investigate these interactions via coupled carbon-climate simulations.The Chinese Academy of sciences Earth System Model version 2(CAS-ESM2.0)has successfully fixed a two-way coupling of atmospheric CO_(2)with the climate and carbon cycle on land and in the ocean.Using CAS-ESM2.0,we conducted a coupled carbon-climate simulation by following the CMIP6 proposal of a historical emissions-driven experiment.This paper examines the modeled CO_(2)by comparison with observed CO_(2)at the sites of Mauna Loa and Barrow,and the Greenhouse Gases Observing Satellite(GOSAT)CO_(2)product.The results showed that CAS-ESM2.0 agrees very well with observations in reproducing the increasing trend of annual CO_(2)during the period 1850-2014,and in capturing the seasonal cycle of CO_(2)at the two baseline sites,as well as over northern high latitudes.These agreements illustrate a good ability of CAS-ESM2.0 in simulating carbon-climate interactions,even though uncertainties remain in the processes involved.This paper reports an important stage of the development of CAS-ESM with the coupling of carbon and climate,which will provide significant scientific support for climate research and China’s goal of carbon neutrality.

关键词： CAS-ESM atmospheric CO_(2) coupled carbon-climate simulation emissions-driven CMIP6 experiment

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Predicting impact forces on pipelines from deep-sea fluidized slides:A comprehensive review of key factors

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International Journal of Mining science and technology 2024年第2期34卷 211-225页

作者： Xingsen Guo Ning Fan Defeng Zheng Cuiwei Fu Hao Wu Yanjun Zhang Xiaolong Song Tingkai Nian State Key laboratory of Coastal and Offshore Engineering Dalian University of TechnologyDalian 116024China Department of Civil Environmentaland Geomatic EngineeringUniversity College LondonLondon WC1E 6BTUnited Kingdom Shandong Provincial Key laboratory of marine Environment and Geological Engineering Ocean University of ChinaQingdao 266100China State Key laboratory of Geohazard Prevention and Geoenvironment Protection Chengdu University of TechnologyChengdu 610059China College of Civil Engineering and Architecture Wenzhou UniversityWenzhou 325035China Key laboratory of Engineering and technology for Soft Soil Foundation and Tideland Reclamation of Zhejiang Province Wenzhou 325035China Zhejiang International science and technology Cooperation Base of Ultra-soft Soil Engineering and Smart Monitoring Wenzhou 325035China School of Geography Liaoning Normal UniversityDalian 116029China China Railway First Survey and Design Institute Group Co. Ltd.Xi’an 710043China Department of Geotechnical Engineering Nanjing Hydraulic Research InstituteNanjing 210024China Wuhan center China Geological Survey(Central South China Innovation Center for Geosciences)Wuhan 430205China State Key laboratory of Mining Response and Disaster Prevention and Control in Deep Coal Mines Anhui University of Science and TechnologyHuainan 232001China

Deep-sea pipelines play a pivotal role in seabed mineral resource development,global energy and resource supply provision,network communication,and environmental protection.However,the placement of these pipelines on the seabed surface exposes them to potential risks arising from the complex deep-sea hydrodynamic and geological environment,particularly submarine slides.Historical incidents have highlighted the substantial damage to pipelines due to slides.Specifically,deep-sea fluidized slides(in a debris/mud flow or turbidity current physical state),characterized by high speed,pose a significant threat.Accurately assessing the impact forces exerted on pipelines by fluidized submarine slides is crucial for ensuring pipeline safety.This study aimed to provide a comprehensive overview of recent advancements in understanding pipeline impact forces caused by fluidized deep-sea slides,thereby identifying key factors and corresponding mechanisms that influence pipeline impact forces.These factors include the velocity,density,and shear behavior of deep-sea fluidized slides,as well as the geometry,stiffness,self-weight,and mechanical model of pipelines.Additionally,the interface contact conditions and spatial relations were examined within the context of deep-sea slides and their interactions with pipelines.Building upon a thorough review of these achievements,future directions were proposed for assessing and characterizing the key factors affecting slide impact loading on pipelines.A comprehensive understanding of these results is essential for the sustainable development of deep-sea pipeline projects associated with seabed resource development and the implementation of disaster prevention measures.

关键词： Deep-sea fluidized slides Pipes Impact forces Shear behavior of slides Interface contact conditions Spatial relation

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Analysis of a simplification strategy in a nonhydrostatic model for surface and internal wave problems

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Acta Oceanologica Sinica 2023年第2期42卷 29-43页

作者： Jinghua Zhang Wensheng Jiang Xueqing Zhang Key laboratory of marine Environment and Ecology of Ministry of Education Ocean University of ChinaQingdao266100China Tianjin Research Institute for Water Transport Engineering Ministry of TransportTianjin300456China physical oceanography laboratory/qingdao collaborative innovation center of marine science and technology Ocean University of ChinaQingdao266100China Pilot National laboratory for marine science and technology(qingdao) Qingdao266237China

This paper examines the simplification strategy of retaining only the nonhydrostatic effect of local acceleration in a three-dimensional fully nonhydrostatic model regarding the submesoscale wave phenomenon in the ocean.Elaborate scale analysis of the vertical component of the Reynold-averaged Navier-Stokes(RANS)equation was performed,confirming the rationalization of this simplification.Then,the simplification was implemented in a RANS equation-based nonhydrostatic model NHWAVE(nonhydrostatic WAVE)to make a simplified nonhydrostatic model.Numerical examples were taken to test its performance,including surface sinusoidal waves propagating on an idealized East China Sea topography,tidally induced internal lee waves and small-scale solitary waves.The results show that in a considerably wide range of nonlinear strengths,the simplified nonhydrostatic model can obtain similar results as those in the fully nonhydrostatic model,even for smaller-scale solitary waves.Nonlinearity influences the applicability of the simplification.The stronger the nonlinearity is,the worse the simplified model describes the nonhydrostatic phenomenon.In general,the simplified nonhydrostatic model can simulate surface waves better than internal waves.Improvement of computational efficiency in the simplified nonhydrostatic model is reasonable,reducing the central processing unit time duration in the fully nonhydrostatic model by 16.4%–20.6%.The specially designed algorithm based on the simplified nonhydrostatic equation can remarkably reduce the computational time.

关键词： simplification of nonhydrostatic model submesoscale wave internal lee wave

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爆破型和聚能型装药水下爆炸载荷特性

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哈尔滨工程大学学报（英文版） 2024年第2期23卷 302-315页

作者：张之凡李海龙张竞元王龙侃张桂勇宗智 State Key laboratory of Structural Analysis Optimization and CAE Software for Industrial EquipmentSchool of Naval Architecture EngineeringDalian University of TechnologyDalian 116024China China Ship Research and Development Academy Beijing 100192China collaborative innovation center for Advanced Ship and Deep-Sea Exploration Shanghai 200240China

Blasting and shaped charges are the main forms of underwater weapons,and their near-field underwater explosions(UNDEX)can severely damage structures.Therefore,it is of great importance to study underwater explosive load characteristics of different forms of charges.The full physical process of a typical underwater explosion of a sphere/column blasting charge and a shaped charge was simulated using the Eulerian method.The loading characteristics of the underwater blast shock wave and bubble,as well as the projectile,were studied.The results show that the shock wave loads of spherical,cylindrical,and polygonal charges propagate outward in spherical,ellipsoidal–spherical and ellipsoidal–spherical wavefronts,respectively.When the shock wave reaches 16 times the distance-to-diameter ratio,its surface is approximately spherical.In addition,in the shaped charge underwater explosion,the shaped charge liner cover absorbs 30°–90°of the shock wave energy and some of the bubble energy to form a high-speed shaped penetrator.Spherical,ellipsoidal,and ellipsoidal bubbles are generated by underwater explosions of spherical,cylindrical,and shaped charges,respectively.The obtained results provide a reference for evaluating the power of underwater weapons.

关键词： Blasting charge Shaped charge Load characteristics Shock wave Bubble

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Exploration of sea anemone-inspired high-performance biomaterials with enhanced antioxidant activity

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Bioactive Materials 2022年第4期7卷 504-514页

作者： Lulu Wang Xiaokang Zhang Pingping Xu Jicheng Yan Yuzhong Zhang Hainan Su Chengjun Sun Qiang Lu Weizhi Liu Sars-Fang Centre MOE Key Laboratory of Marine Genetics and BreedingCollege of Marine Life SciencesOcean University of ChinaQingdao266003China laboratory for marine Biology and Biotechnology Pilot National Laboratory for Marine Science and TechnologyQingdao266071China State Key laboratory of Microbial technology Marine Biotechnology Research CenterShandong UniversityQingdao266237China Key laboratory of marine Eco-environmental science and technology Marine Bioresource and Environment Research CenterFirst Institute of OceanographyMinistry of Natural Resources(MNR)Qingdao266061China National Engineering laboratory for Modern Silk Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou215123China

Antioxidant biomaterials have attracted much attention in various biomedical fields because of their effective inhibition and elimination of reactive oxygen species(ROS)in pathological tissues.However,the difficulty in ensuring biocompatibility,biodegradability and bioavailability of antioxidant materials has limited their further development.Novel bioavailable antioxidant materials that are derived from natural resources are urgently needed.Here,an integrated multi-omics method was applied to fabricate antioxidant biomaterials.A key cysteine-rich thrombospondin-1 type Ⅰ repeat-like(TSRL)protein was efficiently discovered from among 1262 adhesive components and then used to create a recombinant protein with a yield of 500 mg L^(-1).The biocompatible TSRL protein was able to self-assemble into either a water-resistant coating through Ca^(2+)-mediated coordination or redox-responsive hydrogels with tunable physical properties.The TSRL-based hydrogels showed stronger 1,1-diphenyl-2-picrylhydrazyl(DPPH)radical scavenging rates than glutathione(GSH)and ascorbic acid(Aa)and protected cells against external oxidative stress significantly more effectively.When topically applied to mice skin,TSRL alleviated epidermal hyperplasia and suppressed the degradation of collagen and elastic fibers caused by ultraviolet radiation B(UVB)irradiation,confirming that it enhanced antioxidant activity in vivo.This is the first study to successfully characterize natural antioxidant biomaterials created from marine invertebrate adhesives,and the findings indicate the excellent prospects of these biomaterials for great applications in tissue regeneration and cosmeceuticals.

关键词： Sessile marine organisms Antioxidant biomaterials Water-resistant coatings Redox-responsive hydrogels Photoaging

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