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Ammonia pyrolysis oxidation excited by nanosecond pulsed discharge:Global/fluid models hybrid solution

Journal of Energy Chemistry 2025年第1期100卷 385-396页

作者： Mingming Zhang Hanyu Wu Qi Chen Jiaxin Yang Bonan Liu School of Mechanical Electronic and Control Engineering Beijing Jiaotong University China University of petroleum

The kinetic characteristics of plasma-assisted oxidative pyrolysis of ammonia are studied by using the global/fluid models hybrid solution ***,the stable products of plasma-assisted oxidative pyrolysis of ammonia are *** results show that the consumption of NH3/O2and the production of N2/H2change linearly with the increase of voltage,which indicates the decoupling of nonequilibrium molecular excitation and oxidative pyrolysis of ammonia at low ***,the detailed reaction kinetics mechanism of ammonia oxidative pyrolysis stimulated by a nanosecond pulse voltage at low pressure and room temperature is *** on the reaction path analysis,the simplified mechanism is *** detailed and simplified mechanism simulation results are compared with experimental data to verify the accuracy of the simplified ***,based on the simplified mechanism,the fluid model of ammonia oxidative pyrolysis stimulated by the nanosecond pulse plasma is established to study the pre-sheath/sheath behavior and the resultant consumption and formation of key *** results show that the generation,development,and propagation of the pre-sheath have a great influence on the formation and consumption of *** consumption of NH3by the cathode pre-sheath is greater than that by the anode pre-sheath,but the opposite is true for OH and O（1S）.However,within the sheath,almost all reactions do not ***,by changing the parameters of nanosecond pulse power supply voltage,it is found that the electron number density,electron current density,and applied peak voltages are not the direct reasons for the structural changes of the sheath and ***,the discharge interval has little effect on the sheath structure and gas mixture *** research results of this paper not only help to understand the kinetic promotion of non-equilibrium excitation in the process of oxidative pyrolysis but also help to explore th

关键词： Nanosecond pulsed discharge Ammonia Oxidative pyrolysis Fluid model Global model

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Tensor based non-photo realistic rendering for Korean architectural images

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Journal of Central South University 2014年第10期21卷 3805-3810页

作者： Do Kyung Shin Eun Young Ahn deprtment of Computer Science and engineering Hanyang University deprtment of Communication Infromation & Computer engineering Hanbat National University

Existing pen and ink sketch technologies can be applied to general images, but they could not produce optimal output for images of traditional architecture, because most images consist of exquisite straight lined patterns in traditional architecture, such as root tiles and window bars. The lines of roofs and eaves need to be described delicately to express pen and ink sketch most effectively. Therefore, by proposing a method to create white noise for light and shade of input images, to extract input vector directions from the white noise, and to determine the direction and length of stroke, a new expression technique is proposed for pen and ink sketch that could best reflect the characteristics of traditional architecture.

关键词： non-photo realistic rendering pen and ink sketch tensor

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Tuning the interfacial reaction environment via pH-dependent and induced ions to understand C–N bonds coupling performance in NO3- integrated CO2 reduction to carbon and nitrogen compounds over dual Cu-based N-doped carbon catalyst

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Journal of Energy Chemistry 2025年第1期100卷 273-285页

作者： Tianhang Zhou Chen Shen Zhenghao Wu Xingying Lan Yi Xiao College of Carbon Neutrality Future Technology State Key Laboratory of Heavy Oil Processing China University of Petroleum (Beijing) Institute of Materials Science TU Darmstadt Department of Chemistry Xi'an Jiaotong-Liverpool University Department of Mechanical and Mechatronics engineering and Waterloo Institute of Nanotechnology University of Waterloo Waterloo

Dual atomic catalysts （DAC）,particularly copper （Cu2）-based nitrogen （N） doped graphene,show great potential to effectively convert CO2and nitrate （NO3-） into important industrial chemicals such as ethylene,glycol,acetamide,and urea through an efficient catalytical process that involves C–C and C–N ***,the origin of the coupling activity remained unclear,which substantially hinders the rational design of Cu-based catalysts for the N-integrated CO2reduction reaction （CO2RR）.To address this challenge,this work performed advanced density functional theory calculations incorporating explicit solvation based on a Cu2-based N-doped carbon (Cu2N6C10) catalyst for *** calculations are aimed to gain insight into the reaction mechanisms for the synthesis of ethylene,acetamide,and urea via coupling in the interfacial reaction *** to the sluggishness of CO2,the formation of a solvation electric layer by anions （F-,Cl-,Br-,and I-） and cations (Na+,Mg2+,K+,and Ca2+) leads to electron transfer towards the Cu *** process significantly accelerates the reduction of *** results reveal that*CO intermediates play a pivotal role in N-integrated ***,the Cu2-based N-doped carbon catalyst examined in this study has demonstrated the most potential for C–N coupling to *** findings reveal that through the process of a condensation reaction between*CO and NH2OH for urea synthesis,*NO3-is reduced to*NH3,and*CO2to*CCO at dual Cu atom *** dual-site reduction facilitates the synthesis of acetamide through a nucleophilic reaction between NH3and the ketene ***,we found that the I-and Mg2+ions,influenced by pH,were highly effective for acetamide and ammonia synthesis,except when F-and Ca2+were ***,the mechanisms of C–N bond formation were investigated via ab-initio molecular dynamics simulations,and we found that adjusting the micro-environment can change the dominant side reaction,shift

关键词： pH-dependent micro-environments C–N coupling Dual Cu-based nitrogen carbon catalysts Explicit solvation model Ion stabilizer AIMD

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Polymeric artificial solid/electrolyte interphases for Li-ion batteries

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Progress in Natural Science:Materials International 2015年第6期25卷 563-571页

作者： Nae-Lih Wu Yu-Ting Weng Fu-Sheng Li Nai-Hsuan Yang Chin-Lung Kuo Dong-Sheng Li deprtment of Chemical engineering National Taiwan University Department of Materials Science and engineering National Taiwan University

During the operation of Li-ion batteries(LIBs),solvent and electrolyte decomposition takes place at the electrode surface to form a so-called solid-electrode interphase(SEI) *** physical structure and chemical composition of the SEI exert profound effects on various aspects of the electrode performance of the batteries.A new concept of forming polymeric artificial SEIs(A-SEIs) based on rational design of multifunctional polymer-blend coating to achieve favorable electrode/A-SEI/electrolyte interfacial properties is *** examples using binary and ternary polymer blends to form mechanically robust and highly Li-ion permeable surface coatings with selected functionalities in the cases of graphite and silicon–graphite composite electrodes have demonstrated greatly enhanced capacity,rate and cycle *** the rich chemistry available from polymer blends,this surface preconditioning approach holds great promise for improving the performance of various negative electrodes to meet the requirements for advanced LIBs.

关键词： Li ion battery Solid electrolyte interphase Surface modification Polymer blend

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Molecular Structure Tailoring of Organic Spacers for High‑Performance Ruddlesden–Popper Perovskite Solar Cells

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Nano-Micro Letters 2025年第2期17卷 314-357页

作者： Pengyun Liu Xuejin Li Tonghui Cai Wei Xing Naitao Yang Hamidreza Arandiyan Zongping Shao Shaobin Wang Shaomin Liu School of Materials Science and engineering State Key Laboratory of Heavy Oil ProcessingChina University of Petroleum(East China)Qingdao 266580People’s Republic of China School of Chemistry and Chemical engineering Shandong University of TechnologyZibo 255049People’s Republic of China Centre for Applied Materials and Industrial Chemistry(CAMIC) School of ScienceRMIT UniversityMelbourneVic 3000Australia WA School of Mines:Minerals Energy and Chemical Engineering(WASM‑MECE)Curtin UniversityPerthWA 6102Australia School of Chemical engineering The University of AdelaideAdelaideSA 5005Australia School of engineering Great Bay UniversityDongguan 523000People’s Republic of China

Layer-structured Ruddlesden–Popper(RP)perovskites(RPPs)with decent stability have captured the imagination of the photovoltaic research community and bring hope for boosting the development of perovskite solar cell(PSC)***,two-dimensional(2D)or quasi-2D RP PSCs are encountered with some challenges of the large exciton binding energy,blocked charge transport and poor film quality,which restrict their photovoltaic ***,these issues can be readily resolved by rationally designing spacer cations of *** review mainly focuses on how to design the molecular structures of organic spacers and aims to endow RPPs with outstanding photovoltaic *** firstly elucidated the important roles of organic spacers in impacting crystallization kinetics,charge transporting ability and stability of *** we brought three aspects to attention for designing organic ***,we presented the specific molecular structure design strategies for organic spacers of RPPs aiming to improve photovoltaic performance of RP *** proposed strategies in this review will provide new avenues to develop novel organic spacers for RPPs and advance the development of RPP photovoltaic technology for future applications.

关键词： Ruddlesden-Popper perovskites Low-dimensional perovskite solar cells Organic spacers Molecular structure Design strategies

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Mathematical modeling of heat transfer in counter-current multiphase flow found in gas-drilling systems with formation fluid influx

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petroleum Science 2017年第4期14卷 711-719页

作者： Boyun Guo Jun Li Jinze Song Gao Li petroleum engineering Department University of Louisiana at Lafayette College of petroleum engineering Southwest Petroleum University College of petroleum engineering China University of Petroleum

The performance of gas-drilling(drilling oil and gas wells with air, nitrogen, or natural gas) is very unpredictable in many areas due to lack of proper design of drilling parameters because of limited understanding of gas–rock interaction which requires knowledge of heat transfer in the well system. Complete analysis of rock failure requires an accurate mathematical model to predict gas temperature at the bottom hole. The currently available mathematical models are unsuitable for use for the purpose because they do not consider the effects of formation fluid influx, Joule–Thomson cooling, and entrained drill cuttings. A new analytical solution for predicting gas temperature profiles inside the drill string and in the annulus was derived in this study for gas-drilling, considering all these three effects. Results of sensitivity analyses show that formation fluid influx can significantly increase the temperature profiles in both the drill string and the *** Joule–Thomson cooling effect lowers the temperature in the annulus only in a short interval near the bottom *** drill cuttings entrained at the bottom hole can slightly increase the temperature profile in the annulus.

关键词： Gas-drilling Temperature Prediction Influx Joule–Thomson Cuttings

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Experimental assessment of hybrid smart carbonated water flooding for carbonate reservoirs

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petroleum 2021年第1期7卷 80-90页

作者： Payam Soleimani Seyed Reza Shadizadeh Riyaz Kharrat Department of petroleum engineering Ahwaz Faculty of Petroleum EngineeringPetroleum University of TechnologyAhwazIran Department of petroleum engineering Abadan Faculty of Petroleum EngineeringPetroleum University of TechnologyAbadanIran Department petroleum engineering MontanuniversitatLeobenAustria

Different methods of enhanced oil recovery have been used to produce trapped *** of these methods is carbonated water injection in which CO2 contained water is injected in reservoirs in order to decrease free CO2 injection mobility,increase water viscosity and store/remove produced greenhouse CO2 gas *** enhanced oil recovery method is smart water injection at which the ions in brine are modified in order to make controlled reactions with distributed ions on the surface of rock to cause more hydrocarbon ***,combination of these two methods may also have a great effect on enhancing oil recovery or may result in recovery factor less than each method used *** this paper hybrid smart carbonated water injection method is investigated to study its applicability in oil recovery using core flooding *** experimental core flooding setup was designed to perform different types of EOR methods for the sake of recovery comparison with the new hybrid *** effect of both brine content and volume of CO2 is determining in hybrid EOR *** main findings of this work show that the hybrid smart carbonated water results in the highest recovery factor in comparison to the most well-known EOR methods for carbonate cores.

关键词： Hybrid smart carbonated water Carbonated water Smart water Core flooding Carbonate core

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Numerical modeling of simultaneous hydraulic fracturing in the mode of multi-well pads

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Science China(Technological Sciences) 2017年第2期60卷 232-242页

作者： YAO Jun ZENG QingDong HUANG ZhaoQin SUN Hai ZHANG Lei School of petroleum engineering China University of Petroleum (East China) Department of petroleum engineering Colorado School of Mines

In order to investigate propagation regularity of hydraulic fractures in the mode of multi-well pads, numerical modeling of simultaneous hydraulic fracturing of multiple wells was conducted. The mathematical model was established coupling rock deformation with fluid flow in the fractures and wellbores. And then the model was solved by displacement discontinuity method coupling with implicit level set method. The implicit method was based on fracture tip asymptotical solution and used to determine fracture growth length. Simulation results showed that when multiple wells were fractured simultaneously, adjacent fractures might propagate towards each other, showing an effect of attraction other than repulsion. Fracture spacing and well spacing had significant influence on the propagation path and geometry of multiple fractures. Furthermore, when multiple wells were fractured simultaneously, stress reversal regions had a large area, and stress reversal regions were distributed not only in the area between fractures but also on the outside of them. The area of stress reversal regions was related to fracture spacing and well spacing. Results indicated that multi-well fracturing induced larger area of stress reversal regions than one-well fracturing, which was beneficial to generating complex fracture network in unconventional reservoirs.

关键词： hydraulic fracturing multi-well pads displacement discontinuity method implicit level set method stress reversal region

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PRESSURE DISTRIBUTION ON THE WALL OF THE INNER CYLINDER RECIPROCATING AXIALLY TO THE UNSTEADY FLOW OF VISCOELASTIC FLUID IN ECCENTRIC ANNULUS

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Journal of Hydrodynamics 2006年第5期18卷 606-612页

作者： WANG Yan CUI Hai-qing YANG Yuan-jian GUO Jun-hui LI Nan Department of petroleum engineering China University of Petroleum Beijing 102249 China Department of petroleum engineering Daqing Petroleum Institute Daqing 163318 China

In this article, the governing equations for the unsteady flow of viscoelastic fluid in the eccentric annulus with the inner cylinder reciprocating axially and the expression of the pressure distribution on the wall of the inner cylinder of the annulus are established and derived, respectively, under the bipolar coordinate system. The equations and the expression are solved and calculated numerically using the finite difference method, respectively. The curves of the pressure distribution on the wall of the inner cylinder of the aqueous solution of Hydrolyzed Polyacrylamide （HPAM） are plotted and the influences of annular eccentricity, stroke, and stroke frequency on the pressure distribution are analyzed.

关键词： viscoelastic unsteady flow eccentric annulus fluid reciprocating axially pressure distribution

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Corrosion of AISI 4130 Steel Alloy under Hydrodynamic Condition in Ethylene Glycol+Water+NO_2^- Solution

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Journal of Materials Science & Technology 2013年第1期29卷 89-96页

作者： I.Danaee M.Niknejad Khomami A.A.Attar Abadan Faculty of petroleum engineering Petroleum University of Technology

The electrochemical behavior of steel alloy in ethylene glycol-water mixture at different solution rotating speeds was investigated by polarization curves and AC impedance measurements （EIS）. The results obtained showed that corrosion rate was not changed significantly at different rotating speeds and was decreased with increasing ethylene glycol concentration. The effect of nitrite as an inhibitor was studied and high inhibition efficiency was obtained. It was found that surface passivation occurred in the presence of inhibitor. The inhibiting effect of the nitrite was explained on the basis of the competitive adsorption between the inorganic anions and the aggressive CI- ions and the adsorption isotherm basically obeys the Flory-Huggins adsorption isotherm. Thermodynamic parameters for steel corrosion and inhibitor adsorption were determined, which revealed that the adsorption process is spontaneous.

关键词： Steel 4130 Ethylene glycol Corrosion Hydrodynamic Nitrite

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