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In situ tracking of the lithiation and sodiation process of disodium terephthalate as anodes for rechargeable batteries by Raman spectroscopy

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Nano Research 2024年第1期17卷 245-252页

作者： Xiu-Mei Lin Chong Han Xin-Tao Yang Jia-Sheng Lin Wei-Qiang Yang Hong-Xu Guo Yao-Hui Wang Jin-Chao Dong Jian-Feng Li Department of Chemistry and Environment Science Fujian Province University Key Laboratory of Analytical ScienceMinnan Normal UniversityZhangzhou 363000China College of Energy College of Chemistry and Chemical EngineeringCollege of MaterialsState Key Laboratory of Physical Chemistry of Solid SurfacesiChEMXiamen UniversityXiamen 361005China Institute of optical and Electronic Technology China Jiliang UniversityHangzhou 310018China

Organic compounds represent an appealing group of electrode materials for rechargeable batteries due to their merits of biomass,sustainability,environmental friendliness,and *** terephthalate(Na_(2)C_(8)H_(4)O_(4),Na_(2)TP),an organic salt with a theoretical capacity of 255 mAh·g^(-1),is electroactive towards both lithium and ***,its electrochemical energy storage(EES)process has not been directly observed via in situ characterization techniques and the underlying mechanisms are still under ***,in situ Raman spectroscopy was employed to track the de/lithiation and de/sodiation processes of *** appearance and then disappearance of the–COOLi Raman band at 1625 cm^(-1) during the de/lithiation,and the increase and then decrease of the–COONa Raman band at 1615 cm^(-1) during the de/sodiation processes of Na2TP elucidate the one-step with the 2Li+or 2Na+transfer *** also found that the inferior cycling stability of Na2TP as an anode for sodium-ion batteries(SIBs)than lithium-ion batteries(LIBs)could be due to the larger ion radium of Na+than Li+,which results in larger steric resistance and polarization during *** Na2TP,therefore,shows greater changes in spectra during de/sodiation than de/*** expect that our findings could provide a reference for the rational design of organic compounds for EES.

关键词： disodium terephthalate(Na_(2)C_(8)H_(4)O_(4) Na2TP) in situ Raman spectroscopy de/lithiation de/sodiation mechanisms

Robust polarimetric dehazing algorithm based on low-rank approximation and multiple virtual-exposure fusion

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Photonics Research 2024年第8期12卷 1640-1653页

作者： YIFU ZHOU HANYUE WEI JIAN LIANG FEIYA MA RUI YANG LIYONG REN XUELONG LI School of Physics and Information Technology Shaanxi Normal University Xi'an Key Laboratory of optical Information Manipulation and Augmentation(OMA) Robust(Xixian New Area) Opto-Electro Technologies Co. Ltd. Institute of Artificial Intelligence(TeleAI) China Telecom Corp Ltd.

Polarimetric dehazing is an effective way to enhance the quality of images captured in foggy weather. However,images of essential polarization parameters are vulnerable to noise, and the brightness of dehazed images is usually unstable due to different environmental illuminations. These two weaknesses reveal that current polarimetric dehazing algorithms are not robust enough to deal with different scenarios. This paper proposes a novel, to our knowledge, and robust polarimetric dehazing algorithm to enhance the quality of hazy images, where a low-rank approximation method is used to obtain low-noise polarization parameter images. Besides, in order to improve the brightness stability of the dehazed image and thus keep the image have more details within the standard dynamic range, this study proposes a multiple virtual-exposure fusion(MVEF) scheme to process the dehazed image(usually having a high dynamic range) obtained through polarimetric dehazing. Comparative experiments show that the proposed dehazing algorithm is robust and effective, which can significantly improve overall quality of hazy images captured under different environments.

关键词： Deep learning Image enhancement Image metrics Imaging techniques Polarimetric imaging Scattering media

Efficient photocatalytic biomass-alcohol conversion with simultaneous hydrogen evolution over ultrathin 2D NiS/Ni-CdS photocatalyst

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Chinese Chemical Letters 2024年第7期35卷 422-427页

作者： Zongyi Huang Cheng Guo Quanxing Zheng Hongliang Lu Pengfei Ma Zhengzhong Fang Pengfei Sun Xiaodong Yi Zhou Chen State Key Laboratory of Physical Chemistry of Solid surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China College of Materials Key Laboratory of High Performance Ceramic Fibers(Xiamen University)Ministry of EducationXiamen UniversityXiamen 361005China Technology Center China Tobacco Fujian Industrial Co.Ltd.Xiamen 361021 China

The photocatalytic conversion of biomass into high-value chemicals,coupled with simultaneous hydrogen(H_(2))evolution,leveraging the electrons and holes generated by solar energy,holds great promise for addressing energy *** this study,we constructed a dual functional photocatalytic system formed by NiS loaded on Ni doped two-dimensional(2D)CdS nanosheet(NiS/Ni-CdSNS)heterostructure for visible-light-driven H_(2)evolution and ethanol oxidation to ***,the 2D NiS/NiCdSNS exhibited significant activity and selectivity in both photocatalytic H_(2)evolution and ethanol oxidation,achieving yields of 7.98 mmol g^(-1)h^(-1)for H_(2)and 7.33 mmol g^(-1)h^(-1)for *** heterogeneous interface of the composite facilitated efficient charge separation,while NiS provided abundant sites for proton reduction,thereby promoting the overall dual-functional photocatalytic *** functional theory calculations further reveal that both Ni doping and NiS loading can reduce the reaction energy barrier of ethanol oxidation of free radicals,and NiS/Ni-CdSNS composite materials exhibit stronger ethanol C-H activation ability to generate key intermediate·CH(OH)CH_(3)on the *** work serves as a valuable guide for the rational design of efficient dual functional photocatalytic systems that combine H_(2)evolution with the selective conversion of organic compounds into high-value chemicals.

关键词： Photocatalysis Biomass-alcohol oxidation H_(2)evolution Dual-functional catalysis

optical responses of metallic plasmonic arrays under the localized excitation

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Nano Research 2024年第3期17卷 1571-1577页

作者： Sen Yan Hao Ma Yi-Fan Bao Maofeng Cao Chuan Liu Kaifeng Zhang Xiaowei Wu Jianbo He Xiang Wang Bin Ren State Key Laboratory of Physical Chemistry of Solid surfaces Department of ChemistryCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province(IKKEM) Xiamen 361005China Research&Development Group HitachiLtd.Yokohama 244-0817KanagawaJapan Department of Electronic Science and Engineering Kyoto UniversityKyoto 615-8510Japan

The metallic plasmonic array that can support both propagating surface plasmon polaritons(PSPPs)and localized surface plasmon resonance(LSPR)possesses rich optical properties and remarkable optical performance,making it a powerful platform for applications in photonics,chemistry,and *** practical applications,the excitation spot is usually smaller than the area of metal *** is thus imperative to address“how many array units are enough?”towards a rational design of plasmonic ***,we employed focused ion beam(FIB)to precisely fabricate a series of plasmonic array structures with increased unit *** utilizing photoluminescence(PL)and surface-enhanced Raman spectroscopy(SERS),we found that the array units outside the excitation spot still have a significant impact on the optical response within the *** with the numerical simulation,we found that the boundary of the finite array leads to the loss of PSPP outside the excitation point,which subsequently affects the coupling of PSPP and LSPR in the excitation spot,leading to variations in PL and SERS *** on the findings,we further tuned the LSPR mode of the metal arrays by electrodeposition to obtain strong near-field enhancement without any influence on the PSPP *** work advances the understanding of near-field and far-field optical behavior in finite-size array structures and provides guidance for designing highly-efficient photonic devices.

关键词： plasmonic periodic array finite-size effects dark field scattering surface-enhanced Raman spectroscopy(SERS)

Differential interference contrast phase edging net:an all-optical learning system for edge detection of phase objects

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Chinese Optics Letters 2024年第1期22卷 21-27页

作者：李一鸣李然陈泉栾海涛卢海军杨晖顾敏张启明 Institute of Photonic Chips University of Shanghai for Science and TechnologyShanghai 200093China School of optical-Electrical and Computer Engineering University of Shanghai for Science and TechnologyShanghai 200093China Nokia Shanghai Bell Co. Ltd.Shanghai 201206China College of Medical Instruments Shanghai University of Medicine and Health SciencesShanghai 201318China

Edge detection for low-contrast phase objects cannot be performed directly by the spatial difference of intensity *** this work,an all-optical diffractive neural network(DPENet)based on the differential interference contrast principle to detect the edges of phase objects in an all-optical manner is *** information is encoded into an interference light field by dual Wollaston prisms without lenses and light-speed processed by the diffractive neural network to obtain the scale-adjustable *** results show that DPENet achieves F-scores of 0.9308(MNIST)and 0.9352(NIST)and enables real-time edge detection of biological cells,achieving an F-score of 0.7462.

关键词： diffractive neural network edge detection phase objects

Glass-Ceramics with High Strength and High Transmittance Obtained by Multi-Factor Controlling

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Journal of Wuhan University of Technology(Materials Science) 2024年第3期39卷 551-560页

作者：胡云坤 RAO Yu WANG Mingzhong XU Yinsheng XIA Mengling TAO Haizheng 陆平 School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China Xianning CSG Photovoltaic Glass Co. Ltd.Xianning 437100China State Key Laboratory of Silicate Materials for Architectures Wuhan University of TechnologyWuhan 430070China Jincheng optical-mechanical Industry Research Institute Jincheng 048000China

The presence of Li_(2)Si_(2)O_(5) and LiAlSi_(4)O_(10) could effectively improve the elastic modulus and transmittance of lithium disilicate(LD)*** synergistically modulation of the crystal content and grain size,we obtained high strength and high transmittance of LD *** optimal sample had a high transmittance of 90.3%,the hardness was 7.72 GPa,the fracture toughness was 1.07 MPa·m^(1/2),and the elastic modulus was 103.1 GPa.

关键词： lithium disilicate glass-ceramics transmittance mechanical properties

On-chip source-device-independent quantum random number generator

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Photonics Research 2024年第7期12卷 1379-1394页

作者： LANG LI MINGLU CAI TAO WANG ZICONG TAN PENG HUANG KAN WU GUIHUA ZENG State Key Laboratory of Advanced optical Communication Systems and Networks Shanghai Jiao Tong UniversityShanghai 200240China Institute of Quantum Sensing and Information Processing School of Sensing Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China Shanghai Research Center for Quantum Sciences Hefei National LaboratoryShanghai 201315China Shanghai Xun Tai Quantech Co. Ltd.Shanghai 200241China

Quantum resources offer intrinsic randomness that is valuable for applications such as cryptography, scientific simulation, and computing. Silicon-based photonics chips present an excellent platform for the cost-effective deployment of next-generation quantum systems on a large scale, even at room temperature. Nevertheless,the potential susceptibility of these chips to hacker control poses a challenge in ensuring security for on-chip quantum random number generation, which is crucial for enabling extensive utilization of quantum resources.

关键词： temperature. quantum random

Welding depth measurement for different mode lasers using optical coherence tomography

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Chinese Optics Letters 2024年第1期22卷 41-46页

作者：谢冠明王三宏张跃强李由胡彪傅愉于起峰 Institute of Intelligent optical Measurement and Detection Shenzhen UniversityShenzhen 518060China College of Physics and Optoelectronic Engineering Shenzhen UniversityShenzhen 518060China Shenzhen Sincevision Technology Co. Ltd.Shenzhen 518055China National Key Laboratory of Human Factors Engineering China Astronaut Research and Training CenterBeijing 100094China College of Aerospace Science and Engineering National University of Defense TechnologyChangsha 410073China

optical coherence tomography(OCT)allows a direct and precise measurement of laser welding depth by coaxially measuring the keyhole depth and can be used for process monitoring and *** OCT measurement was taken during single-beam laser welding,the keyhole instability of aluminum welding resulted in highly scattered OCT data and complicated the welding depth extraction *** a combination of an inner core beam and an outer ring beam,a novel adjustable ring mode(ARM)laser for producing a stable keyhole was applied to the OCT *** ARM laser power arrangements were conducted on aluminum and *** results indicated that the ring beam greatly improved the stability of the core beam-induced keyhole,and smooth welding depth can be extracted from the concentrated OCT data.

关键词： optical coherence tomography adjustable ring mode laser laser welding welding depth

High-repetition-rate and high-power efficient picosecond thin-disk regenerative amplifier

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High Power Laser Science and Engineering 2024年第2期12卷 16-23页

作者： Sizhi Xu Yubo Gao Xing Liu Yewang Chen Deqin Ouyang Junqing Zhao Minqiu Liu Xu Wu Chunyu Guo Cangtao Zhou Qitao Lue Shuangchen Ruan Key Laboratory of Advanced optical Precision Manufacturing Technology of Guangdong Higher Education Institutes Sino-German College of Intelligent ManufacturingShenzhen Technology UniversityShenzhenChina Han’s Laser Technology Industry Group Co. Ltd.ShenzhenChina Shenzhen Key Laboratory of Laser Engineering College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhenChina Shenzhen Key Laboratory of Ultraintense Laser and Advanced Material Technology College of Engineering PhysicsShenzhen Technology UniversityShenzhenChina

We present an effective approach to realize a highly efficient,high-power and chirped pulse amplification-free ultrafast ytterbium-doped yttrium aluminum garnet thin-disk regenerative amplifier pumped by a zero-phonon line 969 nm laser *** amplifier delivers an output power exceeding 154 W at a pulse repetition rate of 1 MHz with custom-designed 48 pump *** exceptional thermal management on the thin disk through high-quality bonding,efficient heat dissipation and a fully locked spectrum collectively contributes to achieving a remarkable optical-to-optical efficiency of 61%and a near-diffraction-limit beam quality with an M2 factor of *** the best of our knowledge,this represents the highest conversion efficiency reported in ultrafast thin-disk regenerative ***,the amplifier operates at room temperature and exhibits exceptional stability,with root mean square stability of less than 0.33%.This study significantly represents advances in the field of laser amplification systems,particularly in terms of efficiency and average *** advantageous combination of high efficiency and diffraction limitation positions the thin-disk regenerative amplifier as a promising solution for a wide range of scientific and industrial applications.

关键词： high efficiency high power picosecond laser regenerative amplifier thin-disk laser