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Optomechanically-induced-transparency cooling of massive mechanical resonators to the quantum ground state

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Science China(Physics,Mechanics & Astronomy) 2015年第5期58卷 46-51页

作者： LIU Yong-Chun XIAO Yun-Feng LUAN Xing-Sheng WONG Chee Wei State Key laboratory for Mesoscopic Physics and School of Physics Peking University Collaborative Innovation Center of Quantum Matter Optical Nanostructures Laboratory Columbia University

Ground state cooling of massive mechanical objects remains a difficult task restricted by the unresolved mechanical sidebands. We propose an optomechanically-induced-transparency cooling scheme to achieve ground state cooling of mechanical motion without the resolved sideband condition in a pure optomechanical system with two mechanical modes coupled to the same optical cavity mode. We show that ground state cooling is achievable for sideband resolution ωm/κ as low as～0.003. This provides a new route for quantum manipulation of massive macroscopic devices and high-precision measurements.

关键词：机械模式透明度冷却基态量子诱导谐振器光学机械系统

Applications of nanostructures in wide-field, label-free super resolution microscopy

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Chinese Physics B 2018年第11期27卷 186-195页

作者：刘小威孟超徐雪初汤明炜庞陈雷杨青 State Key laboratory of Modern optical Instrumentation College of Optical Science and Engineering Zhejiang University

Super resolution imaging capable of resolving details beyond the diffraction limit is highly desired in many scientific and application fields, including bio-medicine, nanomaterial science, and opto-electronic integration. Up to now, many different methods have been proposed, among which wide-field, label-free super resolution microscopy is indispensable due to its good applicability to diverse sample types, large field of view（FOV）, and high imaging speed. In recent years,nanostructures have made a crucial contribution to the wide-field, label-free subdiffraction microscopy, with various working mechanisms and configuration designs. This review summarizes the recent applications of the nanostructures in the wide-field, label-free super resolution microscopy, with the emphasis on the designs of hyperlens with hyperbolic dispersion, microsphere with ＂nano-jets＂, and nanowire ring illumination microscopy based on spatial frequency shift effect. The bottlenecks of the current techniques and possible solutions are also discussed.

关键词： optical microscopy spatial resolution nanowire metamaterials

"Chameleon-like" optical behavior of lanthanide-doped fluoride nanoplates for multilevel anti-counterfeiting applications

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Nano Research 2019年第6期12卷 1417-1422页

作者： Wenwu You Datao Tu Renfu Li Wei Zheng Xueyuan Chen CAS Key laboratory of Design and Assembly of Functional nanostructures and Fujian Key Laboratory of NanomaterialsFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China

Lanthanide-based luminescent anti-counterfeiting materials are widely used in various kinds of products.However,the emission color of traditional lanthanide-based luminescent materials usually remains nearly unaltered upon different excitation lights,which may only work for single-level anti-counterfeiting.Herein,the NaYbF4∶2%Er@NaYF4 core/shell nanoplates (NPs) with "chameleon-like" optical behavior are developed.These NPs display single-band red or green downshifting (DS) emission upon excitation at 377 or 490 nm,respectively.Upon 980 nm excitation,the color of upconversion (UC) emission can be finely tuned from green to yellow,and to red with increasing the excitation power density from 0.1 to 4.0 W/cm^2.The proposed materials readily integrate the advantages of excitation wavelength-dependent DS single-band emissions and sensitive excitation power-dependent UC multicolor emissions in one and the same material,which has never been reported before.Particularly,the proposed NPs exhibit excellent performance as security labels on trademark tag and security ink on painting,thus revealing the great potential of these lanthanide-doped fluoride NPs in multilevel anti-counterfeiting applications.

关键词： lanthanide-doped chameleon-like upconversion downshifting multilevel anti-counterfeiting

Manipulation of plasmonic wavefront and light–matter interaction in metallic nanostructures: A brief review

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Chinese Physics B 2014年第4期23卷 25-40页

作者：李家方李志远 laboratory of optical Physics Institute of Physics Chinese Academy of Sciences

The control and application of surface plasmons （SPs）, is introduced with particular emphasis on the manipulation of the plasmonic wavefront and light-matter interaction in metallic nanostructures. We introduce a direct design methodology called the surface wave holography method and show that it can be readily employed for wave-front shaping of near-infrared light through a subwavelength hole, it can also be used for designing holographic plasmonic lenses for SPs with complex wavefronts in the visible band. We also discuss several issues of light-matter interaction in plasmonic nanostructures. We show theoretically that amplification of SPs can be achieved in metal nanoparticles incorporated with gain media, leading to a giant reduction of surface plasmon resonance linewidth and enhancement of local electric field intensity. We present an all-analytical semiclassical theory to evaluate spaser performance in a plasmonic nanocavity incorporated with gain media described by the four-level atomic model. We experimentally demonstrate amplified spontaneous emission of SP polaritons and their amplification at the interface between a silver film and a polymer film doped with dye molecules. We discuss various aspects of microscopic and macroscopic manipulation of fluorescent radiation from gold nanorod hybrid structures in a system of either a single nanoparticle or an aligned group of nanoparticles. The findings reported and reviewed here could help others explore various approaches and schemes to manipulate plasmonic wavefront and light-matter interaction in metallic nanostructures for potential applications, such as optical displays, information integration, and energy harvesting technologies.

关键词： surface plasmons surface wave holography surface plasmon amplification fluorescence enhance-ment gold nanorods

Enhanced light absorption of silicon in the near-infrared band by designed gold nanostructures

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Chinese Physics B 2014年第4期23卷 551-556页

作者：刘菊钟晓岚李志远 laboratory of optical Physics Institute of Physics Chinese Academy of Sciences

A scheme to enhance near-infrared band absorption of a Si nanoparticle by placing the Si nanoparticle into a designed gold nanostructure is proposed. Three-dimensional （3D） finite-difference time-domain simulations are employed to calcu- late the absorption spectrum of the Si nanostructure and maximize it by generating alternate designs. The results show that in the near-infrared region over 700 nm, the absorption of a pure Si nanoparticle is very low, but when the same nanoparticle is placed within an optimally designed gold nanostructure, its absorption cross section can be enhanced by more than two orders of magnitude in the near-infrared band.

关键词： surface plasmon resonance near-infrared silicon absorption finite-difference time-domain opti-mization

Unraveling the triplet excited-state dynamics of Bi^(3+)in vacancyordered double perovskite Cs_(2)SnCl_(6) nanocrystals

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Nano Research 2022年第7期15卷 6422-6429页

作者： Mengyao Jin Wei Zheng Zhongliang Gong Ping Huang Renfu Li Jin Xu Xingwen Cheng Wei Zhang Xueyuan Chen CAS Key laboratory of Design and Assembly of Functional nanostructures Fujian Key Laboratory of Nanomaterialsand State Key Laboratory of Structural ChemistryFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China College of Chemistry Fuzhou UniversityFuzhou 350116China Fujian Science&Technology Innovation laboratory for Optoelectronic Information of China Fuzhou 350108China

Luminescent metal halides doped with ns^(2-)metal ions such as 6s^(2-)metal Bi^(3+)have aroused reviving interest owing to their outstanding optical properties;however,the origin of the photoluminescence(PL)remains controversial and unclear.Herein,we report a strategy for the controlled synthesis of Bi^(3+)-doped vacancy-ordered double perovskite Cs_(2)SnCl_(6)nanocrystals(NCs)and unravel the triplet excited-state dynamics of Bi^(3+)through temperature-dependent PL and ultrafast femtosecond transient absorption spectroscopies.Owing to the aliovalent Bi^(3+)doping in the spatially confined zero-dimensional(0D)structure of Cs2SnCl6,Bi^(3+)ions experience an enhancive Jahn-Teller distortion in the excited state,which results in intense broadband blue PL originating from the inter-configurational 3P0,1→1S0 transitions of Bi^(3+)at 450 nm,with a large Stokes shift and a quantum yield of 35.2%.Specifically,an unusual thermal-enhanced Jahn-Teller splitting of the excitation band and a remarkable transition of the PL lifetime from ms at 10 K toμs at 300 K were observed,as solid evidence for the isolated Bi^(3+)emission.These findings clarify the controversy about the PL origin in ns^(2-)metal ion-doped lead-free luminescent metal halides,thereby paving the way for exploring their optoelectronic applications.

关键词： bismuth luminescent nanocrystals metal halide excited-state dynamics electron-phonon coupling

Luminescent nano-bioprobes based on NIR dye/lanthanide nanoparticle composites

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Aggregate 2021年第5期2卷 115-131页

作者： Shan Lu Jianxi Ke Xingjun Li Datao Tu Xueyuan Chen CAS Key laboratory of Design and Assembly of Functional nanostructures and Fujian Key Laboratory of NanomaterialsFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFujianChina Fujian Science&Technology Innovation laboratory for Optoelectronic Information of China FujianChina

Near-infrared(NIR)light,which has ignorable tissue scattering/absorption,minimal photodamage,and no autofluorescence interference,is highly favorable for bioapplications.NIR dye and lanthanide-doped nanoparticle(LnNP),as representative NIR-excited luminescence probes,have attracted increasing interest due to their unique optical property and low biological toxicity.Design of luminescence probes based on NIR dye/LnNP nanocomposites cannot only integrate the advantages but also achieve additional functions via regulating internal energy transfer pathways.In this review,we focus on the most recent advances in the development of NIR dye/LnNP nanocomposites as potential bioprobes,which cover from their fundamental photophysics to bioapplications,including energy transfer mechanisms,interface engineering(involving binding interaction,distance,and aggregation as key factors),and their applications for dye-sensitized upconversion/downshifting luminescent bioimaging,detection of biomolecules,and NIR-triggered diagnosis and therapy.Some future prospects and efforts toward this active research field are also envisioned.

关键词： dye sensitization energy transfer interface engineering lanthanide-doped nanoparticle nano-bioprobe NIR dye

Deep Ultraviolet Emission from Water-Soluble SnO_2 Quantum Dots Grown via a Facile "Top-Down" Strategy

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Journal of Materials Science & Technology 2015年第6期31卷 670-673页

作者： Shusheng Pan Wei Lu Zhaoqin Chu Guanghai Li Department of Applied Physics The Hong Kong Polytechnic University Key laboratory of Materials Physics Anhui Key Laboratory of Nanomaterials and NanostructuresInstitute of Solid State PhysicsChinese Academy of Sciences

Tin oxide（SnO2） is a promising wide bandgap semiconductor for next generation ultraviolet（UV） nonpolar optoelectronic devices applications.The development of SnO2-based optoelectronic devices is obsessed by its low exciton emission efficiency.In this study,quantum confined SnO2nanocrystals have been fabricated via pulsed laser ablation in water.The SnO2quantum dots（QDs） possess high performance exciton emission at 297-300 nm light in water.The exciton emission intensity and wavelength can be slightly tuned by laser pulse energy and irradiation time.optical gain has been observed in SnO2QDs.Therefore,SnO2QDs can be a promising luminescence material for the realization of deep UV nanoemitter and lasing devices.

关键词： SnO2 Wide bandgap semiconductor Deep ultraviolet P

MoS_(2)core-shell nanoparticles prepared through liquid-phase ablation and light exfoliation of femtosecond laser for chemical sensing

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Science China(Technological Sciences) 2023年第3期66卷 853-862页

作者： ZUO Pei JIANG Lan LI Xin TIAN MengYao YUAN YongJiu HAN WeiNa MA Le HU LiFei HE ZhiCong LI Fang School of Mechanical and Electrical Engineering Hubei Key Laboratory of Optical Information and Pattern RecognitionSchool of Optical Information and Energy EngineeringWuhan Institute of TechnologyWuhan 430073China Laser Micro/Nano Fabrication laboratory School of Mechanical EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing Institute of Technology Chongqing Innovation Center Chongqing 401120China

Molybdenum disulfide(MoS_(2))-based nanostructures are highly desirable for applications such as chemical and biological sensing,photo/electrochemical catalysis,and energy storage due to their unique physical and chemical properties.In this work,MoS_(2)core-shell nanoparticles were first prepared through the liquid-phase processing of bulk MoS2by a femtosecond laser.The core of prepared nanoparticles was incompletely and weakly crystalline MoS_(2);the shell of prepared nanoparticles was highly crystalline MoS_(2),which wrapped around the core layer by layer.The femtosecond laser simultaneously achieved liquid-phase ablation and light exfoliation.The formation mechanism of the core-shell nanoparticles is to prepare the nanonuclei first by laser liquid-phase ablation and then the nanosheets by light exfoliation;the nanosheets will wrap the nanonuclei layer by layer through van der Waals forces to form core-shell nanoparticles.The MoS_(2)core-shell nanoparticles,because of Mo-S bond breakage and recombination,have high chemical activity for chemical catalysis.Afterward,the nanoparticles were used as a reducing agent to directly prepare three-dimensional(3D)Au-MoS_(2)micro/nanostructures,which were applied as surface-enhanced Raman spectroscopy(SERS)substrates to explore chemical sensing activity.The ultrahigh enhancement factor(1.06×10^(11)),ultralow detection limit(10-13M),and good SERS adaptability demonstrate highly sensitive SERS activity,great ability of ultralow concentration detection,and ability to detect diverse analytes,respectively.This work reveals the tremendous potential of 3D Au-MoS_(2)composite structures as excellent SERS substrates for chemical and biological sensing.

关键词： MoS_(2)core-shell nanoparticle femtosecond laser liquid-phase ablation light exfoliation 3D Au-MoS_(2)composite structure chemical sensing