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Chinese Chemical Letters 2025年第2期36卷 360-365页

作者： Yi Zhou Wei Zhang Rong Fu Jiaxin Dong Yuxuan Liu Zihang Song Han Han Kang Cai college of Chemistry Nankai University Department of Chemistry Northwestern University Department of Chemistry The University of Hong Kong

Chiral coordination molecular cages/capsules with discrete nanoconfined chiral cavities demonstrate significant potential applications across various fields. In this study, we utilized Tr?ger's base as the building block to design and synthesize two pairs of enantiopure ligands. These ligands were then self-assembled with Pd(II) ions through chiral self-sorting coordination, resulting in the formation of two pairs of homochiral M2L4-type coordination molecular capsules. Notably, due to differences in the substitution positions on the Tr?ger's base, these two pairs of enantiomeric coordination molecular capsules exhibited distinct levels of cavity closures, cavity sizes, and host-guest recognition properties. This research offers valuable insights into the construction of novel chiral molecular capsules and the regulation of confined cavities.

关键词： Chirality Host-guest recognition Metal-organic capsule Self-sorting Tröger's base

Effects of the extrusion parameters on microstructure,texture and room temperature mechanical properties of extruded Mg-2.49Nd-1.82Gd-0.2Zn-0.2Zr alloy

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 136-146页

作者： Chenjin Zhang Guangyu Yang Lei Xiao Zhiyong Kan Jing Guo Qiang Li Wanqi Jie State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an 710072China college of Materials Science and Engineering Fuzhou UniversityFuzhou 350108China college of Chemistry and Environmental Science Qujing Normal UniversityQujing 655011China

Microstructure,texture,and mechanical properties of the extruded Mg-2.49Nd-1.82Gd-0.2Zn-0.2Zr alloy were investigated at different extrusion temperatures(260 and 320℃),extrusion ratios(10:1,15:1,and 30:1),and extrusion speeds(3 and 6 mm/s).The experimental results exhibited that the grain sizes after extrusion were much finer than that of the homogenized alloy,and the second phase showed streamline distribution along the extrusion direction(ED).With extrusion temperature increased from 260 to 320℃,the microstructure,texture,and mechanical properties of alloys changed *** dynamic recrystallization(DRX)degree and grain sizes enhanced as the extrusion ratio increased from 10:1 to 30:1,and the strength gradually decreased but elongation(EL)*** the extrusion speed increased from 3 to 6 mm/s,the grain sizes and DRX degree increased significantly,and the samples presented the typical-rare-earth(RE)*** alloy extruded at 260℃ with extrusion ratio of 10:1 and extrusion speed of 3 mm/s showed the tensile yield strength(TYS)of 213 MPa and EL of 30.6%.After quantitatively analyzing the contribution of strengthening mechanisms,it was found that the grain boundary strengthening and dislocation strengthening played major roles among strengthening *** results provide some guidelines for enlarging the industrial application of extruded Mg-RE alloy.

关键词： Mg-rare earth alloys extrusion temperature extrusion ratio extrusion speed strengthening mechanisms

The resonance effect for the CP asymmetry associated with the process ω→π+π-π0

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Chinese Physics C 2025年第02期 11-22页

作者：原喜亮吕刚王娜王超 Institute of Theoretical Physics College of PhysicsHenan University of Technology School of Ecology and Environment Northwestern Polytechnical University

The direct CP asymmetry in the weak decay process of hadrons is commonly attributed to the weak phase of the CKM matrix and the indeterminate strong *** propose a method to generate a significant phase difference through the interference between ρ and ω mesons,taking into account the G-parity allowed decay process of ω→π+π-π0and the G-parity-suppressed decay process of ρ0→π+π-π0in B meson *** interference can lead to notable changes in the CP asymmetry within the interference ***,we calculate the integral results for different phase space regions of the four-body decay *** hope that our work provides valuable theoretical guidance for future experimental investigations on CP asymmetry in these decays.

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Current development and future prospects of multi-target assignment problem:A bibliometric analysis review

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Defence Technology(防务技术) 2025年第1期43卷 44-59页

作者： Shuangxi Liu Zehuai Lin Wei Huang Binbin Yan college of Aerospace Science and Engineering National University of Defense TechnologyChangsha410073China Hypersonic Technology Laboratory National University of Defense of TechnologyChangsha410073China School of Astronautics Northwestern Polytechnical UniversityXi'an710072China

The multi-target assignment(MTA)problem,a crucial challenge in command control,mission planning,and a fundamental research focus in military operations,has garnered significant attention over the *** studied across various domains such as land,sea,air,space,and electronics,the MTA problem has led to the emergence of numerous models and *** delve deeper into this field,this paper starts by conducting a bibliometric analysis on 463 Scopus database papers using CiteSpace *** analysis includes examining keyword clustering,co-occurrence,and burst,with visual representations of the *** this,the paper provides an overview of current classification and modeling techniques for addressing the MTA problem,distinguishing between static multi-target assignment(SMTA)and dynamic multi-target assignment(DMTA).Subsequently,existing solution algorithms for the MTA problem are reviewed,generally falling into three categories:exact algorithms,heuristic algorithms,and machine learning ***,a development framework is proposed based on the"HIGH"model(high-speed,integrated,great,harmonious)to guide future research and intelligent weapon system development concerning the MTA *** framework emphasizes application scenarios,modeling mechanisms,solution algorithms,and system efficiency to offer a roadmap for future exploration in this area.

关键词： Multi-target assignment Offensive and defensive confrontation Cooperative operation Modeling mechanism Solution algorithm CiteSpace analysis

Sulfur atom occupying surface oxygen vacancy to boost the charge transfer and stability for aqueous Bi2O3 electrode

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Journal of Energy Chemistry 2025年第2期101卷 751-759页

作者： Guangmin Yang Jianyan Lin Guanwu Li Tian Li Dong Wang Weitao Zheng college of Physics Changchun Normal University School of Materials Science and Engineering Northwestern Polytechnical University Key Laboratory of Automobile Materials of MOE School of Materials Science and Engineering and Jilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy Materials Jilin University

Oxygen vacancies（Ov） within metal oxide electrodes can enhance mass/charge transfer dynamics in energy storage ***,construction of surface Ovoften leads to instability in electrode structure and irreversible electrochemical reactions,posing a significant *** overcome these challenges,atomic heterostructures are employed to address the structural instability and enhance the mass/charge transfer dynamics associated with phase conversion mechanism in aqueous electrodes,Herein,we introduce an atomic S-Bi2O3heterostructure(sulfur（S） anchoring on the surface Ovof Bi2O3).The integration of S within Bi2O3lattice matrix triggers a charge imbala nce at the heterointerfaces,ultimately resulting in the creation of a built-in electric field（BEF）.Thus,the BEF attracts OH-ions to be adsorbed onto Bi within the regions of high electron cloud overlap in S-Bi2O3,facilitating highly efficient charge ***,the anchored S plays a pivotal role in preserving structural integrity,thus effectively stabilizing the phase conversion reaction of *** a result,the S-Bi2O3electrode achieves72.3 mA h g-1at 10 A g-1as well as high-capacity retention of 81.9% after 1600 *** innovative SBi2O3design presents a groundbreaking approach for fabricating electrodes that exhibit efficient and stable mass and charge transfer ***,it enhances our understanding of the underlying reaction mechanism within energy storage electrodes.

关键词： Anchoring effect Atomic heterostructure Charge/mass transfer Oxygen vavancy Structural integrity

Combining slow-release fertilizer and plastic film mulching reduced the carbon footprint and enhanced maize yield on the Loess Plateau

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Journal of Environmental Sciences 2025年第1期147卷 359-369页

作者： Xiaoqing Han Pengfei Dang Lechen Liao Fangqi Song Miaomiao Zhang Maoxue Zhang Guoqing Li Shuyue Wen Ning Yang Xiping Pan Xiaofan Wang WenWang Xiaoliang Qin Charles O.Joseph Kadambot H.M.Siddique college of Agronomy Key Laboratory of Crop Physi-ecology and Tillage Science in Northwestern Loess PlateauNorthwest A&F UniversityYanglingShaanxi 712100China Department of Crop Sciences and Beekeeping Technology college of Agricultural Sciences and Food Technology University of Dar es SalaamMwalimu Julius Nyerere Mlimani CampusP.O.Box 35091Dar es SalaamTanzania college of Life Science Yulin UniversityChongwen Road No.4YulinShaanxi719000China The UWA Institute of Agriculture and School of Agriculture&Environment The University of Western AustraliaPerth WA 6001Australia

Agricultural practices significantly contribute to greenhouse gas(GHG)emissions,necessitating cleaner production technologies to reduce environmental pressure and achieve sustainable maize *** film mulching is commonly used in the Loess Plateau *** slow-release fertilizers as a replacement for urea within this practice can reduce nitrogen losses and enhance crop *** these techniques represents a novel agricultural approach in semi-arid ***,the impact of this integration on soil carbon storage(SOCS),carbon footprint(CF),and economic benefits has received limited research ***,we conducted an eight-year study(2015-2022)in the semi-arid northwestern region to quantify the effects of four treatments[urea supplied without plastic film mulching(CK-U),slow-release fertilizer supplied without plastic film mulching(CK-S),urea supplied with plastic film mulching(PM-U),and slow-release fertilizer supplied with plastic film mulching(PM-S)]on soil fertility,economic and environmental *** results revealed that nitrogen fertilizer was the primary contributor to total GHG emissions(≥71.97%).Compared to other treatments,PM-S increased average grain yield by 12.01%-37.89%,water use efficiency by 9.19%-23.33%,nitrogen accumulation by 27.07%-66.19%,and net return by 6.21%-29.57%.Furthermore,PM-S decreased CF by 12.87%-44.31%and CF per net return by 14.25%-41.16%.After eight years,PM-S increased SOCS(0-40 cm)by 2.46%,while PM-U decreased it by 7.09%.These findings highlight the positive effects of PM-S on surface soil fertility,economic gains,and environmental benefits in spring maize production on the Loess Plateau,underscoring its potential for widespread adoption and application.

关键词： Plastic film mulching Slow-release fertilizer Maize grain yield Carbon footprint Economic benefits

Utilizing electronic assisted enhancement:An innovative approach for studying the thermal decomposition and combustion of ionic liquids

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Defence Technology(防务技术) 2025年第2期44卷 179-189页

作者： Cailing Zhang Yutao Wang Baiquan Chen Zhenguo Pang Hongqi Nie Quan Zhu Peijin Liu Wei He college of Chemical Engineering Sichuan UniversityChengdu 610065China School of Aeronautics and Astronautics Sichuan UniversityChengdu 610065China School of Environmental and Safety Engineering North University of ChinaTaiyuan 030051China Science and Technology on Combustion Internal Flow and Thermostructure LaboratoryNorthwestern Polytechnical UniversityXi'an 710072China

Flammable ionic liquids exhibit high conductivity and a broad electrochemical window,enabling the generation of combustible gases for combustion via electrochemical decomposition and thermal *** characteristic holds significant implications in the realm of novel satellite *** a fraction of the electrical energy into energetic ionic liquid fuels,the thermal decomposition process is facilitated by reducing the apparent activation energy required,and electrical energy can trigger the electrochemical decomposition of ionic liquids,presenting a promising approach to enhance combustion efficiency and energy *** study applied an external voltage during the thermal decomposition of 1-ethyl-3-methylimidazole nitrate([EMIm]NO_(3)),revealing the effective alteration of the activation energy of[EMIm]NO_(3).The pyrolysis,electrochemical decomposition,and electron assisted enhancement products were identified through Thermogravimetry-Differential scanning calorimetry-Fourier transform infrared-Mass spectrometry(TG-DSC-FTIR-MS)and gas chromatography(GC)analyses,elucidating the degradation mechanism of[EMIm]NO_(3).Furthermore,an external voltage was introduced during the combustion of[EMIm]NO_(3),demonstrating the impact of voltage on the combustion process.

关键词： Flammable ionic liquids Kinetic methods Electron assisted enhanced thermal decomposition Electron assisted enhanced combustion

Deciphering theαrelaxation and the anelastic-to-plastic transition in the deep glassy state

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Science China(Physics,Mechanics & Astronomy) 2025年第3期68卷 131-138页

作者： Qi Hao Guanghui Xing Eloi Pineda Claudio Fusco Laurent Chazeau Jean-Marc Pelletier Yunjiang Wang Yong Yang Jichao Qiao School of Mechanics Civil Engineering and ArchitectureNorthwestern Polytechnical UniversityXi’an710072China Department of Physics Institute of Energy TechnologiesUniversitat Politècnica de CatalunyaBarcelona08019Spain Univ Lyon INSA LyonUniversitéClaude Bernard Lyon 1CNRSMATEISUMR5510Villeurbanne69621France State Key Laboratory of Nonlinear Mechanics Institute of MechanicsChinese Academy of SciencesBeijing100190China School of Engineering Science University of Chinese Academy of SciencesBeijing100049China Department of Mechanical Engineering College of EngineeringCity University of Hong KongHong Kong999077China Department of Materials Science and Engineering College of EngineeringCity University of Hong KongHong Kong999077China State Key Laboratory of Clean and Efficient Turbomachinery Power Equipment Northwestern Polytechnical UniversityXi’an710072China Key Laboratory of Aircraft Structural Integrity Ministry of Industry and Information TechnologyXi’an710072China

In contrast to their conventional crystalline counterparts,amorphous solids exhibit diverse dynamic relaxation mechanisms under external *** challenge to understanding their behavior lies in unifying microscopic dynamics,relaxation,and macroscopic *** study establishes a potential link by quantifying the characteristic time of the anelastic-to-plastic transition through dynamic mechanical relaxation and stress relaxation tests across a wide temperature range in both the supercooled liquid and the glassy *** is found that the stress relaxation time in the glassy solids follows an Arrhenius relationship,aligning with the mainαrelaxation time,and unveils a finding:αrelaxation continues to govern deformation even below the glass transition,challenging previous assumptions of the role of secondaryβrelaxation.A hierarchically constrained atomic dynamics model rationalizes the temperature dependence ofαrelaxation and the transition fromβtoαrelaxation,also providing evidence that the stretched exponent in the Kohlrausch-Williams-Watts equation can serve as an order *** work highlights the role ofαrelaxation in the glassy state and contributes to elucidating the potential correlation between relaxation and deformation in amorphous materials.

关键词： dynamic relaxation nonelastic deformation metallic glasses aging

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DNA2 knockout aggravates cerebral ischemia/reperfusion injury by reducing postsynaptic Homer1a

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Zoological Research 2025年第01期 87-102页

作者： Ting Ma Yu-Meng Li Peng-Yu Ren Shi-Quan Wang Xiang-Long Liu Wen-Bo Lv Wu-Gang Hou Wen-Qiang Zuo Wei-Qiang Lin Jian Sima An-Qi Geng Laboratory of Aging Neuroscience and Neuropharmacology School of Basic Medicine and Clinical Pharmacy China Pharmaceutical University Research & Development Institute of northwestern Polytechnical University in Shenzhen Xi'an Key Laboratory of Stem Cell and Regenerative Medicine Xi'an Key Laboratory of Special Medicine and Health Engineering Institute of Medical Research Northwestern Polytechnical University Sanhang Institute for Brain Science and Technology Northwestern Polytechnical University Department of Anesthesiology and Perioperative Medicine Xijing Hospital Fourth Military Medical University college of Pharmacy Shaanxi University of Chinese Medicine International Institutes of Medicine Fourth Affiliated Hospital School of Medicine Zhejiang University

DNA2, a multifunctional enzyme with structure-specific nuclease, 5'-to-3' helicase, and DNA-dependent ATPase activities, plays a pivotal role in the cellular response to DNA damage. However, its involvement in cerebral ischemia/reperfusion(I/R) injury remains to be *** study investigated the involvement of DNA2 in cerebral I/R injury using conditional knockout(cKO) mice(Nestin-Cre) subjected to middle cerebral artery occlusion(MCAO), an established model of cerebral I/R. Results demonstrated a gradual up-regulation of DNA2 expression,peaking at 72 h post-MCAO. Notably, DNA2 cKO mice exhibited more pronounced brain injury, neurological deficits, and neuronal apoptosis within the penumbra following MCAO. Additionally, DNA2 expression was elevated in an oxygen-glucose deprivation/reoxygenation(OGD/R) cell culture model, and DNA2 knockdown(KD)exacerbated neuronal apoptosis and oxidative *** analysis of ischemic penumbra tissues via RNA sequencing revealed significant down-regulation of Homer1 in DNA2 cKO mice. Furthermore, in vitro experiments demonstrated that overexpression of Homer1a ameliorated DNA2 KD-induced neuronal apoptosis. Collectively, these findings demonstrate that DNA2 deficiency exacerbates cerebral I/R injury through the down-regulation of Homer1a, highlighting a novel regulatory axis in ischemic neuroprotection.

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Sex differences in aging and injured brain

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Neural Regeneration Research 2025年第10期20卷 2901-2902页

作者： Jordan N.Williamson Yuan Yang University of Illinois Urbana-Champaign Grainger College of EngineeringDepartment of BioengineeringUrbanaILUSA Carle Foundation Hospital Stephenson Family Clinical Research InstituteClinical Imaging Research CenterUrbanaILUSA University of Illinois Urbana-Champaign Beckman Institute for Advanced Science and TechnologyUrbanaILUSA northwestern University Department of Physical Therapy and Human Movement SciencesChicagoILUSA

Background:The prevalence,age of onset,and symptomatology of traumatic brain injury,stroke,and neurodegenerative diseases(such as Alzheimer’s disease(AD),Parkinson’s disease,amyotrophic lateral sclerosis,and Huntington’s disease)differ substantially between males and *** higher prevalence of these brain disorders has been attributed to females having a greater longevity compared with *** one of the greatest risk factors of acquired brain injury(such as stroke,traumatic brain injury caused by fall)and neurodegenerative disease is age.

关键词： Huntington prevalence traumatic