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Long-term functional maintenance of primary hepatocytes in vitro using macroporous hydrogels engineered through liquid-liquid phase separation

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Nano Research 2024年第3期17卷 1725-1736页

作者： Yang Sun Sheng Yin Jian Cui Zhongxia Wang Yueying Han Ding Ma Shuo Wang Junhua Wu Yi Cao Chunping Jiang Xiaosong Gu Jinan Microecological Biomedicine Shandong laboratory Jinan 250021China Collaborative Innovation Center of Advanced Microstructures National Laboratory of Solid State MicrostructureKey Laboratory of Intelligent Optical Sensing and ManipulationMinistry of EducationDepartment of PhysicsNanjing UniversityNanjing 210093China department of Hepatobiliary Surgery The Affiliated Drum Tower Hospital of Nanjing University Medical SchoolNanjing 210093China national Institute of Healthcare Data Science at Nanjing University Nanjing UniversityNanjing 210093China

Preserving the functionality of hepatocytes in vitro poses a significant challenge in liver tissue engineering and bioartificial liver,as these cells rapidly lose their metabolic and functional characteristics after *** by the macroporous structures found in native liver tissues,here we develop synthetic hydrogel scaffolds that closely mimic the liver’s structural organization through the phase separation between polyethylene glycol(PEG)and *** hydrogels exhibit interconnected macroporous structures and appropriate mechanical properties,providing an optimal microenvironment conducive to hepatocyte adhesion and the formation of sizable *** to two-dimensional hepatocyte cultures,enhanced functionalities of hepatocytes cultured in our macroporous hydrogels were observed for 14 days,as evidenced by quantitative reverse-transcription–polymerase chain reactions(qRT-PCR),immunofluorescence,and enzyme linked immunosorbent assay(ELISA)*** sequencing data further confirmed the establishment of cell–cell interactions among hepatocytes when cultured in our ***,these hepatocytes maintained a protein expression lineage that closely resembled freshly isolated hepatocytes,particularly in the Notch and tumor necrosis factor(TNF)signaling *** results suggest that the macroporous hydrogels are attractive scaffolds for liver tissue engineering.

关键词： liver tissue engineering phase separation hepatocytes macroporous hydrogel

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Three-Wave Mixing of Dipole Solitons in One-Dimensional Quasi-Phase-Matched Nonlinear Crystals

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Chinese physics Letters 2024年第1期41卷 25-33页

作者：郭宇欣徐晓喜陈招拼周延桂刘彬和河向黎永耀谢嘉宁 School of physics and Optoelectronic Engineering Foshan UniversityFoshan 528000China physics department and solid-state Institute TechnionHaifa 32000Israel Guangdong-Hong Kong-Macao Joint laboratory for Intelligent Micro-Nano Optoelectronic Technology School of Physics and Optoelectronic EngineeringFoshan UniversityFoshan 528000China

A quasi-phase-matched technique is introduced for soliton transmission in a quadratic[χ^((2))]nonlinear crystal to realize the stable transmission of dipole solitons in a one-dimensional space under three-wave *** report four types of solitons as dipole solitons with distances between their bimodal peaks that can be laid out in different *** study three cases of these solitons:spaced three stripes apart,one stripe apart,and confined to the same *** the case of three stripes apart,all four types have stable results,but for the case of one stripe apart,stable solutions can only be found atω_(1)=ω_(2),and for the condition of dipole solitons confined to one stripe,stable solutions exist only for Type1 and Type3 atω_(1)=ω_(2).The stability of the soliton solution is solved and verified using the imaginary time propagation method and real-time transfer propagation,and soliton solutions are shown to exist in the multistability *** addition,the relations of the transportation characteristics of the dipole soliton and the modulation parameters are numerically ***,possible approaches for the experimental realization of the solitons are outlined.

关键词： soliton solitons dipole

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Embedded Majorana islands

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Science China(physics,Mechanics & Astronomy) 2024年第9期67卷 154-164页

作者： Jin-Xing Hou Alex Weststrom Rui Wang Wen-Li Yang Jian Li Institute of Modern physics Northwest UniversityXi’an 710127China department of physics School of ScienceWestlake UniversityHangzhou 310030China Shaanxi Key laboratory for Theoretical physics Frontiers Xi’an 710127China Institute of Natural Sciences Westlake Institute for Advanced StudyHangzhou 310024China national laboratory of solid state Microstructures and department of physics Nanjing UniversityNanjing 210093China Collaborative Innovation Center for Advanced Microstructures Nanjing 210093China Peng Huanwu Center for Fundamental Theory Xi’an 710127China

Mesoscopic superconducting islands hosting Majorana zero modes(MZMs),or Majorana islands in short,offer a prototype of topological *** this work we investigate theoretically the model of a generic Majorana island tunneling-coupled to a singlepiece metallic substrate,hence an embedded Majorana *** show the crucial consequences of an interplay between the topological ground states nonlocally addressed by the MZMs and the metallic bath with coherent electron propagation:on the one hand,the topological degeneracy on the Majorana island can be preserved,by virtue of the particle-hole symmetry,despite the apparent bath-induced coupling between MZMs;on the other hand,the electronic interference in the metallic bath may lead to profound alterations to the renormalization group behavior of the hybrid system towards low energy/temperature compared with conventional Kondo *** work serves to establish the model of embedded Majorana islands as an experimentally relevant and theoretically intriguing problem particularly in the direction of topological quantum computation.

关键词： topological quantum computation Majorana zero modes topological qubit mesoscopic superconductor topological Kondo effect

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Fully polarized Compton scattering in plane waves and its polarization transfer

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Matter and Radiation at Extremes 2024年第3期9卷 45-56页

作者： Suo Tang Yu Xin Meng Wen Mamat Ali Bake Baisong Xie College of physics and Optoelectronic Engineering Ocean University of ChinaQingdaoShandong 266100China department of physics Hubei UniversityWuhan 430062China Xinjiang Key laboratory of solid state physics and Devices School of Physics Science and TechnologyXinjiang UniversityUrumqi 830017China Key laboratory of Beam Technology of the Ministry of Education and College of Nuclear Science and TechnologyBeijing Normal UniversityBeijing 100875China

Fully polarized Compton scattering from a beam of spin-polarized electrons is investigated in plane-wave backgrounds in a broad intensity region from the perturbative to the nonperturbative *** the perturbative regime,polarized linear Compton scattering is considered for investigating polarization transfer from a single laser photon to a scattered photon,and in the high-intensity region,the polarized locally monochromatic approximation and locally constant field approximation are established and are employed to study polarization transfer from an incoming electron to a scattered *** numerical results suggest an appreciable improvement of about 10%in the scattering probability in the intermediate-intensity region if the electron’s longitudinal spin is parallel to the laser *** longitudinal spin of the incoming electron can be transferred to the scattered photon with an efficiency that increases with laser intensity and collisional *** collision between an optical laser with frequency1 eV and a 10 GeV electron,this polarization transfer efficiency can increase from about 20%in the perturbative regime to about 50%in the nonperturbative regime for scattered photons with relatively high energy.

关键词： polarized scattered transfer

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Finite barrier bound state

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Light(Science & Applications) 2024年第4期13卷 664-671页

作者： Tao Liu Kai Bai Yicheng Zhang Duanduan Wan Yun Lai C.T.Chan Meng Xiao Key laboratory of Artificial Micro-and Nano-structures of Ministry of Education and School of physics and Technology Wuhan University430072 WuhanChina. national laboratory of solid state Microstructures School of Physicsand Collaborative Innovation Center of Advanced MicrostructuresNanjing University210093 NanjingChina. department of physics The Hong Kong University of Science and TechnologyClear Water BayKowloon999077Hong KongChina. Wuhan Institute of Quantum Technology 430206 WuhanChina

A boundary mode localized on one side of a finite-size lattice can tunnel to the opposite side which results in unwanted *** wisdom tells that the tunneling probability decays exponentially with the size of the system which thus requires many lattice sites before eventually becoming negligibly *** we show that the tunneling probability for some boundary modes can apparently vanish at specific ***,similar to bound states in the continuum,a boundary mode can be completely trapped within very few lattice sites where the bulk bandgap is not even *** intriguingly,the number of trapped states equals the number of lattice sites along the normal direction of the *** provide two configurations and validate the existence of this peculiar finite barrier-bound state experimentally in a dielectric photonic crystal at microwave *** work offers extreme flexibility in tuning the coupling between localized states and channels as well as a new mechanism that facilitates unprecedented manipulation of light.

关键词： boundary state eventually

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Ferromagnetism and insulating behavior with a logarithmic temperature dependence of resistivity in Pb_(10-x)Cux(PO_(4))_(6)O

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Science China(physics,Mechanics & Astronomy) 2024年第1期67卷 106-111页

作者： Yuhang Zhang Cong Liu Xiyu Zhu Hai-Hu Wen Center for Superconducting physics and Materials National Laboratory of Solid State Microstructures and Department of PhysicsNational Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China

Recent claim of discovering above-room-temperature superconductivity(Tc≈400 K)at ambient pressure in copper doped apatite Pb10(PO_(4))_(6)O has stimulated world-wide enthusiasm and impulse of motion.A lot of follow-up works have been carried out with controversial *** check whether superconductivity is really present or absent in the material,we need samples which should have a rather pure phase of Pb_(10-x)Cux(PO_(4))_(6)*** we report the characterization results from the Pb_(10-x)Cux(PO_(4))_(6)O with a fraction of about 97 wt.%inferred from the fitting to the X-ray diffraction pattern,if assuming Cu2S as the only *** resistivity measurements show that it is a semiconductor characterized roughly by a ln(1/T)temperature dependence in wide temperature region without trace of *** measurements show that it has a general ferromagnetic signal with a weak superparamagnetic *** grains of the sample show clear interactions with a Nb Fe B *** detected Cu concentration is much lower than the expected nominal *** results show the absence of metallicity and superconductivity in Pb_(10-x)Cux(PO_(4))_(6)O at ambient pressure,and suggest the presence of strong correlation effect.

关键词： superconductivity Pb10(PO4)6O ferromagnetic correlation effect

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Tailoring Electrode–Electrolyte Interface Using an Electron-Deficient Borate-Based Additive in MgTFSI_(2)-MgCl_(2)/DME Electrolyte for Rechargeable Magnesium Batteries

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Energy & Environmental Materials 2024年第6期7卷 167-175页

作者： Haiyan Fan Xinxin Zhang Jianhua Xiao Wenjie Chen Qiyuan Lin Zi Shyun Ng Yitao Lin Yi Su Ludi Pan Yipeng Su Shuaiyang Ren Haowen Liu Xuanzhang Li Yuegang Zhang state Key laboratory of Low Dimensional Quantum physics and department of physics Tsinghua UniversityBeijing 100084China Frontier Science Center for Quantum Information Beijing 100084China

Rechargeable magnesium metal batteries need an electrolyte that forms a stable and ionically conductive solid electrolyte interphase(SEI)on the ***,we used molecular dynamic simulation,density functional theory calculation,and X-ray photoelectron spectroscopy analysis to investigate the solvation structures and SEI compositions in electrolytes consisting of dual-salts,magnesium bis(trifluoromethanesulfonyl)imide(MgTFSI_(2)),and MgCl_(2),with different additives in 1,2-dimethoxyethane(DME)*** found that the formed[Mg_(3)(μ-Cl)_(4)(DME)mTFSI_(2)](m=3,5)inner-shell solvation clusters in MgTFSI_(2)-MgCl_(2)/DME electrolyte could easily decompose and form a MgO-and MgF_(2)-rich *** electron-rich inorganic species in the SEI,especially MgF_(2),turned out to be detrimental for Mg plating/*** reduce the MgF_(2)and MgO contents in SEI,we introduce an electron-deficient tri(2,2,2-trifluoroethyl)borate(TFEB)additive in the ***//Mg cells using the MgTFSI_(2)-MgCl_(2)/DME-TFEB electrolyte could cycle stably for over 400 h with a small polarization voltage of~150 *** with the presence of 800 ppm H_(2)O,the electrolyte with TFEB additive could still preserve its good electrochemical *** optimized electrolyte also enabled stable cycling and high-rate capability for Mg//Mo6S8 and Mg//CuS full cells,showing great potential for future applications.

关键词： electrolyte additives interfacial chemistry magnesium metal batteries solvation structure

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High Density 3D Carbon Tube Nanoarray Electrode Boosting the Capacitance of Filter Capacitor

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Nano-Micro Letters 2024年第11期16卷 242-254页

作者： Gan Chen Fangming Han Huachun Ma Pei Li Ziyan Zhou Pengxiang Wang Xiaoyan Li Guowen Meng Bingqing Wei Key laboratory of Materials physics and Anhui Key Laboratory of Nanomaterials and NanotechnologyInstitute of Solid State PhysicsHFIPSChinese Academy of SciencesHefei 230031People’s Republic of China department of Materials Science and Engineering University of Science and Technology of ChinaHefei 230026People’s Republic of China department of Mechanical Engineering University of DelawareNewarkDE 19716USA Mechano‑X Institute Applied Mechanics LaboratoryDepartment of Engineering MechanicsTsinghua UniversityBeijing 100084People’s Republic of China

Electric double-layer capacitors(EDLCs)with fast frequency response are regarded as small-scale alternatives to the commercial bulky aluminum electrolytic *** carbon-based nanoarray electrodes with precise alignment and smooth ion channels is crucial for enhancing EDLCs’***,controlling the density of macropore-dominated nanoarray electrodes poses challenges in boosting the capacitance of line-filtering ***,a simple technique to finely adjust the vertical-pore diameter and inter-spacing in three-dimensional nanoporous anodic aluminum oxide(3D-AAO)template is achieved,and 3D compactly arranged carbon tube(3D-CACT)nanoarrays are created as electrodes for symmetrical EDLCs using nanoporous 3D-AAO template-assisted chemical vapor deposition of *** 3D-CACT electrodes demonstrate a high surface area of 253.0 m^(2) g^(−1),a D/G band intensity ratio of 0.94,and a C/O atomic ratio of *** a result,the high-density 3D-CT nanoarray-based sandwich-type EDLCs demonstrate a record high specific areal capacitance of 3.23 mF cm^(-2) at 120 Hz and exceptional fast frequency response due to the vertically aligned and highly ordered nanoarray of closely packed CT *** 3D-CT nanoarray electrode-based EDLCs could serve as line filters in integrated circuits,aiding power system miniaturization.

关键词： Compactly arranged Three-dimensional carbon tube nanoarray Dimensional carbon tube nanoarray Fast frequency response Electric double-layer capacitors Layer capacitors AC line-filtering Filtering

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Iron oxide/CNT-based artificial nacre for electromagnetic interference shielding

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Nano Research 2024年第7期17卷 6560-6566页

作者： Cheng-Xin Yu Yu-Feng Meng Bo Yang Jun Pang Xiang-Sen Meng Zi-Ye Zhao Qing-Yue Wang Li-Bo Mao Zhi-Kun Wu Shu-Hong Yu Institute of Physical Science and Information Technology Anhui UniversityHefei 230601China Key laboratory of Materials physics Anhui Key Laboratory of Nanomaterials and NanotechnologyCAS Center for Excellence in NanoscienceInstitute of Solid State PhysicsHFIPSChinese Academy of SciencesHefei 230031China department of Chemistry New Cornerstone Science LaboratoryInstitute of Biomimetic Materials&ChemistryAnhui Engineering Laboratory of Biomimetic MaterialsDivision of Nanomaterials&ChemistryHefei National Research Center for Physical Sciences at the MicroscaleUniversity of Science and Technology of ChinaHefei 230026China

Biological structural materials,despite consisting of limited kinds of compounds,display multifunctionalities due to their complex hierarchical *** some biomimetic strategies have been applied in artificial materials to enhance their mechanical stability,the simultaneous optimization of other functions along with the mechanical properties via biomimetic designs has not been thoroughly ***,iron oxide/carbon nanotube(CNT)-based artificial nacre with both improved mechanical and electromagnetic interference(EMI)shielding performance is fabricated via the mineralization of Fe_(3)O_(4)onto a CNTincorporated *** micro-and nano-structures of the artificial nacre are similar to those of natural nacre,which in turn improves its mechanical *** alternating electromagnetic wave-reflective CNT layers and the wave-absorptive iron oxide layers can improve the multiple reflections of the waves on the surfaces of the reflection layers,which then allows sufficient interactions between the waves and the absorption ***,compared with the reflection-dependent EMI-shielding of the non-structured material,the artificial nacre exhibits strong absorption-dependent shielding behavior even with a very low content of wave-absorptive *** to the high mechanical stability,the shielding effectiveness of the artificial nacre that deeply cut by a blade is still maintained at approximately 70%−96%depending on the incident wave *** present work provides a new way for designing structural materials with concurrently enhanced mechanical and functional properties,and a path to combine structural design and intrinsic properties of specific materials via a biomimetic strategy.

关键词： artificial nacre electromagnetic interference shielding biomineralization biomimetic material hierarchical structure

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Mixed‑Dimensional Assembly Strategy to Construct Reduced Graphene Oxide/Carbon Foams Heterostructures for Microwave Absorption,Anti‑Corrosion and Thermal Insulation

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Nano-Micro Letters 2024年第11期16卷 1-18页

作者： Beibei Zhan Yunpeng Qu Xiaosi Qi Junfei Ding Jiao‑jing Shao Xiu Gong Jing‑Liang Yang Yanli Chen Qiong Peng Wei Zhong Hualiang Lv College of physics Guizhou Province Key Laboratory for Photoelectrics Technology and ApplicationGuizhou UniversityGuiyang City 550025People’s Republic of China College of Materials and Metallurgy Guizhou UniversityGuiyang City 550025People’s Republic of China national laboratory of solid state Microstructures and Jiangsu Provincial laboratory for NanoTechnology Nanjing UniversityNanjing 210093People’s Republic of China department of Materials Science and laboratory of Advanced Materials Fudan UniversityShanghai 200433People’s Republic of China

Considering the serious electromagnetic wave(EMW)pollution problems and complex application condition,there is a pressing need to amalgamate multiple functionalities within a single ***,the effective integration of diverse functions into designed EMW absorption materials still faces the huge ***,reduced graphene oxide/carbon foams(RGO/CFs)with two-dimensional/three-dimensional(2D/3D)van der Waals(vdWs)heterostructures were meticulously engineered and synthesized utilizing an efficient methodology involving freeze-drying,immersing absorption,secondary freeze-drying,followed by carbonization *** to their excellent linkage effect of amplified dielectric loss and optimized impedance matching,the designed 2D/3D RGO/CFs vdWs heterostructures demonstrated commendable EMW absorption performances,achieving a broad absorption bandwidth of 6.2 GHz and a reflection loss of-50.58 dB with the low matching ***,the obtained 2D/3D RGO/CFs vdWs heterostructures also displayed the significant radar stealth properties,good corrosion resistance performances as well as outstanding thermal insulation capabilities,displaying the great potential in complex and variable ***,this work not only demonstrated a straightforward method for fabricating 2D/3D vdWs heterostructures,but also outlined a powerful mixeddimensional assembly strategy for engineering multifunctional foams for electromagnetic protection,aerospace and other complex conditions.

关键词： Multifunctionality Reduced graphene oxide/carbon foams 2D/3D van der Waals heterostructures Electromagnetic wave absorption Thermal insulation

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