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A surface engineering strategy for the stabilization of zinc metal anodes with montmorillonite layers toward long-life rechargeable aqueous zinc ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 94-105页

作者： Wenbo Wang Ruifeng Xu Xu Zhang Peiyu Wang Bao Yang Bingjun Yang Juan Yang Kailimai Su Pengjun Ma Yanan Deng Xianfeng Fan Wanjun Chen Key laboratory for Electronic Materials College of Electrical Engineering Northwest Minzu University Resource Chemistry and Energy Materials Research Center State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences University of Chinese Academy of Sciences Institute for Materials and Processes School of Engineering University of Edinburgh

Rechargeable aqueous zinc-ion batteries （AZIBs） exhibit appreciable potential in the domain of electrochemical energy ***,there are serious challenges for AZIBs,for instance zinc dendrite growth,hydrogen evolution reaction （HER）,and corrosion side ***,we propose a surface engineering modification strategy for coating the montmorillonite （MMT） layer onto the surface of the Zn anode to tackle these issues,thereby achieving high cycling stability for rechargeable *** results reveal that the MMT layer on the surface of the Zn anode is able to provide ordered zincophilic channels for zinc ions migration,facilitating the reaction kinetics of zinc *** functional theory（DFT） calculations and water contact angle （CA） tests prove that MMT@Zn anode exhibits superior adsorption capacity for Zn2+and better hydrophobicity than the bare Zn anode,thereby achieving excellent cycling ***,the MMT@Zn||MMT@Zn symmetric cell holds the stable cycling over 5600 h at 0.5 mA cm-2and 0.125 m A h cm-2,even exceeding 1800 h long cycling under harsh conditions of 5 m A cm-2and 1.25 m A h *** MMT@Zn||V2O5full cell reaches over 3000 cycles at 2 A g-1with excellent rate ***,this surface engineering modification strategy for enhancing the electrochemical performance of AZIBs represents a promising application.

关键词： Surface engineering strategy Montmorillonite layer Protection mechanism of Zn anode Cycling stability Aqueous zinc ion batteries

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二维纳米材料的相变:设计策略和催化应用的最新进展（英文）

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Science China Materials 2025年第1期 65-85页

作者：吴泽棋钮峰陈达黄岳祥刘贵高周勇涂文广朱熹邹志刚 College of Materials and Chemistry China Jiliang University national Special Superfine Powder Engineering Research Center School of Chemistry and Chemical Engineering Nanjing University of Science and Technology school of Science and Engineering The Chinese University of Hong Kong (Shenzhen) Jiangsu Key laboratory for Nano Technology National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced Microstructures School of Physics Nanjing University

二维(2D)纳米材料的相变会导致其电子和光学特性发生重大变化,为其开辟新的应用领域提供可能.最近, 2D纳米材料相工程的有效策略引起了广泛关注.本文综述了2D纳米材料相变的最新进展及其在催化领域的应用.首先,简要介绍了相变的基本概念...

二维(2D)纳米材料的相变会导致其电子和光学特性发生重大变化,为其开辟新的应用领域提供可能.最近, 2D纳米材料相工程的有效策略引起了广泛关注.本文综述了2D纳米材料相变的最新进展及其在催化领域的应用.首先,简要介绍了相变的基本概念,以及相变引起的显著电子和光学特性.以诱导相变的因素不同,将相变材料分为以下几种关键类型:(i)掺杂,(ii)外场,(iii)光照射,(iv)应变效应,(v)高能粒子激发,以及(vi)热处理.此外,还讨论了基于相变的二维纳米材料的催化领域的应用.最后,总结了控制2D纳米材料相变所涉及的技术挑战,并探讨了在该领域开发新应用的潜在机会.

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Bifunctional bridging capping layer enables 24.5% efficiency of perovskite solar cells with polymer-based hole transport materials

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Science China Chemistry 2025年第1期 350-359页

作者： Can Zhu Yiyang Wang Lei Meng Beibei Qiu Jing Li Shucheng Qin Ke Hu Xin Jiang Wenbin Lai Minchao Liu Zhe Liu Chenxing Lu Jinyuan Zhang Yongfang Li Beijing national laboratory for Molecular Sciences CAS Key Laboratory of Organic Solids Institute of Chemistry Chinese Academy of Sciences school of Chemical Science University of Chinese Academy of Sciences Key laboratory of solid state Optoelectronic Devices of Zhejiang Province College of Physics and Electronic Information Engineering Zhejiang Normal University Key laboratory of Photochemical Conversion and Optoelectronic Materials Technical Institute of Physics and ChemistryChinese Academy of Sciences laboratory of Advanced Optoelectronic Materials College of Chemistry Chemical Engineering and Materials ScienceSoochow University

Developing a bridge capping layer between perovskite and hole transport layer materials（HTMs） in the n-i-p perovskite solar cells（pero-SCs） is an effective approach to modify the morphology of HTMs and passivate the perovskite ***, we select the quinoxaline-based bifunctional passivation agent, quinoxalin-6-yl-methylamine hydrochloride（Qx MACl）,as the bridging layer, and a D-A copolymer PBQ12 containing the same quinoxaline unit as an HTM for the n-i-p pero-SCs. Due to the π-π stacking among the common quinoxaline units in the bridge layer and HTM, Qx MACl induces the π-π stacking of the PBQ12 film and improves the film morphology of HTMs with better conductivity. Additionally, Qx MACl can effectively passivate the perovskite surface, and PBQ12 possesses appropriate energy levels and high hole mobility. The pero-SCs based on FAPbI3with PBQ12/Qx MACl treatment showed a higher power conversion efficiency（PCE） of 24.05% and outstanding stability, maintaining 95.4% and 92.1% of its initial PCE after 750 h of storage and after over 800 h of thermal annealing at 85 °C, respectively. To further enhance the PCE of the PBQ12/Qx MACl-based devices, we developed a non-metal ion dopant for the PBQ12 HTM. Through trace doping of PBQ12 HTM by the non-metal ion dopant, the PCE of the PBQ12/Qx MACl-based devices reached 25.24%（the calibrated PCE of 24.55% by the national Institute of Metrology, China）.

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Detection of Majorana fermions in an Aharonov-Bohm interferometer

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Chinese physics B 2014年第5期23卷 478-484页

作者：尚恩明潘义明邵陆兵王伯根 national laboratory of solid state microstructures and school of physics Nanjing University

By using the non-equilibrium Green＇s function technique, we investigate the electronic transport properties in an Aharonov-Bohm interferometer coupling with Majorana fermions. We find a fixed unit conductance peak which is in-dependent of the other factors when the topological superconductor is grounded. Especially, an additional phase appears when the topological superconductor is in the strong Coulomb regime, which induces a new conductance resonant peak compared with the structure of replacing the topological superconductor by a quantum dot, and the conductance oscillation with the magnetic flux reveals a 2π phase shift by raising （lowering） a charge on the capacitor.

关键词： Majorana fermion quantum dot Aharonov-Bohm interferometer Coulomb blockade

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Recent progress in molten salt synthesis of low-dimensional perovskite oxide nanostructures, structural characterization,properties, and functional applications: A review

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Journal of Materials Science & Technology 2018年第6期34卷 914-930页

作者： Piaojie Xue Heng Wu Yao Lu Xinhua Zhu national laboratory of solid state microstructures School of Physics Nanjing University

Molten salt synthesis （MSS） method has advantages of the simplicity in the process equipment, versatile and large-scale synthesis, and friendly environment, which provides an excellent approach to synthesize high pure oxide powders with controllable compositions and morphologies. Among these oxides, perovskite oxides with a composition of ABO3 exhibit a broad spectrum of physical properties and functions （e.g. ferroelectric, piezoelectric, magnetic, photovoltaic and photocatalytic properties）. The downscaling of the spatial geometry of perovskite oxides into nanometers result in novel properties that are different from the bulk and film counterparts. Recent interest in nanoscience and nanotechnology has led to great efforts focusing on the synthesis of low-dimensional perovskite oxide nanostructures （PONs） to better understand their novel physical properties at nanoscale. Therefore, the low-dimensional PONs such as perovskite nanoparticles, nanowires, nanorods, nanotubes, nanofibers, nanobelts, and two dimensional oxide nanostructures, play an important role in developing the next generation of oxide electronics. In the past few years, much effort has been made on the synthesis of PONs by MSS method and their structural characterizations. The functional applications of PONs are also explored in the fields of storage memory, energy harvesting, and solar energy conversion. This review summarizes the recent progress in the synthesis of low-dimensional PONs by MSS method and its modified ways. Their structural char- acterization and physical properties are also scrutinized. The potential applications of low-dimensional PONs in different fields such as data memory and storage, energy harvesting, solar energy conversion, are highlighted. Perspectives concerning the future research trends and challenges of low-dimensional PONs are also outlined. ~ 2017 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science ＆ Technology.

关键词： Low-dimensional perovskite nanostructures Molten salt synthesis Structural characterization Physical properties Functional applications

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Resolution of ghost imaging with entangled photons for different types of momentum correlation

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Science China(physics,Mechanics & Astronomy) 2016年第7期59卷 9-13页

作者： MaLin Zhong Ping Xu LiangLiang Lu ShiNing Zhu national laboratory of solid state microstructures and school of physics Nanjing University

We present an analytical analysis of the spatial resolution of quantum ghost imaging implemented by entangled photons from a general, spontaneously parametric, down-conversion process. We find that the resolution is affected by both the pump beam waist and the nonlinear crystal length. Hence, we determined a method to improve the resolution for a certain imaging setup. It should be noted that the resolution is not uniquely related to the degree of entanglement of the photon pair since the resolution can be optimized for a certain degree of entanglement. For certain types of Einstein-Podolsky-Rosen(EPR) states——namely the momentum-correlated or momentum-positively correlated states——the resolution exhibits a simpler relationship with the pump beam waist and crystal length. Further, a vivid numerical simulation of ghost imaging is presented for different types of EPR states,which supports our analysis. This work discusses applicable references to the applications of quantum ghost imaging.

关键词： resolution of ghost imaging entangled photons momentum correlation

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Using monochromatic light to measure attenuation length of liquid scintillator solvent LAB

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Nuclear Science and Techniques 2019年第2期30卷 11-18页

作者： Rui Zhang De-Wen Cao Chang-Wei Loh You-Hang Liu Fang-Liang Wu Jia-Liang Zhang Ming Qi national laboratory of solid state microstructures and school of physics Nanjing University

Linear alkylbenzene(LAB) will be used as solvent for the liquid scintillator in the central detector of Jiangmen Underground Neutrino Observatory. The sheer size of the detector imposes significant challenges and the necessity to further improve the optical transparency of high-quality LAB. In order to study high optical transparencies, we continuously improve our measurement setup and use monochromatic light to measure the attenuation lengths of LAB samples. Moreover, the effects of organic impurities on LAB samples are studied to understand their interaction mechanisms and further improve the optical transparency of LAB.

关键词： Neutrino detector Linear alkylbenzene Light absorption

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A novel superhard tungsten nitride predicted by machine-learning accelerated crystal structure search

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Science Bulletin 2018年第13期63卷 817-824页

作者： Kang Xia Hao Gao Cong Liu Jianan Yuan Jian Sun Hui-Tian Wang Dingyu Xing national laboratory of solid state microstructures School of Physics and Collaborative Innovation Center of Advanced MicrostructuresNanjing University

Transition metal nitrides have been suggested to have both high hardness and good thermal stability with large potential application value, but so far stable superhard transition metal nitrides have not been synthesized. Here, with our newly developed machine-learning accelerated crystal structure searching method, we designed a superhard tungsten nitride, h-WN6, which can be synthesized at pressure around 65 GPa and quenchable to ambient pressure. This h-WN6 is constructed with single-bonded armchair-like N6 rings and presents ionic-like features, which can be formulated as W^2.4＋N^2.4-. It has a band gap of 1.6 eV at 0GPa and exhibits an abnormal gap broadening behavior under pressure. Excitingly, this h-WN6 is found to be the hardest among transition metal nitrides known so far （Vickers hardness around 57 GPa） and also has a very high melting temperature （around 1,900 K）. Additionally, the good gravimet- ric （3.1 kJ/g/and volumetric （28.0 kJ/cm3） energy densities make this nitrogen-rich compound a potential high-energy-density material, These predictions support the designing rules and may stimulate future experiments to synthesize superhard and high-energy-density material.

关键词： Tungsten nitride Transition metal nitrides Machine-learning accelerated crystal structure searching method Superhard tungsten nitride

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Reconfigurable vertical field-effect transistor based on graphene/MoTe2/graphite heterostructure

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Science China(Information Sciences) 2020年第10期63卷 211-218页

作者： Cong WANG Chen PAN Shi-Jun LIANG Bin CHENG Feng MIAO national laboratory of solid state microstructures School of PhysicsCollaborative Innovation Center of Advanced MicrostructuresNanjing University

Reconfigurable field-effect transistors have attracted enormous attention over the past decades because of their potential in implementing logic and analog circuit functions with fewer resources of transistors compared with complementary metal-oxide-semiconductor transistors. However, the miniaturization of traditional reconfigurable transistors is still a challenge owing to their inherent planar multi-gate ***, we fabricated a dual-gate vertical transistor based on graphene/MoTe2/graphite van der Waals heterostructure and demonstrated a switchable n-type, V-shape ambipolar and p-type field-effect characteristics by varying the voltages of the top gate and drain electrodes. According to the band diagram analysis, we reveal that the reconfiguring ability of the field-effect characteristics stems from the asymmetric injection efficiency of the carriers through the gate-tunable barriers at the interfaces. Our results offer a potential approach to achieve device miniaturization of reconfigurable transistors.

关键词： reconfigurable field-effect transistor vertical transistor graphene/MoTe2 van der Waals heterostructure ambipolar transistor dual-gate transistor

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High-pressure phases of Weyl semimetals NbP, NbAs, TaP,and TaAs

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Science China(physics,Mechanics & Astronomy) 2018年第3期61卷 47-55页

作者： ZhaoPeng Guo PengChao Lu Tong Chen JueFei Wu Jian Sun DingYu Xing national laboratory of solid state microstructures School of Physics and Collaborative Innovation Center of Advanced MicrostructuresNanjing University

In this study, we used the crystal structure search method and first-principles calculations to systematically explore the highpressure phase diagrams of the TaAs family （NbP, NbAs, TaP, and TaAs）. Our calculation results show that NbAs and TaAs have similar phase diagrams, the same structural phase transition sequence I41md→Pδm2→}P21/c→Pm3m, and slightly different transition pressures. The phase transition sequence of NbP and TaP differs somewhat from that of NbAs and TaAs, in which new structures emerge, such as the Cmcm structure in NbP and the Pmmn structure in TaP. Interestingly, we found that in the electronic structure of the high-pressure phase Pδm2-NbAs, there are coexisting Weyl points and triple degenerate points, similar to those found in high-pressure Pδm2-TaAs.

关键词： high pressure phase transition crystal structure prediction topological materials Dirac/Weyl/node-line semimetals Fermi arc

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