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Lattice water fuels acidic water oxidation

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Science China Chemistry 2024年第7期67卷 2132-2133页

作者： Minyue Zhao Jianyong Feng Zhaosheng Li Zhigang Zou Collaborative Innovation Center of Advanced microstructures National Laboratory of Solid State MicrostructuresCollege of Engineering and Applied SciencesNanjing UniversityNanjing 210093China Jiangsu key laboratory for Nano Technology Nanjing UniversityNanjing 210093China

In comparison to commercial alkaline water electrolysis technologies,proton-exchange membrane water electrolyzers(PEMWEs)offer intriguing advantages for hydrogen production,such as high current density,compact system ... 详细信息

关键词： Lattice alkaline system

Beating the Fault-Tolerance Bound and Security Loopholes for Byzantine Agreement with a Quantum Solution

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Research 2024年第3期2023卷 445-455页

作者： Chen-Xun Weng Rui-Qi Gao Yu Bao Bing-Hong Li Wen-Bo Liu Yuan-Mei Xie Yu-Shuo Lu Hua-Lei Yin Zeng-Bing Chen national laboratory of Solid State microstructures and School of Physics Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China Department of Physics and Beijing key laboratory of Opto-electronic Functional Materials and Micro-nano Devices Key Laboratory of Quantum State Construction and Manipulation(Ministry of Education)Renmin University of ChinaBeijing 100872China.

Byzantine agreement,the underlying core of blockchain,aims to make every node in a decentralized network reach *** Byzantine agreements unavoidably face two major *** is 1/3 fault-tolerance bound,which means that the system to tolerate f malicious players requires at least 3f+1 *** other is the security loopholes from its classical cryptography ***,we propose a Byzantine agreement framework with unconditional security to break this bound with nearly 1/2 fault tolerance due to multiparty correlation provided by quantum digital *** is intriguing that quantum entanglement is not necessary to break the 1/3 fault-tolerance bound,and we show that weaker correlation,such as asymmetric relationship of quantum digital signature,can also *** work strictly obeys two Byzantine conditions and can be extended to any number of players without requirements for multiparticle *** experimentally demonstrate three-party and five-party consensus for a digital *** work indicates the quantum advantage in terms of consensus problems and suggests an important avenue for quantum blockchain and quantum consensus networks.

关键词： methods. quantum signature

Unraveling role of double-exchange interaction in electrochemical water oxidation by external magnetic field

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Rare Metals 2024年第1期43卷 289-297页

作者： Jun Li Jun-Ming Li Hong Hong Dong-Xue Liu Qing-Qi Cao Dun-Hui Wang national laboratory of Solid State microstructures and Jiangsu Provincial key laboratory for Nanotechnology Nanjing UniversityNanjing 210093China School of Electronics and Information Hangzhou Dianzi UniversityHangzhou 310018China

Double-exchange(DE) interaction plays an important role in electrocatalytic oxygen evolution reaction(OER).However,precise achievement of DE interaction often requires foreign dopants or vacancy engineering,leading to destabilization of the catalysts and deterioration of *** contrast,the utilization of environmentally friendly,contactless,and continuously adjustable magnetic fields to study the OER process is profitable to avoid aforementioned interference factors and further elucidate the direct relationship_(0.5)between DE interaction and OER ***,by using cobalt hydroxide carbonate(Co(OH)(CO_(3))·xH_(2)O,CoHC) nanostructures as a proof-of-concept study,external magnetic fields are carefully implemented to verify the role of DE interaction during water oxidation *** studies reveal that external magnetic fields effectively enhance the reaction rate of the catalyst,the overpotential decreases from 386 to 355 mV(100 mA·cm^(-2)),while Tafel slopes drastically decline from 93 to 67 mV·dec^(-1)(1.0 T).Moreover,magnetic field increment exhibits robust *** in situ Raman and impedance measurements under external field,it can be found that magnetic field promotes the electron migration between Co^(2+) and Co^(3+) in the CoHC catalysts with the assistance of DE interactions,thus boosting the OER efficiency.

关键词： Magnetic field Double-exchange(DE)interaction Electrocatalysis Oxygen evolution reaction(OER) Cobalt hydroxide carbonate

In-phase and out-of-phase spin pumping effects in Py/Ru/Pysynthetic antiferromagnetic structures

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Chinese Physics B 2024年第9期33卷 541-545页

作者： Zhaocong Huang Xuejian Tang Qian Chen Wei Jiang Qingjie Guo Milad Jalali Jun Du Ya Zhai key laboratory of Quantum Materials and Devices of Ministry of Education School of PhysicsSoutheast UniversityNanjing 211189China national laboratory of Solid microstructures Nanjing UniversityNanjing 210093China

The spin pumping effect in magnetic heterostructures and multilayers is a highly effective method for the generationand transmission of spin currents. In the increasingly prominent synthetic antiferromagnetic structures, the two ferromagneticlayers demonstrate in-phase and out-of-phase states, corresponding to acoustic and optical precession modes. Withinthis context, our study explores the spin pumping effect in Py/Ru/Py synthetic antiferromagnetic structures across differentmodes. The heightened magnetic damping resulting from the spin pumping effect in the in-phase state initially decreaseswith increasing Py thickness before stabilizing. Conversely, in the out-of-phase state, the amplified damping exceeds thatof the in-phase state, suggesting a greater spin relaxation within this configuration, which demonstrates sensitivity to alterationsin static exchange interactions. These findings contribute to advancing the application of synthetic antiferromagneticstructures in magnonic devices.

关键词： spin pumping spin transmission synthetic antiferromagnetic structures spin dynamics

Quantized bound states around a vortex in anisotropic superconductors

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Science China(Physics,Mechanics & Astronomy) 2024年第6期67卷 146-155页

作者： Ke Xiang Da Wang Qiang-Hua Wang national laboratory of Solid State microstructures&School of Physics Nanjing UniversityNanjing 210093China Collaborative Innovation Center of Advanced microstructures Nanjing 210093China

The bound states around a vortex in anisotropic superconductors is a longstanding yet important *** this work,we develop a variational theory on the basis of the Andreev approximation to obtain the energy levels and wave functions of the low-energy quantized bound states in superconductors with anisotropic pairing on arbitrary Fermi *** the case of circular Fermi surface,the effective Schr¨odinger equation yielding the bound state energies gets back to the theory proposed by Volovik and Kopnin many years *** generalization here enables us to prove the equidistant energy spectrum inside a vortex in a broader class of *** importantly,we are now able to obtain the wave functions of these bound states by projecting the quasiclassical wave function on the eigenmodes of the effective Schr¨odinger equation,going beyond the quasiclassical Eilenberger results,which,as we find,are sensitive to the scattering *** the case of isotropic Fermi surface,the spatial profile of the low-energy local density of states is dominated near the vortex center and elongates along the gap antinode directions,in addition to the ubiquitous Friedel oscillation arising from the quantum inteference neglected in the Eilenberger ***,as a consequence of the pairing anisotropy,the quantized wave functions develop a peculiar distribution of winding number,which reduces stepwise towards the vortex *** work provides a flexible way to study the vortex bound states in the future.

关键词： vortex bound state anisotropic superconductor Andreev approximation

Robust and Tunable Ferroelectricity in Ba/Co Codoped (K_(0.5)Na_(0.5))NbO_(3) Ceramics

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Chinese Physics Letters 2024年第7期41卷 152-160页

作者：刘佳讯查节林杨玉龙吕笑梅胡雪莉阎朔吴子敬黄凤珍 national laboratory of Solid State microstructures and School of Physics Nanjing UniversityNanjing 210093China Collaborative Innovation Center of Advanced microstructures Nanjing UniversityNanjing 210093China

The 0.98(K_(0.5)Na_(0.5))NbO_(3)-0.02Ba(Nb_(0.5)Co_(0.5))O_(3-δ) ceramics with doped Ba^(2+) and Co^(2+) ions are fabricated,and the impacts of the thermal process are *** with the rapidly cooled (RC) sample,the slowly cooled (SC) sample possesses superior dielectric and ferroelectric properties,and an 11 K higher ferroelectricparaelectric phase transition temperature,which can be attributed to the structural characteristics such as the grain size and the degree of *** treatment can reversibly modulate the content of the oxygen vacancies,and in turn the ferroelectric hysteresis loops of the ***,robust and tunable ferroelectric property is achieved in SC samples with good structural integrity.

关键词： ceramics ferroelectric treatment

Heralded entanglement between error-protected logical qubits for fault-tolerant distributed quantum computing

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Science China(Physics,Mechanics & Astronomy) 2024年第2期67卷 25-33页

作者： Jialun Li Zhihao Xie Yachen Li Yansen Liang Zhenhua Li Tao Li MIIT key laboratory of Semiconductor Microstructure and Quantum Sensing School of PhysicsNanjing University of Science and TechnologyNanjing 210094China national laboratory of Solid State microstructures Nanjing UniversityNanjing 210093China

Quantum error correction is essential for achieving reliable quantum information processing tasks,as it can mitigate the detrimental effects of noise by encoding single-qubit information into a larger quantum ***,the generation of distributed entanglement between logical qubits located within two spatially separated nodes presents a significant resource-intensive challenge that has yet to be *** we present a heralded protocol for generating distributed entanglement between two nonlocal error-protected logical qubits.A high-dimensional single photon can evolve physical qubits into a logical qubit that entangles with the photon and then converts logical qubit-photon entanglement into entanglement between two logical qubits,when the photon state is properly tuned and an effective photon-spin interface between single photons and individual spins is ***,the success of the entanglement generation is heralded by the detection of the photon,and the corresponding efficiency can,in principle,approach *** distinguished features make our protocol highly appealing for future large-scale quantum technologies.

关键词： quantum networks distributed entanglement error-protected logical qubits high-dimensional photons

Coexistence of All-Order Topological States in a Three-Dimensional Phononic Topological Crystalline Insulator

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Research 2024年第2期2023卷 511-518页

作者： Hua-Shan Lai Hao Chen Chu-Hao Xia Si-Yuan Yu Cheng He Yan-Feng Chen national laboratory of Solid State microstructures&Department of Materials Science and Engineering Nanjing UniversityNanjng 210093China Collaborative Innovation Center of Advanced microstructures Nanjing University Nanjng 210093China Jiangsu key laboratory of Artificial Functional Materials Nanjing University Nanjing 210093China

Classical-wave topological materials lacking intrinsic half-integer spins are less robust while more ***,we explore a single 3-dimensional phononic topological crystalline insulator that simultaneously exhibits a whole family of first-order quadratic surface,second-order hinge,and third-order corner states within the same *** a topological crystalline insulator hosting all-order phases originates from the different topological nature when hierarchically projected onto different facets and lower dimensions,thus free from trivial cladding *** work offers an ideal platform for either robust wave propagation or localization in on-demand dimensions and may facilitate dimension division multiplexing technology.

关键词： topological dimensions crystalline

Conceptual transition from molecular to atomic: unleashing a new era in hydrogen therapy for chronic disease

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national Science Review 2024年第04期11卷 17-18页

作者： Zhigang Zou Eco-materials and Renewable Energy Research Center (ERERC) Jiangsu Key Laboratory for Nano Technology National Laboratory of Solid State Microstructures and Department of PhysicsNanjing University

The dysregulated overexpression of reactive oxygen and nitrogen species (RONS)intricately links to the occurrence and development of diverse chronic diseases[1–3]. Hydrogen therapy stands out as a promising treatment methodology recognized for effectively mitigating RONS and maintaining intracellular redox equilibrium, thereby yielding therapeutic benefits [4,5].

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