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Quantitative geochemical reconstruction of Eocene paleoenvironment in Fushun Basin,northeast China

Acta Geochimica 2024年第3期43卷 571-587页

作者： Yuanji Li Pingchang Sun Qiang Zhang Junxian Wang Department of safety engineering Heilongjiang University of Science and TechnologyHarbin 150022China national Professional center Lab of safety Basic research for Hydrocarbon gas pipeline transportation Network Harbin 150022China College of Earth Sciences Jilin UniversityChangchun 130061JilinChina Beijing research Institute of Uranium Geology Beijing 100029China

The quantitative estimation of key parameters of paleotemperature and paleoprecipitation is crucial for paleoclimate reconstruction.Geochemical data from mod-ern sediments are highly consistent with climate data,and their relationship can provide an important reference for the quantitative reconstruction of the paleoclimate.In this study,detailed inorganic geochemical analysis was carried out using high-precision sampling of the Paleogene(LFD-1 well)Guchengzi,Jijuntun and Xiloutian Formations in the Fushun Basin located in the mid-latitudes of the Northern Hemisphere.The Eocene Guchengzi Formation(54.51–47.8 Ma)and Jijuntun Formation(47.8–41.2 Ma)in the Fushun Basin were found to have been deposited under a humid climate.The lower(41.2–40.1 Ma)and upper(40.1–37.8 Ma)parts of the Xiloutian Formation were character-ized by semiarid and semihumid–semiarid climates,respec-tively,which is very similar to the paleoclimatic information reflected by organic carbon isotopes.The Eocene Thermal Maximum 2(ETM2,~53.7 Ma),Early Eocene Climatic Optimum(EECO,~53.1–46.5 Ma),Eocene Thermal Maxi-mum 3(ETM 3,~52.8 Ma),and Middle Eocene Climatic Optimum(MECO,~40.7–40.1 Ma)events significantly enhanced chemical weathering during these periods.The rapid increase in pCO_(2)concentration leads to an increase in temperature,precipitation,and surface runoff,exhibiting strong chemical weathering.The mean annual temperature(MATa)and mean annual precipitation(MAPa,MAPb,and MAPc)were estimated using parameters,such as the corrosion index without potassium(CIA-K),CaO/Al_(2)O_(3),and(Na_(2)O+K_(2)O)/Al_(2)O_(3).Comparing MAPa,MAPb,and MAPc with the MAP estimated using pollen data,MAPa and MAPb were found to be more sensitive to the climate during high precipitation periods(precipitation>1000 mm,Guchengzi Formation),and the recovered average precipi-tation was similar to MAP.In contrast,MAPc was more sensitive to the climate during low precipitation periods(precipitation<1000 mm,Jijuntun,and Xiloutian Forma-tions),with higher accuracy.To fully co

关键词： Eocene Fushun Basin Major element Paleoclimate Geochemical reconstruction

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Review of the evolution and prevention of friction,wear,and noise for water-lubricated bearings used in ships

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Friction 2024年第1期12卷 1-38页

作者： Zhuo ZHANG Wu OUYANG Xingxin LIANG Xinping YAN Chengqin YUAN Xincong ZHOU Zhiwei GUO Conglin DONG Zhenglin LIU Yong JIN Jinhua XIAO School of transportation and Logistics engineering Wuhan University of TechnologyWuhan 430063China Reliability engineering Institute National Engineering Research Center for Water Transport SafetyWuhan 430063China School of Naval Architecture Ocean and Energy Power EngineeringWuhan University of TechnologyWuhan 430063China East Lake Laboratory Wuhan 420202China

With the development of green tribology in the shipping industry,the application of water lubrication gradually replaces oil lubrication in stern bearings and thrust bearings.In terms of large-scale and high-speed ships,water-lubricated bearings with high performance are more strictly required.However,due to the lubricating medium,water-lubricated bearings have many problems such as friction,wear,vibration,noise,etc.This review focuses on the performance of marine water-lubricated bearings and their failure prevention mechanism.Furthermore,the research of marine water-lubricated bearings is reviewed by discussing its lubrication principle,test technology,friction and wear mechanism,and friction noise generation mechanism.The performance enhancement methods have been overviewed from structure optimization and material modification.Finally,the potential problems and the perspective of water-lubricated bearings are given in detail.

关键词： water-lubricated bearings lubrication principles test techniques friction and wear friction noise evolution and prevention

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research on a TOPSIS energy efficiency evaluation system for crude oil gathering and transportation systems based on a GA-BP neural network

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Petroleum Science 2024年第1期21卷 621-640页

作者： Xue-Qiang Zhang Qing-Lin Cheng Wei Sun Yi Zhao Zhi-Min Li Key Lab of Ministry of Education for Enhancing the oil and gas Recovery Ratio Northeast Petroleum UniversityDaqing163318HeilongjiangChina China Petroleum pipeline Material and Equipment Co. LtdLangfang065000HebeiChina research Institute of Petroleum engineering and Technology Sinopec Northwest Oilfield CompanyUrumqi830011XinjiangChina

As the main link of ground engineering,crude oil gathering and transportation systems require huge energy consumption and complex structures.It is necessary to establish an energy efficiency evaluation system for crude oil gathering and transportation systems and identify the energy efficiency gaps.In this paper,the energy efficiency evaluation system of the crude oil gathering and transportation system in an oilfield in western China is established.Combined with the big data analysis method,the GA-BP neural network is used to establish the energy efficiency index prediction model for crude oil gathering and transportation systems.The comprehensive energy consumption,gas consumption,power consumption,energy utilization rate,heat utilization rate,and power utilization rate of crude oil gathering and transportation systems are predicted.Considering the efficiency and unit consumption index of the crude oil gathering and transportation system,the energy efficiency evaluation system of the crude oil gathering and transportation system is established based on a game theory combined weighting method and TOPSIS evaluation method,and the subjective weight is determined by the triangular fuzzy analytic hierarchy process.The entropy weight method determines the objective weight,and the combined weight of game theory combines subjectivity with objectivity to comprehensively evaluate the comprehensive energy efficiency of crude oil gathering and transportation systems and their subsystems.Finally,the weak links in energy utilization are identified,and energy conservation and consumption reduction are improved.The above research provides technical support for the green,efficient and intelligent development of crude oil gathering and transportation systems.

关键词： Crude oil gathering and transportation system GA-BP neural network Energy efficiency evaluation TOPSIS evaluation method Energy saving and consumption reduction

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Modulating the degree of O vacancy defects to achieve selective control of electrochemical CO_(2) reduction products

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Chinese Chemical Letters 2024年第5期35卷 482-486页

作者： Tianbo Jia Lili Wang Zhouhao Zhu Baikang Zhu Yingtang Zhou Guoxing Zhu Mingshan Zhu Hengcong Tao School of Petrochemical engineering&Environment Zhejiang Ocean UniversityZhoushan 316022China Department of General Practice First Medical CenterChinese PLA General HospitalBeijing 100853China national&Local Joint engineering research center of Harbor oil&gas Storage and transportation Technology Zhoushan 316022China School of Chemistry and Chemical engineering Jiangsu UniversityZhenjiang 212013China Guangdong Key Laboratory of Environmental Pollution and Health School of EnvironmentJinan UniversityGuangzhou 511443China

Conversion of CO_(2) into high-value products using electrochemical CO_(2) reduction(ECR)technology is an effective way to alleviate global warming and reach carbon neutrality.The oxygen vacancies in heterogenous catalysis are generally considered as a powerful method to enhance the performance of ECR by promoting CO_(2) adsorption and activation.However,the extent of defects in oxygen vacancies-activity relation has rarely been studied.Herein,we prepared Cu-Cd bimetallic catalysts with adjustable oxygen defect degree by controlling the amount of cadmium addition.Fourier transform infrared spectroscopy characterization results reveal that the formation of oxygen vacancies is attributed to the asymmetric stretching of Cu-O by the addition of cadmium.Electrochemical results show that the oxygen defect degree can modulate the selectivity of ECR products.A low degree of oxygen defects(CuO)is generally associated with lower product Faraday efficiency(FE_(C2)/FE_(C1)≈114%),but overabundant oxygen vacancies(CuO_(2.625)-CdO_(0.375))are not entirely favorable to improving ECR activity(FE_(C2)/FE_(C1)≈125%)and single selectivity,while an appropriate degree of oxygen vacancies(CuO_(2.75)-CdO_(0.25))can facilitate the ECR process toward single product selective production(FE_(C2)/FE_(C1)≈296%).The theoretical calculation showed that the O vacancy formed on CuO and the interface between CdO and CuO were conducive to enhancing the formation of ^(*)COOH intermediate and promoting the generation of ethylene products.This study provides a new approach and insight into the selective production of single products for future industrial applications of ECR.

关键词： CO_(2) O-vacancies Bimetallic catalysts Copper oxide Cadmium oxide Selective

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research on the falling film flow and heat transfer characteristics of FLNG spiral wound heat exchanger under sea conditions

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Petroleum Science 2022年第3期19卷 1276-1290页

作者： Chong-Zheng Sun Liang Liu Yu-Xing Li Jian-Lu Zhu College of pipeline and Civil engineering/Shandong Provincial Key Laboratory of oil&gas Storage and transportation safety/Qingdao Key Laboratory of Circle Sea oil&gas Storage and transportation Technology China University of PetroleumQingdaoShandong266580China

As the key equipment of floating liquefied natural gas(FLNG)process,the performance of spiral wound heat exchanger(SWHE)influences operation costs and reliability of the whole system.The sea conditions destroy the falling film flow state of the refrigeration and then affect the heat transfer performance of FLNG SWHE.In order to design and optimize the SWHE,a cryogenic experimental device of FLNG process and a numerical model of falling film flow have been constructed to study the effects of sea conditions on the falling film flow and heat transfer characteristics of SWHE.The cryogenic experimental results show that the pitching conditions have larger effects on the heat transfer performance than yawing.Under the pitching angle of 7°,the natural gas temperature and gaseous refrigerant temperature increase by 3.22°C and 7.42°C,respectively.The flow rates of refrigerant and feed natural gas have a great impact on the heat transfer performance of SWHE under pitching and compound sloshing conditions.When the tilt angle increases to 9°,the tube structure with outer diameter D=8 mm and pipe spacing S=4 mm is recommended to reduce the drying area of the pipe wall surface.

关键词： FLNG Spiral wound heat exchanger Falling film flow Cryogenic heat transfer Sea condition

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A further investigation to mechanism of the electrorheological effect of waxy oils:Behaviors of charged particles under electric field

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Petroleum Science 2023年第2期20卷 1247-1254页

作者： Yi-Wei Xie Hong-Ying Li Chao-Yue Zhang Yang Su Qian Huang Feng Jiang Chao-Hui Chen Shan-Peng Han Jin-Jun Zhang national engineering research center of oil and gas pipeline transportation safety China University of PetroleumBeijing 102249China MOE Key Laboratory of Petroleum engineering China University of PetroleumBeijing 102249China Beijing Key Laboratory of Urban oil&gas Distribution Technology China University of PetroleumBeijing 102249China PetroChina Planning and engineering Institute Beijing 100083China

Exposing waxy oils to an electric field may significantly improve their cold flowability.Our previous study has shown that interfacial polarization,i.e.,charged particle accumulation on the wax particle surface,is the primary mechanism of the electrorheological behavior of waxy oils.However,the way that charged particles interact with wax particles under an electric field remains unknown.In this study,we found no viscosity and impedance change for two waxy crude oils after their exposure to a high-voltage electric field.However,the yield stresses were reduced obviously.We thus proposed that the collision of colloidal particles such as resins and asphaltenes with the wax particles could be an essential mechanism that the wax particle structure was weakened.To verify this hypothesis,a series of ad hoc experiments were carried out,i.e.,by performing electrorheological tests on model waxy oils containing additives removable under an electric field,including electrically-neutral colloidal particles(Fe3O4),charged colloidal particles(resins),and oil-soluble electrolyte(C22H14CoO4),respectively,and demonstrated that upon application of a high-voltage electric field,charged particles in a waxy oil may move and thus collide with wax particles,and consequently adhere to the wax particle surface.The particle collision results in damage to the wax particle network,and the electrostatic repulsion arising from the adhesion of the charged particle on the wax particle diminishes attraction between wax particles.This study clarifies the process of interfacial polarization.

关键词： Waxy oil Electrorheological effect Interfacial polarization Charged particle motion

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Investigation on hydrate growth at the oil–water interface:In the presence of asphaltene

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Chinese Journal of Chemical engineering 2022年第5期35卷 211-218页

作者： Guangchun Song Yuanxing Ning Yuxing Li Wuchang Wang Shandong Key Laboratory of oil-gas Storage and transportation safety College of Pipeline and Civil EngineeringChina University of PetroleumQingdao 266580China State Key Laboratory of Natural gas Hydrates Beijing 100028China

Natural gas hydrates can readily form in deep-water oil production processes and pose a great threat to the oil industry.Moreover,the coexistence of hydrate and asphaltene can result in more severe challenges to subsea flow assurance.In order to study the effects of asphaltene on hydrate growth at the oil-water interface,a series of micro-experiments were conducted in a self-made reactor,where hydrates nucleated and grew on the surface of a water droplet immersed in asphaltene-containing oil.Based on the micro-observations,the shape and growth rate of the hydrate shell formed at the oil-water interface were mainly investigated and the effects of asphaltene on hydrate growth were analyzed.According to the experimental results,the shape of the water droplet and the interfacial area changed significantly after the formation of the hydrate shell when the asphaltene concentration was higher than a certain value.A mechanism related to the reduction of the interfacial tension caused by the absorption of asphaltenes on the interface was proposed for illustration.Moreover,the growth rate of the hydrate shell decreased significantly with the increasing asphaltene concentration under experimental conditions.The conclusions of this paper could provide preliminary insight how asphaltene affect hydrate growth at the oil-water interface.

关键词： Hydrate Asphaltene Interface Growth Shape

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Microscopic morphology evolution of the crystal structure of tetrahydrofuran hydrate under flowing condition

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Chinese Journal of Chemical engineering 2022年第5期35卷 103-110页

作者： Jialu Zhang Xiang Liu Shuai Liu Yuxing Li Qihui Hu Wuchang Wang Shandong Key Laboratory of oil-gas Storage and transportation safety College of Pipeline and Civil EngineeringChina University of Petroleum(East China)Qingdao 266580China State Key Loboratory of Natural gas Hydrates Beijing 100028China

The evolution of the hydrate particle structure during growth and agglomeration under flowing condition affects the particle as well as flow characteristic,which plays an important role in the flow assurance as well as heat transfer in refrigeration systems.Therefore,this article conducts experiments to study and observe the growth and agglomeration process in the main forming stage of hydrate.It was found that the growth of tetrahydrofuran hydrate was anisotropic and in a layered growth pattern.Single crystals generally transformed from octahedral structure to octahedral skeleton structure with growth,however some single crystals also deformed into plate type particles.The thickness of the plate type particles increased gradually during growth,and the edge part increased earlier than the middle part.During agglomeration,the hydrate particles contacted and sintered together.Sand as the impurity didn’t serve as the nucleation center but affected the agglomeration of hydrate particles by collisions.In addition,the effect increased as the sand size decreased.Finally,a microstructure model for hydrate growth and agglomeration was proposed,which showed the hydrate structure evolution in these processes and could lay a foundation for studying the flow assurance of hydrate slurry.

关键词： Tetrahydrofuran hydrate Growth Agglomeration Morphology Microstructure Microstructure model

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Investigation on synergistic deposition of wax and hydrates in waxy water-in-oil(W/O) flow systems

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Petroleum Science 2022年第4期19卷 1840-1852页

作者： Yang Liu Xiao-Fang Lv Qian-Li Ma Shi-Dong Zhou Bo-Hui Shi Hui Du Yun Lei Peng-Fei Yu Shang-Fei Song Jing Gong Bing-Cai Sun Jiangsu Key Laboratory of oil and gas Storage and transportation Technology Changzhou UniversityChangzhouJiangsu213164China Institute of Petroleum engineering Technology Sinopec Northwest Oil Field CompanyUrumqiXinjiang830011China national engineering Laboratory for pipeline safety/State Key Laboratory of Natural gas Hydrate China University of Petroleum-BeijingBeijing102249China CNPC safety and Environmental Protection Technology research Institute Co.Ltd Beijing102206China

Elucidating the synergistic effect of wax and hydrates, involving formation, aggregation and deposition,is imperative to the operation and transportation safety for offshore petroleum fields. To understand the characteristics and mechanism of synergistic deposition of wax and hydrates, flow and deposition experiments of systems with different wax contents(0-2.89 wt%), initial flow rates, pressures and temperatures were conducted in a high pressure visual flow loop. According to the flow rate and pressure drop data as well as the visual window observation, four different types of plugging scenarios of waxhydrate coexisting systems with different flow properties and wall deposition state were summarized,including rapid plugging, transition plugging, gradual plugging type I and gradual plugging type II.Compared with the wax-free system after hydrate formation, even with the addition of anti-agglomerant(AA) with the same concentration, wax-hydrate coexisting systems could not reach stable hydrate slurry flow state, indicating that the existence of wax deteriorated the performance of AA. Aside from the influence of wax crystals on hydrate agglomeration, it was found that wax deposition layer would alter the adhesion and bedding of hydrates, resulting in the variation of flow properties and wall deposition state.For low wax content systems(0.75 wt%) where rapid plugging occurred, the synergistic effect between wax and hydrates promoted the formation of wax-hydrate coupling aggregates, resulting in severe local deposition when the coupling aggregates attained critical deposition size and consequently decreasing flow rate, forming a vicious circle of decreasing transportability. Since bedding of coupling aggregates was hindered by the uniformly coated wax deposition layer on pipe wall, gradual plugging rather than rapid plugging occurred in medium wax content systems(1-1.25 wt%), predominately caused by the gradual increment in viscosity of waxy hydrate slurry. For relatively high wax content systems(2.89 wt%), hydrate f

关键词： Flow assurance Wax Hydrates Flow properties Synergistic deposition

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Optimization design of multi-gathering mode for the surface system in coalbed methane field

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Petroleum 2023年第2期9卷 237-247页

作者： Jun Zhou Tiantian Fu Kunyi Wu Yunxiang Zhao Lanting Feng Petroleum engineering School Southwest Petroleum UniversityChengduChina research Institute of Gathering and transportation engineering Technology PetroChina Southwest Oil&Gas Field CompanyChengduChina Pipechina Southwest pipeline Company ChengduChina

As a potential resource for emerging clean energy with abundant reserves,coalbed methane(CBM)has risen rapidly in recent years,and the construction of rational and economical CBM gathering system plays a vital role in the development of the oil and gas industry.At present,there is no literature that considers the optimization of the multi-gathering mode of coalbed methane pipe network system.Due to the complexity and high investment,this paper establishes a unified mixed-integer nonlinear programming model to determine the gathering modes(including liquified natural gas,compressed natural gas,and gas gathering station)of gathering system to reduce the cost of coalbed methane collection and export.The objective function is the maximization of total profit during the period of the whole project,and such constraints,like network structure,facility number,location,node flow balance,capacity and variable value,are taken into consideration.The solution strategy and heuristic algorithm is proposed and verified by the field data from Shanxi province(China).The results show that the model can solve the problem for optimization design of the surface system in complicated CBM fields.

关键词： Coalbed methane Multi-gathering mode Optimization pipeline network

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