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Journal of Energy Chemistry 2024年第3期90卷 496-503,I0011页

作者： Junjie Qian Jingjing He Qihang Zhang Chenyue Zhu Shilin Chen Zhanpeng Wei Xuesong Leng Ziren Zhou Benben Shen Yu Peng Qiang Niu Shuang Yang Yu Hou Key Laboratory for Ultrafine Materials of Ministry of Education Shanghai Engineering Research Center of Hierarchical NanomaterialsSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China national Enterprise Technology center Inner Mongolia Erdos Electric Power and Metallurgy Group Company LimitedOrdos 016064Inner MongoliaChina

Inverted perovskite solar cells(PSCs) have attracted broad research and industrial interest owing to their suppressed hysteresis,cost-effectiveness,and ***,the issue of non-radiative recombination losses at the n-type interface between the perovskite and fullerene has impeded further improvement of photovoltaic ***,we modify the n-type interface of FAPbI_(3) perovskite films by constructing a stereochemical two-dimensional(2D) perovskite interlayer,in which the organic cations comprise both pyridine and ammonium *** pyridine N donor can create stable bonding with the surface-uncoordinated Pb on the perovskite,thereby passivating the shallow-level defects and enhancing the air stability of the ***,the pyridine N donor also offers a positive polar interface to decrease the surface work function of the perovskite film,enabling n-type ***,we employ a p-i-n photovoltaic(PV) device with the positive dipole interlayer at perovskite/fullerene contact and achieve remarkable photoelectric conversion efficiency(PCE) of 22.0%.

关键词： Perovskite solar cells Dipole interlayer Stereochemistry Non-radiative recombination

Understanding microstructure-property relationships of HPDC Al-Si alloy based on machine learning and crystal plasticity simulation

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Advances in Manufacturing 2024年第3期12卷 497-511页

作者： Qiang-Qiang Zhai Zhao Liu Ping Zhu State Key Laboratory of Mechanical System and Vibration Shanghai Jiao Tong UniversityShanghai200240People’s Republic of China national engineering research center of Automotive Power and Intelligent Control Shanghai Jiao Tong UniversityShanghai200240People’s Republic of China School of Design Shanghai Jiao Tong UniversityShanghai200240People’s Republic of China

Al-Si alloys manufactured via high-pressure die casting(HPDC)are suitable for a wide range of ***,the heterogeneous microstructure and unpredictable pore distribution of Al-Si high-pressure die castings result in significant variations in the mechanical properties,thus leading to a complicated microstructure-property relationship that is difficult to ***,a computational framework incorporating machine learning and crystal plasticity method is *** framework aims to provide a systematic and comprehensive understanding of this relationship and enable the rapid prediction of macroscopic mechanical properties based on the ***,we select eight variables that can effectively characterize the microstructural features and then obtain their statistical ***,based on 160 samples obtained via the Latin hypercube sampling method,representative volume elements are constructed,and the crystal plasticity fast Fourier transformation method is executed to obtain the macroscopic mechanical ***,the yield strength,elastic modulus,strength coefficient,and strain-hardening exponent are used to characterize the stress-strain curve,and Gaussian process regression models and microstructural variables are ***,sensitivity and univariate analyses based on these machine-learning models are performed to obtain insights into the microstructure-property relationships of the HPDC Al-Si *** results show that the Gaussian process regression models exhibit high accuracy(R2 greater than 0.84),thus confirming the viability of the proposed *** results of sensitivity analysis indicate that the pore size exerts the most significant effect on the mechanical ***,the proposed framework can not only be transferred to other alloys but also be employed for material design.

关键词： High-pressure die casting(HPDC) Machine learning Crystal plasticity Aluminum alloys

Potential therapeutic role of spermine via Rac1 in osteoporosis:Insights from zebrafish and mice

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Zoological research 2024年第2期45卷 367-380页

作者： Rui-Xue Jiang Nan Hu Yu-Wei Deng Long-Wei Hu Hao Gu Nan Luo Jin Wen Xin-Quan Jiang Department of Prosthodontics Shanghai Ninth People’s HospitalShanghai Jiao Tong University School of MedicineShanghai 200011China College of Stomatology Shanghai Jiao Tong UniversityNational Center for StomatologyNational Clinical Research Center for Oral DiseasesShanghai Key Laboratory of StomatologyShanghai Research Institute of StomatologyShanghai Engineering Research Center of Advanced Dental Technology and MaterialsShanghai 200125China Department of Endodontics Shanghai Ninth People’s HospitalShanghai Jiao Tong University School of MedicineShanghai Jiao Tong UniversityShanghai 200011China Department of Oral and Maxillofacial-Head and Neck Oncology Shanghai Ninth People’s HospitalSchool of MedicineShanghai Jiao Tong UniversityShanghai 200011China Department of Preventive Dentistry Shanghai Ninth People’s HospitalShanghai Jiao Tong University School of MedicineShanghai Jiao Tong UniversityShanghai 200011China

Osteoporosis(OP)is a prevalent metabolic bone *** drug therapy is essential to prevent bone loss in osteoporotic patients,current treatments are limited by side effects and high costs,necessitating the development of more effective and safer targeted *** a zebrafish(Danio rerio)larval model of osteoporosis,we explored the influence of the metabolite spermine on bone *** showed that spermine exhibited dual activity in osteoporotic zebrafish larvae by increasing bone formation and decreasing bone *** not only demonstrated excellent biosafety but also mitigated prednisolone-induced embryonic neurotoxicity and ***,spermine showcased protective attributes in the nervous systems of both zebrafish embryos and *** the molecular level,Rac1 was identified as playing a pivotal role in mediating the antiosteoporotic effects of spermine,with P53 potentially acting downstream of *** findings were confirmed using mouse(Mus musculus)models,in which spermine not only ameliorated osteoporosis but also promoted bone formation and mineralization under healthy conditions,suggesting strong potential as a bonestrengthening *** study underscores the beneficial role of spermine in osteoporotic bone homeostasis and skeletal system development,highlighting pivotal molecular *** their efficacy and safety,human endogenous metabolites like spermine are promising candidates for new anti-osteoporotic drug development and daily bone-fortifying agents.

关键词： Osteoporosis Spermine Rac1 Zebrafish Mice

Stretchable poly[2]rotaxane elastomers

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Fundamental research 2024年第2期4卷 300-306页

作者： Kai Liu Xinhai Zhang Dong Zhao Ruixue Bai Yongming Wang Xue Yang Jun Zhao Hao Zhang Wei Yu Xuzhou Yan School of Chemistry and Chemical engineering Frontiers Science Center for Transformative MoleculesShanghai Key Laboratory of Electrical Insulation and Thermal AgingShanghai Jiao Tong UniversityShanghai 200240China College of Chemistry and Chemical engineering National Engineering Research Center for Dyeing and Finishing of TextilesDonghua UniversityShanghai 201620China

Mechanically interlocked polymers(MIPs)are promising candidates for the construction of elastomeric materials with desirable mechanical performance on account of their abilities to undergo inherent rotational and translational mechanical movements at the molecular ***,the investigations on their mechanical properties are lagging far behind their structural fabrication,especially for linear polyrotaxanes in ***,we report stretchable poly[2]rotaxane elastomers(PREs)which integrate numerous mechanical bonds in the polymeric backbone to boost macroscopic mechanical ***,we have synthesized a hydroxyfunctionalized[2]rotaxane that subsequently participates in the condensation polymerization with diisocyanate to form *** from the peculiar structural and dynamic characteristics of the poly[2]rotaxane,the representative PRE exhibits favorable mechanical performance in terms of stretchability(∼1200%),Young’s modulus(24.6 MPa),and toughness(49.5 MJ/m^(3)).Moreover,we present our poly[2]rotaxanes as model systems to understand the relationship between mechanical bonds and macroscopic mechanical *** is concluded that the mechanical properties of our PREs are mainly determined by the unique topological architectures which possess a consecutive energy dissipation pathway including the dissociation of host−guest interaction and consequential sliding motion of the wheel along the axle in the[2]rotaxane motif.

关键词： Polyrotaxanes Mechanically interlocked polymers Mechanically interlocked molecules Dynamic materials Elastomers

Description of martensitic transformation kinetics in Fe-C-X(X = Ni,Cr,Mn,Si) system by a modified model

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International Journal of Minerals,Metallurgy and Materials 2024年第5期31卷 1026-1036页

作者： Xiyuan Geng Hongcan Chen Jingjing Wang Yu Zhang Qun Luo Qian Li State Key Laboratory of Advanced Special Steels&shanghai Key Laboratory of Advanced Ferrometallurgy&School of Materials Science and engineering Shanghai UniversityShanghai 200444China Ansteel Beijing research Institute Co. LtdBeijing 102211China national engineering research center for Magnesium Alloys Chongqing UniversityChongqing 400044China College of Materials Science and engineering Chongqing UniversityChongqing 400044China national Key Laboratory of Advanced Casting Technologies Chongqing UniversityChongqing 400044China

Controlling the content of athermal martensite and retained austenite is important to improving the mechanical properties of high-strength steels,but a mechanism for the accurate description of martensitic transformation during the cooling process must be *** present,frequently used semi-empirical kinetics models suffer from huge errors at the beginning of transformation,and most of them fail to exhibit the sigmoidal shape characteristic of transformation *** describe the martensitic transformation process accurately,based on the Magee model,we introduced the changes in the nucleation activation energy of martensite with temperature,which led to the varying nucleation rates of this model during martensitic *** to the calculation results,the relative error of the modified model for the martensitic transformation kinetics curves of Fe-C-X(X = Ni,Cr,Mn,Si) alloys reached 9.5% compared with those measured via the thermal expansion *** relative error was approximately reduced by two-thirds compared with that of the Magee *** incorporation of nucleation activation energy into the kinetics model contributes to the improvement of its precision.

关键词： Fe-C-X system martensitic transformation kinetics curve semi-empirical model nucleation activation energy

Simulation extractable SNARKs based on target linearly collision-resistant oracle

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Science China(Technological Sciences) 2024年第9期67卷 2853-2866页

作者： WANG LiGuan LI Yuan ZHANG ShuangJun CAI DongLiang KAN HaiBin shanghai Key Laboratory of Intelligent Information Processing School of Computer ScienceFudan UniversityShanghai 200433China shanghai engineering research center of Blockchain Shanghai 200433China Yiwu research Institute of Fudan University Yiwu 322000China

The famous zero-knowledge succinct non-interactive arguments of knowledge(zk-SNARK) was proposed by Groth in ***, the construction is based on quadratic arithmetic programs which are highly efficient concerning the proof length and the verification complexity. Since then, there has been much progress in designing zk-SNARKs, achieving stronger security,and simulated extractability, which is analogous to non-malleability and has broad applications. In this study, following Groth's pairing-based zk-SNARK, a simulation extractability zk-SNARK under the random oracle model is constructed. Our construction relies on a newly proposed property named target linearly collision-resistant, which is satisfied by random oracles under discrete logarithm assumptions. Compared to the original Groth16 zk-SNARK, in our construction, both parties are allowed to use such a random oracle, aiming to get the same random number. The resulting proof consists of 3 group elements and only 1 pairing equation needs to be verified. Compared to other related works, our construction is shorter in proof length and simpler in verification while preserving simulation extractability. The results also extend to achieve subversion zero-knowledge SNARKs.

关键词： quadratic arithmetic program simulation extractability subversion zero-knowledge succinct non-interactive arguments of knowledge target linearly collision-resistant

Lactobacillus plantarum AR113 attenuates liver injury in D-galactose-induced aging mice via the inhibition of oxidative stress and endoplasmic reticulum stress

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Food Science and Human Wellness 2024年第2期13卷 885-897页

作者： Yongjun Xia Yujie Gong Xiangna Lin Yijin Yang Xin Song Guangqiang Wang Zhiqiang Xiong Yangyang Qian Zhuan Liao Hui Zhang Lianzhong Ai School of Health Science and engineering Shanghai Engineering Research Center of Food MicrobiologyUniversity of Shanghai for Science and TechnologyShanghai 200093China College of Life Sciences Linyi UniversityLinyi 276000China Department of Gastroenterol. Digestive Endoscopy CenterChanghai HospitalShanghai 200082China

Probiotics could effectively eliminate excess reactive oxygen species(ROS)generated during aging or lipid metabolism disorders,but their mechanism is *** major purpose of this study was to investigate the mechanism of Lactiplantibacillus plantarun AR113 alleviating oxidative stress injury in the D-galactose induced aging *** result showed that pretreatment with *** AR113 significantly relieving H_(2)O_(2)induced cytotoxicity in HepG2 cells by maintain cell membrane integrity and increasing antioxidant enzyme *** D-galactose induced aging mice,*** AR113 could significantly attenuate liver damage and inflammatory infiltration by promoting endogenous glutathione(GSH)synthesis and activating the Nrf2/Keap1 signaling pathway in mice,and increasing the expression of regulated phaseⅡdetoxification enzymes and antioxidant *** analysis shown that gavage of *** AR113 could significantly reduce the expression of G protein-coupled receptor 78(GPR78)and C/EBP homologous protein(CHOP)proteins,and promote the restoration of endoplasmic reticulum(ER)homeostasis,thereby activating cell anti-apoptotic *** results were also confirmed in H_(2)O_(2)-treated HepG2 *** indicated that *** AR113 could inhibit D-galactose-induced liver injury through dual inhibition of ER stress and oxidative *** AR113 have good application potential in anti-aging and alleviating metabolic disorders.

关键词： Lactiplantibacillus plantarun AR113 HepG2 D-galactose Oxidative stress ER stress

New insights into the pre-lithiation kinetics of single-crystalline Ni-rich cathodes for long-life Li-ion batteries

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Green Energy & Environment 2024年第3期9卷 556-564页

作者： Qiang Han Lele Cai Zhaofeng Yang Yanjie Hu Hao Jiang Chunzhong Li shanghai engineering research center of Hierarchical Nanomaterials School of Chemical EngineeringEast China University of Science and TechnologyShanghai200237China Key Laboratory for Ultrafine Materials of Ministry of Education School of Materials Science and EngineeringEast China University of Science and TechnologyShanghai200237China

Developing single-crystalline Ni-rich cathodes is an effective strategy to improve the safety and cycle life of Li-ion batteries(LIBs).However,the easy-to-loss of Li and O in high-temperature lithiation results in unsatisfactory ordered layered structure and ***,we demonstrate the synthesis of highly-ordered and fully-stoichiometric single-crystalline LiNi_(0.83)Co_(0.12)Mn_(0.05)O_(2)(SC-NCM83)cathodes by the regulation of pre-lithiation *** well-balanced pre-lithiation kinetics have been proved to greatly improve the proportion of layered phase in the intermediate by inhibiting the formation of metastable spinel phase,which promoted the rapid transformation of the intermediate into highly-ordered layered SC-NCM83 in the subsequent lithiation *** coating a layer of Li_(2)O–B_(2)O_(3),the resultant cathodes deliver superior cycling stability with 90.9%capacity retention at 1C after 300 cycles in pouch-type full *** enhancement mechanism has also been *** findings exhibit fundamental insights into the pre-lithiation kinetics process for guiding the synthesis of high-quality singlecrystalline Ni-rich cathodes.

关键词： Single-crystalline cathode Ni-rich oxides Pre-lithiation Li-ion batteries Surface modification

Experimental Study on engineering Behavior of Solidified Soil for Scour Repair and Protection

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China Ocean engineering 2024年第4期38卷 625-635页

作者： WU Xiao-ni LI Ru-yu SHU Jian TANG Chao CHEN Jin-jian WANG Hui-li JIANG Hai-li WANG Xiao State Key Laboratory of Ocean engineering Department of Civil EngineeringShanghai Jiao Tong UniversityShanghai 200240China shanghai Road and Bridge Group Co. Ltd.Shanghai 200433China shanghai engineering research center of Urban Infrastructure Renewal Shanghai 200032China Jiangsu Kunze Technology Co. Ltd.Nanjing 210000China

A new scour countermeasure using solidified slurry for offshore foundation has been proposed *** solidified slurry is pumped to seabed area around foundation for scour protection or pumped into the developed scour holes for scour repair as the fluidized material solidifies *** the pumping operation and solidification,the engineering behaviors of solidified slurry require to be considered synthetically for the reliable application in scour repair and protection of ocean engineering such as the pumpability related flow value,flow diffusion behavior related rheological property,anti-scour performance related retention rate in solidification and bearing capacity related strength property after *** this study,a series of laboratory tests are conducted to investigate the effects of mix proportion(initial water content and binder content)on the flow value,rheological properties,density,retention rate of solidified slurry and unconfined compressive strength(UCS).The results reveal that the flow value increases with the water content and decreases with the binder *** the solidified slurry exhibits Bingham plastic behavior when the shear rate is larger than 5 s^(-1).The Bingham model has been employed to fit the rheology test results,and empirical formulas for obtaining the density,yield stress and viscosity are established,providing scientific support for the numerical assessment of flow and diffusion of solidified *** rate of solidified slurry decreases with the water flow velocity and flow value,which means the pumpability of solidified slurry is contrary to anti-scour *** unconfined compressive strength after solidification reduces as the water content increases and binder content decreases.A design and application procedure of solidified soil for scour repair and protection is also proposed for engineering reference.

关键词： scour repair and protection solidified soil pumpability strength flow properties anti-scour performance

On-chip source-device-independent quantum random number generator

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Photonics research 2024年第7期12卷 1379-1394页

作者： LANG LI MINGLU CAI TAO WANG ZICONG TAN PENG HUANG KAN WU GUIHUA ZENG State Key Laboratory of Advanced Optical Communication Systems and Networks Shanghai Jiao Tong UniversityShanghai 200240China Institute of Quantum Sensing and Information Processing School of Sensing Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China shanghai research center for Quantum Sciences Hefei National LaboratoryShanghai 201315China shanghai Xun Tai Quantech Co. Ltd.Shanghai 200241China

Quantum resources offer intrinsic randomness that is valuable for applications such as cryptography, scientific simulation, and computing. Silicon-based photonics chips present an excellent platform for the cost-effective deployment of next-generation quantum systems on a large scale, even at room temperature. Nevertheless,the potential susceptibility of these chips to hacker control poses a challenge in ensuring security for on-chip quantum random number generation, which is crucial for enabling extensive utilization of quantum resources.

关键词： temperature quantum random