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Electrochemical conversion of methane to bridge the gap in the artificial carbon cycle

Journal of Energy Chemistry 2025年第1期100卷 286-308页

作者： Yuhao Peng Yuefeng Song Ihar Razanau Juanxiu Xiao Wei Xiao Di Hu Guoxiong Wang College of Chemistry and Molecular Sciences Hubei Key Laboratory of Electrochemical Power Sources Wuhan University State Key Laboratory of Catalysis Dalian National Laboratory for Clean Energy iChEM (Collaborative Innovation Center of Chemistry for Energy Materials) Dalian Institute of Chemical Physics Chinese Academy of Sciences Laboratory of Physical-Chemical Technologies SSPA Scientific and Practical Materials Research Centre of NAS of Belarus State Key Laboratory of Marine Resources Utilization in South China Sea Collaborative Innovation Center of Marine Science and Technology School of Marine Science and Engineering Hainan University Department of Chemical and Environmental Engineering University of Nottingham Ningbo China

Methane, an abundant one-carbon（C1） resource, is extensively used in the industrial production of vital fuels and value-added chemicals. However, current industrial methane conversion technologies are energy-and carbon-intensive, mainly due to the high activation energy required to break the inert C–H bond, low selectivity, and problematic side reactions, including CO2emissions and coke deposition. Electrochemical conversion of methane（ECM） using intermittent renewable energy offers an attractive solution, due to its modular reactor design and operational flexibility across a broad spectrum of temperatures and pressures. This review emphasizes conversion pathways of methane in various reaction systems, highlighting the significance and advantages of ECM in facilitating a sustainable artificial carbon cycle. This work provides a comprehensive overview of conventional methane activation mechanisms and delineates the complete pathways of methane conversion in electrolysis contexts. Based on surface/interface chemistry, this work systematically analyzes proposed reaction pathways and corresponding strategies to enhance ECM efficiency towards various target products, including syngas, hydrocarbons, oxygenates, and advanced carbon materials. The discussion also encompasses opportunities and challenges for the ECM process, including insights into ECM pathways, rational electrocatalyst design, establishment of benchmarking protocols, electrolyte engineering, enhancement of CH4conversion rates, and minimization of CO2emission.

关键词： Activation energy

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A deep learning approach for spatial error correction of numerical seasonal weather prediction simulation data

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Big Earth Data 2023年第2期7卷 231-250页

作者： Stelios Karozis Iraklis A.Klampanos Athanasios Sfetsos Diamando Vlachogiannis Environmental research Laboratory(EREL) INRaSTESNational Centre for Scientific Research“Demokritos”AthensGreece Institute of Informatics and Telecommunications National Centre for Scientific Research“Demokritos”AthensGreece

Numerical Weather Prediction(NWP)simulations produce meteorological data in various spatial and temporal scales,depending on the application *** the current study,a deep learning approach,based on convolutional autoencoders,is explored to effectively correct the error of the NWP *** undercomplete convolutional autoencoder(CAE)is applied as part of the dynamic error correction of NWP *** work is an attempt to improve the seasonal forecast(3-6 months ahead)data accuracy for Greece using a global reanalysis dataset(that incorporates observations,satellite imaging,etc.)of higher spatial *** specifically,the publically available Meteo France Seasonal(Copernicus platform)and the national Centers for Environmental Prediction(NCEP)Final Analysis(FNL)(NOAA)datasets are *** addition,external information is used as evidence transfer,concerning the time conditions(month,day,and season)and the simulation characteristics(initialization of simulation).It is found that convolutional autoencoders help to improve the resolution of the seasonal data and successfully reduce the error of the NWP data for 6-months ahead ***,the month evidence yields the best agreement indicating a seasonal dependence of the performance.

关键词： Seasonal weather prediction neural networks convolutional autoencoder evidence transfer

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Energy Efficiency of a Solar Green Building Using Bio-Sourced Materials for Indoor Temperature and Humidity Optimization

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Energy Engineering 2025年第1期122卷 41-62页

作者： SoumiaMounir Youssef Maaloufa Abdelhamid Khabbazi ElinaMohd Husini Nurul SyalaAbdul Latip YakubuAminuDodo Rime ELHarrouni MinaAmazal Asma Souidi Malika Atigui Ahmed Aharoune national School of Architecture Agadir New Complex Ibn ZohrAgadirBP 20732Morocco EMDD CERNE2DUniversity of Mohammed V in RabatEst SaleSaleBP 227Morocco Thermodynamics and Energetics Laboratory Faculty of ScienceIbn Zohr UniversityAgadirBP 8106Morocco Faculty of Built Environment University Sains Islam MalaysiaNilaiBP 71800Malaysia Architectural Engineering Department Najran UniversityNajranBP 1988Saudi Arabia The centre of scientific and Engineering research Najran UniversityNajranBP 1988Saudi Arabia Euro-Mediterranean School of Architecture Design and UrbanismEuro-Mediterranean University of FezFezBP 51Morocco

A clean environment with low carbon emissions is the goal of research on the development of green and sustainable buildings that use bio-sourced materials in conjunction with solar energy to create more sustainable *** is particularly true in Africa,where there aren’t many studies on the *** current study suggests a 90 m^(2) model of a sustainable building in a dry climate that is movable to address the issue of housing in remote areas,ensures comfort in harsh weather conditions,uses solar renewable resources—which are plentiful in Africa—uses biosourced materials,and examines how these materials relate to temperature and humidity control while emitting minimal carbon *** order to solve the topic under consideration,the work is split into two sections:numerical and experimental *** TRNSYS and Revit,the suggested prototype building is examined numerically to examine the impact of orientation,envelope composition made of bio-sourced materials,and carbon *** a hygrothermal investigation,experiments are conducted to evaluate this prototype’s ***,an examination of the photovoltaic system’s production,consumption,and several scenarios used tomaximize battery life is included in the *** the biosourcedmaterial achieves a thermal transmittance of 0.15(W.m^(-2).K^(-1)),the results demonstrate an intriguing finding in terms of *** value satisfies the requirements of passive building,energy autonomy of the dwelling,and injection in-network with an annual value of 15,757 ***,compared to the literature,the heating needs ratio is 6.38(kWh/m^(2).an)and the cooling needs ratio is 49(kWh/m^(2).an),both of which are good *** to international norms,the inside temperature doesn’t go above 26℃,and the humidity level is within a comfortable range.

关键词： Bio-sourced materials energy sustainability green architecture built environment

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The influence of canopy-layer composition on understory plant diversity in southern temperate forests

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Forest Ecosystems 2017年第2期4卷 154-166页

作者： Luciana Mestre Monica Toro-Manriquez Rosina Soler Alejandro Huertas-Herrera Guillermo Martinez-Pastur Maria Vanessa Lencinas national scientific and technical research Council (CONICET) Austral Center for Scientific Research (CADIC-CONICET) Houssay 200 9410 Ushuaia Tierradel Fuego Argentina

Background： Understory plants represents the largest component of biodiversity in most forest ecosystems and plays a key role in forest *** their importance, the influence of overstory-layer composition on understory plant diversity is relatively poorly understood within deciduous-evergreen broadleaved mixed *** aim of this work was to evaluate how tree overstory-layer composition influences on understory-layer diversity in three forest types（monospecific deciduous Nothofagus pumilio（Np）, monospecific evergreen Nothofagus betuloides（Nb）, and mixed ***（M） forests）, comparing also between two geographical locations（coast and mountain） to estimate differences at landscape ***： We recorded 46 plant species： 4 ferns, 12 monocots, and 30 ***-layer composition influences the herb-layer structure and diversity in two different ways： while mixed forests have greater similarity to evergreen forests in the understory structural features, deciduous and mixed were similar in terms of the specific composition of plant *** pure stands were the most diverse, meanwhile evergreen stands were least *** of exclusive species of mixed forest could represent a transition where evergreen and deciduous communities meet and ***, landscape has a major influence on the structure, diversity and richness of understory vegetation of pure and mixed forests likely associated to the magnitude and frequency of natural disturbances, where mountain forest not only had highest herb-layer diversity but also more exclusive ***： Our study suggests that mixed Nothofagus forest supports coexistence of both pure deciduous and pure evergreen understory plant species and different assemblages in coastal and mountain *** the mixture of canopy patch types within mixed stands will be important for conserving the natural patterns of understory plant composition in southern beech mixe

关键词： Landscape Understory communities Understory structure Forest structure Nothofagus Conservation

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A catalyst-free new polyol method synthesized hot-pressed Cu-doped Bi2S3 nanorods and their thermoelectric properties

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Nano research 2016年第11期9卷 3291-3304页

作者： Tarachand Vikash Sharma Ranu Bhatt Vedachalaiyer Ganesan Gunadhor Singh Okram UGC-DAE Consortium for scientific research Indore 452001 India technical Physics Division Bhabha Atomic Research Centre Mumbai 400085 India

This is the first report on the thermoelectric properties of a catalyst-free polyol method used to prepare stoichiometric Bi2-xCuxS3 samples, x = 0.1, 0.2, 0.3, 0.4, via hot pressing. Various systematic approaches to arrive at in their stoichiometric compositions are explored precisely with introduction of excess precursor of S. X-ray diffraction data analysis using Rietveld refinement confirms a polyhedral orthorhombic crystal structure with a space group Pnma, in contrast to Pbnm reported earlier. Raman data further substantiates this. X-ray photoelectron spectroscopy confirms the valence states of the constituent elements （Bi^3＋, Cu^2＋, and S^2-） and energy dispersive X-ray analysis corroborates their compositions. The particle sizes of the pure Bi2S3 nanoparticles were 20, 35, and 82 nm as determined from the Scherrer formula, atomic force microscopy, and dynamic light scattering, respectively. Their transmission electron microscopy image shows rod-like nanostructures elongated in the 〈010〉 direction with an average diameter of 23 nm and a length of several hundreds of nanometers. A 34% improvement in the thermoelectric figure of merit is observed for Bi.6Cu0.4S3 as compared to pure Bi2S3 at 300 K.

关键词： Bi2S3 polyol nanorods thermoelectrics

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Simulation of erosion-deposition processes at basin scale by a physically-based mathematical model

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International Journal of Sediment research 2010年第2期25卷 91-109页

作者： Pedro A. BASILE Gerardo A. RICCARDI Erik D. ZIMMERMANN Hernán R. STENTA Hydraulics Department School of Civil EngineeringNational University of Rosario research Scientist Centre for Hydro-Environmental ResearchNational University of Rosario research Scientist Research Council of National University of Rosario(CIUNR) research Scientist National Council of Scientific and Technical Research(CONICET)

The development and application of the physically-based and spatially-distributed mathematical model CTSS8-SED is presented. The model simulates hydrologic-hydraulic processes produced by storm events and related soil erosion and sediment transport processes at basin scale in lowland areas. The model simulates (i) storm runoff,(ii) soil detachment by raindrop impact and overland flow (gross sediment yield),(iii) sediment transport by overland flow and associated erosion-deposition processes and (iv) sediment transport by stream flow and riverbed erosion-deposition processes. A quasi two-dimensional representation of water flow and sediment transport routing is made by means of interconnected cells approach. The model is applied to simulate two flooding events in the Luduea Creek basin (Santa Fe, Argentina) occurred in April 1994 and March 2007 due to extraordinary rainfalls.

关键词： Mathematical modeling Erosion Sedimentation Ludue?a Creek Argentina

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Protective effects of D-002 on experimentally induced gastroesophageal reflux in rats

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World Journal of Gastroenterology 2014年第8期20卷 2085-2090页

作者： Zullyt Zamora Vivian Molina Rosa Mas Yazmin Ravelo Yohany Perez Ambar Oyarzabal Department of Pharmacology Centre of Natural ProductsNational Centre for Scientific ResearchHavana 10600Cuba

AIM: To investigate the effects of beeswax alcohols (D-002) on the esophageal damage induced by gastroesophageal reflux (GER) in rats.

关键词： D-002 Beeswax alcohols Esophagitis Gastroesophageal reflux Oxidative stress

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Effectiveness of sodium silicate as gangue depressants in iron ore slimes flotation

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International Journal of Minerals,Metallurgy and Materials 2011年第5期18卷 515-522页

作者： Danda Srinivas Rao Tadiparthi Venkata VijayaKumar Sripada Subba Rao Swarna Prabhakar Guntamadugu Bhaskar Raju national Metallurgical Laboratory-Madras centre Council of Scientific and Industrial Research-Madras ComplexChennai 600 113India

The recovery of iron from the screw classifier overflow slimes by direct flotation was studied. The relative effectiveness of sodium silicates with different silica-to-soda mole ratios as depressants for silica and silicate bearing minerals was investigated. Silica-to-soda mole ratio and silicate dosage were found to have significant effect on the separation efficiency. The results show that an increase of Fe content in the concentrate is observed with concomitant reduction in SiO2 and A1203 levels when a particular type of sodium silicate at a proper dosage is used. The concentrate of 58.89wt% Fe, 4.68wt% SiO2, and 5.28wt% A1203 with the weight recovery of 38.74% and the metal recovery of 41.13% can be obtained from the iron ore slimes with 54.44wt% Fe, 6.72wt% SiO2, and 6.80wt% A1203, when NazSiO3 with a silica-to-soda mole ratio of 2.19 is used as a depressant at a feed rate of 0.2 kg/t.

关键词： iron ores sodium silicate depressants flotation

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Repurposing drugs to target nonalcoholic steatohepatitis

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World Journal of Gastroenterology 2019年第15期25卷 1783-1796页

作者： Silvia Sookoian Carlos J Pirola Department of Clinical and Molecular Hepatology National Scientific and Technical Research Council (CONICET) University of Buenos Aires Institute of Medical Research (IDIM) Department of Molecular Genetics and Biology of Complex Diseases National Scientific and Technical Research Council (CONICET) University of Buenos Aires Institute of Medical Research (IDIM)

Nonalcoholic fatty liver disease(NAFLD) is a complex disorder that has evolved in recent years as the leading global cause of chronic liver damage. The main obstacle to better disease management pertains to the lack of approved pharmacological interventions for the treatment of nonalcoholic steatohepatitis(NASH) and NASH-fibrosis-the severe histological forms. Over the past decade,tremendous advances have been made in NAFLD research, resulting in the discovery of disease mechanisms and novel therapeutic targets. Hence, a large number of pharmacological agents are currently being tested for safety and efficacy. These drugs are in the initial pharmacological phases(phase 1 and 2),which involve testing tolerability, therapeutic action, and pharmacological *** is thus reasonable to assume that the next generation of NASH drugs will not be available for clinical use for foreseeable future. The expected delay can be mitigated by drug repurposing or repositioning, which essentially relies on identifying and developing new uses for existing drugs. Here, we propose a drug candidate selection method based on the integration of molecular pathways of disease pathogenesis into network analysis tools that use OMICs data as well as multiples sources, including text mining from the medical literature.

关键词： Drug discovery Drug repositioning Fibrosis Genetics Treatment Systems biology

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Kairomonal effect of sex pheromone components of two lepidopteran olive pests on Trichogramma wasps

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Insect Science 2009年第2期16卷 131-136页

作者： Panos Milonas Basilios E. Mazomenos Maria A. Konstantopoulou Chemical Ecology and Natural Products Laboratory Institute of Biology National Centre of Scientific Research 'Demokritos' Attikis Greece

Egg parasitoids are known to use a wide range of chemicals, emitted by plants, host eggs or adults, for host selection. The effect of the sex pheromone components of the lepidopteran olive pests Prays oleae （Lepidoptera： Yponomeutidae） and Palpita unionalis （Lepidoptera： Pyralidae） was studied under laboratory conditions, on the foraging behaviour of the egg parasitoid Trichogramma oleae （Hymenoptera： Trichogrammatidae）. The re- sponse of T. oleae wasps to （Z）-7-tetradecenal and （E）-1 l-hexadecenal, major sex phero- mone components ofP. oleae and P. unionalis respectively, depended on the dose of the pheromone used in a Y-tube olfactometer bioassay. （E）-11-hexadecenal elicited maximum attraction （70%） at a dose of 1 pg, while a dose of 100 pg （Z）-7-tetradecenal attracted 80% of the tested wasps. （E）-11-hexadecenyl acetate, the second sex pheromone component of P. unionalis, and the binary blend of（E）-i 1-hexadecenyl acetate：（E）-11-hexadecenal （7：3） were not attractive at these doses. The results of this research are discussed in view that they may be considered as alternatives in the biological control of these pests.

关键词： egg parasitoids olive pest semiochemicals Y-tube olfactometer

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