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Degradation of carbamazepine by the UVA-LED_(365)/ClO_(2)/NaClO process:Kinetics,mechanisms and DBPs yield

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Journal of Environmental Sciences 2025年第2期148卷 399-408页

作者： Chenyan Hu Yihui Wu Zhengyu Dong Ziyi Dong Shengjie Ji Lili Hu Xinyu Yang Hao Liu College of Environmental and Chemical engineering Shanghai Engineering Research Center of EnergySaving in Heat Exchange SystemsShanghai University of Electric PowerShanghai 200090China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China

A mixed oxidant of chlorine dioxide(ClO_(2))and NaClO was often used in water treatment.A novel UVA-LED(_(365) nm)-activated mixed ClO_(2)/NaClO process was proposed for the degradation of micropollutants in this ***(CBZ)was selected as the target *** with the UVA_(365)/ClO_(2) process,the UVA_(365)/ClO_(2)/NaClO process can improve the degradation of CBZ,with the rate constant increasing from 2.11×10^(−4) sec^(−1) to 2.74×10^(−4) sec^(−1).In addition,the consumption of oxidants in the UVA_(365)/ClO_(2)/NaClO process(73.67%)can also be lower than that of UVA_(365)/NaClO(86.42%).When the NaClO ratio increased,both the degradation efficiency of CBZ and the consumption of oxidants can increase in the UVA_(365)/ClO_(2)/NaClO *** solution pH can affect the contribution of NaClO in the total oxidant *** the pH range of 6.0-8.0,the combination process can generate more active species to promote the degradation of *** change of active species with oxidant molar ratio was investigated in the UVA_(365)/ClO_(2)/NaClO *** ClO_(2) acted as the main oxidant,HO·and Cl·were the main active species,while when NaClO was the main oxidant,ClO·played a role in the *** chloride ion(Cl^(-)),bicarbonate ion(HCO_(3)^(-)),and nitrate ion(NO_(3)^(-))can promote the reaction *** the concentration of NaClO in the reaction solution increased,the generation of chlorates will *** UVA_(365)/ClO_(2)/NaClO process can effectively control the formation of volatile disinfection by-products(DBPs),and with the increase of ClO_(2) dosage,the formation of DBPs can also decrease.

关键词： UVA Chlorine dioxide(ClO_(2)) NaClO Carbamazepine(CBZ) Disinfection by-products

Coordinated Control Strategy of New Energy Power Generation System with Hybrid Energy Storage Unit

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Energy engineering 2025年第1期122卷 167-184页

作者： Yun Zhang Zifen Han Biao Tian Ning Chen Yi Fan School of Mechano-Electronic engineering Xidian UniversityXi’an710071China electric Power Control center State Grid Gansu Electric Power CompanyLanzhou730030China electric Power Control center State Grid Gansu Electric Power Company Zhangye Power Supply BranchZhangye734000China

The new energy power generation is becoming increasingly important in the power *** as photovoltaic power generation has become a research hotspot,however,due to the characteristics of light radiation changes,photovoltaic power generation is unstable and random,resulting in a low utilization rate and directly affecting the stability of the power *** solve this problem,this paper proposes a coordinated control strategy for a newenergy power generation system with a hybrid energy storage unit based on the lithium iron phosphate-supercapacitor hybrid energy storage ***,the variational mode decomposition algorithm is used to separate the high and low frequencies of the power signal,which is conducive to the rapid and accurate suppression of the power fluctuation of the energy storage ***,the fuzzy control algorithm is introduced to balance the power between energy *** this paper,the actual data is used for simulation,and the simulation results show that the strategy realizes the effective suppression of the bus voltage fluctuation and the accurate control of the internal state of the energy storage unit,effectively avoiding problems such as overshoot and over-discharge,and can significantly improve the stability of the photovoltaic power generation systemand the stability of the Direct Current *** is of great significance to promote the development of collaborative control technology for photovoltaic hybrid energy storage units.

关键词： Photovoltaic power suppression hybrid energy storage unit variationalmodal decomposition fuzzy control power distribution control

Co-production of hydrogen, oxygen, and electricity via an integrated solar-driven system with decoupled water electrolyzer and Na-Zn ion battery

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Journal of Energy Chemistry 2025年第1期100卷 621-627页

作者： Fei Lv Longjie Liu Jiazhe Wu Pengfei Wang Lixia Pan Dengwei Jing Yubin Chen International research center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049ShaanxiChina

Combining water electrolysis and rechargeable battery technologies into a single system holds great promise for the co-production of hydrogen (H_(2)) and ***,the design and development of such systems is still in its ***,an integrated hydrogen-oxygen (O_(2))-electricity co-production system featuring a bipolar membrane-assisted decoupled electrolyzer and a Na-Zn ion battery was established with sodium nickelhexacyanoferrate (NaNiHCF) and Zn^(2+)/Zn as dual redox *** decoupled electrolyzer enables to produce H_(2)and O_(2)in different time and space with almost 100%Faradaic efficiency at 100 mA cm^(-2).Then,the charged NaNiHCF and Zn electrodes after the electrolysis processes formed a Na-Zn ion battery,which can generate electricity with an average cell voltage of 1.75 V at 10 m A cm^(-2).By connecting Si photovoltaics with the modular electrochemical device,a well-matched solar driven system was built to convert the intermittent solar energy into hydrogen and electric energy with a solar to hydrogen-electricity efficiency of 16.7%,demonstrating the flexible storage and conversion of renewables.

关键词： Hydrogen electricity Decoupled water electrolyzer Na-Zn ion battery Solar energy

Lattice distortion enhanced self-trapped excitons emission in antimony halide crystalline clusters

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Science China Materials 2025年第1期68卷 132-140页

作者： Da Liu Jingjing He Yuting Sun Xinyi Liu Yu Peng Qing Li Hua Gui Yang Qiang Niu Shuang Yang Yu Hou Key Laboratory for Ultrafine Materials of Ministry of Education Shanghai Engineering Research Center of Hierarchical NanomaterialsSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China China national Enterprise Technology center Inner Mongolia Erdos Electric Power and Metallurgy Group Company LimitedOrdos 016064China

Zero-dimensional perovskite materials,characterized by broadband emission caused by self-trapped excitons,are promising materials for stimuli-responsive and photo-writeable ***,existing research is focused on the effects of structural phase transitions on photophysical properties,and lacks in-depth understanding of the mechanisms of self-trapped excitons ***,we demonstrate that the dehydration reaction in zero-dimensional antimony halide clusters significantly enhances the self-trapped excitons emission without inducing structural phase transition,resulting in a substantial increase in photoluminescence(PL)quantum yield from 3.5%to 91.4%.In-situ X-ray diffraction and PL techniques were employed to shed light on the relationship between the crystal structure and radiative recombination,demonstrating the introduction of rich lattice distortion during the dehydration ***-dependent PL spectra and transient absorption spectra suggest that the lattice distortion causes the moderate electron-phonon coupling strength and high exciton binding energy,facilitating self-trapped excitons to relax from the non-radiative recombination singlet state to the radiative recombination triplet state,corresponding to the enhanced emission *** a proof of concept,several switchable PL applications have been established in scenarios such as anti-counterfeiting,rewritable luminescent paper,and humidity *** finding elucidates the emission mechanism of self-trapped excitons and provides a novel avenue for designing switchable luminescent materials.

关键词： self-trapped excitons zero-dimensional perovskite antimony halides lattice distortion photoluminescence quantum yield

Status analysis on sputtering and erosion evaluation methods of ion optic systems

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Chinese Journal of Aeronautics 2025年第1期38卷 254-270页

作者： Long MIAO Tongxun YANG Zhengxi ZHU Chang LU Zhiwen WU Ningfei WANG School of Aerospace engineering Beijing Institute of TechnologyBeijing 100081China Chongqing Innovation center Beijing Institute of TechnologyChongqing 404100China Advanced Aerospace Power and Energy research center Beijing Institute of TechnologyZhuhai 519088China

In the past few decades,ion engines have been widely used in deep-space propulsion and satellite *** aim of extending the thruster lifetime is still one of the most important parts during the design stage of ion *** one of the core components of ion engine,the grid assembly of ion optic systems may experience long-term ion sputtering in extreme electro-thermal environments,which will eventually lead to its structural and electron-backstreaming *** this paper,the current studies of the grid assembly erosion process are systematically analyzed from the aspects of sputtering damage process of grid materials,numerical simulations,and measurements of erosion characteristics of grid *** advantages and disadvantages of various erosion prediction models are highlighted,and the key factors and processes affecting the prediction accuracy of grid assembly erosion patterns are *** different types of experimental methods of grid assembly erosion patterns are *** analysis in this paper is of great importance for selecting the sputter-resistant grid materials,as well as establishing the erosion models and measurement methods to accurately determine the erosion rate and failure modes of grid ***,the working conditions and structure parameters of ion optic systems could be optimized based on erosion models to promote the ion engine lifetime.

关键词： electric propulsion Ion optic systems Sputtering yield Erosion characteristics Erosion pattern measurement Lifetime evaluation

Intermetallic compounds for nitrogen electrochemistry

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Green Energy & Environment 2025年第2期10卷 268-291页

作者： Haohong Wei Cheng Tang Yanyun Wang Yongcheng Feng Huancong Shi Mingjin Cui Huakun Liu Shixue Dou Laiquan Li Institute of Energy Materials Science School of Energy and Power EngineeringUniversity of Shanghai Science and TechnologyShanghai200093China Tsinghua center for Green Chemical engineering Electrification(CCEE) Department of Chemical EngineeringTsinghua UniversityBeijing100084China State Grid New Energy Cloud Carbon Neutralization Innovation center State Grid Zhejiang Electric Power Co.LtdHuzhou Power Supply CompanyZhejiang313000China Shanghai Marine Diesel Engine research Institute.Shanghai 201108China

Electrochemical nitrogen transformation techniques represent a burgeoning avenue for nitrogen pollutant remediation and synthesizing valuable nitrogenous products from atmospheric *** compounds(IMCs)nanocrystals,featured with unique geometric,electronic and functional properties,have emerged as promising *** review discusses various synthesis approaches for IMCs,including thermal annealing,wet chemical synthesis,electrochemical synthesis,and other emerging methods,analyzing their advantages and *** we summarized the recent advances of IMCs in electrocatalytic nitrogen transformation reactions,such as nitrate reduction reaction,nitric oxide reduction reaction,nitrogen reduction reaction,and hydrazine oxidation *** significant progress,challenges remain in the field,particularly in adopting more refined strategies to improve catalyst performance and *** review aims to comprehensively understand the structural properties of IMCs and their structure-performance relationship,guiding the development of more efficient and stable catalysts for future nitrogen electrochemistry.

关键词： Intermetallic compounds Electrocatalysis Nitrogen transformation reactions Synthesis methods Catalyst design

Multi-Stage Voltage Control Optimization Strategy for Distribution Networks Considering Active-Reactive Co-Regulation of electric vehicles

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Energy engineering 2025年第1期122卷 221-242页

作者： Shukang Lyu Fei Zeng Huachun Han Huiyu Miao Yi Pan Xiaodong Yuan electric Power research Institute State Grid Jiangsu Electric Power Co.Ltd.Nanjing211103China

The high proportion of uncertain distributed power sources and the access to large-scale random electric vehicle(EV)charging resources further aggravate the voltage fluctuation of the distribution network,and the existing research has not deeply explored the EV active-reactive synergistic regulating characteristics,and failed to realize themulti-timescale synergistic control with other regulatingmeans,For this reason,this paper proposes amultilevel linkage coordinated optimization strategy to reduce the voltage deviation of the distribution ***,a capacitor bank reactive power compensation voltage control model and a distributed photovoltaic(PV)activereactive power regulationmodel are ***,an external characteristicmodel of EVactive-reactive power regulation is developed considering the four-quadrant operational characteristics of the *** optimization model of the distribution network is then constructed considering the time-series coupling constraints of multiple types of voltage regulators.A multi-timescale control strategy is proposed by considering the impact of voltage regulators on active-reactive EV energy consumption and PV energy ***,a four-stage voltage control optimization strategy is proposed for various types of voltage regulators with multiple time ***-objective optimization is solved with the improvedDrosophila algorithmto realize the power fluctuation control of the distribution network and themulti-stage voltage control *** results validate that the proposed voltage control optimization strategy achieves the coordinated control of decentralized voltage control resources in the distribution *** effectively reduces the voltage deviation of the distribution network while ensuring the energy demand of EV users and enhancing the stability and economic efficiency of the distribution network.

关键词： electric vehicle(EV) distribution network multi-stage optimization active-reactive power regulation voltage control

Mapping the territories of the mountain-foothill zone of Tajikistan exposed to mudflows

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Journal of Mountain Science 2025年第1期22卷 16-30页

作者： SAFAROV Mustafo KANG Shichang FAZYLOV Ali GULAYOZOV Majid NAVRUZSHOEV Hofiz BANERJEE Abhishek MAMADJANOV Yunus Key Laboratory of Cryospheric Science and Frozen Soil engineering Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China research center for Ecology and Environment of Central Asia(Dushanbe) Dushanbe 734063Tajikistan University of Chinese Academy of Sciences Beijing 100049China Institute of Water Problems Hydropower and Ecology of the National Academy of Sciences of TajikistanDushanbe 734042Tajikistan Mountain Societies research Institute University of Central AsiaDushanbe 734000Tajikistan State Scientific Institution“center for research of Glaciers of the national Academy of Sciences of Tajikistan” Dushanbe 734025Tajikistan

In recent years,mudflows have emerged as a significant threat to infrastructure and lives,exhibiting increased frequency and *** study collectively addresses the rising threat of natural hazards,specifically mudflows in mountain-foothill zones in Tajikistan,utilizing UAV and remote sensing technologies to monitor their *** 2020 to 2023,we employed a QC-2 Micro UAV and a DJI Phantom 4 quadcopter to capture high-resolution aerial imagery across multiple affected districts,supplemented by pre-and post-event Sentinel-2 images analyzed using the Normalized Difference Water Index(NDWI)and Normalized Difference Vegetation Index(NDVI).Our analysis revealed that 49 districts and cities experienced significant mudflow events,resulting in estimated damages and economic losses of 30.2 million USD,with particularly severe impacts noted in the Khuroson,Tojikobod,Vakhsh,Panjakent,Lakhsh,and *** composition of mudflows in the six studied areas predominantly consisted of clay,with some regions featuring mudstone and a few exhibiting a mixture of both *** findings indicate the predominance of rain-induced mudflows in foothill areas,contrasting with rain-snow,glacial,and lake-outburst-induced mudflows in mountainous *** underscores the urgent need for effective disaster risk management strategies in vulnerable *** UAV and remote sensing technologies provides crucial information for analyzing damages,identifying vulnerable areas,and advising emergency response efforts,thereby enhancing disaster risk management in Tajikistan.

关键词： Disaster Mudflows Remote sensing Unmanned aerial vehicles Tajikistan

Design of a cationic accelerator enabling ultrafast ion diffusion kinetics in aqueous zinc-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 377-384页

作者： Yawei Xiao Qianqian Gu Haoyu Li Mengyao Li Yude Wang national center for International research on Photoelectric and Energy Materials School of Materials and EnergyYunnan UniversityKunming 6500504YunnanChina Key Laboratory of Ministry of Education for Advanced Materials in Tropical Island Resources School of Chemistry and Chemical EngineeringHainan UniversityHaikou 570228HainanChina College of Chemical engineering Fuzhou UniversityFuzhou 350108FujianChina Yunnan Key Laboratory of Carbon Neutrality and Green Low-carbon Technologies Yunnan UniversityKunming 6500504YunnanChina

Aqueous zincion batteries are highly favored for grid-level energy storage owing to their low cost and high safety,but their practical application is limited by slow ion *** address this,a strategy has been developed to create a cation-accelerating electric field on the surface of the cathode to achieve ultrafast Zn^(2+)diffusion *** employing electrodeposition to coat MoS_(2)on the surface of BaV_(6)O_(16)·3H_(2)O nanowires,the directional builtin electric field generated at the heterointerface acts as a cation accelerator,continuously accelerating Zn^(2+)diffusion into the active *** optimized Zn^(2+)diffusion coefficient in CC@BaV-V_(6)O_(16)·3H_(2)@MoS_(2)(7.5×10^(8)cm^(2)s^(-1)) surpasses that of most reported V-based ***,MoS_(2)serving as a cathodic armor extends the cycling life of the Zn-CC@BaV_(6)O_(16)·3H_(2)@MoS_(2)full batteries to over 10000 *** work provides valuable insights into optimizing ion diffusion kinetics for high-performance energy storage devices.

关键词： Internal electric field Cationic accelerator lon diffusion kinetics Cathode modification strategy Aqueous zinc ion battery