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Interfacial engineering through lead binding using crown ethers in perovskite solar cells

Journal of Energy Chemistry 2024年第5期92卷 263-270页

作者： Sun-Ju Kim YeonJu Kim Ramesh Kumar Chitumalla Gayoung Ham Thanh-Danh Nguyen Joonkyung Jang Hyojung Cha Jovana Milić Jun-Ho Yum Kevin Sivula Ji-Youn Seo Department of Nano Fusion Technology Pusan National UniversityBusan 46241Republic of Korea Laboratory for Molecular Engineering of Optoelectronic Nanomaterials Institute of Chemical Sciences and EngineeringÉcole Polytechnique Fédérale de Lausanne(EPFL)1015 LausanneSwitzerland Department of Energy Convergence and Climate Change Kyungpook National UniversityDaegu 41566Republic of Korea Department of Hydrogen and Renewable Energy Kyungpook National UniversityDaegu 41566Republic of Korea Adolphe merkle Institute University of FribourgCH-1700 FribourgSwitzerland

In the domain of perovskite solar cells(PSCs),the imperative to reconcile impressive photovoltaic performance with lead-related issue and environmental stability has driven innovative *** study pioneers an approach that not only rectifies lead leakage but also places paramount importance on the attainment of rigorous interfacial *** ethers,notably benzo-18-crown-6-ether(B18C6),were strategically integrated at the perovskite-hole transport material *** ethers exhibit a dual role:efficiently sequestering and immobilizing Pb^(2+)ions through host-guest complexation and simultaneously establishing a robust interfacial passivation *** crown ether candidates,guided by density functional theory(DFT)calculations,demonstrated proficiency in binding Pb2+ions and optimizing interfacial *** devices incorporating these materials achieved exceptional power conversion efficiency(PCE),notably 21.7%for B18C6,underscoring their efficacy in lead binding and interfacial *** techniques,including time-of-flight secondary ion mass spectrometry(ToF-SIMS),ultraviolet photoelectron spectroscopy(UPS),time-resolved photoluminescence(TRPL),and transient absorption spectroscopy(TAS),unequivocally affirmed Pb^(2+)ion capture and suppression of non-radiative ***,these PSCs maintained efficiency even after enduring 300 h of exposure to 85%relative *** research underscores the transformative potential of crown ethers,simultaneously addressing lead binding and stringent interfacial passivation for sustainable PSCs poised to commercialize and advance renewable energy applications.

关键词： Perovskite solar cells Interfacial passivation Crown ether materials Stability

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Data Secure Storage Mechanism for IIoT Based on Blockchain

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Computers, Materials & Continua 2024年第3期78卷 4029-4048页

作者： Jin Wang Guoshu Huang R.Simon Sherratt Ding Huang Jia Ni School of Computer science and Mathematics Fujian University of TechnologyFuzhou350118China School of Computer&Communication Engineering Changsha University of Science&TechnologyChangsha410004China School of Systems Engineering The University of ReadingReadingRG66AYUK School of Computer Nanjing University of Information Science and TechnologyNanjing210044China

With the development of Industry 4.0 and big data technology,the Industrial Internet of Things(IIoT)is hampered by inherent issues such as privacy,security,and fault tolerance,which pose certain challenges to the rapid development of *** technology has immutability,decentralization,and autonomy,which can greatly improve the inherent defects of the *** the traditional blockchain,data is stored in a merkle *** data continues to grow,the scale of proofs used to validate it grows,threatening the efficiency,security,and reliability of blockchain-based ***,this paper first analyzes the inefficiency of the traditional blockchain structure in verifying the integrity and correctness of *** solve this problem,a new Vector Commitment(VC)structure,Partition Vector Commitment(PVC),is proposed by improving the traditional VC ***,this paper uses PVC instead of the merkle tree to store big data generated by *** can improve the efficiency of traditional VC in the process of commitment and ***,this paper uses PVC to build a blockchain-based IIoT data security storage mechanism and carries out a comparative analysis of *** mechanism can greatly reduce communication loss and maximize the rational use of storage space,which is of great significance for maintaining the security and stability of blockchain-based IIoT.

关键词： Blockchain IIoT data storage cryptographic commitment

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A Novel High-Efficiency Transaction Verification Scheme for Blockchain Systems

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Computer Modeling in Engineering & sciences 2024年第5期139卷 1613-1633页

作者： Jingyu Zhang Pian Zhou Jin Wang Osama Alfarraj Saurabh Singh Min Zhu School of Computer&Communication Engineering Changsha University of Science&TechnologyChangsha410015China science and Technology on Information Systems Engineering Laboratory School of Systems EngineeringNational University of Defense TechnologyChangsha410073China Computer science Department King Saud UniversityRiyadh11437Saudi Arabia Department of Artificial Intelligence and Big Data Woosong UniversityDaejeon34606South Korea College of Information science and Technology Zhejiang Shuren UniversityHangzhou310015China

Blockchain can realize the reliable storage of a large amount of data that is chronologically related and verifiable within the *** technology has been widely used and has developed rapidly in big data systems across various *** increasing number of users are participating in application systems that use blockchain as their underlying *** the number of transactions and the capital involved in blockchain grow,ensuring information security becomes *** the verification of transactional information security and privacy has emerged as a critical ***-based verification methods can effectively eliminate the need for centralized third-party ***,the efficiency of nodes in storing and verifying blockchain data faces unprecedented *** address this issue,this paper introduces an efficient verification scheme for transaction ***,it presents a node evaluation module to estimate the activity level of user nodes participating in transactions,accompanied by a probabilistic analysis for all ***,this paper optimizes the conventional transaction organization form,introduces a heterogeneous merkle tree storage structure,and designs algorithms for constructing these heterogeneous *** analyses and simulation experiments conclusively demonstrate the superior performance of this *** verifying the same number of transactions,the heterogeneous merkle tree transmits less data and is more efficient than traditional *** findings indicate that the heterogeneous merkle tree structure is suitable for various blockchain applications,including the Internet of *** scheme can markedly enhance the efficiency of information verification and bolster the security of distributed systems.

关键词： Blockchain architecture transaction verification information security heterogeneous merkle tree distributed systems

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Unconventional bound states in the continuum from metamaterial-induced electron acoustic waves

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Advanced Photonics 2023年第5期5卷 77-85页

作者： Wenhui Wang Antonio Günzler Bodo D.Wilts Ullrich Steiner Matthias Saba University of Fribourg Adolphe Merkle InstituteFribourgSwitzerland University of Salzburg Department of Chemistry and Physics of MaterialsSalzburgAustria

Photonic bound states in the continuum(BICs)are spatially localized modes with infinitely long lifetimes,which exist within a radiation continuum at discrete energy *** states have been explored in various systems,including photonic and phononic crystal slabs,metasurfaces,waveguides,and integrated *** and availability of the BICs are important aspects for fully taming the BICs toward practical ***,we propose a generic mechanism to realize BICs that exist by first principles free of fine parameter tuning based on non-Maxwellian double-net metamaterials(DNMs).An ideal warm hydrodynamic double plasma(HDP)fluid model provides a homogenized description of DNMs and explains the robustness of the BICs found *** the HDP model,these are standing wave formations made of electron acoustic waves(EAWs),which are pure charge oscillations with vanishing electromagnetic *** BICs have various advantages,such as(i)frequency-comb-like collection of BICs free from normal resonances;(ii)robustness to symmetry-breaking perturbations and formation of quasi-BICs with an ultrahigh Q-factor even if subject to disorder;and(iii)giving rise to subwavelength microcavity resonators hosting quasi-BIC modes with an ultrahigh Q-factor.

关键词： bound states in the continuum double-net metamaterial metamaterial electron acoustic wave hydrodynamical plasma

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A Blockchain-Based Efficient Cross-Domain Authentication Scheme for Internet of Vehicles

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Computers, Materials & Continua 2024年第7期80卷 567-585页

作者： Feng Zhao Hongtao Ding Chunhai Li Zhaoyu Su Guoling Liang Changsong Yang Guangxi Engineering Research Center of Industrial Internet Security and Blockchain Guilin University of Electronic TechnologyGuilin541004China School of Information and Communication Guilin University of Electronic TechnologyGuilin541004China School of Computer science and Information Security Guilin University of Electronic TechnologyGuilin541004China

The Internet of Vehicles(IoV)is extensively deployed in outdoor and open environments to effectively address traffic efficiency and safety issues by connecting vehicles to the ***,due to the open and variable nature of its network topology,vehicles frequently engage in cross-domain *** such processes,directly uploading sensitive information to roadside units for interaction may expose it to malicious tampering or interception by attackers,thus compromising the security of the cross-domain authentication ***,IoV imposes high real-time requirements,and existing cross-domain authentication schemes for IoV often encounter efficiency *** mitigate these challenges,we propose CAIoV,a blockchain-based efficient cross-domain authentication scheme for *** scheme comprehensively integrates technologies such as zero-knowledge proofs,smart contracts,and merkle hash tree *** divides the cross-domain process into anonymous cross-domain authentication and safe cross-domain authentication phases to ensure efficiency while maintaining a balance between efficiency and ***,we evaluate the performance of *** results demonstrate that our proposed scheme reduces computational overhead by approximately 20%,communication overhead by around 10%,and storage overhead by nearly 30%.

关键词： Blockchain cross-domain authentication internet of vehicle zero-knowledge proof

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Identifying malicious accounts in blockchains using domain names and associated temporal properties

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Blockchain(Research and Applications) 2023年第3期4卷 39-51页

作者： Rohit Kumar Sachan Rachit Agarwal Sandeep Kumar Shukla C3i Hub Indian Institute of Technology KanpurKanpur 208016India CSE Department Indian Institute of Technology KanpurKanpur 208016India Bennet University Greater Noida 201310India merkle science Bangalore 560102India

The rise in the adoption of blockchain technology has led to increased illegal activities by cybercriminals costing billions of *** machine learning algorithms are applied to detect such illegal *** algorithms are often trained on the transaction behavior and,in some cases,trained on the vulnerabilities that exist in the *** our approach,we study the feasibility of using the Domain Name(DN)associated with the account in the blockchain and identify whether an account should be tagged malicious or ***,we leverage the temporal aspects attached to the *** approach achieves 89.53%balanced-accuracy in detecting malicious blockchain *** our results identify 73769 blockchain DNs that show malicious behavior at least once,out of these,34171 blockchain DNs show persistent malicious behavior,resulting in 2479 malicious blockchain DNs over ***,none of these identified malicious DNs were reported in new officially tagged malicious blockchain DNs.

关键词： Blockchain Machine learning Suspect identification Domain name Temporal properties

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Perovskites for Laser and Detector Applications

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Energy & Environmental Materials 2019年第2期2卷 146-153页

作者： Saunak Das Somayeh Gholipour Michael Saliba Institute of Physical Chemistry(IPC) Friedrich Schiller University JenaHelmholtzweg 4Jena 07743Germany Leibniz Institute of Photonic Technology(IPHT) Albert-Einstein-Str.907745Jena Germany Adolphe merkle Institute University of Fribourg CH 1700Switzerland Institute of Materials science Technical University of DarmstadtD-64287Germany

Perovskite materials have triggered a renewed interest in photovoltaic research in the recent *** display crystal forms with 0D,1D and 2D,3D motifs,and several chemical forms,namely inorganic(titanates,rubidiates,nobiates,tantalates etc.),organic/inorganic metal halides with single to multiple cations,and even organic polymer or quantum dot-infused *** crystal type and chemical form are endowed with specific physicochemical,optical,electronic,and morphological *** unique properties render them suitable for targeted applications,namely photovoltaics,LEDs,photocatalysis/electrolysis/solar fuels/solar and Li-ion batteries,gas-sensors,ferroelectrics,capacitors,transistors and memristors,photodetectors,and lasers,for advanced quantum cryptography and outer space *** first,the crystal and material types,and physicochemical,morphological,and optoelectronic properties of perovskite materials are ***,we focus on those properties which cumulatively contribute to their application in the abovementioned ***,a comprehensive discussion about the advances in each field is ***/property/application relationships with key advances demonstrate the versatility of perovskites in modern optoelectronic technologies.

关键词： 2D perovskites hybrid perovskites micro-lasers X-ray detectors c-ray detectors

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High refractive index of melanin in shiny occipital feathers of a bird of paradise

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Light(science & Applications) 2015年第1期4卷 518-523页

作者： Doekele G Stavenga Hein L Leertouwer Daniel C Osorio Bodo D Wilts Computational Physics University of Groningen9747 AGThe Netherlands School of Life sciences University of SussexBrightonBN19QGUK Adolphe merkle Institute University of FribourgCH-1700 FribourgSwitzerland

Male Lawes’s Parotia,a bird of paradise,use the highly directional reflection of the structurally colored,brilliant-silvery occipital feathers in their courtship *** in other birds,the structural coloration is produced by ordered melanin *** barbules of the Parotia’s occipital feathers,with thickness,3 μm,contain 6–7 layers of densely packed melanin rodlets(diameter,0.25 μm,length,2 μm).The effectively,0.2 μm thick melanin layers separated by,0.2 μm thick keratin layers create a multilayer interference *** measurements yielded peak wavelengths in the near-infrared at,1.3 μm,i.e.,far outside the visible wavelength *** the Jamin-Lebedeff interference microscopy method recently developed for pigmented media,we here determined the refractive index of the intact *** thus derived the wavelength dependence of the refractive index of the barbules’melanin to be 1.7–1.8 in the visible wavelength *** the anatomical and refractive index data in an optical multilayer model,we calculated the barbules’reflectance,transmittance and absorptance spectra,thereby confirming measured spectra.

关键词： bird of paradise interference reflector iridescence Jamin-Lebedeff microscopy multilayer

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Blockchain merkle-Tree Ethereum Approach in Enterprise Multitenant Cloud Environment

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Computers, Materials & Continua 2023年第2期74卷 3297-3313页

作者： Pooja Dhiman Santosh Kumar Henge Sartaj Singh Avinash Kaur Parminder Singh Mustapha Hadabou School of Computer Applications Lovely Professional UniversityPhagwara144001India School of Computer science and Engineering Lovely Professional UniversityPhagwara144001India School of Computer science Mohammed VI Polytechnic UniversityBen Guerir43150Morocco

This research paper puts emphasis on using cloud computing with Blockchain(BC)to improve the security and privacy in a *** security of data is not guaranteed as there is always a risk of leakage of users’*** can be used in a multi-tenant cloud environment(MTCE)to improve the security of data,as it is a decentralized *** is saved in unaltered ***,Blockchain is not owned by a single *** encryption process can be done using a Homomorphic encryption(HE)algorithm along with hashing technique,hereby allowing computations on encrypted data without the need for *** research paper is composed of four objectives:Analysis of cloud security using Blockchain technology;Exceptional scenario of Blockchain architecture in an enterprise-level MTCE;Implementation of cipher-text policy attribute-based encryption(CPABE)algorithm;Implementation of merkle tree using Ethereum(MTuE)in a Multi-tenant *** of these four objectives,the main focus is on the implementation of CP-ABE ***-ABE parameters are proposed for different levels of *** levels include inner tenant,outer tenant,Inner-Outer-Tenant,Inner-Outer-External-Tenant,Outer-Inner-Tenant,External-Outer-Inner-Tenant and the parameters such as token,private key,public key,access tree,message,attribute set,node-level,cipher-text,salting which will help in providing better security using CP-ABE algorithm in a multitenant environment(MTE)where tenants can be provided with different levels of security and achieved 92 percentage of authenticity and access-control of the data.

关键词： Blockchain(BC) merkle tree using ethereum(MTuE) multi-tenant environment(MTE) homomorphic encryption(HE) ciphertext policy attribute-based encryption(CP-ABE)

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Data Security Storage Mechanism Based on Blockchain Network

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Computers, Materials & Continua 2023年第3期74卷 4933-4950页

作者： Jin Wang WeiOu Wenhai Wang RSimon Sherratt Yongjun Ren Xiaofeng Yu School of Computer&Communication Engineering Changsha University of Science&TechnologyChangsha410004China School of Control science and Engineering Zhejiang UniversityHangzhou310058China School of Systems Engineering The University of ReadingReadingRG66AYUK School of Computer Engineering Research Center of Digital Forensics of Ministry of EducationNanjing University of Information Science&TechnologyNanjing210044China School of Business Nanjing UniversityNanjing210093China

With the rapid development of information technology,the development of blockchain technology has also been deeply *** performing block verification in the blockchain network,if all transactions are verified on the chain,this will cause the accumulation of data on the chain,resulting in data storage *** the same time,the security of data is also challenged,which will put enormous pressure on the block,resulting in extremely low communication efficiency of the *** traditional blockchain system uses themerkle Tree method to store *** verifying the integrity and correctness of the data,the amount of proof is large,and it is impossible to verify the data in batches.A large amount of data proof will greatly impact the verification efficiency,which will cause end-to-end communication delays and seriously affect the blockchain system’s stability,efficiency,and *** order to solve this problem,this paper proposes to replace the merkle tree with polynomial commitments,which take advantage of the properties of polynomials to reduce the proof size and communication *** realizing the ingenious use of aggregated proof and smart contracts,the verification efficiency of blocks is improved,and the pressure of node communication is reduced.

关键词： Blockchain cryptographic commitment smart contract data storage

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