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A New Chirality Invertible Photoswitch:Light-Driven Axially Chiral Hydrazone Enabling Dynamic Handedness Inversion of Self-Organized Helical Superstructure

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CCS Chemistry 2024年第8期6卷 2011-2020页

作者： Ruochen Lan Jinying Bao Zhaozhong Li Zizheng Wang Zichen Wang Qian Wang Lanying Zhang Jiumei Xiao Huai Yang Institute of Advanced Materials College of Chemistry and Chemical EngineeringJiangxi Normal UniversityNanchang 330022 Beijing Advanced Innovation Center for Materials Genome Engineering School of Materials Science and EngineeringPeking UniversityBeijing 100871 School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083 Beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing 100083 Key Laboratory of Polymer Chemistry and Physics of Ministry of Education Peking UniversityBeijing 100871 School of Mathematics and Physics University of Science and Technology BeijingBeijing 100083

Inspired by nature,dynamic self-organized helical superstructures are becoming attractive as building blocks in soft photonic crystals and advanced chiroptical ***,a chirality invertible hydrazone photoswitch,possessing high helical twisting power(HTP)was judiciously designed and *** to the photoinduced configuration changes of the hydrazone photoswitch,it displayed superior thermal stability and strikingly reversible HTP *** incorporating a novel chiral hydrazone(CH)into the liquid crystal(LC)host,a handedness invertible cholesteric liquid crystal(CLC)helical superstructure with high thermal stability and light-modulated photonic bandgap was *** inferred that the mechanism of chirality inversion of the novel CH photoswitch derived from changes in the dihedral angle between the two naphthalene rings induced by hydrazone ***,the influence of chemical structures on its photoresponsiveness was ***,the potential applications of this advanced light-driven CLC in soft photonic crystals,showing erasable and rewritable colorful patterns and chiroptical templates to induce handedness invertible circularly polarized luminescence were illustrated.

关键词： chirality inversion hydrazone photoswitch cholesteric liquid crystals dynamic photonic crystals dynamic circularly polarized luminescence

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Redundant Data Detection and Deletion to Meet Privacy Protection Requirements in Blockchain-Based Edge Computing Environment

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China Communications 2024年第3期21卷 149-159页

作者： Zhang Lejun Peng Minghui Su Shen Wang Weizheng Jin Zilong Su Yansen Chen Huiling Guo Ran Sergey Gataullin Cyberspace Institute Advanced technology Guangzhou UniversityGuangzhou 510006China College of Information Engineering Yangzhou UniversityYangzhou 225127China School Math&Computer Science Quanzhou Normal UniversityQuanzhou 362000China Computer Science Department City University of Hong KongHong Kong 999077China School of Computer and Software Nanjing University of Information Science and TechnologyNanjing 21004China Key Laboratory of Intelligent Computing and Signal Processing of Ministry of Education School of Computer Science and TechnologyAnhui UniversityHefei 230601China Department of Computer Science and Artificial Intelligence Wenzhou UniversityWenzhou 325035China Guangzhou university Library Guangzhou UniversityGuangzhou 510006China Central Economic and Mathematics Institute Russian Academy of Sciences MIREA-Russian Technological university Moscow RegionRussia

With the rapid development of information technology,IoT devices play a huge role in physiological health data *** exponential growth of medical data requires us to reasonably allocate storage space for cloud servers and edge *** storage capacity of edge nodes close to users is *** should store hotspot data in edge nodes as much as possible,so as to ensure response timeliness and access hit rate;However,the current scheme cannot guarantee that every sub-message in a complete data stored by the edge node meets the requirements of hot data;How to complete the detection and deletion of redundant data in edge nodes under the premise of protecting user privacy and data dynamic integrity has become a challenging *** paper proposes a redundant data detection method that meets the privacy protection *** scanning the cipher text,it is determined whether each sub-message of the data in the edge node meets the requirements of the hot *** has the same effect as zero-knowledge proof,and it will not reveal the privacy of *** addition,for redundant sub-data that does not meet the requirements of hot data,our paper proposes a redundant data deletion scheme that meets the dynamic integrity of the *** use Content Extraction Signature(CES)to generate the remaining hot data signature after the redundant data is *** feasibility of the scheme is proved through safety analysis and efficiency analysis.

关键词： blockchain data integrity edge computing privacy protection redundant data

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High speed laser cladding as a new approach to prepare ultra-high temperature ceramic coatings

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Journal of Advanced Ceramics 2024年第2期13卷 143-154页

作者： Qiyao Deng Pengfei He Chuan Sun Yang Li Yue Xing Yujie Wang Jinglong Li Xiubing Liang Xin Wang Yujie Zhou Yujun Cai National-Local Joint Engineering Laboratory of Intelligent Manufacturing Oriented Automobile Die&Mould Tianjin University of Technology and EducationTianjin 300222China Defense Innovation Institute Academy of Military ScienceBeijing 100071China School of mechanical engineering Tianjin University of Technology and EducationTianjin 300222China Scientific and Technological Innovation Center Beijing 100012China

Ultra-high temperature ceramic(UHTC)coatings are used to protect the hot-end components of hypervelocity aerocrafts from thermal *** study provides a new approach to fabricate UHTC coatings with high speed laser cladding(HSLC)technology,and places more emphasis on investigating the formation mechanism,phase compositions,and mechanical properties of HSLC-UHTC *** show that a well-bonded interface between the coating and the tantalum alloy substrate can be *** coating is mainly composed of(Zr,Ta)C ceramic solid solution phase with a content of higher than 90% by volume and Ta(W)metal solid solution *** a relatively high powder feeding rate,the ZrC ceramic phase appears in the coating while a dense ZrC UHTC top layer with a thickness of up to~50μm is successfully *** for the mechanical properties of the HSLC coatings,the fracture toughness of the coating decreases with the increase of powder feeding *** increase of carbide solid solution phase can significantly improve the high temperature microhardness(552.7±1.8 HV0.5@1000℃).The innovative design of HSLC ZrC-based coatings on refractory alloys accomplishes continuous transitions on microstructure and properties from the substrate to the UHTC top layer,which is a very promising candidate scheme for thermal protection coating.

关键词： high speed laser cladding(HSLC) ultra-high temperature ceramic(UHTC) thermal protection coating microstructure mechanical properties

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Recent progress and perspective on electrocatalysis in neutral media:Mechanisms,materials,and advanced characterizations

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Interdisciplinary Materials 2024年第4期3卷 492-529页

作者： Fayuan Lai Haochuan Shang Yuchao Jiao Xinyi Chen Tianran Zhang Xiangfeng Liu College of Materials Science and Opto-Electronic technology University of Chinese Academy of SciencesBeijingChina

Electrocatalysis,which involves oxidation and reduction reactions with direct electron transfer,is essential for a variety of clean energy conversion ***,the vast majority of studies regarding electrocatalysis reactions focus on strong acidic or alkaline media because of the higher catalytic ***,some inherent drawbacks,including the corrosive environment,expensive proton exchange membranes,and side effects,are still hard to break through.A sustainably promising way to overcome these shortcomings is to deploy neutral/near-neutral electrolytes for electrocatalysis ***,insufficient research in this area due to the lack of attention to related issues has slowed down the development *** this review,we systematically review the catalytic reaction mechanisms,neutral electrolytes,electrocatalysts,and modification strategies carried out in neutral media on the three most common electrocatalytic reactions,that is,hydrogen evolution reaction,oxygen reduction reaction,and oxygen evolution ***,the advanced characterization tools for guiding catalyst synthesis and mechanistic studies are also ***,we propose some challenges and perspectives on electrocatalysis reactions in neutral media and hope it will attract more research interest and provide guidance in neutral electrocatalysis.

关键词： advanced characterizations electrocatalysis HER/ORR/OER mechanism studies neutral/near-neutral electrolyte

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Dynamics of perinuclear actin ring regulating nuclear morphology

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Applied Mathematics and Mechanics(English Edition) 2024年第8期45卷 1415-1428页

作者： Haoxiang YANG Houbo SUN Jinghao SHEN Hao WU Hongyuan JIANG CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern MechanicsUniversity of Science and Technology of ChinaHefei 230026China

Cells are capable of sensing and responding to the extracellular mechanical microenvironment via the actin *** vivo,tissues are frequently subject to mechanical forces,such as the rapid and significant shear flow encountered by vascular endothelial ***,the investigations about the transient response of intracellular actin networks under these intense external mechanical forces,their intrinsic mechanisms,and potential implications are very ***,we observe that when cells are subject to the shear flow,an actin ring structure could be rapidly assembled at the periphery of the *** gain insights into the mechanism underlying this perinuclear actin ring assembly,we develop a computational model of actin *** demonstrate that this perinuclear actin ring assembly is triggered by the depolymerization of cortical actin,Arp2/3-dependent actin filament polymerization,and myosin-mediated actin network ***,we discover that the compressive stress generated by the perinuclear actin ring could lead to a reduction in the nuclear spreading area,an increase in the nuclear height,and a decrease in the nuclear *** present model thus explains the mechanism of the perinuclear actin ring assembly under external mechanical forces and suggests that the spontaneous contraction of this actin structure can significantly impact nuclear morphology.

关键词： mechanical force actin dynamics perinuclear actin ring compressive stress nucleus

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e^(+)e^(-)→Λ_(c)+Λ_(c)^(- ) Cross Sections and the Λ_(c)^(+) Electromagnetic Form Factors within the Extended Vector Meson Dominance Model

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Chinese Physics Letters 2024年第2期41卷 36-41页

作者：陈诚闫冰谢聚军 Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China School of Nuclear Sciences and technology University of Chinese Academy of SciencesBeijing 101408China College of Mathematics and Physics Chengdu University of TechnologyChengdu 610059China Southern Center for Nuclear-Science Theory(SCNT) Institute of Modern PhysicsChinese Academy of SciencesHuizhou 516000China

Within the extended vector meson dominance model,we investigate the𝑒e^(+)e^(-)→Λ_(c)+Λ_(c)^(- ) reaction and the electromagnetic form factors of the charmed baryon𝛬 Λ_(c)^(+)𝑐.The model parameters are determined by fitting them to the cross sections of the process𝑒e^(+)e^(-)→Λ_(c)+Λ_(c)^(- ) and the magnetic form factor|G_(M)|of Λ_(c)^(+) .By considering four charmonium-like states,called𝜓(4500),𝜓(4660),𝜓(4790),and𝜓(4900),we can well describe the current data on the𝑒e^(+)e^(-)→Λ_(c)+Λ_(c)^(- ) reaction from the reaction threshold up to 4.96 *** addition to the total cross sections and|𝐺M|,the ratio|G_(E)/G_(M)|and the effective form factor|Geff|for Λ_(c)^(+) 𝑐are also calculated,and found that these calculations are consistent with the experimental *** the fitted model parameters,we have also estimated the charge radius of the charmed Λ_(c)^(+) baryon.

关键词： fitted radius meson

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Nonlinear uncertainty impact of geometric variations on aerodynamic performance of low-pressure turbine blades with ultra-high loading under extreme operational conditions

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Chinese Journal of Aeronautics 2024年第5期37卷 281-300页

作者： Xiaojing WANG Zhengping ZOU Chao FU Pengcheng DU School of Energy and Power Engineering Beihang UniversityBeijing 100191China National Key Laboratory of Science and technology on Aero-Engine Aero-Thermodynamics Beihang UniversityBeijing 100191China Research Institute of Aero-Engine Beihang UniversityBeijing 100191China

Uncertainty impact of random geometric variations on the aerodynamic performance of low-pressure turbine blades is considerable,which is further amplified by the current ultra-high-lift design trend for weight ***,this uncertainty impact on ultra-highly loaded blades under extreme operational conditions near the margins with potential large-scale open separation is focused on in this *** is demonstrated that this impact is significant,unfavourable,and nonlinear,which is clearly severer under extreme *** addition to the overall attenuation and notable scattering of specific performance,the operational margins with open separation are also notably scattered with great risk of significant *** scattering and nonlinearity are dominated by the variations in leading-edge *** thinning of leading edge triggers local transition,enhancing downstream friction and reducing resistance to open separation,which is further exacerbated by operational ***,the opposite thickening yields less benefit,implying *** unfavourable impact highlights the need for robust aerodynamic design,where both a safer operational condition and a more robust blade are indispensable,i.e.,a compromise among performance,weight,and *** the necessary limitation of loading levels,a mid-loaded design is recommended to reduce adverse pressure gradients in both the leading edge and rear region of the suction side,which helps to decrease the susceptibility of the transition and open separation to random *** improvements can also be achieved by appropriately thickening the leading edge.

关键词： Ultra-highly loaded turbine blade Geometric variations Uncertainty analysis Operational margins Robust aerodynamic design Nonlinearity

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Upcycling the spent graphite/LiCoO_(2) batteries for high-voltage graphite/LiCoPO_(4)-co-workable dual-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1745-1751页

作者： Miao Du Hongyan Lü Kaidi Du Shuohang Zheng Xiaotong Wang Xiaotong Deng Ronghua Zeng Xinglong Wu Key Laboratory for UV Light-Emitting Materials and technology of Ministry of Education Northeast Normal UniversityChangchun 130024China Faculty of Chemistry Northeast Normal UniversityChangchun 130024China School of Chemistry South China Normal UniversityGuangzhou 510006China

The worldwide proliferation of portable electronics has resulted in a dramatic increase in the number of spent lithium-ion batteries(LIBs).However,traditional recycling methods still have limitations because of such huge amounts of spent ***,we proposed an ecofriendly and sustainable double recycling strategy to concurrently reuse the cathode(LiCoO_(2))and anode(graphite)materials of spent LIBs and recycled LiCoPO_(4)/graphite(RLCPG)in Li^(+)/PF^(-)_(6) co-de/intercalation dual-ion *** recycle-derived dualion batteries of Li/RLCPG show impressive electrochemical performance,with an appropriate discharge capacity of 86.2 mAh·g^(-1) at25 mA·g^(-1) and 69%capacity retention after 400 *** recycling of the cathode and anode from spent LIBs avoids wastage of resources and yields cathode materials with excellent performance,thereby offering an ecofriendly and sustainable way to design novel secondary batteries.

关键词： recycle lithium cobalt oxide lithium cobalt phosphate graphite dual-ion batteries spent lithium-ion batteries

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Neutrophils in Atlantic salmon(Salmo salar L.)are MHC class II^(+)and secret IL-12p40 upon bacterial exposure

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Aquaculture and Fisheries 2024年第2期9卷 144-153页

作者： Gyri Teien Haugland Anita Rønneseth Lene Gundersen Harald SæbøLunde Kaja Nordland Heidrun Inger Wergeland Department of Biological Sciences Bergen High-Technology CentreUniversity of BergenBergen5020Norway

Antigen-presentation via major histocompatibility complex(MHC)to T cells is the key event to initiate adaptive immune *** teleosts,as in mammals,the main types of professional antigen-presenting cells(APCs)are dendritic cells(DCs),monocytes/macrophages,and B *** the current study,flow cytometry,immunostaining and qPCR have been used to show that neutrophils in the teleost fish Atlantic salmon(Salmo salar L.)have antigen-presenting *** neutrophils were positive for MHC class II,CD83 and CD80/86,and upon in vitro bacterial exposure,gene expression analysis of purified neutrophils showed that IL-12p40,which is essential for proliferation of naïve T cells,was highly upregulated at both 6 and 24 h post bacterial *** on presence of MHC class II and upregulation of molecules involved in antigen presentation and T cell activation,we suggest that neutrophils in Atlantic salmon have potential to function as professional *** work makes an important basis for further exploring the potential of using neutrophils to develop new,targeted immunoprophylactic measures.

关键词： Granulocytes Antigen presenting cells Major histocompatibility complex T cell activation B cells CD83 CD80/86 MHC classⅡ

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Recent progress in MOFs-based nanozymes for biosensing

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Nano Research 2024年第1期17卷 39-64页

作者： Imamdin Chandio Yongjian Ai Lei Wu Qionglin Liang MOE Key Laboratory of Bioorganic Phosphorus Chemistry&Chemical Biology Department of ChemistryLaboratory of Flexible Electronics TechnologyCenter for Synthetic and Systems BiologyTsinghua University-Peking University Joint Centre for Life SciencesTsinghua UniversityBeijing 100084China

Nanozymes are nanomaterials with enzyme-mimicking catalytic *** to natural enzymes,nanozymes show various properties such as easy to manufacture,stable,adjustable,and *** play key roles in biosensing,biocatalysis,and disease *** an important kind of nanozymes,metal-organic framework(MOF)-based nanozymes are receiving a lot of attention due to their structural properties and *** developing MOF with enzymes-like catalytic properties has opened new perspectives in *** review summarizes the up-to-date developments in synthesizing two-dimensional and three-dimensional MOF-based nanozymes and their applications in ***,classification of nanozymes obtained by MOFs is categorized,and different properties of MOF-based nanozymes are ***,the distinctive applications of MOF-based nanozymes in identifying various analytes are thoroughly ***,the recent challenges and progressive directions in this area are highlighted.

关键词： metal-organic frameworks nanozymes metal-organic framework (MOF)-based nanozymes biosensing analytes

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