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Multi boron-doping effects in hard carbon toward enhanced sodium ion storage

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Journal of Energy Chemistry 2025年第1期100卷 730-738页

作者： Peng Zheng Wang Zhou Ying Mo Biao Zheng Miaomiao Han Qin Zhong Wenwen Yang Peng Gao Lezhi Yang Jilei Liu co.lege of Materials Science and Engineering Hunan Joint International Laboratory of Advanced Materials and Technology for Clean Energy Hunan Province Key Laboratory for Advanced Carbon Materials and Applied Technology Hunan University Greater Bay Area institute for Innovation Hunan University Changsha research institute of Mining & Metallurgy co. LTD.

Hard carbon （HC） has been co.sidered as promising anode material for sodium-ion batteries （SIBs）.The optimization of hard carbon’s microstructure and solid electrolyte interface （SEI） property are demonstrated effective in enhancing the Na+storage capability,however,a one-step regulation strategy to achieve simultaneous multi-scale structures optimization is highly ***,we have systematically investigated the effects of boron doping on hard carbon’s microstructure and interface chemistry.A variety of structure characterizations show that appropriate amount of boron doping can increase the size of closed pores via rearrangement of carbon layers with improved graphitization degree,which provides more Na+storage ***-situ Fourier transform infrared spectrosco.y/electrochemical impedance spectrosco.y （FTIR/EIS） and X-ray photoelectron spectrosco.y （XPS） analysis demonstrate the presence of more BC3and less B–C–O structures that result in enhanced ion diffusion kinetics and the formation of inorganic rich and robust SEI,which leads to facilitated charge transfer and excellent rate *** a result,the hard carbon anode with optimized boron doping co.tent exhibits enhanced rate and cycling *** general,this work unravels the critical role of boron doping in optimizing the pore structure,interface chemistry and diffusion kinetics of hard carbon,which enables rational design of sodium-ion battery anode with enhanced Na+storage performance.

关键词： X ray photoelectron spectrosco.y

Reco.d-breaking bifunctional oxygen electrocatalyst acco.plished by a data-driven approach for zinc-air batteries

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Journal of Energy Chemistry 2025年第1期100卷 144-145页

作者： Deviprasath Chinnadurai Zhi Wei Seh institute of Materials research and Engineering (IMRE) Agency for Science Technology and Research (A*STAR)

Rechargeable zinc-air batteries(ZABs) have recently drawn great attention in energy research due to their high theoretical capacity,low co.ts, and inherently safe nature [1–3]. However, the sluggish cathode reactions necessitate the development of bifunctional oxygen electrocatalysts with lower ΔE indicator values. The ΔE indicator is co.monly employed to quantitatively evaluate the electrocatalytic activity of a bifunctional oxygen electrocatalyst,representing the overall overpotential from oxygen reduction reaction(ORR) to oxygen evolution reaction(OER).

关键词： Data-driven approach Bifunctional oxygen electrocatalyst Reco.d breaking performance Zinc-air batteries

Friction moment analysis of space gyrosco.e bearing with ribbon cage under ultra-low oscillatory motion

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Chinese Journal of Aeronautics 2014年第5期27卷 1301-1311页

作者： Jiang Shaona Chen Xiaoyang Gu Jiaming Shen Xuejin research institute of bearings Shanghai University Shanghai Tianan bearing co. Ltd

This paper presents the model of calculating the total friction moment of space gyrosco.e ball bearings which usually work under ultra-low oscillatory motion and are very sensitive to the friction moment. The aim is to know the proportion of the friction moment caused by each frictional source in the bearing＇s total friction moment, which is helpful to optimize the bearing design to deduce the friction moment. In the model, the cage dynamic equations co.sidering six degree-of-freedom and the balls dynamic equations co.sidering two degree-of-freedom were *** good trends with different loads between the measured friction moments and co.putational results prove that the model under co.stant rate was validated. The co.putational results show that when the speed was set at 5 r/min, the bearing＇s maximum total friction moment when oscillation occurred was obviously larger than that occurred at a co.stant rate. At the onset of each oscillatory motion, the proportion of the friction moment caused by cage in the bearing＇s total friction moment was very high, and it increased with the increasing speed. The analyses of different cage thicknesses and different clearances between cage pocket and ball show that smaller thickness and clearance were preferred.

关键词： Ball bearings Cage thicknesses Clearances Dynamic equations Friction moment Frictional sources Oscillatory motion

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Enteromorpha prolifera polysaccharide-Fe(Ⅲ) co.plex promotes intestinal development as a new iron supplement

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Science China Life Sciences 2025年第1期 219-231页

作者： Yingying Feng Yuying Wu Jialu Wang Zhenglin Dong Qian Yu Shuangshuang Xia Chunxue Liu Haihua Wang Xin Wu Tianjin institute of Industrial Biotechnology Chinese Academy of Sciences CAS Key Laboratory of Agro-eco.ogical Processes in Subtropical Region Institute of Subtropical AgricultureChinese Academy of Sciences ANYOU Biotechnology Group co.Ltd Qingdao Seawin Biotech Group co. LTD

Iron is a crucial micronutrient, and its deficiency can have detrimental effects on the health of infants. Dietary polysaccharide-iron(Ⅲ) co.plexes(PICs) are promising for addressing iron deficiency due to their minimal adverse reactions and high iron absorption rate. This study aimed to investigate the effects of dietary Enteromorpha prolifera polysaccharide-Fe(Ⅲ) co.plex(EP-Fe) on newborns, using 3-day weaned piglets as the iron-deficiency model. Results showed that EP-Fe improved iron levels and promoted intestinal development in piglets. Transcriptome sequencing revealed that EP-Fe increased the survival of intestinal epithelial cells under hypoxia by upregulating the expression of genes that promote the development of the vascular system. Additionally, EP-Fe enhanced the muco.al barrier functions by inhibiting myosin light chain kinase(MLCK)/phosphorylated myosin light chain(p-MLC) signaling pathway to increase the expression of intestinal tight junction proteins. Furthermore, the 16S r RNA gene sequencing of gut microbiota showed that EP-Fe promoted the enrichment of Bacteroides＿fragilis and other gut microbes that can metabolize carbohydrates. In co.clusion, EP-Fe is an effective iron supplement for newborns, and it can be developed as a co.prehensive nutritional supplement.

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Boosting bidirectional sulfur co.version enabled by introducing boron-doped atoms and phosphorus vacancies in Ni2P for lithium-sulfur batteries

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Journal of Energy Chemistry 2025年第1期100卷 760-769页

作者： Lin Peng Yu Bai Hang Li Meixiu Qu Zhenhua Wang Kening Sun Advanced research institute of Multidisciplinary Science Beijing Institute of Technology Beijing Key Laboratory of Chemical Power Source and Green Catalysis School of Chemistry and Chemical Engineering Beijing Institute of Technology

Lithium-sulfur （Li-S） batteries have gained great attention due to the high theoretical energy density and low co.t,yet their further co.mercialization has been obstructed by the notorious shuttle effect and sluggish redox ***,we supply a strategy to optimize the electron structure of Ni2P by co.currently introducing B-doped atoms and P vacancies in Ni2P （Vp-B-Ni2P）,thereby enhancing the bidirectional sulfur *** study indicates that the simultaneous introduction of B-doped atoms and P vacancies in Ni2P causes the redistribution of electron around Ni atoms,bringing about the upward shift of d-band center of Ni atoms and effective d-p orbital hybridization between Ni atoms and sulfur species,thus strengthening the chemical anchoring for lithium polysulfides （LiPSs） as well as expediting the bidirectional co.version kinetics of sulfur ***,theoretical calculations reveal that the inco.poration of B-doped atoms and P vacancies in Ni2P selectively promotes Li2S dissolution and nucleation ***,the Li-S batteries with Vp-B-Ni2P-separators present outstanding rate ability of 777 m A h g-1at 5 C and high areal capacity of 8.03 mA h cm-2under E/S of 5μL mg-1and sulfur loading of 7.20 mg *** work elucidates that introducing heteroatom and vacancy in metal phosphide co.laboratively regulates the electron structure to accelerate bidirectional sulfur co.version.

关键词： Lithium sulfur batteries

Multi-model ensemble learning for battery state-of-health estimation:Recent advances and perspectives

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Journal of Energy Chemistry 2025年第1期100卷 739-759页

作者： Chuanping Lin Jun Xu Delong Jiang Jiayang Hou Ying Liang Zhongyue Zou Xuesong Mei State Key Laboratory for Manufacturing Systems Engineering Xi'an Jiaotong University Shaanxi Key Laboratory of Intelligent Robots School of Mechanical Engineering Xi'an Jiaotong University Department of Electrical Engineering and Automation Luoyang Institute of Science and Technology School of Mechanical Engineering Hangzhou Dianzi University

The burgeoning market for lithium-ion batteries has stimulated a growing need for more reliable battery performance monitoring. Accurate state-of-health(SOH) estimation is critical for ensuring battery operational performance. Despite numerous data-driven methods reported in existing research for battery SOH estimation, these methods often exhibit inco.sistent performance across different application scenarios. To address this issue and overco.e the performance limitations of individual data-driven models,integrating multiple models for SOH estimation has received co.siderable attention. Ensemble learning(EL) typically leverages the strengths of multiple base models to achieve more robust and accurate outputs. However, the lack of a clear review of current research hinders the further development of ensemble methods in SOH estimation. Therefore, this paper co.prehensively reviews multi-model ensemble learning methods for battery SOH estimation. First, existing ensemble methods are systematically categorized into 6 classes based on their co.bination strategies. Different realizations and underlying co.nections are meticulously analyzed for each category of EL methods, highlighting distinctions, innovations, and typical applications. Subsequently, these ensemble methods are co.prehensively co.pared in terms of base models, co.bination strategies, and publication trends. Evaluations across 6 dimensions undersco.e the outstanding performance of stacking-based ensemble methods. Following this, these ensemble methods are further inspected from the perspectives of weighted ensemble and diversity, aiming to inspire potential approaches for enhancing ensemble performance. Moreover, addressing challenges such as base model selection, measuring model robustness and uncertainty, and interpretability of ensemble models in practical applications is emphasized. Finally, future research prospects are outlined, specifically noting that deep learning ensemble is poised to advance ens

关键词： Lithium-ion battery State-of-health estimation Data-driven Machine learning Ensemble learning Ensemble diversity

High-energy-density lithium manganese iron phosphate for lithium-ion batteries: Progresses, challenges, and prospects

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Journal of Energy Chemistry 2025年第1期100卷 1-17页

作者： Bokun Zhang Xiaoyun Wang Shuai Wang Yan Li Libo Chen Handong Jiao Zhijing Yu Jiguo Tu State Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing research institute for Intelligent Wearable Systems The Hong Kong Polytechnic University institute of Advanced Structure Technology Beijing Institute of Technology

The soaring demand for smart portable electronics and electric vehicles is propelling the advancements in high-energy–density lithium-ion *** manganese iron phosphate (LiMnxFe1-xPO4) has garnered significant attention as a promising positive electrode material for lithium-ion batteries due to its advantages of low co.t,high safety,long cycle life,high voltage,good high-temperature performance,and high energy *** LiMnxFe1-xPO4has made significant breakthroughs in the past few decades,there are still facing great challenges in poor electronic co.ductivity and Li-ion diffusion,manganese dissolution affecting battery cycling performance,as well as low tap *** review systematically summarizes the reaction mechanisms,various synthesis methods,and electrochemical properties of LiMnxFe1-xPO4to analyze reaction processes accurately and guide material ***,the main challenges currently faced are co.cluded,and the co.responding various modification strategies are discussed to enhance the reaction kinetics and electrochemical performance of LiMnxFe1-xPO4,including multi-scale particle regulation,heteroatom doping,surface co.ting,as well as microsco.ic morphology ***,in view of the current research challenges faced by intrinsic reaction processes,kinetics,and energy storage applications,the promising research directions are *** importantly,it is expected to provide key insights into the development of high-performance and stable LiMnxFe1-xPO4materials,to achieve practical energy storage requirements.

关键词： Lithium manganese iron phosphate High energy density Lithium-ion batteries Reaction mechanism Tap density

Tackling the microlensing wave effects of strong lensing gravitational waves with TAAH

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 257-258页

作者： Zuhui Fan South-Western institute for Astronomy research Yunnan University

The rapid development of gravitational wave（GW） observations since their first detection in 2015 [1] has opened a co.pletely new window for exploring the Universe. co.sequently, astronomical research has entered the multimessenger era, allowing us to use different tracers to view the co.mos from various perspectives. Among others, the appealing application of gravitational wave events from co.pact binary mergers is that they can act as standard sirens to determine absolute co.mic distances entirely independent of standard candles. This approach is one of the most promising means to solve the current H0tension problem.

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Ultrabroad band microwave absorption from hierarchical MoO_(3)/TiO_(2)/Mo_(2)TiC_(2)Tx hybrids via annealing treatment

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Journal of Advanced Ceramics 2022年第9期11卷 1466-1478页

作者： Feiyue HU Fan ZHANG Xiaohan WANG Yaya LI Hailong WANG Rui ZHANG Hongxia LI Bingbing FAN School of Material Science and Engineering Zhengzhou UniversityZhengzhou 450001China School of Materials Science and Engineering Luoyang Institute of Science and TechnologyLuoyang 471023China Sinosteel luoyang institute of Refractories research co. Ltd.Luoyang 471039China

Two-dimensional(2D)transition metal carbide MXene-based materials hold great potentials applied for new electromagnetic wave(EMW)***,the application of MXenes in the field of electromagnetic wave absorption(EMA)is limited by the disadvantages of poor impedance matching,single loss mechanism,and easy *** this work,MoO_(3)/TiO_(2)/Mo_(2)TiC_(2)T_(x)hybrids were prepared by the annealing-treated Mo_(2)TiC_(2)T_(x)MXene and uniform MoO_(3)and TiO_(2)oxides in-situ grew on Mo_(2)TiC_(2)T_(x)*** the annealing temperature of 300℃,the minimum reflection loss(RLmin)value of MoO_(3)/TiO_(2)/Mo_(2)TiC_(2)T_(x)reaches-30.76 dB(2.3 mm)at 10.18 GHz with a significantly broadening effective absorption bandwidth(EAB)of 8.6 GHz(1.8 mm).The in-situ generated oxides creating numerous defects and heterogeneous interfaces enhance dipolar and interfacial polarizations and optimize the impedance matching of Mo_(2)TiC_(2)T_(x).co.sidering the excellent overall performance,the MoO_(3)/TiO_(2)/Mo_(2)TiC_(2)T_(x)hybrids can be a promising candidate for EMA.

关键词： MoO_(3)/TiO_(2)/Mo_(2)TiC_(2)T_(x)co.posites Mo_(2)TiC_(2)T_(x)MXene electromagnetic wave absorption(EMA) impedance matching interfacial polarization dielectric loss