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Precise phase adjustment and antibacterial property of copper sulfide particles in confined mesoporous silica nanoreactor

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Particuology 2024年第2期85卷 113-121页

作者： Shiyu Xu Jinyong Wu Zhongzhen Ren Dechao Niu low dimensional materials Chemistry Laboratory Key Laboratory for Ultrafine Materials of Ministry of EducationFrontier Science Center of the Materials Biology and Dynamic ChemistryShanghai Engineering Research Center of Hierarchical NanomaterialsSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai200237China

Bacteria-caused wound infection greatly threatens human health,thus developing an efficient and safe antibacterial agent without drug resistance is still a great ***,a confined vulcanization strategy is proposed to construct copper sulfides-loaded dual-mesoporous silica nanospheres(Cux-Sy@DMSNs)with various crystal phases for reactive oxygen species(ROS)-mediated and photothermal antibacterial *** the pore confinement of DMSNs,the crystal phases of copper sulfides including CuS,Cu_(9)S_(5)and Cui.96S can be easily controlled by changing the vulcanization *** relationships between the crystal phases and photothermal properties as well as peroxidase-like activity of copper sulfides were systematically *** show that the obtained CuS@DMSNs exhibited higher photothermal ability with remarkable photothermal conversion efficiency of 36.86%in the second near-infrared region(NIR-II)and better peroxidase-like activity,compared to those of Cu_(9)S_(5)@DMSNs and Cu_(1.96)S@*** a result,the in vitro experiments showed the good antibacterial effect against both gram-negative *** and gram-positive *** under 1064 nm laser irradiation and the presence of H_(2)O_(2).Besides,the CCK-8 assay indicated that CuS@p-DMSNs have minimal cytotoxicity against normal human umbilical vein endothelial cells at the ranged ***,the resultant CuS@p-DMSNs could act as a promising antibacterial agent for deep wound bacterial infection treatment.

关键词： Copper sulfides Mesoporous silica Photothermal Reactive oxygen species Antibacterial agent

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Ultrathin surface coating of Cu enabling long-life Zn metal anodes

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Rare Metals 2024年第5期43卷 2125-2135页

作者： Sang-Sang Liu Ya-Ru Liang Wen-Long Chen Ze-Hua Wang Yi-Long Dai Fu-Gang Qi Zeng-Sheng Ma Xiao-Ping Ouyang School of materials Science and Engineering Xiangtan UniversityXiangtan 411105China Key Laboratory of low dimensional materials and Application Technology of Ministry of Education Xiangtan UniversityXiangtan 411105China

Aqueous zinc-ion batteries(AZIBs)are regarded as promising energy storage devices due to their low cost,high capacity,and ecological ***,the severe dendritic growth and side reactions hinder their practical applicability ***,an ultrathin Cu coating layer(~200 nm)is decorated on zinc foils via filtered cathodic vacuum arc deposition technology,aiming to achieve high-performance *** Cu layer effectively suppresses chemical corrosion and hydrogen evolution reactions and enables preferential(002)Zn deposition during the stripping/plating ***,the Cu@Zn anode represents an elongated cycle life over 4,000 h at 2 mA·cm^(-2)/2 mAh·cm^(-2).Even in conditions of high current density of 5 and 10 mA·cm^(-2),the Cu@Zn anode shows prolonged cycling stability exceeding 4000 and 2000 h,*** advantages also bring high Coulombic efficiency of 99.87%under 5 mAh·cm^(-2)in Cu@Ti||Zn half-cell over 1500 ***,the Cu@Zn||MnO_(2)full cell demonstrates a superior cyclability with a specific capacity of 203 mAh·g^(-1)after 500 cycles a1 A·g^(-1).

关键词： Zn ion battery Zn metal anode Zn(002)plane Cu coating

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Mode-switchable dual-color infrared quantum cascade detector

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Photonics research 2024年第2期12卷 253-259页

作者： YIXUAN ZHU SHENQIANG ZHAI KUN LI KAI GUO QIANGQIANG GUO JINCHUAN ZHANG SHUMAN LIU LIJUN WANG FENGQI LIU JUNQI LIU Key Laboratory of Semiconductor materials Science Beijing Key Laboratory of Low Dimensional Semiconductor Materials and DevicesInstitute of SemiconductorsChinese Academy of SciencesBeijing 100083China Center of materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

In this paper,a patch-antenna-array enhanced quantum cascade detector with freely switchable operating modes among mid-wave,long-wave,and dual-color was proposed and *** dual-color absorption occurs in a single active region through an optimized coupled miniband diagonal-transition subbands arrangement,and a successful separation of the operation regimes was realized by two nested antenna arrays with different patch sizes up to room *** 77 K,the 5.7-μm channel achieved a peak responsivity of 34.6 mA/W and exhibited a detectivity of 2.0×10^(10)Jones,while the 10.0-μm channel achieved a peak responsivity of 87.5 mA/W,giving a detectivity of 5.0×10^(10)*** a polarization modulation of the incident light,the minimum cross talk of the mid-wave and the long-wave operating modes was 1:22.5 and 1:7.6,*** demonstration opens a new prospect for multicolor infrared imaging chip integration technology.

关键词： antenna polarization quantum

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Critical behavior of quasi-two-dimensional ferromagnet Cr1.04Te2

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Chinese Physics B 2024年第7期33卷 97-105页

作者：钮伟宋沁心常世琦王敏袁奎高嘉程王硕王振东刘凯斐刘萍徐永兵张晓倩普勇 Jiangsu Provincial Engineering research Center of low dimensional Physics and New Energy & School of Science Nanjing University of Posts and Telecommunications School of Electronic Science and Engineering Nanjing University Key Laboratory of Quantum materials and Devices of Ministry of Education School of Physics Southeast University

The self-intercalation of Cr into pristine two-dimensional（2D） van der Waals ferromagnetic CrTe2,which forms chromium tellurides（CrxTe2）,has garnered interest due to their remarkable magnetic characteristics and the wide variety of chemical compositions ***,comprehensive basic characterization and magnetic studies are conducted on quasi-2D ferromagnetic *** of the isothermal magnetization curves are conducted around the critical temperature to systematically investigate the critical ***,the critical exponents β=0.2399,γ=0.859,and δ=4.3498,as well as the Curie temperature TC=249.56 K,are determined using various methods,including the modified Arrott plots,the Kouvel-Fisher method,the Widom scaling method,and the critical isotherm *** results indicate that the tricritical mean-field model accurately represents the critical behavior of Cr1.04Te2.A magnetic phase diagram with tricritical phenomenon is thus *** investigations confirm that the critical exponents obtained conform to the scalar equation near TC,indicating their self-consistency and *** work sheds light on the magnetic properties of quasi-2D Cr1.04Te2,broadening the scope of the van der Waals crystals for developments of future spintronic devices operable at room temperature.

关键词： critical behavior magnetic measurement self-intercalation van der Waals magnets

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Band structures of strained kagome lattices

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Chinese Physics B 2024年第2期33卷 456-463页

作者：徐露婷杨帆 Center for Joint Quantum Studies and Department of Physics School of ScienceTianjin UniversityTianjin 300354China Tianjin Key Laboratory of low dimensional materials Physics and Preparing Technology Department of PhysicsTianjin UniversityTianjin 300354China

materials with kagome lattices have attracted significant research attention due to their nontrivial features in energy *** theoretically investigate the evolution of electronic band structures of kagome lattices in response to uniaxial strain using both a tight-binding model and an antidot model based on a periodic muffin-tin *** is found that the Dirac points move with applied ***,the flat band of unstrained kagome lattices is found to develop into a highly anisotropic shape under a stretching strain along y direction,forming a partially flat band with a region dispersionless along ky direction while dispersive along kx *** results shed light on the possibility of engineering the electronic band structures of kagome materials by mechanical strain.

关键词： kagome lattice strain band structure engineering

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Overcoming side reaction effects in the colloidal synthesis of ZnSe/ZnS core/shell quantum dots with an etching strategy

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Nano research 2024年第8期17卷 7020-7026页

作者： Jinhua He Chenhui Wang Mingrui Liu Muhammad Ramzan Zhiwei Long Xian-gang Wu Yu Chen Haizheng Zhong MIIT Key Laboratory for low-dimensional Quantum Structure and Devices School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing Engineering research Center for Mixed Reality and Advanced Display Technology School of Optics and PhotonicsBeijing Institute of TechnologyBeijing 100081China

The potential use of large-size ZnSe quantum dots as blue emitters for display applications has greatly inspired the colloidal ***,we report the negative effects of side reactions of large-size ZnSe quantum *** side reactions between oleic acid and oleylamine generated amidation products and H_(2)O,which led to the hydrolysis of Zn(OA)2 to Zn(OH)2 and the subsequent formation of zinc oxide(ZnO)and zinc bis[diphenylphosphinate](Zn(DPPA)2)*** side reactions resulted in the formation of a defective surface including a Se-rich surface and oxygen-related *** negative effects can be overcome by adopting an etching strategy using potassium fluoride and myristic acid in *** overcoating a ZnS shell,blue emissive ZnSe/ZnS quantum dots with a maximum photoluminescence quantum yield of up to 91%were *** further fabricated ZnSe quantum dots-based blue light-emitting diodes with an emission peak at 456 *** device showed a turn-on voltage of 2.7 V with a maximum external quantum efficiency of 4.2%and a maximum luminance of 1223 cd·m^(−2).

关键词： quantum dots ZnSe side reactions surface etching light-emitting diodes

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Enhanced activation of peroxymonosulfate on layered molybdenum disulfide loaded with Co–La bimetallic oxide for efficient degradation of chloramphenicol

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Rare Metals 2024年第9期43卷 4628-4635页

作者： Yu-Ning Fan Yun-Qiu Zhang San-Shuang Gao Zeng-Hui Bi Yin Wang Shu-Xing Zhou Qian Liu Tian-Ping Lv Guang-Zhi Hu Institute for Ecological research and Pollution Control of Plateau Lakes School of Ecology and Environmental ScienceYunnan University Hubei Key Laboratory of low dimensional Optoelectronic materials and Devices Hubei University of Arts and Science Institute for Advanced Study Chengdu University

The use of transition metal-activated peroxymonosulfate（PMS） as an advanced oxidation technology has gained recognition. This study developed a catalyst using cobaltDlanthanum bimetallic oxide supported on layered molybdenum disulfide （Mo S2） as a carrier. The CoDLa/Mo S2catalyst was synthesised through coprecipitation, followed by calcination with an optimised metal ratio of Co:La=2:1 to activate PMS and degrade trace chloramphenicol（CAP） in water. The chemical composition of the catalyst was confirmed using X-ray diffraction （XRD） and X-ray photoelectron spectroscopy （XPS）. At catalyst and PMS dosages of 0.1 and 0.5 g·L-1, respectively, the degradation rate of CAP was 95% with in 30 min. The catalyst exhibitedstrong resistance to most interfering anions and maintained a high degradation rate at p H 3D11. Liquid chromatographyDmass spectrometry analysis revealed the potential degradation pathways of CAP in the CoDLa/Mo S2（2:1）/PMS system. For other pollutants, such as oxytetracycline,complete degradation was achieved within 20 min,demonstrating the broad applicability of the CoDLa/Mo S2（2:1）/PMS system for the degradation and removal of antibiotic organic contaminants. This study offers a feasible approach for the degradation of antibiotic organic pollutants, including CAP, in natural water bodies.

关键词： Catalysts

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Lensless opto-electronic neural network with quantum dot nonlinear activation

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Photonics research 2024年第4期12卷 682-690页

作者： WANXIN SHI XI JIANG ZHENG HUANG XUE LI YUYANG HAN SIGANG YANG HAIZHENG ZHONG HONGWEI CHEN Beijing National research Center for Information Science and Technology(BNRist) Department of Electronic EngineeringTsinghua UniversityBeijing 100084China China Mobile research Institute Beijing 100053China MIIT Key Laboratory for low-dimensional Quantum Structure and Devices School of Materials Sciences&EngineeringBeijing Institute of TechnologyBeijing 100081China

With the swift advancement of neural networks and their expanding applications in many fields, optical neural networks have gradually become a feasible alternative to electrical neural networks due to their parallelism, high speed, low latency, and power consumption. Nonetheless, optical nonlinearity is hard to realize in free-space optics, which restricts the potential of the architecture.

关键词： network neural networks

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Side ionic-gated perovskite/graphene heterojunction synaptic transistor with bipolar photoresponse for neuromorphic computing

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Photonics research 2024年第6期12卷 1167-1174页

作者： XIAOYING HE MINGHAO XU SHILIN LIU KUN WANG BOWEN CAO LAN RAO XIANGJUN XIN School of Electronic Engineering and Beijing Key Laboratory of Space-Ground Interconnection and Convergence Beijing University of Posts and TelecommunicationsBeijing 100876China Key Laboratory of Semiconductor materials Science Beijing Key Laboratory of Low Dimensional Semiconductor Materials and DevicesInstitute of SemiconductorsChinese Academy of SciencesBeijing 100083China

By combining the good charge transport property of graphene and the excellent photo-carrier generation char-acteristic of perovskite nanocrystal,we propose and demonstrate an ionic-gated synaptic transistor based on CsPbBr_(3)∕graphene heterojunction for bipolar *** the potential barrier of the CsPbBr_(3)∕graphene heterojunction by the ionic-gate of the electrical double-layer effect can promote the sepa-ration of photogenerated carriers and effectively retard their *** the ionic-gate-tunable Fermi level of graphene and the pinning effect of perovskite nanocrystal,the bipolar photocurrent responses correspond-ing to the excitatory and inhibitory short-term and long-term plasticity are realized by adjusting the negative gate bias.A series of synaptic functions including logic operation,Morse coding,the optical memory and electrical erasure effect,and light-assisted re-learning have also been demonstrated in an optoelectronic collaborative ***,the excellent optical synaptic behaviors also contribute to the handwritten font recognition accuracy of-95%in artificial neural network *** results pave the way for the fabrication of bipolar photoelectric synaptic transistors and bolster new directions in the development of future integrated human ret-inotopic vision neuromorphic systems.

关键词： perovskite ionic Morse

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High-performance carbon-electrode-based self-powered optoelectronic synaptic devices

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Science China(Information Sciences) 2024年第5期67卷 339-340页

作者： Wen HUANG Xuwen XIA Huixing ZHANG Tenglong GUO Pengjie HANG Bin LI Jiawei TANG Biao LI Chen ZHU Lei WANG Deren YANG Xuegong YU Xing'ao LI Jiangsu Provincial Engineering research Center of low dimensional Physics and New Energy & School of Science Nanjing University of Posts and Telecommunications College of Integrated Circuit Science and Engineering Nanjing University of Posts and Telecommunications State Key Laboratory of Silicon and Advanced Semiconductor materials Zhejiang University

A two-terminal self-powered optoelectronic structure could mimic synaptic functions of a human brain synapse unit(Figure 1(a)) based on the photovoltaic effects [1], demonstrating the potential for decreasing energy consumption for future computing. However, current self-powered optoelectronic synaptic devices face issues of stability and cost,which mainly arise from noble metal electrodes and independent hole transport layers used in these structures. Substituting low-cost carbon for these metal electrodes and carrier transport layers may promise to solve these challenges.

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