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Journal of environmental Sciences 2024年第6期140卷 91-102页

作者： Ruxian Hou Jiewen Xiao Qian Wu Tianyu Zhang Qiang Wang Beijing Key Lab for Source control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China Engineering Research Center for Water Pollution Source control&Eco-remediation College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China

CO_(2)hydrogenation to methanol has become one of the most promising ways for CO_(2)utilization,however,the CO_(2)conversion rate and methanol selectivity of this reaction still need to be improved for industrial *** we investigated the structure-activity relationship for CO_(2)conversion to methanol of In_(2)O_(3)-based catalysts by modulating morphology and decorating *** different Au/In_(2)O_(3)catalysts were prepared,their activity follow the sequence of Au/In_(2)O_(3)-nanosphere(Au/In_(2)O_(3)-NS)>Au/In_(2)O_(3)-nanoplate(Au/In_(2)O_(3)-NP)>Au/In_(2)O_(3)-hollow microsphere(Au/In_(2)O_(3)-HM).Au/In_(2)O_(3)-NS exhibited the best performance with good CO_(2)conversion of 12.7%,high methanol selectivity of 59.8%,and large space time yield of 0.32 g CH_(3)OH/(hr·gcat)at 300℃.The high performance of Au/In_(2)O_(3)-NS was considered as the presence of *** contributes to the creation of more surface oxygen vacancies,which further promoted the CO_(2)adsorption and facilitated CO_(2)activation to form the formate intermediates towards *** work clearly suggests that the activity of In_(2)O_(3)catalyst can be effective enhanced by structure engineering and Au decorating.

关键词： CO_(2)hydrogenation Methanol Au/In_(2)O_(3) Morphology Oxygen vacancies

Characteristics of rural domestic sewage discharge and their driving mechanisms: evidence from the Northern Region, China

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Frontiers of environmental Science & Engineering 2024年第7期18卷 47-58页

作者： Jianguo Liu Ziyu Zhou Pengyu Li Zixuan Wang Ying Yan Xuezheng Yu Wenkai Li Tianlong Zheng Yingnan Cao Wenjun Wu Wenqian Cai Zhining Shi Junxin Liu Key laboratory of environmental Pollution control and Remediation at Universities of Inner Mongolia Autonomous Region College of Resources and Environmental EngineeringInner Mongolia University of TechnologyHohhot 010051China State Key laboratory of environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China SCEGC No.12 Construction Engineering Group Co. Ltd.Ankang 725000China State environmental Protection Key laboratory of environmental Planning and Policy Simulation Chinese Academy of Environmental PlanningBeijing 100041China Technical Centre for Soil Agriculture and Rural Ecology and EnvironmentMinistry of Ecology and EnvironmentBeijing 100012China Sustainable Infrastructure and Resource Management(SIRM) UniSA STEMUniversity of South AustraliaSouth AustraliaMawson LakesSA 5095Australia

The traits of rural domestic sewage emission are unclear,negatively affecting rural domestic sewage treatment and sewage *** study used data from the Second National Pollution Source Census Bulletin to establish a data *** spatial distribution characteristics and main factors influencing rural sewage discharge in the Northern Region were studied using spatial autocorrelation analysis and structural *** findings demonstrated that(l)a significant Spearman correlation between drainage water volume(DwV),chemical oxygen demand(COD),ammonia nitrogen(NH_(3)-N),total nitrogen(TN),and total phosphorus(TP)and that the correlation coefficients between DWV and COD,NH,-N,TNand TP were 0.87**,1.0**,0.99**,0.99**,respectively;(2)rural sewage discharge showed spatial autocorrelation,and rural domestic sewage discharge in the districts and counties with an administration was significantly higher than in the surrounding areas;and(3)social development was the main driver rural domestic sewage changes(path coefficient was 0.407**),and the main factors influencing rural domestic sewage discharge were the urbanization rate,years of education,and population age *** study obtained the spatial variation law and clarified the main influencing factors of rural domestic sewage to provide data support and a theoretical basis for subsequent rural sewage collection and *** of the Inner Mongolia Autonomous Region in northern China as a typical case,provides a theoretical foundation for scientific decision-making on rural domestic sewage treatment at the national and regional levels and offers new perspectives for managing pollutants.

关键词： Rural domestic sewage Emission characteristics Spatial autocorrelation analysis Influencing factors

Unraveling the role of formate in improving nitrogen removal via coupled partial denitrification-anammox

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Frontiers of environmental Science & Engineering 2024年第9期18卷 79-90页

作者： Wanlu Zhu Rui Xiao Min Xu Wenbo Chai Wenlong Liu Zhengyu Jin David Ikumi Huijie Lu Key laboratory of environmental Remediation and Ecological Health(Ministry of Education) College of Environmental and Resource SciencesZhejiang UniversityHangzhou 310058China China National Nuclear Corporation Beijing Research Institute of Chemical Engineering and MetallurgyBeijing 100029China College of Environment Zhejiang University of TechnologyHangzhou 310014China Key laboratory of Ecology and Environment in Minority Areas National Ethnic Affairs CommissionCollege of Life&Environmental SciencesMinzu University of ChinaBeijing 100081China Water Research Group Department of Civil EngineeringUniversity of Cape TownRondebosch 7700South Africa Key laboratory of Water Pollution control and environmental Safety Hangzhou 310058China

The addition of traditional carbon sources(e.g.,acetate)could favor heterotrophic overgrowth in partial denitrification coupled with anammox(PD–A)systems,thus hindering the performance and stability of this novel wastewater nitrogen removal ***,it is necessary to develop an effective,environmentally friendly,and inexpensive *** study demonstrated the potential of formate to enhance the performance and community stability of PD–A under mainstream *** a laboratory-scale biofilm reactor,formate addition(COD/NO_(3)^(–)–N=1.75)improved nitrogen removal efficiency(from 72.1±3.5%to 81.7±2.7%),EPS content(from 106.3±8.1 to 163.0±15.5 mg/gVSS)and increased anammox bacteria growth(predominantly Candidatus Brocadia,from 29.5±0.7%to 34.5±5.4%)while maintaining stable heterotrophs dominated by methylotrophic ***–NanoSIMS revealed a formate uptake using *** and Desulfobacillus,with *** being the major contributor to partial nitrate reduction to *** can synthesize diverse hydrophobic amino acids and provide key nutrients for *** achieve comparable nitrogen removal,the cost of the formate-driven PD–A process should be 11.2%lower than that of *** results greatly enrich our understanding of C1 metabolism represented by formate in anammox communities and its application in the context of coupling partial denitrification–anammox toward enhanced nitrogen removal in global wastewater treatment systems.

关键词： Formate Mixotrophic growth Partial denitrification-anammox Metabolic interaction FISH-NanoSIMS

Leaching kinetics and permeability of polyethyleneimine added ammonium sulfate on weathered crust elution-deposited rare earth ores

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Journal of Rare Earths 2024年第8期42卷 1610-1619,I0008页

作者： Huifang Yang Aoyang Sha Zhengyan He Chenjie Wu Yuanlai Xu Jingjing Hu Zhigao Xu Ru'an Chi Key laboratory for Green Chemical Process of Ministry of Education School of Resources&Safety EngineeringWuhan Institute of TechnologyWuhan 430073China Key laboratory of Resources Conversion and Pollution control of the State Ethnic Affairs Commission College of Resources and Environmental ScienceSouth-Central MinzuUniversityWuhan430074China

At present,in-situ leaching of weathered crust elution-deposited rare earth ores(WCE-DREOs) encounter with problems such as long leaching cycles,slow infiltration rate and low product *** order to solve the above problems,the conventional leaching agent ammonium sulfate((NH_(4))_(2)SO_(4)) was compounded with polymeric surfactant polyethyleneimine(PEI) to form a composite leaching *** effects of leaching temperature,PEI *** rate and pH on leaching kinetics and permeability of rare earths(RE) and aluminum(AI) in orebody were *** is found that with temperature increasing,the time required to reach leaching equilibrium for both RE and Al is shortened,the apparent activation energies of RE and AI are 14.79 and 13.45 kJ/mol,respectively,and the leaching processes are in accordance with the outer diffusion control,When the concentrations of(NH_(4))_(2)SO_(4) and PEI in the composite leaching agent are 2.0 wt% and 0.4 wt%;the time required to reach leaching equilibrium for RE and AI is about 50% shorter than that using(NH_(4))_(2)SO_(4) alone,and the leaching efficiencies of RE are slightly higher than that of *** increasing the temperature and flow rate of the composite leaching agent can improve the leaching efficiencies of RE and Al,but pH has neglected effects on the leaching efficiencies of *** PEI concentrations below 0,4 wt%, the addition of PEI promotes the leaching of RE and *** column leaching studies of the WCE-DREO,the addition of 0.4 wt% PEI to the traditional leaching agent(NH_(4))_(2)SO_(4) has no impact on the leaching efficiencies of ***,it can significantly increase the infiltration rate of WCE-DREO,shortening the leaching time per 10 mL effluent from about 30 min for(NH_(4))_(2)SO_(4) leaching system to 20 min for the composite leaching *** leaching time is shortened by one-third,and the leaching cost is reduced,which can provide theoretical guidance for the development and commercial implementa

关键词： Polyethyleneimine Kinetics Rare earths Permeability Activation energy

Green manufacturing for achieving carbon neutrality goal requires innovative technologies:A bibliometric analysis from 1991 to 2022

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Journal of environmental Sciences 2024年第6期140卷 255-269页

作者： Sheng Zhang Xintian Wang Jiayu Xu Qinqin Chen Meng Peng Jiming Hao School of Environment Tsinghua UniversityBeijing 100084China School of Environment&Natural Resources Renmin University of ChinaBeijing 100872China State environmental Protection Key laboratory of Sources and control of Air Pollution Complex Beijing 100084China

Recent years have seen a significant increase in interest in green manufacturing as a key driver of global carbon-neutral efforts and sustainable *** find the research hotspots of green manufacturing and reveal future research trends,this study reviewed and analyzed research articles from the Web of Science database on green manufacturing from1991 to 2022 using a bibliometric *** findings indicate a significant rise in the number of articles related to green manufacturing since the ***,there has been an increase in the involvement of scholars from developing countries such as China and India in this *** on the literature review and bibliometric cluster analysis on green manufacturing,we believed that future research may continue following the lines of intelligent technology integration,adoption of frontier engineering techniques,and industry development in line with carbon reduction targets.A framework for future green manufacturing development is proposed,with a focus on Chinese *** framework could provide policy implications for developing countries looking to pursue opportunities for development in green manufacturing.

关键词： Green manufacturing Carbon neutrality Sustainable development Innovative technologies China

Enhanced degradation of florfenicol by microscale SiC/Fe:Dechlorination via hydrogenolysis

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Chinese Chemical Letters 2024年第7期35卷 218-221页

作者： Yun-Fei Zhang Chun-Hui Zhang Jian-Hui Xu Lei Li Dan Li Jin-Hong Fan Jiale Gao Xin Quan Qi Wu Yue Zou Yan-Ling Liu Dongguan University of Technology School of Environment and Civil EngineeringDongguan 523830China State Key laboratory of Pollution control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China

Herein,the degradation of florfenicol(FLO)over zero-valent iron(ZVI)enhanced by SiC was systematically *** was found that 5 g/L of ZVI/SiC(1:3)at pH 3.0 could completely degrade 20 mg/L of FLO within 1 h,with a Kobsvalue of 0.0873 min^(-1),12.5 times greater than that of pure ZVI(0.0069 min^(-1)).Vibrating sample magnetometer(VSM)characterizations revealed that the use of SiC supporter reduces the magnetic intensity of ZVI,which mitigates iron particle agglomeration,increases Brunauer-Emmett-Teller(BET)surface area,and enhances FLO degradation ***,ZVI/SiC exhibits a much lower hydrogen evolution potential(HEP)and significantly higher corrosion currents compared to pure *** was proposed to undergo degradation via reductive dechlorination,involving a hydrogenolysis mechanism that entails the cleavage of theσ*** study provides new insights into the reduction hydrogenation mechanism of ZVI.

关键词： Zero-valent iron Silicon carbide Reductive dechlorination Hydrogenolysis Florfenicol

Single-atom Ag-loaded carbon nitride photocatalysts for efficient degradation of acetaminophen:The role of Ag-atom and O_(2)

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Journal of environmental Sciences 2024年第5期139卷 12-22页

作者： Yi Yuan Wen-Long Wang Zhi-Wei Wang Jin Wang Qian-Yuan Wu Key laboratory of Microorganism Application and Risk control of Shenzhen Guangdong Provincial Engineering Research Center for Urban Water Recycling and Environmental SafetyInstitute of Environment and EcologyShenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China Shenzhen environmental Science and New Energy Technology Engineering laboratory Tsinghua-Berkeley Shenzhen InstituteShenzhen 518055China College of Materials Science and Engineering Shenzhen UniversityShenzhen 518071China

Carbon nitride has been extensively used as a visible-light photocatalyst,but it has the disadvantages of a low specific surface area,rapid electron-hole recombination,and relatively low light *** this study,single-atom Ag was successfully anchored on ultrathin carbon nitride(UTCN)via thermal polymerization,the catalyst obtained is called *** Ag hardly changed the carbon nitride's layered and porous physical *** exhibited efficient visible-light photocatalytic performances in the degradation of various recalcitrant pollutants,eliminations of 85% were achieved by visible-light irradiation for *** with Ag improved the photocatalytic performance of UTCN by narrowing the forbidden band gap from 2.49 to 2.36 e V and suppressing electron-hole pair *** addition,Ag doping facilitated O_(2) adsorption on UTCN by decreasing the adsorption energy from -0.2 to -2.22 e V and favored the formation of O_(2)^(·-).Electron spin resonance and radical-quenching experiments showed that O_(2)^(·-)was the major reactive species in the degradation of Acetaminophen(paracetamol,APAP).

关键词： Ag single atom Carbon nitride Photocatalysis Visible light Adsorption energy Reactive species

The development of local ambient air quality standards: A case study of Hainan Province, China

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Eco-Environment & Health 2024年第1期3卷 11-20页

作者： Qian Song Nannan Zhang Yanning Zhang Dejia Yin Jiming Hao Shuxiao Wang Shengyue Li Wenshuai Xu Weijun Yan Xinxin Meng Xinghong Xu Xiaochen Wu Donghai Xie Yun Zhu Qipeng Qu Xuan Hou Yueqi Jiang Zhaoxin Dong Haotian Zheng Yisheng Sun Zeqi Li Bin Zhao State Key Joint laboratory of environmental Simulation and Pollution control School of EnvironmentTsinghua UniversityBeijing 100084China State environmental Protection Key laboratory of Sources and control of Air Pollution Complex Beijing 100084China Institute of Strategic Planning Chinese Academy of Environmental PlanningBeijing 100041China Hainan Research Academy of environmental Sciences Haikou 571126China Hainan Provincial Ecological and environmental Monitoring Center Haikou 570206China Hainan Radiation environmental Monitoring Station Haikou 571126China Guangdong Provincial Key laboratory of Atmospheric Environment and Pollution control College of Environment and EnergySouth China University of TechnologyGuangzhou Higher Education Mega CenterGuangzhou 510006China

The ambient air quality standard(AAQS)is a vital policy instrument for protecting the environment and human *** Province is at the forefront of China's efforts to protect its ecological environment,with an official goal to achieve world-leading air quality by ***,neither the national AAQS nor the World Health Organization guideline offers sufficient guidance for improving air quality in Hainan because Hainan has well met the former while the latter is excessively ***,the establishment of Hainan's local AAQS becomes ***,research regarding the development of local AAQS is scarce,especially in comparatively more polluted countries such as *** relatively high background values and significant interannual fluctuations in air pollutant concentrations in Hainan present challenges in the development of local *** research proposes a world-class local AAQS of Hainan Province by reviewing the AAQS in major countries or regions worldwide,analyzing the influence of different statistical forms,and carefully evaluating the attainability of the *** the proposed AAQS,the annual mean concentration limit for PM2.5,the annual 95th percentile of daily maximum 8-h mean(MDA8)concentration limit for O_(3),and the peak season concentration limit for O_(3) are set at 10,120,and 85μg/m^(3),*** study indicates that,with effective control policies,Hainan is projected to achieve compliance with the new standard by *** implementation of the local AAQS is estimated to avoid 1,526(1,253–1,789)and 259(132–501)premature deaths attributable to longterm exposure to PM2.5 and O_(3) in Hainan in 2035,respectively.

关键词： Local ambient air quality standard Statistical form Feasibility Health effects Hainan province

Unveiling microplastic distribution and interactions in the benthic layer of the Yangtze River Estuary and East China Sea

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environmental Science and Ecotechnology 2024年第4期20卷 114-122页

作者： Xinyu Ge Feng Xu Bo Li Lili Liu Xiao Lu Lijuan Wang Yunxiao Zhang Jiangpeng Li Jiawei Li Yuanyuan Tang School of environmental Science and Engineering College of EngineeringSouthern University of Science and TechnologyShenzhen518055China State environmental Protection Key laboratory of environmental Risk Assessment and control on Chemical Process School of Resource and Environmental EngineeringEast China University of Science and TechnologyShanghai200237China School of Marine Science and Technology Zhejiang Ocean UniversityZhoushan316004China

Microplastics(MPs),recognized as an emerging global environmental concern,have been extensively detected worldwide,with specific attention directed towards the Yangtze River Estuary(YRE)and East China Sea(ECS)*** their critical research significance,there remains a knowledge gap concerning the distribution of MPs in the benthic layer within this area,particularly regarding interactions governing their *** we illuminate the distribution of MPs within the benthic layer and unravel the intricate interplay between bottom water and sediment in the YRE and *** find that MPs are notably more abundant in bottom water,ranging from 8 to 175 times higher than in surface *** MPs predominantly consist of polyester fibers,exhibit a size range between 0.5 and 5.0 mm,and display distinct ***-occurrence network analysis and Principal Coordinate Analysis confirm a robust correlation between MPs in bottom water and sediment,signifying the pivotal role of bottom water in mediating the distribution and transportation of MPs within the benthic ***,a positive correlation between MPs in sediment and bottom water turbidity underscores the impact of surface sediment resuspension and upwelling on MPs *** study clarifies the intricate interactions within the benthic layer and highlights the crucial role of bottom water as a mediator in the vertical distribution of MPs,advancing our understanding of the“source-to-sink”transport processes governing MPs within water-sediment systems.

关键词： Microplastics Bottom water Sediment Distribution Correlation analysis

Influences of clean fracturing fluid viscosity and horizontal in-situ stress difference on hydraulic fracture propagation and morphology in coal seam

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International Journal of Coal Science & Technology 2024年第3期11卷 159-175页

作者： Gang Wang Shuxin Wang Yixin Liu Qiming Huang Shengpeng Li Shuliang Xie Jinye Zheng Jiuyuan Fan College of Safety and environmental Engineering Shandong University of Science and TechnologyQingdao266590China Mine Disaster Prevention and control-Ministry of State Key laboratory Breeding Base Shandong University of Science and TechnologyQingdao266590China

The viscosity of fracturing fluid and in-situ stress difference are the two important factors that affect the hydraulic fracturing pressure and propagation morphology. In this study, raw coal was used to prepare coal samples for experiments, and clean fracturing fluid samples were prepared using CTAB surfactant. A series of hydraulic fracturing tests were conducted with an in-house developed triaxial hydraulic fracturing simulator and the fracturing process was monitored with an acoustic emission instrument to analyze the influences of fracturing fluid viscosity and horizontal in-situ stress difference on coal fracture propagation. The results show that the number of branched fractures decreased, the fracture pattern became simpler, the fractures width increased obviously, and the distribution of AE event points was concentrated with the increase of the fracturing fluid viscosity or the horizontal in-situ stress difference. The acoustic emission energy decreases with the increase of fracturing fluid viscosity and increases with the increase of horizontal in situ stress difference. The low viscosity clean fracturing fluid has strong elasticity and is easy to be compressed into the tip of fractures, resulting in complex fractures. The high viscosity clean fracturing fluids are the opposite. Our experimental results provide a reference and scientific basis for the design and optimization of field hydraulic fracturing parameters.

关键词： Clean fracturing fluid Hydraulic fracturing Viscosity Horizontal in-situ stress difference Hydraulic fracture morphology Acoustic emission