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The risk factors and threshold level of subchronic inhalation exposure of reclaimed water

Journal of environmental Sciences 2024年第3期137卷 639-650页

作者： Jiayang Kong Yun Lu Yunru Ren Menghao Chen Gang Liu Liangliang Shi State Key Joint laboratory of environment Simulation and Pollution Control State Environment Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

Inhalation of reclaimed water is known to cause lung infammation,and free endotoxins have been shown to be a major risk factor for acute *** exposure has also been shown to induce infammatory responses with visible tissue ***,subchronic risk factors have yet to be identified,and a threshold for the protection of occupational populations during urban reuse is *** this study,potential risk factors in reclaimed water were examined by subchronic exposure with fractionated reclaimed water,and the health risk threshold was tested with a series of diluted reclaimed ***,following a 12-week exposure,macromolecules and microorganisms were found to be two major risk factors in reclaimed water that could cause pulmonary infammation,including increased proportion of polymorphonuclear leukocytes in bronchoalveolar fuid,formation of inducible bronchus-associated lymphoid tissue,and elevation of Immunoglobulin A ***,infammation persisted after a 4-week recovery *** calculated threshold of reclaimed water exposure for mice was 31.8 Endotoxin Unit(EU)/(kg·day)under when exposed to 50%additional relative humidity from reclaimed water at 25℃ for 2 hr/***,the subchronic threshold estimate for humans under the same exposure conditions was found to be 12.2 EU/(kg·day),corresponding to endotoxin levels of 61.7 EU/mL in reclaimed *** threshold level of endotoxin was lower than that in most non-potable reclaimed *** findings of this study suggest that occupational exposure of reclaimed water can serve as a potential risk to workers.

关键词： Reclaimed water Inhalation exposure Risk factor Threshold Infammation Endotoxin

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Selective adsorption of tetracycline by β-CD-immobilized sodium alginate aerogel coupled with ultrafiltration for reclaimed water

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Chinese Journal of Chemical Engineering 2024年第4期68卷 27-34页

作者： Xi Quan Jun Zhang Linlin Yin Wei Zuo Yu Tian State Key laboratory of Urban Water Resource and environment(SKLUWRE) School of EnvironmentHarbin Institute of TechnologyHarbin 150090China

In this work,a novel composite material based on β-cyclodextrin-immobilized sodium alginate aerogel(β-CD/NaAlg) was developed utilizing cross-linker of epichlorohydrin and applied as an adsorbent to remove tetracycline antibiotics from reclaimed wastewater.A series of characterizations were utilized to confirm the successful synthesis of the adsorbent and this β-CD/NaAlg presented a three-dimensional network at the nanoscale or *** optimal conditions(pH=4,t=8 h,β-CD:NaAlg=9,adsorbent dosage = 1.5 g·L-1),the maximum removal rate of β-CD/NaAlg to tetracycline was 70%.The adsorption behavior of tetracycline on β-CD/NaAlg conformed to the Freundlich isotherm model(R2=0.9977) and the pseudo-second-order kinetic model(R^(2)=0.9993).Moreover,the adsorbent still removed 55.3% of tetracycline after five ***,the adsorbent was integrated with ultrafiltration to adsorb tetracycline antibiotics from simulated reclaimed wastewater,and the removal rate of tetracycline reached 78.9% within 2 *** existence of Cr(Ⅵ) had a negligible impact on tetracycline removal,while the presence of humic acid exhibited a promoting *** possible adsorption mechanisms were also elucidated through X-ray photoelectron spectroscopy and density functional theory *** summary,β-CD/NaAlg represents an environmentally friendly,efficient,and sustainable adsorbent for removing tetracycline antibiotics from reclaimed water.

关键词： b-CD/NaAlg aerogel Covalent grafting Tetracycline antibiotics Ultrafiltration Selective adsorption Reclaimed water

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Exploring plant adaptation strategies to phosphorus limitation induced by nitrogen addition:foliar phosphorus allocation and root functional traits analysis in two dominant subalpine tree species

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Journal of Plant Ecology 2024年第4期17卷 154-166页

作者： Yan Su Yongfeng Tang Yi Hu Meiyu Liu Xuyang Lu Baoli Duan Institute of Mountain Hazards and environment Chinese Academy of SciencesChengdu 610041China Sichuan Ecological environment construction Engineering Supervision Co. Ltd.Chengdu 610084China

Plants adapt to the limitation of soil phosphorus(P)induced by nitrogen(N)deposition through a complex interaction of various root and leaf functional *** this study,a pot experiment was conducted to explore the effects of different levels of N addition(control,low N[LN]:25 kg N ha^(-1) yr^(-1),high N[HN]:50 kg N ha^(-1) yr^(-1))on tree growth,leaf nutrient content,foliar P fractions and root characteristics of two dominant tree species,the pioneer species Salix rehderiana Schneid and the climax species Abies fabri(Mast.)Craib,in a subalpine forest in southwestern *** results demonstrated that LN addition had a minimal impact on leaf N and P ***,HN addition significantly decreased the leaf P content in both *** rehderiana exhibited more pronounced increases in specific root length and specific root area under P deficiency triggered by HN addition when compared with *** contrast,*** showed weaker morphological responses to N addition but had a higher proportion of foliar P to metabolic P,as well as higher root exudates rate and root phosphatase activity in response to HN *** fabri employs a synergistic approach by allocating a greater amount of leaf P to metabolite P and extracting P from the soil through P-mobilizing exudates and root phosphatase activity,while *** exhibits higher flexibility in modifying its root morphology in response to P limitation induced by HN *** study provides insights into subalpine tree species adaptation to N-induced P limitation,emphasizing its significance for guiding forest management and conservation in the context of global climate change.

关键词： N deposition root functional traits root morphology root exudation P-scavenging strategy

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Towards experimental studying the airborne sound insulation of light frame walls with staggered studs

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Science China(Technological Sciences) 2024年第7期67卷 2230-2243页

作者： ZHANG YuCai YUE Kong XIE YiFan CHENG XiangYu SHI XinLei WU Peng ZHAO Hui College of Civil Engineering Nanjing Tech UniversityNanjing 211800China Key laboratory of Architectural Acoustic environment of Anhui Higher Education Institutes Hefei 230601China Nanjing Gongda construction Technology Co.Ltd. Nanjing 211800China

Light frame walls(LFWs) serve as common partition walls in prefabricated buildings due to their lightweight nature, costeffectiveness, energy efficiency, and adaptability for rapid on-site assembly. However, their acoustic insulation capability is hindered by issues such as sound bridges, resonance, and coincidence dips, resulting in inadequate sound insulation. This study aims to propose LFW designs with superior acoustic insulation suitable for practical engineering while meeting prevailing national standards. Nine full-scale LFW configurations were subjected to laboratory testing to evaluate the impact of staggered stud arrangements, stud types, and incorporation of compounded materials. The tests were performed between 100 and 5000 Hz,and the sound pressure level and reverberation time at 1/3 octave band were measured and used to calculate the weighted sound insulation index(Rw). Results demonstrated that the outlined design modifications significantly enhanced the sound insulation of the LFW. These modifications effectively mitigate the influence of sound bridges while addressing resonance and coincidence dips inherent in the wall system. Particularly noteworthy was the superior sound insulation achieved by staggered-stud LFWs with compounded materials, surpassing that of autoclaved lightweight concrete walls commonly used in prefabricated constructions despite having lesser thickness and surface density. Rwvalues increased from 43 to 54 dB compared to conventional LFWs, translating to a notable elevation in airborne sound insulation level from 4 to 7 as an internal separation component,meeting the requisite standards for most applications.

关键词： light frame wall staggered stud airborne sound insulation weighted sound insulation index

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From ore to MOF: A case of MIL-100(Fe) production from iron ore concentrates

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Progress in Natural Science:Materials International 2024年第1期34卷 66-73页

作者： Miao Chang Chiyao Tang Chong-Chen Wang Chen Zhao Beijing Key laboratory of Functional Materials for Building Structure and environment Remediation School of Environment and Energy Engineering Beijing University of Civil Engineering and Architecture

Within this work, iron ore concentrates instead of elemental iron Fe0and iron salts like Fe（NO3）3and FeCl3were selected as iron source to prepare MIL-100（Fe）(labeled as MIL-100（Fe）-ore). The corresponding synthesis cost is reduced to half of the MIL-100（Fe） produced from elemental iron and iron salts. As well, the unreacted iron ore concentrates can be easily separated from the as-prepared MIL-100（Fe）-ore by magnetic to facilitate the purification process, free of the strong acids to wash the residual iron. The as-obtained MIL-100（Fe）-ore with Langmuir surface area up to 2281.6 m2g-1displayed long-term chemical stability. Furthermore, the sorption capacity of MIL-100（Fe）-ore towards malachite green（MG） is up to 522.3 mg g-1at 25℃ and initial pH = 3.2, higher than that of MIL-100（Fe） yielded by conventional hydrothermal process. Finally, the production cost and life cycle assessment of MIL-100（Fe）-ore were compared with other traditional production procedures. The results revealed that our work greatly reduced the synthesis cost and enhanced the environmental sustainability.

关键词： Metal-organic framework Iron ore concentrates Adsorption Life cycle assessment

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Experimental Study on Towing Characteristics of Composite Bucket Wellhead Platform

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China Ocean Engineering 2024年第3期38卷 531-542页

作者： ZHANG Pu-yang LIU Ying-fei LE Cong-huan DING Hong-yan BAI Yu State Key laboratory of Hydraulic Engineering Intelligent construction and Operation Tianjin UniversityTianjin 300072China

With the rapid development of large-scale development of marginal oilfields in China,simple wellhead platforms that are simple in structure and easy to install have become an inevitable choice in the process of oilfield ***,traditional simple wellhead platforms are often discarded after a single *** pursuit of a more costeffective approach to developing marginal oilfields,this paper proposes a new offshore oil field development facility—an integrated bucket foundation for wellhead *** verify the safety of its towing behavior and obtain the dynamic response characteristics of the structure,this paper takes a bucket integrated bucket foundation for wellhead platform with a diameter of 40 m as the research *** combining physical model tests and numerical simulations,it analyzes the static stability and dynamic response characteristics of the structure during towing,complete with the effects of the draft,wave height,wave period,and towing point height,which produce the dynamic responses of the structure under different influence factors,such as roll angle,pitch angle,heave acceleration and towing force as well as the sensibility to transport *** results show that the integrated bucket foundation for wellhead platform is capable of self-floating towing,and its movement is affected by the local environment,which will provide a reference for actual projects.

关键词： composite bucket foundation wellhead platform air flotation towing model test

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Causal Analysis Between Rice Growth and Cadmium Accumulation and Transfer under Arbuscular Mycorrhizal Inoculation

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Rice science 2024年第2期31卷 226-236页

作者： ZHAO Ting WANG Li YANG Jixian MA Fang State Key laboratory of Urban Water Resource and environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China

Cadmium(Cd)contamination in rice has been a serious threat to human *** investigate the effects of arbuscular mycorrhizal fungi(AMF)on the Cd translocation in rice,a controlled pot experiment was *** results indicated that AMF significantly increased rice biomass,with an increase of up to 40.0%,particularly in root biomass by up to 68.4%.Notably,the number of prominent rice individuals also increased,and their plasticity was enhanced following AMF *** led to an increase in the net photosynthetic rate and antioxidant enzyme activity of *** the AMF treatment group,the Cd concentration in the rice roots was significantly higher(19.1%‒68.0%)compared with that in the control ***,the Cd concentration in the rice seeds was lower in the AMF treatment group,indicating that AMF facilitated the sequestration of Cd in rice roots and reduced Cd accumulation in the *** coefficients varied across different treatments,suggesting that AMF inoculation reduced the direct impact of soil Cd concentration on the total Cd accumulation in *** translocation of Cd was consistently associated with simultaneous growth dilution and compensatory accumulation as a result of mycorrhizal *** study quantitatively analyzed this process through path analysis and clarified the causal relationship between rice growth and Cd transfer under the influence of AMF.

关键词： cadmium transfer dilution effect heavy metal immobilization mycorrhizal effect path analysis phenotypic plasticity

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Comparison of antimony and arsenic behaviour at the river-lake junction in the middle of the Yangtze River Basin

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Journal of environmental Sciences 2024年第2期136卷 189-200页

作者： Huiji Liu Wei Zeng Ziyang Lai Mengchang He Chunye Lin Wei Ouyang Xitao Liu State Key laboratory of Water environment Simulation School of EnvironmentBeijing Normal UniversityBeijing 100875China Advanced Interdisciplinary Institute of environment and Ecology Beijing Normal UniversityZhuhai 519087China

As typical metalloid toxic elements widely distributed in environmental media,the geochemical behaviour of antimony(Sb)and arsenic(As)affects environmental *** selected the surface waters and sediments at the river-lake junction of Dongting Lake as the research objects,analysed the concentration and chemical partitioning of Sb and As,assessed its contamination and ecological risk levels,and discussed its sources and potential influencing *** concentrations of dissolved Sb and As in surface waters were low(environmental behaviour of metalloids in specific hydrological conditions,such as river-lake junctions.

关键词： Contamination Ecological risks Antimony(Sb) Arsenic(As) River-lake junction Dongting Lake

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Uncovering the dominant contribution of intermediate volatility compounds in secondary organic aerosol formation from biomass-burning emissions

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National Science Review 2024年第3期11卷 150-158页

作者： Kun Li Jun Zhang David M.Bell Tiantian Wang Houssni Lamkaddam Tianqu Cui Lu Qi Mihnea Surdu Dongyu Wang Lin Du Imad El Haddad Jay G.Slowik Andre S.H.Prevot environment Research Institute Shandong University laboratory of Atmospheric Chemistry Paul Scherrer Institute

Organic vapors from biomass burning are a major source of secondary organic aerosols(SOAs). Previous smog chamber studies found that the SOA contributors in biomass-burning emissions are mainly volatile organic compounds(VOCs). While intermediate volatility organic compounds(IVOCs) are efficient SOA precursors and contribute a considerable fraction of biomass-burning emissions, their contribution to SOA formation has not been directly observed. Here, by deploying a newly-developed oxidation flow reactor to study SOA formation from wood burning, we find that IVOCs can contribute ～70% of the formed SOA, i.e.>2 times more than VOCs. This previously missing SOA fraction is interpreted to be due to the high wall losses of semi-volatile oxidation products of IVOCs in smog chambers. The finding in this study reveals that SOA production from biomass burning is much higher than previously thought, and highlights the urgent need for more research on the IVOCs from biomass burning and potentially other emission sources.

关键词： atmospheric chemistry biomass burning secondary organic aerosol intermediate volatility organic compounds

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Challenges and opportunities in Quaternary palynology

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Science China Earth Sciences 2024年第7期67卷 2148-2161页

作者： Qinghai XU Houyuan LU Zhuo ZHENG College of Geographical Sciences Hebei Key Laboratory of Environmental Change and Ecological ConstructionHebei Normal UniversityShijiazhuang 050024China Key laboratory of Cenozoic Geology and environment Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China School of Earth Sciences and Engineering Sun Yat-sen UniversityZhuhai 519082China

Quaternary palynology plays a pivotal role in investigating global climate change and various other research fields,serving as an essential tool for the quantitative analysis of paleoenvironment ***,due to the vast diversity of terrestrial ecosystems and intricate interactions between vegetation,climate,and human activities,further advancements are required in the following aspects within this discipline.(1)The accuracy of classification in pollen morphology and fossil pollen identification needs improvement,particularly at the species *** represents a significant challenge in present Quaternary ***-aided intelligent recognition holds promise as a solution for species identification based on more detail pollen morphology.(2)Most pollen-based vegetation and climate reconstructions overlook the significance of bare *** bare ground can lead to substantial inaccuracies when quantitatively reconstructing past vegetation and climate.(3)While pollen records provide reliable information on paleoclimate changes,current quantitative climate reconstruction models heavily rely on modern pollen datasets derived from present-day vegetation disturbed more or less by human *** introduces bias and uncertainties into paleoclimate reconstruction.(4)Although pollen can serve as an indicator of human activities,accurately quantifying the intensity of human influence remains *** accurate identification of crop pollen,reconstructing reliable land cover/use data,and integrating multidisciplinary data may enhance the identification and quantification of signals related to human activity in pollen records.

关键词： Quaternary palynology Paleoclimate Paleovegetation Human activity

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