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Evolution Mechanism of Carbon Covalent Bond during Coal Activation Using Mixed Atmosphere of H_(2)O and CO_(2)

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Journal of Thermal Science 2024年第5期33卷 1961-1973页

作者： WANG Mingyue ZHANG Siyuan HAN Shaobo ZHANG Chi REN Qiangqiang institute of Engineering thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China State Key Laboratory of Coal Conversion Institute of Engineering ThermophysicsChinese Academy of SciencesBeijing 100190China

Adequate destruction of the aromatic structure in coal is key to further reducing the emission of *** this research,activation reactions of Shenmu coal powder were carried out in a vertical tube *** study investigated the evolution mechanism of carbon covalent bonds during the activation process by altering the ratio of H_(2)O to CO_(2)in the activation *** theoretical validation was conducted through density functional *** two gas molecules follow different pathways to increase the reactivity of ***_(2)mainly participates in the cross-linking reaction by intensifying branching,while H_(2)O and char have lower adsorption energy barriers and are more likely to generate oxygen-containing functional *** molecules partially compete for active sites in a mixed gas atmosphere,but there is a synergism between the two *** synergism can be attributed to two *** inclusion of H_(2)O mitigates the generation of five-membered rings to a limited extent,while concurrently enhances the development of oxygen-containing functional *** oxygen-containing functional groups can effectively diminish the adsorption energy barrier associated with the interaction between gas molecules and char,consequently leading to a reduction in the energy demand for subsequent bond cleavage.

关键词： activation reaction carbon structure char CO_(2)/H_(2)O atmosphere density functional theory

Flame Synthesis of Zr/ZSM-5 Catalysts with Tunable Acidity for the Oxidative Dehydrogenation of Propane to Propene

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Journal of Thermal Science 2024年第1期33卷 268-283页

作者： DANIEL Samuel FONZEU MONGUEN Cedric Karel WU Lingnan TIAN Zhenyu institute of Engineering thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

Tuning the surface acidity of ZSM-5 catalyst is essential to achieve desired propene selectivity and *** several ratios of Zr were utilized to modify ZSM-5 via flame spray pyrolysis technique coupled with a pulse spray evaporation *** interaction between Zr and ZSM-5 in the flame influenced the physicochemical and acidity properties of the Zr/*** increasing Zr ratio in ZSM-5 shows coated layers of irregular nano-sized Zr with an increase in crystallite sizes due to the synergetic effect between Zr and *** surface chemical analysis revealed increased lattice oxygen on the Zr modified ZSM-5(1:4) sample compared to other *** acidity analysis revealed the Lewis and Br?nsted acid distribution in the weak and medium acid sites on the catalyst ***,the increase in Zr loading decreased the concentration of Br?nsted acid sites and tuned the catalyst surface to more Lewis acidity,promoting propene selectivity and hindering the over-oxidation of *** modified ZSM-5 catalysts were examined in a fixed bed reactor within 300℃-700℃ at a gas hourly space velocity(GHSV) of 6000 mL·g(catalysts)^(-1)·h^(-1) for the oxidative dehydrogenation of propane(ODHP) to *** the catalysts,Zr/ZSM-5(1:4) exhibited the best propene yield, with 57.19% propane conversion and 75.54% selectivity to propene and the highest *** work provides a promising strategy for tuning the surface acidity of ZSM-5 with Zr for ODHP applications.

关键词： flame synthesis Zr modified ZSM-5 catalyst ODHP surface acidity lattice oxygen

Exciting broadband thermochromic transmission property opposite to vanadium dioxide in the atmospheric window

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Science China(Technological Sciences) 2024年第7期67卷 2244-2254页

作者： GONG YiQuan GUO YanMing CHEN ShuNi LI Meng PAN QingHui SHUAI Yong Ministry of Industry and Information Technology Key Laboratory of Aerospace thermophysics School of Energy Science and EngineeringHarbin Institute of TechnologyHarbin 150001China

The traditional telecommunications band performs poorly in harsh weather conditions due to atmospheric absorption. In recent years, researchers have begun to study optical communication through atmospheric windows, and optical switches are an essential component of optical communication. A broadband atmospheric window optical switch was proposed based on Vanadium dioxide and magnetic polaritons(MP). It is formed by the stacking of two metal-dielectric-metal structures. The simulation results show that the modulation depth can reach 98.38%, and the extinction ratio is 17.93 dB. By calculating the magnetic field, we confirmed that the reason for the “off” mode is the coupling between the different MP modes, while the “on”mode is the excitation of MP. The optical switch we proposed may be applied to radiation cooling and optical satellite communication.

关键词： optical communication thermochromic property atmospheric window optical switch magnetic polariton

Experimental and Numerical Investigations of Shock-Wave Boundary Layer Interactions in a Highly Loaded Transonic Compressor Cascade

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Journal of Thermal Science 2024年第1期33卷 158-171页

作者： MENG Fanjie LI Kunhang GUO Penghua GAN Jiuliang LI Jingyin School of Energy and Power Engineering Xi'an Jiaotong UniversityXi'an 710049China institute of Engineering thermophysics Chinese Academy of SciencesBeijing 100190China

Experimental and numerical investigations were conducted to investigate the variations of shock-wave boundary layer interaction(SBLI) phenomena in a highly loaded transonic compressor cascade with Mach *** schlieren technique was used to observe the shock structure in the cascade and the pressure tap method to measure the pressure distribution on the blade *** unsteady pressure distribution on blade surface was measured with the fast-response pressure-sensitive paint(PSP) technique to obtain the unsteady pressure distribution on the whole blade surface and to capture the shock oscillation characteristics caused by *** addition,the Reynolds Averaged Navier Stokes simulations were used to compute the three-dimensional steady flow field in the transonic *** was found that the shock wave patterns and behaviors are affected evidently with the increase in incoming Mach number at the design flow angle,especially with the presence of the separation bubble caused by *** time-averaged pressure distribution on the blade surface measured by PSP technique showed a symmetric pressure filed at Mach numbers of 0.85,while the pressure field on the blade surface was an asymmetric one at Mach numbers of 0.90 and *** oscillation of the shock wave was closely with the flow separation bubble on the blade surface and could transverse over nearly one interval of the pressure *** oscillation of the shock wave may smear the pressure jump phenomenon measured by the pressure taps.

关键词： transonic flow transonic compressor cascade shock-wave boundary-layer interaction shock oscillation

Comparative Study on Different Methods for Prediction of Thermal Insulation Performance of Thermal Barrier Coating Used on Turbine Blades

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Journal of Thermal Science 2024年第1期33卷 172-189页

作者： ZHANG Zhixin ZENG Wu ZHANG Xiaodong ZENG Yuntao Advanced Gas Turbine Laboratory Institute of Engineering ThermophysicsChinese Academy of SciencesBeijing 100190China Key Laboratory of Advanced Energy and Power Institute of Engineering ThermophysicsChinese Academy of SciencesBeijing 100190China Innovation Academy for Light-duty Gas Turbine Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

As turbine inlet temperature gets higher and higher,thermal barrier coating(TBC) is more and more widely used in turbine *** turbine blades with TBC,it is of great significance to evaluate the temperature distribution of its substrate metal quickly and accurately,especially during the design *** different degrees of simplification such as whether to consider the change of the geometric size of the fluid domain by TBC and whether to consider the planar heat conduction in TBC,three different methods used in conjugate heat transfer(CHT) simulation to model the TBC of the turbine blades have been developed and widely used by ***,little research has been conducted to investigate the influence of the three methods on the temperature distribution of turbine *** fill this gap,three geometric models were *** are a solid conduction model with a substrate metal layer and a TBC layer,a transonic turbine vane with internal cooling and TBC,and a plate cylindrical film hole cooling model with *** methods were used in these geometric models and their differences were carefully analyzed and *** result shows that for the conduction model used in this paper,with the same TBC surface temperature distribution,the difference between the three methods is very small and can be *** a transonic turbine vane with internal cooling,regarding the local maximum temperature of the substrate-TBC interface,the largest difference between the method in which TBC is considered as a thermal resistance or a virtual layer of cells and the method in which three-dimensional heat conduction equation of TBC is solved occurs at the trailing *** difference near the leading edge is below *** employed to the film cooling model,the difference of the laterally averaged temperature of the substrate-TBC interface can be 8 K which is mainly due to the change of the length to diameter ratio of the film cooling hole by *** the substrate

关键词： turbine blade thermal barrier coating conjugate heat transfer film cooling hole

Efficient and robust CNN-LSTM prediction of flame temperature aided light field online tomography

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Science China(Technological Sciences) 2024年第1期67卷 271-284页

作者： NIU ZhiTian QI Hong SUN AnTai REN YaTao HE MingJian GAO BaoHai School of Energy Science and Engineering Harbin Institute of TechnologyHarbin 150001China Key Laboratory of Aerospace thermophysics Ministry of Industry and Information TechnologyHarbin 150001China

Light field tomography,an optical combustion diagnostic technology,has recently attracted extensive attention due to its easy implementation and ***,the conventional iterative methods are high data throughput,low efficiency and time-consuming,and the existing machine learning models use the radiation spectrum information of the flame to realize the parameter field measurement at the current *** is still an offline measurement and cannot realize the online prediction of the instantaneous structure of the actual turbulent combustion *** this work,a novel online prediction model of flame temperature instantaneous structure based on deep convolutional neural network and long short-term memory(CNN-LSTM)is *** method uses the characteristics of local perception,shared weight,and pooling of CNN to extract the threedimensional(3D)features of flame temperature and outgoing radiation ***,the LSTM is used to comprehensively utilize the ten historical time series information of high dynamic combustion flame to accurately predict 3D temperature at three future moments.A chaotic time-series dataset based on the flame radiation forward model is built to train and validate the performance of the proposed CNN-LSTM *** is proven that the CNN-LSTM prediction model can successfully learn the evolution pattern of combustion flame and make accurate predictions.

关键词： temperature prediction convolutional neural network long short-term memory light field imaging online tomography

A review on current development of thermophotovoltaic technology in heat recovery

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International Journal of Extreme Manufacturing 2024年第2期6卷 297-323页

作者： Shuni Chen Yanming Guo Qinghui Pan Yong Shuai Ministry of Industry and Information Technology Key Laboratory of Aerospace thermophysics School of Energy Science and EngineeringHarbin Institute of TechnologyHarbin 150001People’s Republic of China

The burning of fossil fuels in industry results in significant carbon emissions,and the heat generated is often not fully *** high-temperature industries,thermophotovoltaics(TPVs)is an effective method for waste heat *** review covers two aspects of high-efficiency TPV systems and industrial waste heat *** the system level,representative results of TPV complete the systems,while selective emitters and photovoltaic cells in the last decade are *** key points of components to improve the energy conversion efficiency are further analyzed,and the related micro/nano-fabrication methods are *** the application level,the feasibility of TPV applications in high-temperature industries is shown from the world waste heat utilization *** potential of TPV in waste heat recovery and carbon neutrality is illustrated with the steel industry as an example.

关键词： thermophotovoltaic waste heat recovery micro/nano-fabrication carbon neutrality

Effect of structural characteristics on the transport characteristics of solid particles in the thermal storage and release system of circulating fluidized bed

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Particuology 2024年第6期89卷 22-31页

作者： Zengcai Ji Guoliang Song Zihua Tang Liwei Sun institute of Engineering thermophysics Chinese Academy of SciencesBeijing100190China University of Chinese Academy of Sciences Beijing100049China Dalian National Laboratory for Clean Energy Dalian116023China

Coal-fired power generation stands as the most economically viable modulating power source in present-day *** holds the potential to offer prospective solutions to the challenges posed by the rapid expansion of intermittent,unpredictable,and unstable renewable energy *** particle thermal storage technology emerges as an effective means to enhance the flexibility of coal-fired circulating fluidized bed power *** attain an optimized structure for the solid particle thermal storage and release system in circulating fluidized bed units,experimental research was conducted on a 0.1 MWth circulating fluidized bed test *** study delved into the impact of ash storage bin geometries and the shapes of their feed-discharge valves on the control properties of solid particle *** experimental outcomes reveal that employing inverted m-shaped valve and dual U-shaped valves for feed control,alongside U-shaped valves and N-shaped valves for discharge control,both enable efficient and rapid storage and release of solid particles within the circulating fluidized *** similar air distribution conditions,the inverted m-shaped valve exhibits lower conveying energy consumption than the dual U-shaped valves,while the N-shaped valve excels in control characteristics over the U-shaped ***,the inverted m-shaped valve and the N-shaped valve demonstrate optimal overflow port heights,and the ash storage bin exhibits an optimum height-to-diameter ratio.

关键词： Solid particle Thermal storage System structure Transport regulation

A Comprehensive Review of Thermal Performance Improvement of High-Temperature Heat Pipes

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Journal of Thermal Science 2024年第2期33卷 625-647页

作者： CHEN Qihan ZHOU Jingzhi ZHOU Guohui CHENG Keyong HUAI Xiulan WEI Gaosheng School of Energy Power and Mechanical EngineeringNorth China Electric Power UniversityBeijing100096China Nanjing institute of Future Energy System Nanjing211135China institute of Engineering thermophysics Chinese Academy of SciencesBeijing100190China

Energy efficiency issues are being focused on the growing concern of global warming and environmental *** high-temperature heat pipe(HTHP) is an effective and environmental-friendly heat transfer device employed in many industries,including solar power generation,high-temperature flue gas waste heat recovery,industrial furnaces,nuclear industries,and *** a critical factor in HTHPs,thermal performance is mainly introduced in the entire *** date,most reviews have been published concerning one or several application ***,to the best of authors' knowledge,it is hard to find a review discussing how to improve the thermal performance of HTHPs ***,the impact on the performance of three main components of HTHPs over the past 30 years is introduced:the working fluid,the HTHP structure,and the wick ***,it is a considerable review of the optimal operating conditions for each direction,and we expect this paper contribute to improving the thermal performance of ***,current numerical simulations and theoretical research on the heat transfer limit of HTHPs are *** significant hypotheses used in numerical simulations and the present theoretical studies are compiled ***,some potential future directions and tentative suggestions for HTHP research are put forward.

关键词： high-temperature heat pipe review alkali metal heat pipe thermal performance