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Geoscience Frontiers 2024年第3期15卷 166-179页

作者： Shuoqin Hou Di Li Dengfa He Yu Lu Yu Zhen Hao Yang Dan Fan key Laboratory of Marine Reservoir Evolution and Hydrocarbon accumulation mechanism the Ministry of Educationand School of Energy ResourcesChina University of Geosciences(Beijing)Beijing 100083China

The Carboniferous to Permian tectono-sedimentary evolution of the southern Junggar area brings new insights into understanding the subduction-collision processes in the northern Tianshan *** geophysics,geochemistry,and geochronology approaches,this study investigates the Carboniferous-Permian strata in the southern Junggar *** results have revealed three distinct tectono-stratigraphic evolutionary stages,each marked by a distinctive volcano-sedimentary *** Early Carboniferous strata suggest intense volcanic activities in the southern Junggar *** the Late Carboniferous,the southern Junggar Basin was controlled by normal faulting in an extensional setting,receiving sedimentary inputs from the Junggar *** Lower Permian,unconformably overlying the Upper Carboniferous,was shaped by an extensional regime and is comprised by volcano-clastic sequences that received detritus from the Yili-Central Tianshan *** findings indicate that a Late Carboniferous forearc basin developed in the southern Junggar area,and it evolved into a post-collisional rift in the Early *** period marked a dynamic shift from bidirectional subduction(rollback)to the detachment of the North Tianshan oceanic *** propose that the collision between the YiliCentral Tianshan block and the Junggar terrane,along with the closure of the North Tianshan Ocean,likely occurred in the Late Carboniferous(ca.306-303 Ma).

关键词： Tectono-sedimentary evolution Tectonic transition Carboniferous-Permian Junggar Basin North Tianshan Ocean

Electrocatalytic Multicomponent Cascade Cross-Coupling for the Synthesis of Chalcogenosulfonates

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Chinese Journal of Chemistry 2024年第17期42卷 2049-2055页

作者： Zhiheng Zhao Hongyan Yan Yaqin Zhou Wei Xue Lijun Gu Shengyong Zhang State key laboratoryof Green Pesticide Key Laboratoryof Green Pesticide and Agricultural BioengineeringMinistry of EducationCenter for R&D of Fine Chemicals of Guizhou UniversityGuiyangGuizhou 550025China Schoolof Pharmacy Air Force Medical UniversityShaanxiXi'anShaanxi 710032China

An electrocatalytic multicomponent cascade cross-coupling for the synthesis of chalcogenosulfonates has been *** approach does not require the use of transition metals,acids,and external *** gentle conditions and tole... 详细信息

关键词： Electrochemical catalysis Synthetic methods Radical Multi-component reaction Chalcogenosulfonates Tellurium

Multi-locomotion transition of tensegrity mobile robot under different terrains

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Science China(Technological Sciences) 2024年第2期67卷 536-557页

作者： YANG Qi LIU XinYu WANG PanFeng SONG YiMin SUN Tao key Laboratory of mechanism Theory and Equipment Design(Tianjin University) Ministry of EducationTianjin UniversityTianjin 300350China

Knowing how to make a multi-locomotion robot achieve locomotion transition under different terrains is a challenging problem,especially for tensegrity robots with multi-locomotion *** this study,a motion planning method for the transition of a multi-locomotion tensegrity robot(hereafter TJUBot)under different terrains is *** robot can achieve four locomotion modes:earthworm-like,inchworm-like,tumbling,and sliding locomotion with only two *** models of the four locomotion modes under five typical terrains,including flat ground,confined space,obstacle,gap,and descending slope,are established using the energy ***,the kinematic characteristics(driving law and initial position)of the robot under these terrains are *** this basis,motion planning for the locomotion transition of TJUBot is conducted,which includes a perception strategy based on three laser sensors and a transition strategy under different *** driving laws of the two motors that can ensure the effective locomotion transition of TJUBot under different terrains are naturally ***,experiments are *** demonstrate that the robot can achieve effective locomotion transition when the motion planning method is used.

关键词： multi-locomotion robot tensegrity kinematic modeling locomotion transition

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Synthetic Studies toward Pseudolaric Acids:Radical Cyclization to Form Bridged Scaffold

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Chinese Journal of Chemistry 2024年第15期42卷 1699-1705页

作者： Yujie Niu Minggui Lin Hao Cui Yanji Huang Yang Shen Yandong Zhang State key laboratoryof Physical Chemistry of Solid Surfaces Key Laboratory of Chemical Biology of Fujian ProvinceicHEMCollege of Chemistryand Chemical EngineeringXiamen UniversityXiamenFujian 361005China

Pseudolaric acids are a family of diterpenoid natural products that exhibit a broad spectrum of biological *** main structural feature of their framework is a trans-fused perhydroazulene bearing a bridged lactone positioned at the junction of the ***,we have developed a radical cyclization strategy that allows flexible tuning of the cyclization process through diverse silicon substitutions on the *** strategy can assist in constructing a series of skeletons with structural resemblance to pseudolaric acids and expedites the construction of the bridged ***,it facilitates the synthesis of the entire skeletal structure of the pseudolaric acidfamily of natural products,excludingthe B-ringfunctionalization.

关键词： Terpenoids Total synthesis Radical cyclization Bridged cycles Regioselectivity

Sedimentary paleoenvironment and its control on organic matter enrichment in the Mesoproterozoic hydrocarbon source rocks in the Ordos Basin, southern margin of the North China Craton

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Petroleum Science 2024年第4期21卷 2257-2272页

作者： Zhi-Chen Wu Ju-Ye Shi Tai-Liang Fan Ming Jiang School of Energy Resources China University of Geosciences (Beijing) key Laboratory of Marine Reservoir Evolution and Hydrocarbon Enrichment mechanism Ministry of Education China University of Geosciences (Beijing)

The black shale of the Mesoproterozoic Cuizhuang Formation in the Changcheng System in Yongji city,North China Craton, is a potential source rock. Understanding the organic matter enrichment mechanism is crucial for evaluating source rock resources and understanding oil and gas accumulation *** this study, we evaluated the sedimentary paleoenvironment and organic matter enrichment mechanisms of shale using thin section observations, mineral composition analysis, organic geochemistry, and elemental geochemistry. We found significant differences in the sedimentary paleoenvironment and organic matter enrichment mechanisms between the lower Cuizhuang Formation and the Beidajian Formation shale. The Cuizhuang Formation was deposited in a late-stage, restricted basin environment during the rift phase, and elemental and geochemical indicators showed that the Cuizhuang Formation was in a suboxic-anoxic water environment, that was influenced by a warm and humid paleoclimate and submarine hydrothermal activities, which promoted the accumulation of organic matter. However, the enrichment of organic matter in the Cuizhuang Formation was mainly controlled by redox *** formation of suboxic-anoxic water environments may be closely related to the warm and humid paleoclimate and submarine hydrothermal activities. Warm conditions promote continental weathering and increase marine productivity, thereby consuming oxygen in the bottom water. Moreover, acidic hydrothermal activity also helps to establish an anoxic environment. Our results reveal the effects controlling various coupled mechanisms dominated by redox conditions, which may explain the development of source rocks in the Cuizhuang Formation.

关键词： Cuizhuang formation Paleoproterozoic source rocks Marine productivity Paleoenvironments Submarine hydrothermal activity Organic matter enrichment

Injectable chitosan hydrogels loaded with antioxidant agent as first-aid dressings for second-degree burn wounds

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Science China(Technological Sciences) 2024年第3期67卷 891-901页

作者： REN Hui ZHANG Zhen LU KaiLun SHEN YuanYuan HE ChaoLiang CHEN XueSi CAS key laboratoryof Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China

Burn wounds are destructive skin traumas typically of irregular shape and large area. Prone to infection, they require frequent dressing replacement, and painless removal of dressings from burn wounds remains a major challenge. This study focuses on the dynamic characteristics and treatment difficulty of burn wounds. Hydrogel dressings based on glycol chitosan and propionaldehyde-or benzaldehyde-terminated 4-arm poly(ethylene glycol) were designed on the basis of Schiff base cross-linking networks. The hydrogels exhibited shape-adaptability, self-healing and fast-degradation properties, which makes these hydrogels suitable for burn wounds. Salvianolic acid B(SaB)-loaded hydrogel exhibited good antioxidant properties in vitro. In a rat model of deep second-degree burn wounds, the SaB-loaded hydrogel could quickly reduce wound temperature, regulate wound oxidant microenvironment, promote angiogenesis, and accelerate wound healing. Thus, the drug-loaded hydrogel shows significant potential as a first-aid dressing for treatment of burn wounds.

关键词： hydrogel dressing fast-degradation shape-adaptability stress relaxation burn wound treatment

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Fractal Characteristics and Main Controlling Factors of High-Quality Tight Sandstone Reservoirs in the Southeastern Ordos Basin

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Journal of Earth Science 2024年第2期35卷 631-641页

作者： Ruilin Hao Wenhui Huang Jiu Bo Li Yuan key Laboratory for Marine Reservoir Evolution and Hydrocarbon Abundance mechanism School of Energy ResourcesChina University of GeosciencesMinistry of EducationBeijing100083China

Due to the complex conditions and strong heterogeneity of tight sandstone reservoirs,the reservoirs should be classified and the controlling factors of physical properties should be *** thin section observations,cathodoluminescence,scanning electron microscopy(SEM),X-ray diffraction(XRD),and high-pressure mercury injection(HPMI)were used to classify and optimize the *** Brooks-Corey model and stepwise regression were used to study the fractal dimension and main controlling factors of the physical properties of the high-quality *** results show that the reservoirs in the study area can be divided into four types,and the high-quality reservoir has the best physical properties and pore-throat *** the high-quality reservoir,the homogeneity of transitional pores was the best,followed by that of micropores,and the worst was *** porosity was controlled by depth and *** model with standardized coefficients is y=12.454−0.778×(Depth)+0.395×(Kaolinite).The permeability was controlled by depth,illite/montmorillonite,and siliceous cement,and the model with standardized coefficients is y=1.689−0.683×(Depth)−0.395×(Illite/Montmorillonite)−0.337×(Siliceous Cement).The pore-throat evolutionary model shows that the early-middle diagenetic period was when the reservoir physical properties were at their best,and the kaolinite intercrystalline pores and residual intergranular pores were the most important.

关键词： fractal dimension main controlling factors stepwise regression high-quality tight sandstone reservoir Ordos Basin petroleum geolgoy

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Modeling and analysis for material removal and surface roughness in fluid jet polishing of optical glass

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Friction 2024年第7期12卷 1548-1563页

作者： Zhongchen CAO Ming WANG Haitao LIU Tian HUANG key Laboratory of mechanism Theory and Equipment Design of Ministry of Education Tianjin UniversityTianjin 300072China School of Engineering The University of WarwickCoventry CV47ALUK

luid jet polishing(FJP)is a non-contact polishing technology that can fabricate free-form optical surfaces with sub-micron-level form accuracy and nano-level surface roughness,especially for hard and brittle *** surface generation model of FJP can be used to guide the determination and optimization of process parameters and is of great significance for understanding the evolution mechanism of surface ***,predictive models for the microscopic topography of polished surfaces are still *** study established a macroscopic surface profile model for predicting 3D material removal characteristics and surface texture by combining the 3D computer fluid dynamics(CFD)simulation model and single-particle erosion mechanism.A fractal theory-based erosion model has been built to calculate the material removal caused by the erosion of a single abrasive particle on the rough surface;thus,it predicts the micro-topography and surface roughness of the polished samples.A series of polishing experiments were conducted to analyze the feasibility and accuracy of the model quantitatively and study the influence mechanism of process parameters on the material removal characteristics and surface *** indicated that the models could well predict material removal and surface *** prediction accuracy of the surface roughness Ra and maximum removal depth is better than 91.6%and 90%,*** is also found that the material removal rate of FJP could reach 0.517 mm3/min,and the surface roughness convergence rate could reach 62.9%.

关键词： fluid jet polishing(FJP) computational fluid dynamics(CFD) material removal mechanism surface roughness theoretical model

Quantitative liquid storage by billiards-like droplet collision on surfaces with patterned wettability

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Droplet 2024年第3期3卷 80-90页

作者： Minghao Li Haoxu Yu Zhirui Liu Ziyue Gao Faze Chen School of Mechanical Engineering Tianjin UniversityTianjinChina key Laboratory of mechanism Theory and Equipment Design of Ministry of Education Tianjin UniversityTianjinChina

There has been significant interest in researching droplet transport behavior on com-posite wetting ***,current research is primarily focused on modifying individual droplets and lacks an in-depth investigation into high-precision droplet *** study introduces a“billiard ball”droplet transport and storage platform(TSP)with differentiated *** this platform,the volume of droplets stored in the area reaches a consistent threshold through droplet“scrambling,”inspired by the water-gathering behavior of *** TSP involves connecting two regions of different sizes using a three-dimensional stepped wedge angle ***-ever,this connection is not seamless,leaving a 2-mm gap between the *** gap is intentionally designed to enable continuous droplet transfer while preventing any static *** systematic experimental and simulation analysis,we investigated the influence of superhydrophilic pattern structures and parameters on quantitative droplet *** established a functional relationship between the pattern area and the stored volume,and analyzed the intrinsic mechanism of droplet collision *** enabled us to achieve on-demand quantitative droplet stor-age and autonomize the storage ***“billiard ball”droplet transport–storage platform proposed in this study holds promising applications in the fields of biomedical and organic chemistry.

关键词： structure. process. collision

One-Pot Stereoselective Synthesis of Different Fused Multicyclic Iminosugars Based on the Iminium-lon Intermediate

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Chinese Journal of Chemistry 2024年第2期42卷 142-150页

作者： Song Xie Jilai Wu Likai Zhou Chao Wei Xiaoliu Li Hua Chen key laboratoryof Chemical Biology of Hebei Province College of Chemistry and Material ScienceHebei UniversityBaodingHebei 071002China College of Chemistry and Chemical Engineering Xingtai UniversityXingtaiHebei 054001China

Different novel fused multicyclic iminosugars were synthesized from D-ribose tosylate,aniline and vinyl ethyl ether by one-pot three-component stereoselective[4+2]reaction at different *** iminium-ion is the key intermediate for the *** a result,several complex fused iminosugars 3a were obtained by aza-Diels-Alder mechanism at 60℃,while a series of aza-C-glycosides 5a were prepared by Mannich reaction at room temperature accompanied by another tetrahydroquinoline-fused iminosugars 4a(tricyclic derivatives)through aza-Diels-Alder *** strategy will help to construct structurally diverse and bioactive iminosugar analogues.

关键词： Fused multicyclic iminosugar Aza-Diels-Alder cycloaddition Mannich reaction Tetrahydroquinoline Multicomponent reactions Enantioselectivity Cyclization