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Experimental study on reactions between alkaline basaltic melt and orthopyroxenes: constraints on the evolution of lithospheric mantle in the North China Craton

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Acta Geochimica 2024年第2期43卷 354-365页

作者： Hanqi He Mingliang Wang Hongfeng Tang key laboratory for High Temperature and High Pressure study of the earth’s interior Institute of GeochemistryChinese Academy of SciencesGuiyang 550081China University of Chinese Academy of sciences Beijing 100049China school of Resource and Civil Engineering Suzhou UniversitySuzhou 234000AnhuiChina

The experimental results of the reactions between an alkaline basaltic melt and mantle orthopyroxenes under high-temperature and high-pressure conditions of 1300–1400℃ and 2.0–3.0 GPa using a six-anvil apparatus are reported in this paper.The reactions are proposed to simulate the interactions between melts from the asthenospheric mantle and the lithospheric mantle.The starting melt in the experiments was made from the alkaline basalt occurring in Fuxin,Liaoning Province,and the orthopyroxenes were separated from the mantle xenoliths in Damaping,Hebei Province.The results show that clinopyroxenes were formed in all the reactions between the alkaline basaltic melt and orthopyroxenes under the studied P–T conditions.The formation of clinopyroxene in the reaction zone is mainly controlled by dissolution–crystallization,and the chemical compositions of the reacted melt are primarily infl uenced by the diff usion eff ect.Temperature is the most important parameter controlling the reactions between the melt and orthopyroxenes,which has a direct impact on the melting of orthopyroxenes and the diff usion of chemical components in the melt.Temperature also directly controls the chemical compositions of the newly formed clinopyroxenes in the reaction zone and the reacted melt.The formation of clinopyroxenes from the reactions between the alkaline basaltic melt and orthopyroxenes can result in an increase of CaO and Al_(2)O_(3) contents in the rocks containing this mineral.Therefore,the reactions between the alkaline basaltic melt from the asthenospheric mantle and orthopyroxenes from the lithospheric mantle can lead to the evolution of lithospheric mantle in the North China Craton from refractory to fertile with relatively high CaO and Al 2 O 3 contents.In addition,the reacted melts in some runs were transformed from the starting alkaline basaltic into tholeiitic after reactions,indicating that tholeiitic magma could be generated from alkaline basaltic one via reactions between the latter and orthopyroxene.

关键词： Alkaline basaltic melt Orthopyroxene Melt–mineral reaction High-temperature and high-pressure experiment Genesis of basalt Evolution of lithospheric mantle in the North China Craton

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Response of ocean acidification to atmospheric carbon dioxide removal

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Journal of Environmental sciences 2024年第6期140卷 79-90页

作者： Jiu Jiang Long Cao Xiaoyu Jin Zechen Yu Han Zhang Jianjie Fu Guibin Jiang school of Environment Hangzhou Institute for Advanced StudyUniversity of Chinese Academy of SciencesHangzhou 310024China state key laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China key laboratory of Geoscience Big Data and deep Resources of Zhejiang Province School of Earth SciencesZhejiang UniversityHangzhou 310058China Zhejiang Climate Center Hangzhou 310052China

Artificial CO_(2)removal from the atmosphere(also referred to as negative CO_(2)emissions)has been proposed as a potential means to counteract anthropogenic climate change.Here we use an earth system model to examine the response of ocean acidification to idealized atmospheric CO_(2)removal scenarios.In our simulations,atmospheric CO_(2)is assumed to increase at a rate of 1%per year to four times its pre-industrial value and then decreases to the pre-industrial level at a rate of 0.5%,1%,2%per year,respectively.Our results show that the annual mean state of surface ocean carbonate chemistry fields including hydrogen ion concentration([H^(+)]),pH and aragonite saturation state respond quickly to removal of atmospheric CO_(2).However,the change of seasonal cycle in carbonate chemistry lags behind the decline in atmospheric CO_(2).When CO_(2)returns to the pre-industrial level,over some parts of the ocean,relative to the pre-industrial state,the seasonal amplitude of carbonate chemistry fields is substantially larger.simulation results also show that changes in deep ocean carbonate chemistry substantially lag behind atmospheric CO_(2)change.When CO_(2)returns to its pre-industrial value,the whole-ocean acidity measured by[H^(+)]is 15%-18%larger than the pre-industrial level,depending on the rate of CO_(2)decrease.Our study demonstrates that even if atmospheric CO_(2)can be lowered in the future as a result of net negative CO_(2)emissions,the recovery of some aspects of ocean acidification would take decades to centuries,which would have important implications for the resilience of marine ecosystems.

关键词： Carbon dioxide removal Net negative CO_(2)emission Ocean acidification Climate change earth system modeling

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Implementation of a particle-in-cell method for the energy solver in 3D spherical geodynamic modeling

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earth and Planetary Physics 2024年第3期8卷 549-563页

作者： Hao Dong ZeBin Cao LiJun Liu YanChong Li sanZhong Li LiMing Dai XinYu Li Frontiers science Center for deep Ocean Multispheres and earth system Key Laboratory of Submarine Geosciences and Prospecting TechniquesMinistry of Education and College of Marine GeosciencesOcean University of ChinaQingdao 266100China state key laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China laboratory for Marine Geology Laoshan LaboratoryQingdao 266237China Department of earth science&Environmental Change University of Illinois at Urbana-ChampaignUrbanaIL 61801USA laboratory of seismology and Physics of earth’s interior School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China

The thermal evolution of the earth’s interior and its dynamic effects are the focus of earth sciences.However,the commonly adopted grid-based temperature solver is usually prone to numerical oscillations,especially in the presence of sharp thermal gradients,such as when modeling subducting slabs and rising plumes.This phenomenon prohibits the correct representation of thermal evolution and may cause incorrect implications of geodynamic processes.After examining several approaches for removing these numerical oscillations,we show that the Lagrangian method provides an ideal way to solve this problem.In this study,we propose a particle-in-cell method as a strategy for improving the solution to the energy equation and demonstrate its effectiveness in both one-dimensional and three-dimensional thermal problems,as well as in a global spherical simulation with data assimilation.We have implemented this method in the open-source finite-element code Citcoms,which features a spherical coordinate system,distributed memory parallel computing,and data assimilation algorithms.

关键词： numerical oscillation overshooting and undershooting particle-in-cell method three-dimensional spherical geodynamic modeling energy solver finite element method

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High-Pressure Behavior of Ferromagnesite(Mg_(0.81)Fe_(0.19))CO_(3)by synchrotron X-Ray Diffraction and Raman spectroscopy up to 53 GPa

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Journal of earth science 2024年第2期35卷 525-535页

作者： Lin Liang Guibin Zhang shengxuan Huang Jingjing Niu Dongzhou Zhang Jingui Xu Wen Liang shan Qin key laboratory of Orogenic Belts and Crustal Evolution MOEand School of Earth and Space SciencesPeking UniversityBeijing100871China CAs Center of Excellence in Tibetan Plateau earth sciences and key laboratory of Continental Collision and Plateau Uplift Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing100101China Hawai’i Institute of Geophysics and Planetology School of Ocean and Earth Science and TechnologyUniversity of Hawai’i at ManoaHawai’i96822USA key laboratory of High Temperature and High Pressure study of the earth’s interior Institute of GeochemistryChinese Academy of SciencesGuiyang550081China

Ferromagnesite(Mg,Fe)CO_(3)with 20 mol%iron is a potential host mineral for carbon transport and storage in the earth mantle.The high-pressure behavior of synthetic ferromagnesite(Mg_(0.81)Fe_(0.19))CO_(3)up to 53 GPa was investigated by synchrotron X-ray diffraction(XRD)and Raman spectroscopy.The iron bearing carbonate underwent spin transition at around 44–46 GPa accompanied by a volume collapse of 1.8%,which also demonstrated a variation in the dνi/dP slope of the Raman modes.The pressure-volume data was fitted by a third-order Birch-Murnaghan equation of state(BM-Eos)for the high spin phase.The best-fit K_(0)=108(1)GPa and K_(0)'=4.2(1).Combining the dνi/dP and the K_(0),the mode Grüneisen parameters of each vibrational mode(T,L,ν4 andν1)were calculated.The effects of iron concentration on the Mg_(1−x)Fe_(x)CO_(3)system related to high-pressure compressibility and vibrational properties are discussed.These results expand the knowledge of the physical properties of carbonates and provide insights to the potential deep carbon host.

关键词： ferromagnesite synchrotron XRD Raman spectroscopy high pressure geochemistry mineral

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Comparative Experimental study on Heat Transfer Characteristics of Building Exterior surface at High and Low Altitudes

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Journal of Thermal science 2024年第3期33卷 1119-1131页

作者： JIA Yonghong GUO shurui LI Jin GUO Lei CHENG Zhu ZHANG Yin YANG Hanyu LONG Enshen Institute for Disaster Management and Reconstruction Sichuan UniversityChengdu610065China MOE key laboratory of deep earth science and Engineering College of Architecture and EnvironmentSichuan UniversityChengdu610065China

The external surface heat transfer coefficient of building envelope is one of the important parameters necessary for building energy saving design,but the basic data in high-altitude area are scarce.Therefore,the authors propose a modified measurement method based on the heat balance of a model building,and use the same model building to measure its external surface heat transfer coefficient under outdoor conditions in Chengdu city,China at an altitude of 520 m and Daocheng city at an altitude of 3750 m respectively.The results show that the total heat transfer coefficient(h_(t))of building surface in high-altitude area is reduced by 34.48%.The influence of outdoor wind speed on the convective heat transfer coefficient(h_(c))in high-altitude area is not as significant as that in low-altitude area.The fitting relation between convection heat transfer coefficient and outdoor wind speed is also obtained.Under the same heating power,the average temperature rise of indoor and outdoor air at highaltitude is 41.9%higher than that at low altitude,and the average temperature rise of inner wall is 25.8%higher than that at low altitude.It shows that high-altitude area can create a more comfortable indoor thermal environment than low-altitude area under the same energy consumption condition.It is not appropriate to use the heat transfer characteristics of the exterior surface of buildings in low-altitude area for building energy saving design and related heating equipment selection and system terminal matching design in high-altitude area.

关键词： altitude heat transfer characteristics convective heat transfer coefficient(h_(c)) radiative heat transfer coefficient(h_(r)) external building envelope

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A novel box-counting method for quantitative fractal analysis of threedimensional pore characteristics in sandstone

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International Journal of Mining science and Technology 2024年第4期34卷 479-489页

作者： Huiqing Liu Heping Xie Fei Wu Cunbao Li Renbo Gao state key laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing 400030China school of Resources and safety Engineering Chongqing UniversityChongqing 400030China Guangdong Provincial key laboratory of deep earth sciences and Geothermal Energy Exploitation and Utilization Shenzhen UniversityShenzhen 518060China shenzhen key laboratory of deep Underground Engineering sciences and Green Energy College of Civil and Transportation EngineeringShenzhen UniversityShenzhen 518060China

Fractal theory offers a powerful tool for the precise description and quantification of the complex pore structures in reservoir rocks,crucial for understanding the storage and migration characteristics of media within these rocks.Faced with the challenge of calculating the three-dimensional fractal dimensions of rock porosity,this study proposes an innovative computational process that directly calculates the three-dimensional fractal dimensions from a geometric perspective.By employing a composite denoising approach that integrates Fourier transform(FT)and wavelet transform(WT),coupled with multimodal pore extraction techniques such as threshold segmentation,top-hat transformation,and membrane enhancement,we successfully crafted accurate digital rock models.The improved box-counting method was then applied to analyze the voxel data of these digital rocks,accurately calculating the fractal dimensions of the rock pore distribution.Further numerical simulations of permeability experiments were conducted to explore the physical correlations between the rock pore fractal dimensions,porosity,and absolute permeability.The results reveal that rocks with higher fractal dimensions exhibit more complex pore connectivity pathways and a wider,more uneven pore distribution,suggesting that the ideal rock samples should possess lower fractal dimensions and higher effective porosity rates to achieve optimal fluid transmission properties.The methodology and conclusions of this study provide new tools and insights for the quantitative analysis of complex pores in rocks and contribute to the exploration of the fractal transport properties of media within rocks.

关键词： 3D fractal analysis Fractal dimension Rock pore structure Box-counting method Permeability simulation Computational geosciences

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Fe-Mn interdiffusion in aluminosilicate garnets

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Geoscience Frontiers 2024年第1期15卷 118-125页

作者： Yanjun Yin Baohua Zhang Xinzhuan Guo key laboratory of High-temperature and High-pressure study of the earth’s interior Institute of GeochemistryChinese Academy of SciencesGuiyang 550081GuizhouChina University of Chinese Academy of sciences Beijing 100049China key laboratory of Big Data in Geosciences and deep earth Resources of Zhejiang Province School of Earth SciencesZhejiang UniversityHangzhou 310058China

Precise determination of cation diffusivity in garnet can provide critical information for quantitatively understanding the timescales and thermodynamics of various geological processes,but very few studies have been performed for Fe-Mn interdiffusion.In this study,Fe-Mn interdiffusion rates in natural single crystals of Mn-bearing garnet with 750 ppm H2O are determined at 6 GPa and 1273-1573 K in a Kawai-type multi-anvil apparatus.Diffusion profiles were acquired by electron microprobe and fitted using Boltzmann-Matano equation.The experimental results show that the Fe-Mn interdiffusion coefficient(DFe-Mn)slightly decreases with increasing XFe.The experimentally determined DFe-Mn in Mn-bearing garnet can be fitted by the Arrhenius equation:DFe-Mn(m2/s)=D0XFenexp(-E*/RT),where E*=(1-XFe)E*Mn+XFeE*Fe,D0=8.06-6.04+9.87×10-9 m2/s,E*Mn=248±27 KJ/mol,E*Fe=226±59 KJ/mol,n=-1.36±0.51.The comparing the present results with previous experimental data suggest that water can greatly enhance the DFe-Mn in garnet.Our results indicate that the time required for homogenization of the compositional zoning of a garnet is much shorter than previously thought.

关键词： Fe-Mn interdiffusion Diffusion coefficient Garnet High pressure experiment Water

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Geochronological and geochemical constraints on the petrogenesis and geodynamic process of Hemler,Vlinder,and Il'ichev seamount lavas in NW Pacific

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science China earth sciences 2024年第6期67卷 1856-1871页

作者： Xun WEI Yan ZHANG Xuefa sHI Hui ZHANG key laboratory of Marine Geology and Metallogeny First Institute of OceanographyMinistry of Natural ResourcesQingdao 266061China laboratory for Marine Geology Qingdao Marine Science and Technology CenterQingdao 266237China shandong key laboratory of deep sea Mineral Resources Development(Preparatory) Qingdao 266061China

Oceanic intraplate volcanoes with linear age progressions are usually accepted to be derived from melting of an upwelling mantle plume.several seamount groups in NW Pacific,however,show complex age-distance relationships that are difficult to explain using the classic“mantle plume hypothesis”,and thus their origins are controversial.In this study,we present ^(40)Ar-^(39)Ar age,geochemical,and sr-Nd-Pb-Hf isotopic data of lavas from Hemler,Vlinder,and Il’ichev seamounts in NW Pacific,to elucidate their petrogenesis and geodynamic process.The lavas from Hemler,Vlinder,and Il’ichev seamounts are classified as alkali basalt,basanite/nephelinite,and trachyte.Lavas with Mg O>8 wt.%exhibit high contents of CaO,FeO^(T),and TiO_(2),similar to the composition of melts formed from reaction between carbonated eclogite-derived melts and fertile peridotite.These lavas have elevated Zr/Hf ratios(40.6-45.2)and negative Zr and Hf anomalies,indicating the presence of a carbonate component in the mantle source.They are enriched in incompatible trace elements and have enriched mantle 1(EM1)-like srNd-Pb-Hf isotopic compositions.The isotopic compositions of Vlinder,Il’ichev basanite,and Hemler lavas in this study are similar to the Rarotonga hotspot.Although occurring at the same seamount,the Il’ichev alkali basalts display more depleted srNd-Hf isotopic compositions compared to Il’ichev basanite.According to plate tectonic reconstruction results,the ages of Hemler(100.1 Ma),Vlinder pre-(100.2 Ma)and post-shield(87.5 Ma),and Il’ichev(56.4 Ma)lavas clearly deviate from the Macdonald,Arago,Rarotonga,and samoa hotspot tracks,indicating that they cannot directly originate from mantle plumes.We propose that in the mid-Cretaceous,when the Pacific plate passed over Rarotonga hotspot,melting of Rarotonga plume formed the Vlinder(main-shield stage),Pako,and Ioah seamounts.The Rarotonga(and possibly samoa)plume materials would have been dispersed into the surrounding asthenosphere by mantle convection.These diffuse plume materials would underg

关键词： Mantle plume Magellan seamount trail Carbonated mantle component Hotspot Lithosphere extension

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RB-DEM Modeling and simulation of Non-Persisting Rough Open Joints Based on the IFs-Enhanced Method

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Computer Modeling in Engineering & sciences 2024年第4期139卷 337-359页

作者： Hangtian song Xudong Chen Chun Zhu Qian Yin Wei Wang Qingxiang Meng key laboratory of Ministry of Education for Geomechanics and Embankment Engineering Hohai UniversityNanjing210098China Research Institute of Geotechnical Engineering Hohai UniversityNanjing210098China school of earth sciences and Engineering Hohai UniversityNanjing210098China state key laboratory for Geomechanics and deep Underground Engineering China University of Mining and TechnologyXuzhou221116China

When the geological environment of rock masses is disturbed,numerous non-persisting open joints can appear within it.It is crucial to investigate the effect of open joints on the mechanical properties of rock mass.However,it has been challenging to generate realistic open joints in traditional experimental tests and numerical simulations.This paper presents a novel solution to solve the problem.By utilizing the stochastic distribution of joints and an enhanced-fractal interpolation system(IFs)method,rough curves with any orientation can be generated.The Douglas-Peucker algorithm is then applied to simplify these curves by removing unnecessary points while preserving their fundamental shape.subsequently,open joints are created by connecting points that move to both sides of rough curves based on the aperture distribution.Mesh modeling is performed to construct the final mesh model.Finally,the RB-DEM method is applied to transform the mesh model into a discrete element model containing geometric information about these open joints.Furthermore,this study explores the impacts of rough open joint orientation,aperture,and number on rock fracture mechanics.This method provides a realistic and effective approach for modeling and simulating these non-persisting open joints.

关键词： Non-persisting rough open joints stochastic distribution of joints enhanced-IFs method RB-DEM

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Characteristics,origins,and significance of pyrites in deep-water shales

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science China earth sciences 2024年第2期67卷 313-342页

作者： Chao LIANG shichao JI Yingchang CAO keyu LIU Jing WU Fang HAO National key laboratory of deep Oil and Gas China University of Petroleum(East China)Qingdao266580China school of Geosciences China University of PetroleumQingdao266000China laboratory for Marine Mineral Resource Qingdao National Laboratory for Marine Science and TechnologyQingdao266071China College of earth science and Engineering Shandong University of Science and TechnologyQingdao266590China

As important metal sulfides in the geochemical cycle of sulfur,the characteristics and formation processes of pyrites can provide useful clues regarding their environment.Based on previous findings,shale pyrites were divided into three major classes(euhedral pyrites,framboidal pyrites(framboids)and metasomatic pyrites)and six sub-classes in this study.At the microscopic scale,each type of pyrite is associated with a different formation process.Framboids are formed by burst nucleation in environments with a homogeneous distribution of nutrients while euhedral pyrites are usually formed on pre-existing sites(such as=Fes on the minerals surface)in the heterogeneous system.Metasomatic pyrites formed by the replacement of other ions in accountable material by iron ions and hydrogen sulfide ions in hydrothermal events.The morphology and isotope value of pyrite provide information to track the origins of their nutrient and characteristics of sulfur and iron pools.In addition,the trace element content of pyrite can serve as a proxy for paleo-ocean trace element abundance,indicating changes in atmospheric oxygen content.Additionally,pyrite can also serves as an indicator of shale gas reservoirs.

关键词： shale Pyrite sulfate reduction reaction Isotope fractionation Pyrite element

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