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Constructing a 3D multichannel structure to enhance performance of Ni–Co–Mn hydroxide electrodes for flexible supercapacitors

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Rare metals 2024年第1期43卷 148-163页

作者： Zhi-Hui Xu Shi-Shuai Sun Xue-Lei Li Zhi-Hui Zhang Hai-Ying Li Shuang-Ting Ruan Shou-Gen Yin key laboratory of Display materials and Photoelectric Devices(ministry of education)and Tianjin key laboratory for Photoelectric materials and Devices School of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China College of science Tianjin University of TechnologyTianjin 300384China School of materials science and engineering Inner Mongolia University of TechnologyHohhot 010051China

The balancing of the electrochemical performance,mechanical stability,and processing technology for applying supercapacitors to flexible and wearable electronics continues to encounter severe ***,we prepare Ni-Co-Mn hydroxide electrodes with a threedimensional multichannel structure via a simple hydrothermal *** are constructed using vertically contiguous nano sheets with a uniform thickness and rough *** electrodes can provide numerous electroactive sites and accelerate the transmission of electrolyte *** relationship between the structure and electrochemical performances is verified by experiments and theoretical ***-dimensional(2D)planar and one-dimensional(1D)fiber electrodes are prepared using a flexible carbon cloth(CC)and carbon fiber(CF),respectively,as *** assembled quasi-solid-state flexible asymmetric supercapacitor(FASC)with a twodimensional sandwich structure using NiCoMn-OH/CC as the electrode achieves a remarkable energy density of73.8 Wh·kg^(-1)at a power density of 1.03 kW·kg^(-1).The quasi-solid-state FASC with a 1D linear structure using NiCoMn-OH/CF as the electrode also attains a high energy density(12.9 Wh·kg^(-1)at a power density of0.75 W·kg^(-1)).Moreover,the electrochemical performances of the NiCoMn/CC//AC/CC and NiCoMn/CF//AC/CF FASCs are not disturbed at different bending angles(0°,45°,90°,135°and 180°),This indicates the superior flexibility of the *** also assemble a self-powered energy-harvesting storage system by integrating FASCs and commercial solar cells to verify its *** displays sustainable development potential for energy storage.

关键词： Supercapacitors Flexible Ni–Co–Mn hydroxide 3D multichannel structure High performances

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Phase-field simulation of precipitation kinetics and creep properties of Ni-Al-Cr/Ta superalloys

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science China(Technological sciences) 2024年第4期67卷 1139-1150页

作者： YANG ShuaiGe ZHANG Zan ZHUO JiCheng LONG HongLi LI YongSheng National key laboratory of Advanced Casting Technologies MIIT Key Laboratory of Advanced Metallic and Intermetallic Materials TechnologyEngineering Research Center of Materials Behavior and DesignMinistry of EducationNanjing University of Science and TechnologyNanjing 210094China

The precipitation kinetics ofγ'-Ni_(3)(Al,Ta)phase and creep properties of Ni-15Al-x Ta at.%superalloys are investigated by the crystal plasticity phase-field *** results show that the high Ta content brings a lower creep strain for the deceleration and steady creep stage,while the creep lifetime is *** large external strain intensifies the creep damage and shortens the creep life of Ni-15Al-3Ta at.%*** kinetics evolution and elements distribution are revealed in the quaternary Ni-10Al-8.5Cr-xT a(x=1.5 at.%,2.0 at.%,2.5 at.%)superalloys by the multi-component phase-field *** anti-phase boundary(APB)changes the coarsening mechanism ofγ'phase,and Ta promotes the precipitation ofγ'phase with an increasing volume fraction and particle *** composition difference betweenγ'andγphases increases with the rising of Ta content,the strong partitioning of Ta toγ'phase strengthens the partitioning of Ni and Cr toγmatrix,and Ta shows a superiority than Al in the lattice site occupation of L1_(2)-Ni_(3)(Al,X)*** an importantγ'phase forming element,the optimization of Ta content is essential for improving the mechanical properties of Ni-based superalloys.

关键词： Ni-Al-Ta alloys creep properties kinetics phase-field

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Enhancing thermoelectric performance in P-type Mg_(3)Sb_(2)-based Zintls through optimization of band gap structure and nanostructuring

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Journal of materials science & Technology 2024年第3期170卷 25-32页

作者： Yi-bo Zhang Ji-Sheng Liang Chengyan Liu Qi Zhou Zhe Xu Hong-bo Chen Fu-cong Li Ying Peng Lei Miao Guangxi key laboratory of Information Material Engineering Research Center of Electronic Information Materials and DevicesMinistry of EducationSchool of Material Science and EngineeringGuilin University of Electronic TechnologyGuilin 541004China Guangxi key laboratory for Relativity Astrophysics Center on Nanoenergy ResearchGuangxi Key Laboratory of Processing for Nonferrous Metal and Featured MaterialsSchool of Physical Science&TechnologyGuangxi UniversityNanning 530004China Guangxi key laboratory of Precision Navigation Technology and Application Guilin University of Electronic TechnologySchool of Information and CommunicationGuilin 541004China

P-type Mg_(3)Sb_(2)-based Zintls have attracted considerable interest in the thermoelectric(TE)field due to their environmental friendliness and low ***,compared to their n-type counterparts,they show relatively low TE performance,limiting their application in TE *** this work,we simultaneously introduce Bi alloying at Sb sites and Ag doping at Mg sites into the Mg_(3)Sb_(2)to coopera-tively optimize the electrical and thermal properties for the first time,acquiring the highest ZT value of∼0.85 at 723 K and a high average ZT of 0.39 in the temperature range of 323-723 K in sample Mg_(2.94)Ag_(0.06)Sb_(1.9)Bi_(0.1).The first-principle calculations show that the codoping of Ag and Bi can shift the Fermi level into the valence band and narrow the band gap,resulting in the increased carrier concentration from 3.50×10^(17)cm^(-3)in the reference Mg 3 Sb 0.9 Bi 0.1 to∼7.88×10^(19)cm^(-3)in sample Mg 2.94 Ag 0.06 Sb 0.9 Bi *** a result,a remarkable power factor of∼778.9μW m^(-1)K^(-2)at 723 K is achieved in sample Mg 2.94 Ag 0.06 Sb 0.9 Bi ***,a low lattice thermal conductivity of∼0.48 W m^(-1)K^(-1)at 723 K is also obtained with the help of phonon scattering at the distorted lattice,point defects,and nano-precipitates in sample Mg 2.94 Ag 0.06 Sb 0.9 Bi *** synergistic effect of using the multi-element co-doping/-alloying to optimize electrical properties in Mg_(3)Sb_(2)holds promise for further improving the TE performance of Zintl phase materials or even others.

关键词： Thermoelectric materials Band engineering Nanostructuring P-type Mg_(3)Sb_(2) Ag and Bi Co-doping

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Distinct Electrical and Mechanical Responses of a Cu-10Fe Composite Prepared by Hot-Pressed Sintering and Post Treatment

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Acta metallurgica Sinica(English Letters) 2024年第2期37卷 255-265页

作者： X.Y.Yue S.Y.Peng X.Zhang C.N.He Y.Z.Tian key laboratory for Anisotropy and Texture of materials(ministry of education) School of Materials Science and EngineeringNortheastern UniversityShenyang110819China School of materials science and engineering and Tianjin key laboratory of Composite and Functional materials Tianjin UniversityTianjin300350China Research Centre for metallic Wires Northeastern UniversityShenyang110819China

A Cu-10wt%Fe composite was prepared through hot-pressed sintering,and the material was subsequently solution *** hot-pressed sintered and solution treated materials were rolled and *** precipitation behavior and performance changes were systematically studied by using scanning electron microscopy and transmission electron *** contrast to the hot-pressed sintered specimen,the solution treatment significantly affects the thermal stability and properties of the Cu-10wt%Fe *** Cu-10wt%Fe composite was prepared after solid solution,cold rolling and aging at 773 K for 1 h,and it obtained excellent tensile strength of 494 MPa,uniform elongation of 16.3%,electrical conductivity of 51.1%IACS and softening temperature of 838 *** for the distinct difference in thermal stability and properties between hot-pressed sintered and solution treated specimens were *** findings provide a theoretical basis for designing high-performance Cu-based in-situ composites by post treatment.

关键词： Cu-Fe composite Hot-pressed sintering Thermal stability Strength Electrical conductivity

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Vacancy healing for stable perovskite solar cells via bifunctional potassium tartrate

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Journal of Energy Chemistry 2024年第1期88卷 64-70,I0002页

作者： Jing Dou Yue Ma Xiuxiu Niu Wentao Zhou Xueyuan Wei Jie Dou Zhenhua Cui Qizhen Song Tinglu Song Huanping Zhou Cheng Zhu Yang Bai Qi Chen Experimental Centre for Advanced materials School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing key laboratory for Theory and Technology of Advanced Battery materials Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationBIC-ESATSchool of Materials Science and EngineeringPeking UniversityBeijing 100871China

Perovskite solar cell has gained widespread attention as a promising technology for renewable ***, their commercial viability has been hampered by their long-term stability and potential Pb leakage. Herein, we demonstrate a bifunctional passivator of the potassium tartrate(PT) to address both challenges. PT minimizes the Pb leakage in perovskites and also heals cationic vacancy defects, resulting in improved device performance and stability. Benefiting from PT modification, the power conversion efficiency(PCE) is improved to 23.26% and the Pb leakage in unencapsulated films is significantly reduced to 9.79 ppm. Furthermore, the corresponding device exhibits no significant decay in PCE after tracking at the maximum power point(MPP) for 2000 h under illumination(LED source, 100 mW cm^(-2)).

关键词： Perovskite Potassium tartrate Lead leakage Long-term stability

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Stabilization of cathode electrolyte interphase for aqueous zinc-ion batteries

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Journal of Energy Chemistry 2024年第9期96卷 359-386页

作者： Zhenjie Yao Wenyao Zhang Junwu Zhu key laboratory for Soft Chemistry and Functional materials ministry of education Nanjing University of Science and TechnologyNanjing 210094JiangsuChina

Aqueous zinc-ion battery systems are attractive for next-generation energy storage devices,however,the unstable electrode electrolyte interphase,especially cathode electrolyte interphase(CEI),has induced rapid capacity attenuation,insufficient cycle life,and severe safety *** the researching of CEI formation,composition,dynamic structure,and reaction mechanisms would help in understanding the fundamental electrochemistry at CEI such as electron and ion transport processes,further strengthening the specific capacity,rate,and cycle performance of the cathode *** this review,we summarized the latest progress in understanding interfacial reaction mechanisms and ion dynamic behavior,emphasizing the impact of surface-specific adsorption and solvation behaviors on the interface's ultimate structure and chemical ***,the significant challenges that persist in CEI formation mechanisms,such as cathodic dissolution,by-product formation,electrostatic interactions,constrained electrochemical windows,oxygen evolution reaction,overpotentials,phase transitions,and additional factors,were *** challenges are explored to identify triggers contributing to the depletion of active materials and alterations in the composition or state of the ***,with a deep comprehension of interfacial behaviors,the review articulates innovative optimization strategies through a detailed categorization of approaches in electrolyte engineering,cathode engineering,and artificial CEI ***,future challenges and development directions of CEI are *** hope to offer insights for constructing robust CEI films to achieve high performance aqueous zinc-ion batteries.

关键词： Aqueous zinc-ion batteries Cathode-electrolyte interphase Energy storage

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Sulfate-assisted Ni/Fe-based electrodes for anion exchange membrane saline splitting

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Nano Research 2024年第7期17卷 5985-5995页

作者： Yujun Han Li Shao Yuhang Liu Guodong Li Tongzhou Wang Xuerong Zheng Jihong Li Xiaopeng Han Wenbin Hu Yida Deng School of materials science and engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin UniversityTianjin 300072China State key laboratory of Marine Resource Utilization in South China Sea School of Materials Science and EngineeringHainan UniversityHaikou 570228China State key laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012China key laboratory of Advanced Energy materials Chemistry(ministry of education) Nankai UniversityTianjin 300071China

Saline water electrolysis is an appealing strategy for hydrogen production,attracting more attention in recent ***-based electrodes exhibit promise as catalysts for saline water ***,they suffer from the inferior service life of the oxygen evolution reaction(OER).Herein,we report an oxygen-evolution electrode consisting of a sulfate-modulated nickel-iron hydroxide(NiFeOOH)affording as the catalytic active layer and Fe-Ni_(3)S_(2) as the corrosion-proof *** developed electrode only requires overpotentials of 220 and 292 mV to deliver the current density of 10 and 500 mA·cm^(−2),*** importantly,it presents long-term stability exceeding 140 and 100 h in 1 M KOH at high current densities of 500 and 1000 mA·cm^(−2),respectively,as well as 120 h for saline water electrolysis at 100 mA·cm^(−2).Experimental results reveal that the generated sulfate plays an indispensable role in improving stability and corrosion *** assembled and tested an anion exchange membrane electrolyzer with Pt/C and NiFeS/NIF as the cathode and anode,respectively,under industrial *** overall water-splitting electrolyzer achieves an impressive energy conversion efficiency of 75%±0.5%.This report offers fresh insights into the design of stable NiFe-based electrodes,which may further promote its practical applications for saline water electrolysis.

关键词： saline water electrolysis oxygen evolution reaction anode material water splitting

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Boosting high-rate Li-ion storage properties by La(Ⅲ)ion doping in spinel(Co_(0.2)Cr_(0.2)Fe_(0.2)Mn_(0.2)Ni_(0.2))_(3)O_(4)high-entropy oxide anode

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Journal of Advanced Ceramics 2024年第6期13卷 769-779页

作者： Shijie Chen Mengfan Bao Yanggang Jia Pengpeng Wang Dan Wei Yuhuan Guo Jie Tan Aiqin Mao Advanced Ceramics Research Center School of Materials Science and EngineeringAnhui University of TechnologyMa’anshan 243032China key laboratory of Green Fabrication and Surface Technology of Advanced metal materials(Anhui University of Technology) Ministry of EducationMa’anshan 243032China

The present work aims to create lattice distortion and optimize the surface oxygen vacancy(OV)concentration in a model spinel(Co_(0.2)Cr_(0.2)Fe_(0.2)Mn_(0.2)Ni_(0.2))_(3)O_(4)high-entropy oxide(HEO)through a heteroatom La^(3+)doping *** demonstrated,La^(3+)with a large radius can be doped successfully into the spinel lattice of(Co_(0.2)Cr_(0.2)Fe_(0.2)Mn_(0.2)Ni_(0.2))_(3)O_(4),thereby not only causing lattice distortion to increase oxygen vacancies but also refining crystalline grains and improving the specific *** with the(Co_(0.2)Cr_(0.2)Fe_(0.2)Mn_(0.2)Ni_(0.2))_(3)O_(4)anode,the(La_(0.01)CoCrFeMnNi)_(3/5.01)O_(4) anode with moderate doping exhibits excellent cycling performance(1228 mAh·g^(−1)after 400 cycles at 0.2 A·g^(−1))and yields an increase of 75%rate capability at 3 A·g^(−1)(420 mAh·g^(−1)at 3 A·g^(−1)).The desirable kinetic transport of electrons and diffusion of Li+within the moderately La^(3+)-doped anode and the synergistic interfacial pseudocapacitive behavior satisfy the redox reaction at a high rate,thus increasing rate capability.

关键词： lithium-ion battery(LIB) anode lattice distortion high-entropy oxide(HEO) high-rate performance La^(3+)doping oxygen vacancy(OV)

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Hierarchical FeO_(χ)H_(y)@Ni_(3)B hybrid for efficient alkaline oxygen evolution at high current density

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Journal of Energy Chemistry 2024年第7期94卷 599-607页

作者： Fuxi Liu Qing Liang Zhenyu Li Meiqi Liu Nailin Yue Zizhun Wang Xu Zou Wei Zhang key laboratory of Automobile materials ministry of education School of Materials Science&EngineeringElectron Microscopy CenterInternational Center of Future ScienceJilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsJilin UniversityChangchun 130012JilinChina

Electrocatalysts with high activity and long-term durability are vital toward large-scale hydrogen pro-duction from electrocatalytic water ***,the self-supported electrode(FeO_(χ)H_(y)@Ni_(3)B/NF)with hierarchical heterostructure was simply prepared by using Ni_(3)B chunks grown on nickel foam as sub-strate to in situ form vertical FeO_(χ)H_(y)*** hybrid shows efficient oxygen evolution reaction activity with overpotentials as low as 267 and 249 mV at 100 mA cm^(-2)in 1 M KOH solution and 30 wt%KOH solution,***,it also exhibits excellent catalytic stability,sustaining catalysis at 500 mA cm^(-2)in 1 M KOH solution for 200 h,and even for 200 h at 1000 mA cm^(-2)in 30 wt%KOH *** experimental results reveal that the FeO_(χ)H_(y)@Ni_(3)B/NF is endowed with superhydrophilic and superaerophobic surface properties,which not only provide more mass transport channels,as well as facilitated the diffusion of reaction intermediates and gas ***,it holds faster reaction kinetics,more accessible active sites and accelerated electron transfer rates due to strong synergistic interactions attheheterogeneous interface.

关键词： FeO_(χ)H_(y)@Ni_(3)B/NF hybrid Heterostructure Oxygen evolution reaction Electrocatalytic

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Constructing a fluorinated interface layer enriched with Ge nanoparticles and Li-Ge alloy for stable lithium metal anodes

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Nano Research 2024年第6期17卷 5148-5158页

作者： Fulu Chu Jinwei Zhou Jiamin Liu Fengcheng Tang Liubin Song Feixiang Wu School of metallurgy and Environment Engineering Research Center of the Ministry of Education for Advanced Battery MaterialsHunan Provincial Key Laboratory of Nonferrous Value-added MetallurgyCentral South UniversityChangsha 410083China Hunan Provincial key laboratory of materials Protection for Electric Power and Transportation School of Chemistry and Chemical EngineeringChangsha University of Science and TechnologyChangsha 410004China School of materials science&engineering University of JinanJinan 250022China

Lithium metal batteries(LMBs)based on metallic Li exhibit high energy density to be competent for advanced energy storage ***,the unstable solid electrolyte interphase(SEI)layer due to continuous decomposition of electrolytes,and the attendant problem of Li dendrite growth frustrate their commercialization ***,a hybrid SEI comprising abundant LiF,lithiophilic Li-Ge alloy,and Ge nanoparticles is constructed via a simple brush coating *** fluorinated interface layer with embedded Ge-containing components isolates the Li anode from the corrosive electrolyte and facilitates homogenous Li nucleation as well as uniform ***,the modified Li anode exhibits remarkable stability without notorious Li dendrites,delivering stable cycling lives of more than 1000 h for symmetric Li||Li cells and over 600 cycles for Li||Cu cells at 1 mA·cm^(−2).Moreover,the reinforced Li anodes endow multiple full-cell architectures with dramatically improved cyclability under different test *** work provides rational guidance to design an artificial hybrid SEI layer and would stimulate more ideas to solve the dendrite issue and promote the further development of advanced LMBs.

关键词： lithium metal anode artificial solid electrolyte interphase(SEI) dendrite suppression lithium fluoride Li-Ge alloy

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