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Self-Powered Piezo-Supercapacitors Based on ZnO@Mo-Fe-MnO2 Nanoarrays

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Energy & Environmental materials 2024年第4期7卷 304-314页

作者： Luo Sun Zhiguo Ye Xinyuan Peng Shaojie Zhuang Duosheng Li Zhong Jin School of materials Science and Engineering Nanchang Hangkong University State key laboratory of Coordination Chemistry MOE Key Laboratory of Mesoscopic Chemistry MOE Key Laboratory of High Performance Polymer Materials and Technology Jiangsu Key Laboratory of Advanced Organic Materials School of Chemistry and Chemical Engineering Nanjing University

The development of self-charging supercapacitor power cells （SCSPCs） has profound implications for smart electronic devices used in different ***,we epitaxially electrodeposited Mo-and Fe-codoped MnO2films on piezoe... 详细信息

关键词： MnO2 piezoelectric self-charging supercapacitors ZnO nanoarray

DLP printing of BT/HA nanocomposite ceramic scaffolds using low refractive index BT crystals

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Journal of Materiomics 2024年第5期10卷 1036-1048页

作者： Ruixuan Xue Peimei Yuan Bo Zhao Fei Jing Xuyuan Kou Wangyang Yue Yan wang Dongmei Wang Galhenage Asha Sewvandi Dengwei Hu Faculty of Chemistry and Chemical Engineering Baoji University of Arts and SciencesKey Laboratory of Functional Materials of Baoji Engineering Research Center for Titanium Based Functional Materials and DevicesUniversities of Shaanxi Province1 Hi-Tech AvenueBaoji721013ShaanxiChina Department of materials Science and Engineering Faculty of EngineeringUniversity of MoratuwaKatubeddaSri Lanka

Biological piezoelectric materials have significant potential for bone repair and energy harvesting owing to their excellent biocompatibility and piezoelectric *** BaTiO3/Ca10(PO4)6(OH)2(BT/HA)composite material is an outstanding representative of biological piezoelectric materials,which has not been individually designed using digital light processing(DLP)3D printing because of the large difference in the refractive index of its ***,in this work,double-sided-tooth plate-like BT crystals with high curvature were prepared via a hydrothermal process,and BT/HA ceramic slurries were grinded out using dispersed intermittent ball milling scheme,and BT/HA nanocomposite ceramic scaffolds were fabricated by DLP 3D printing *** nanostructure,dielectric properties,and piezoelectric energy harvesting performance of the BT/HA nanocomposite ceramic scaffolds were *** influences of different morphologies and contents for BT on the piezoelectric potential and stress distribution were analyzed based on a multi-physics coupling finite element *** cell proliferation and adhesion abilities were investigated *** BT/HA nanocomposite ceramic scaffolds present excellent dielectric properties,cell proliferation and adhesion abilities,and an open circuit voltage of 8 V during piezoelectric energy *** material properties and multi-physics coupling finite element analysis imply that the double-sided-tooth plate-like BT plays an important role for the fastness structure and electric field distribution in the BT/HA ***,this work provides a strategy for the application of the customized BT/HA nanocomposite ceramic scaffolds in new-generation orthopedic implants and biological energy harvesting.

关键词： 3D printing BT/HA nanocomposite ceramics Bio-piezoelectric scaffolds Energy harvesting

Indentation behavior of a semi-infinite piezoelectric semiconductor under a rigid flat-ended cylindrical indenter

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Applied Mathematics and Mechanics(English Edition) 2024年第4期45卷 649-662页

作者： Shijing GAO Lele ZHANG Jinxi LIU Guoquan NIE Weiqiu CHEN State key laboratory of Mechanical Behavior and System Safety of Traffic Engineering Structures Shijiazhuang Tiedao UniversityShijiazhuang 050043China School of Mechanical Engineering Shijiazhuang Tiedao UniversityShijiazhuang 050043China Hebei key laboratory for Mechanics of Intelligent materials and Structures Department of Engineering MechanicsShijiazhuang Tiedao UniversityShijiazhuang 050043China State key laboratory of Computer Aided Design and Computer Graphics Key Laboratory of Soft Machines and Smart Devices of Zhejiang ProvinceDepartment of Engineering MechanicsZhejiang UniversityHangzhou 310027China

This paper theoretically studies the axisymmetric frictionless indentation of a transversely isotropic piezoelectric semiconductor(PSC)half-space subject to a rigid flatended cylindrical *** contact area and other surface of the PSC half-space are assumed to be electrically *** the Hankel integral transformation,the problem is reduced to the Fredholm integral equation of the second *** equation is solved numerically to obtain the indentation behaviors of the PSC half-space,mainly including the indentation force-depth relation and the electric potential-depth *** results show that the effect of the semiconductor property on the indentation responses is limited within a certain range of variation of the steady carrier *** dependence of indentation behavior on material properties is also analyzed by two different kinds of *** element simulations are conducted to verify the results calculated by the integral equation technique,and good agreement is demonstrated.

关键词： piezoelectric semiconductor(PSC) insulating indenter electromechanical response singular integral equation finite element simulation

Temperature/electric field induced photoluminescence-modulation effect in dysprosium-doped barium titanate ferroelectric ceramics

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Journal of Materiomics 2024年第5期10卷 1117-1125页

作者： Lei Xia Xiao Liu Zhan Mao Yanbin Cai Jing Zhu Jiyang Xie Wanbiao Hu Yunnan key laboratory of Electromagnetic materials and devices National Center for International Research on Photoelectric and Energy MaterialsSchool of Materials and EnergyYunnan UniversityKunming650091China Electron Microscopy Center Yunnan UniversityKunming650091China University of Science and Technology of China Hefei230026China

Lanthanide(Ln^(3+))based ferroelectric phosphors,with an integration of PL emission and ferroelectric effect,are unveiling an exciting realm of possibilities for multifunctional ferroelectric-optic ***,how the ferroelectric host enables the tuning on the PL emissions through modulating the local structure(e.g.,lattice site,symmetry,strains etc.)of the Ln^(3+)activator is not established *** this work,a luminescent-ferroelectric material,***^(3+)doped BaTiO_(3) ceramic(Ba_(1–x)Dy_(x)TiO_(3)(x=0–0.07),abbr:BTO:Dy^(3+)),was explored to address the aforementioned *** BTO:Dy^(3+)ceramics were synthesized by a solid-state reaction *** crystal structure,photoluminescence(PL)and electric properties(dielectric constant,ferroelectric hysteresis and piezoelectric hysteresis loop)were systematically *** BTO:Dy^(3+)ceramics show two predominant emission peaks,corresponding to the blue magnetic dipole transition(477 nm,4F_(7/2)→6H_(15/2))and yellow electric dipole transition(573 nm,4F_(7/2)→6H_(13/2)),the intensity ration of which can be modulated by the ferroelectric polarization that causes the slight lattice *** a polarization-emission modulation combining with the Dy3+doping could accelerate the color change,from yellow to blue,which is characterized to detect the phase transition,with a method and mechanism were proposed,that is,the phase change is reflected by the PL characteristic peak intensity ***,the current results offer a convenient photoluminescence method for detecting the ferroelectric phase transition and a feasible approach to study the interaction between the photoluminescence and polarization in ferroelectric materials,for providing new insights for the development of multifunctional materials.

关键词： Photoluminescence Barium titanate Modulation ferroelectric ceramics

Self-fueling ferroptosis-inducing microreactors based on p H-responsive Lipiodol Pickering emulsions enable transarterial ferro-embolization therapy

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National Science Review 2024年第1期11卷 74-85页

作者： Chunjie Wang Lei Zhang Zhijuan Yang Dongxu Zhao Zheng Deng Jialu Xu Yumin Wu Yu Hao Ziliang Dong Liangzhu Feng Zhuang Liu Institute of Functional Nano & Soft materials (FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices Soochow University Center of Interventional Radiology & Vascular Surgery Department of Radiology Zhongda Hospital Medical School Southeast University Department of Interventional Radiology The First Afflliated Hospital of Soochow University

Lipiodol chemotherapeutic emulsions remain one of the main choices for the treatment of unresectable hepatocellular carcinoma(HCC) via transarterial chemoembolization(TACE). However, the limited stability of Lipiodol chemotherapeutic emulsions would lead to rapid drug diffusion, which would reduce the therapeutic benefit and cause systemic toxicity of administrated chemotherapeutics. Therefore, the development of enhanced Lipiodol-based formulations is of great significance to enable effective and safe TACE treatment. Herein, a stable water-in-oil Lipiodol Pickering emulsion(LPE) stabilized by pH-dissociable calcium carbonate nanoparticles and hemin is prepared and utilized for efficient encapsulation of lipoxygenase(LOX). The obtained LOX-loaded CaCO3&hemin-stabilized LPE(LHCa-LPE) showing greatly improved emulsion stability could work as a pH-responsive and self-fueling microreactor to convert polyunsaturated fatty acids(PUFAs), a main component of Lipiodol, to cytotoxic lipid radicals through the cascading catalytic reaction driven by LOX and hemin, thus inducing ferroptosis of cancer cells. As a result, such LHCa-LPE upon transcatheter embolization can effectively suppress the progression of orthotopic N1S1 HCC in rats. This study highlights a concise strategy to prepare pH-responsive and stable LPE-based self-fueling microreactors, which could serve as bifunctional embolic and ferroptosis-inducing agents to enable proof-of-concept transarterial ferro-embolization therapy of HCC.

关键词： CaCO3 nanoparticles Pickering emulsion ferroptosis lipid peroxidation transarterial ferro-embolization

Convenient folding-hot-pressing fabrication and enhanced piezoelectric properties of highβ-phasecontent poly(vinylidene fluoride)films

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Interdisciplinary materials 2024年第5期3卷 715-725页

作者： Jie Shen Yicheng Zeng Qiangzhi Li Jing Zhou Wen Chen State key laboratory of Advanced Technology for materials Synthesis and Processing School of Materials Science and EngineeringWuhan University of TechnologyWuhanChina Sanya Science and Education Innovation Park Wuhan University of TechnologySanyaChina hubei Longzhong laboratory Wuhan University of Technology Xiangyang Demonstration ZoneXiangyangChina

Poly(vinylidene fluoride)(PVDF)is the most attractive piezoelectric polymer for application in flexible *** attain excellent piezoelectric properties,a substantial amount of spontaneous polarβ-phase content is highly ***,the current reported manufacturing methods to increaseβ-phase contents are inconvenient and complex,hindering progress in PVDF's *** work proposes a folding-hot-pressing method to fabricate highβ-phase-content PVDF *** characterization indicates that the films haveαandβphases and the folding-hot-pressing process transforms theαphase into theβ*** to the 97.5%β-phase content and aligned structure,a piezoelectric constant of 20 pC/N is achieved in the three-times folded ***,the process method enhances the tensile strength(126.2 MPa)of the films,with a low Young's modulus(0.87 GPa)remaining,making the films applicable for flexible piezoelectric ***,sensors based on the achieved films were assembled and applied for human physiological activity *** work offers a scalable new melt-processing strategy for developing high-performance PVDF-based piezo-electric composite films for wearable electronic devices.

关键词： flexible sensors highβ-phase content piezoelectric properties PVDF film

Fourth-order phase-field modeling for brittle fracture in piezoelectric materials

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Applied Mathematics and Mechanics(English Edition) 2024年第5期45卷 837-856页

作者： Yu TAN Fan PENG Chang LIU Daiming PENG Xiangyu LI State key laboratory of Geohazard Prevention and Geoenvironment Protection Chengdu University of TechnologyChengdu 610059China College of Science Chang'an UniversityXi'an 710064China Applied Mechanics and Structure Safety key laboratory of Sichuan province School of Mechanics and Aerospace EngineeringSouthwest Jiaotong UniversityChengdu 610031China

Failure analyses of piezoelectric structures and devices are of engineering and scientific *** this paper,a fourth-order phase-field fracture model for piezoelectric solids is developed based on the Hamilton *** typical electric boundary conditions are involved in the present model to characterize the fracture behaviors in various physical situations.A staggered algorithm is used to simulate the crack *** polynomial splines over hierarchical T-meshes(PHT-splines)are adopted as the basis function,which owns the *** numerical simulations are performed to study the influence of the electric boundary conditions and the applied electric field on the fracture behaviors of piezoelectric *** electric boundary conditions may influence crack paths and fracture loads *** present research may be helpful for the reliability evaluation of the piezoelectric structure in the future applications.

关键词： isogeometric analysis(IGA) brittle fracture fourth-order phase-field model piezoelectric solid

Giant negative electrocaloric effect measured by indirect method in X-ray irradiated P(VDF-TrFE)films

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Journal of Materiomics 2024年第3期10卷 624-631页

作者： Bo Li Bin Yang Hong Zhang Jiajia Zhang Qianjin Wang Weishu Liu Department of materials Science and Engineering Southern University of Science and TechnologyShenzhenGuangdong 518055China Guangdong Provincial key laboratory of Functional Oxide materials and devices Southern University of Science and TechnologyShenzhenChina College of Physics and Electronic Information Yunnan Normal UniversityYunnan Kunming 650500China The Science and Technology on Reliability Physics and Application of Electronic Component laboratory China Electronic Product Reliability and Environmental Testing Research InstituteGuangzhou 510610China

Flexible solid-state cooling devices with high efficiency are attracted to ferroelectric polymers with excellent negative electrocaloric(EC)*** is challenging to obtain a large negative EC effect in ferroelectric polymers due to the lack of tunable techniques.A giant negative EC response was obtained in the poly(vinylidene fluoride-trifluoroethylene)copolymers(P(VDF-TrFE),70/30,in mole ratio)irra-diated with high-energy *** irradiated P(VDF-TrFE)films showed an adiabatic temperature change of-13.5 K at 40 MV/m under a dose of 5 Mrad(1 Mrad=10^(4) J/kg)obtained by the indirect *** significant negative EC effect is attributed to the enhancement of crystalline due to the entry of polymer molecules into the amorphous to crystalline structure and the reduction of heat ca-pacity due to the increase of *** addition,X-ray irradiation improves the dielectric coefficient from 15 to *** research indicates that irradiation can modify the negative EC properties of ferro-electric polymers for solid-state cooling.

关键词： Negative electrocaloric effects X-rays radiation P(VDF-TrFE)films

Single‑Layer ZnO Hollow Hemispheres Enable High‑Performance Self‑Powered Perovskite Photodetector for Optical Communication

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Nano-Micro Letters 2021年第4期13卷 259-270页

作者： Xiyan Pan Jianqiang Zhang Hai Zhou Ronghuan Liu Dingjun Wu Rui Wang Liangping Shen Li Tao Jun Zhang Hao Wang hubei key laboratory of ferro and piezoelectric materials and devices School of Microelectronics and Faculty of Physics and Electronic ScienceHubei UniversityWuhan 430062People’s Republic of China

The carrier transport layer with reflection reduction morphology has attracted extensive attention for improving the utilization of ***,we introduced single-layer hollow ZnO hemisphere arrays(ZHAs)behaving light trapping effect as the electron transport layer in perovskite photodetectors(PDs).The singlelayer hollow ZHAs can not only reduce the reflection,but also widen the angle of the effective incident light and especially transfer the distribution of the optical field from the ZnO/FTO interface to the perovskite active layer confirmed by the 3D finitedifference time-domain *** merits benefit for the generation,transport and separation of carriers,improving the light utilization ***,our optimized FTO/ZHA/CsPbBr3/carbon structure PDs showed high self-powered performance with a linear dynamic range of 120.3 dB,a detectivity of 4.2×10^(12) Jones,rise/fall time of 13/28μs and the f_(−3) dB of up to 28 *** from the high device performance,the PD was demonstrated to the application in the directional transmission of encrypted files as the signal receiving port with super high *** work uniquely utilizes the features of high-performance self-powered perovskite PDs in optical communication,paving the path to wide applications of all-inorganic perovskite PDs.

关键词： Hemisphere array Perovskite Photodetector Reflection reduction Optical communication