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Trace elements in magmatic and hydrothermal quartz:Implications on the genesis of the Xingluokeng Tungsten Deposit,South China

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Acta Geochimica 2024年第3期43卷 441-458页

作者： Qing-Qing Zhang You-Wei Chen Jian-Feng Gao State key laboratory of Ore Deposit geochemistry Institute of GeochemistryChinese Academy of SciencesGuiyang 550081China University of Chinese Academy of Sciences Beijing 100049China

The Xingluokeng deposit is the largest gran-ite-related tungsten deposit within the Wuyi metallogenic belt in South *** Xingluokeng intrusion primarily consists of porphyritic biotite granite,biotite granite,andfine-grained *** deposit is represented by veinlet-disseminated mineralization with K-feldspathization and biotitization,alongside quartz-vein mineralization with gre-isenization and *** study investigates in-situ analyses of quartz compositions from both the intrusion and hydrothermal veinlets and *** element correlations indicate that trivalent Al^(3+)and Fe^(3+)replace Si^(4+)within the quartz lattice,with monovalent cations(such as Li^(+),Na^(+),and K^(+))primarily serving as charge *** Ge/Al ratios(<0.013)of quartz from granites suggest a mag-matic *** low Al/Ti and Ge/Ti ratios,accompanied by high Ti contents in quartz,suggest that the porphyritic biotite granite and biotite granite are characterized by rela-tively low levels of differentiation and high crystallization *** contrast,thefine-grained granite exhibits a higher degree of fractionation,lower crystallization tem-peratures,and a closer association with tungsten *** contents in quartz from quartz veins indicate Qz-Ⅰformed at temperatures above 400°C,while Qz-Ⅱto Qz-Ⅴformed at temperatures below 350°*** in different generations of quartz,as indicated by Al content and(Al+Fe)/(Li+Na+K)ratio,suggest that Qz-Ⅰprecipi-tated from a less acidicfluid with a stable pH,whereas Qz-Ⅱto Qz-Ⅴoriginated from a more acidicfluid with notable pH ***,alkaline alteration and acidic alteration supplied the essential Ca and Fe for the precipita-tion of scheelite and wolframite,respectively,highlighting a critical mechanism in tungsten mineralization at the Xin-gluokeng deposit.

关键词： Quartz Xingluokeng Tungsten deposit Trace elements South China

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Linkage of mineral inclusions and zoning of magnetite with fluid evolution of hydrothermal systems: A case study of the Fenghuangshan Cu-Fe-Au skarn deposit， Eastern China

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Journal of Earth Science 2024年

作者： Xiao-Wen Huang Yiping Yang Mei-Fu Zhou Yu-Miao Meng Jian-Feng Gao Liang Qi State key laboratory of Ore Deposit geochemistry， Institute of geochemistry， Chinese Academy of Sciences CAS key laboratory of Mineralogy and Metallogeny/Guangdong Provincial key laboratory of Mineral Physics and Materials， Guangzhou Institute of geochemistry， Chinese Academy of Sciences

Magnetite from hydrothermal deposits may show compositional zoning with various mineral inclusions in response to the evolution of hydrothermal fluids. Magnetite from the Fenghuangshan Cu-Fe-Au skarn deposit (Eastern China) is a common mineral formed in the earlier stage of skarnization. Magnetite grains have dark gray and light gray zones and contain diverse mineral inclusions. Dark gray zones have higher Si， Ca， Al， and Mg contents than light gray zones. The magnetite matrix from dark gray zones shows superstructure along the [0-11] zone axis in fast Fourier transform patterns， different from magnetite from light gray zones with normal structure. Three types of mineral inclusions are identified within magnetite: nano-， micron- and submicron-nanometer inclusions. Nanoinclusions hosted in dark gray zones are actinolite， diopside， and trace element-rich magnetite， and these are likely formed by growth entrapment during magnetite crystallization at the skarn stage. The chain-width order-disorder intergrowths of diopside nanoinclusion likely indicate fluctuating fluid compositions in a lattice scale. Submicron to nanometer inclusions at the boundary between dark gray and light gray zones are quartz， titanite， and Ti-rich magnetite， which were formed via a dissolution and reprecipitation process at the quartz-sulfide stage. Micron-inclusions randomly distributed in both dark and light gray zones include calcite， ankerite， quartz， and chlorite， and these were formed via penetration of fluids at the carbonate stage. Zoned magnetite was formed by fluid replacement， overgrowth， and fluid infilling. Our study highlights the importance of mineral inclusion assemblages， and textural and chemical zonation of magnetite in constraining fluid evolution.

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Revisiting the Mg isotopic systematics of siliciclastic components of sediments and sedimentary rocks:A new geochemical proxy of continental weathering in Earth's history

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Science China Earth Sciences 2024年第2期67卷 620-633页

作者： Tianzheng HUANG Bing SHEN Kangjun HUANG Meng NING Chao LI Jinzhuang XUE Yuanlin SUN Baoqi HUANG key laboratory of Orogenic Belt and Crustal Evolution MOESchool of Earth and Space SciencesPeking UniversityBeijing100871China State key laboratory of Continental Dynamics Shaanxi Key Laboratory of Early Life and EnvironmentsDepartment of GeologyNorthwest UniversityXi’an710069China Institute of Sedimentary Geology Chengdu University of TechnologyChengdu610059China key laboratory of Rhenium-Osmium Isotopic geochemistry Chinese Academy of Geological SciencesBeijing100037China

The Mg isotopic compositions of siliciclastic components(δ^(26)Mg_(sili))of sediments and sedimentary rocks have been commonly used to constrain the intensity of continental weathering,based on observations of,(1)an upward enrichment of26Mg in modern weathering profiles,(2)preferential uptake of26Mg in soil clays,and(3)general positive correlations between weathering intensities andδ^(26)Mg_(sili)***,not all weathering profiles display an upward increase ofδ^(26)Mg_(sili),and not all soil clays enrich in26Mg,complicating the interpretations ofδ^(26)Mg_(sili)data of sediments and sedimentary *** further explore the controls ofδ^(26)Mg_(sili)of sediments and sedimentary rocks,here we measuredδ^(26)Mg_(sili),mineralogical compositions and major element compositions of deep sea sediments from South China Sea(SCS)and carbonate rock samples from two late Paleozoic sections in South *** samples show decreasing trends of both normalized Mg concentration(Mgnorm)andδ^(26)Mg_(sili)values with the increase of weathering intensity,while SCS sediments samples do not show any correlation between Mgnormorδ^(26)Mg_(sili)values and weathering intensity.A three-stages weathering model is developed to explain the observed Mgnorm andδ^(26)Mg_(sili)*** the new model,weathering can be divided into three stages,(1)the preliminary weathering stage characterized by dissolution of primary minerals and formation of secondary clay minerals in saprolite,(2)the transitional stage with massive vermiculite and chlorite formation on the bottom of soil,and(3)the advanced stage showing dissolution of vermiculite and chlorite in the top of *** new model explains anδ^(26)Mg_(sili)increase and Mgnormdecrease with an increase weathering intensity in preliminary weathering stage and decrease of Mgnormandδ^(26)Mg_(sili)with increase weathering intensity in advanced weathering *** revised weathering model warrants the application of Mg isotope in the study of contin

关键词： Clay mineral Chemical weathering CIA Soil Weathering model

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Trace element Mobility in Subducted Marble and Associated Eclogite:Constraints from UHP Rocks in the Shuanghe Area,Central-East China

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Journal of Earth Science 2024年第1期35卷 1-15页

作者： Xingao Hou Zhiqiang Yu Shefa Chen Lei Liu Yilin Xiao key laboratory of Metallogenic Prediction of Nonferrous Metals and Geological Environment Monitoring Ministry of EducationSchool of Geosciences and Info-PhysicsCentral South UniversityChangsha 410083China key laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China CAS key laboratory of Crust-Mantle Materials and Environments School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China

In order to decipher element mobility in UHP meta-sedimentary rocks in the continental subduction zone,major and trace element compositions are investigated for a continuous profile from a representative UHP region in the Dabie *** the lithologic contact zone,contents of K,Ca,LREE,and LILE exhibit varying degrees of downward trends in both marble and eclogite toward the contact zone,indicating that marble and their associated eclogite can release a large amount of K,Ca,and a small number of LILEs and *** is the main Ti phase in both marble and *** rims around rutile can occasionally be seen in *** of Ti and HFSE exhibit a well-coupled relation among marble and eclogite,indicating that substantial Ti and HFSEs were migrated from eclogite to marble,in accord with the capacity of a melt *** and titanites in marble exhibit a relatively limited variation in Nb/Ta ratios(12.9-16.2),similar to those of titanites in eclogite(14.2-16.7),which demonstrates that rutiles and titanites in marble were sourced from eclogite because of short-distance migrations of Ti and *** to the P-T path and the temperature and pressure conditions of the peak metamorphism reported by previous studies,the eclogite associated with marble may not form supercritical fluids in the subduction zone because of the addition of carbonate minerals.

关键词： UHP metamorphism eclogite marble element migration fluid actions geochemistry

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Age and petrogenesis of the newly discovered Early Permian granite in the Kumtor gold field， Kyrgyz Tien-Shan

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Journal of Earth Science 2024年

作者： Kyiazbek Asilbekov Rustam Orozbaev Etienne Skrzypek Christoph Hauzenberger Elena Ivleva Daniela Gallhofer Jian-Feng Gao Nikolay Pak Anatoliy Shevkunov Anatoliy Bashkirov Aizat Zhaanbaeva Institute of Geology， National Academy of Sciences of the Kyrgyz Republic Institute of Earth Sciences， University of Graz State key laboratory of Ore Deposit geochemistry， Institute of geochemistry， Chinese Academy of Sciences Kumtor Gold Company CJSC

Permian intrusions are widespread in the Middle and Southern Tien Shan， with fewer occurrences in the Northern Tien-Shan. Notably， many of these intrusions are spatially associated with a variety of ore deposits， indicating a significant link between magmatic activity and mineralization processes in these areas. We studied granite samples recently recovered from drilling in the Kumtor gold field to evaluate their potential relationships with gold mineralization. We report major and trace element geochemistry， zircon U-Pb age and Hf isotope data for this so-called Kumtor granite. The Kumtor granite is metaluminous to peraluminous and belongs to the high-K and calc-alkaline series with I-type geochemical characteristics. The relatively high K2O and Na2O concentrations and low high field strength elements （HFSE） and heavy rare earth elements （HREE）， the presence of biotite within these I-type granites， together with their low zircon saturation temperatures （731–779 °C）， suggest that they were likely derived from a hydrous source formed by dehydration melting of mica-bearing， medium- to high-K metabasaltic rocks. Our zircon U-Pb dating results indicate that the Kumtor granite intruded at 293 ± 1.7 Ma， which is consistent with the age range of other Middle Tien-Shan granitoids. The zircon Hf isotopic composition is εHf（t）= –7.56 to –5.05， indicating an ancient （1.39 to 1.52 Ga） crustal origin. Petrographical， geochemical and geochronological data indicate that the Kumtor granite is similar to leuco-granites of the Terekty complex. Our results indicate that the Kumtor granite was emplaced in the early Permian in a post-collision setting and may have temporal and genetic relationships with gold mineralization.

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Insight of enriched basalts into the nature and evolution of mantle lithosphere beneath craton margins

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Science China Earth Sciences 2024年第10期67卷 3128-3142页

作者： Hong-Kun DAI Jianping ZHENG Qing XIONG Linlin HU Xiang ZHOU State key laboratory of Geological Processes and Mineral Resources School of Earth Sciences China University of Geosciences

Refractory lithospheric deep roots are the cornerstone for the prolonged stability of cratons and mantle xenoliths are normally the key targets for study on the evolution of such deep roots. In regions with few mantle xenoliths, the basalts enriched in radiogenic isotopic compositions due to marked lithospheric mantle contribution are crucial to unmask the lithospheric mantle evolution based on a comprehensive study involving petrology, geochemistry and thermodynamic modelling. Here, the Early Cretaceous basalts from the northwest North China Craton with few mantle xenoliths are taken as an example to show the significance of enriched basalts on the study of lithospheric mantle. These basalts are characterized by high silica and alkali contents（SiO2=45.8–59.8 wt.%, K2O+Na2O=4.81–9.88 wt.%）, arc-type trace-element patterns and enriched radiogenic isotope compositions(e.g., εNd=-2.64–-12.88,87Sr/86Sr=0.7063–0.7093). The TiO2and FeO（total） contents are higher than those of natural and experimental melts from refractory mantle peridotite but comparable to those of partial melts of fertile mantle *** high contents of fluid-loving elements（e.g., Rb and Ba） suggest source metasomatism by aqueous fluids. Combined with thermodynamic modelling and regional tectonic history, these enriched basalts likely record simultaneous decompression melting of asthenosphere and low-extent melting of thin and fertile lithospheric mantle fluxed by aqueous fluids from the subducted Paleo-Asian oceanic slab. The newly unmasked lithospheric mantle under the western NCC contrasts with the coeval thick and refractory one supporting the eastern NCC, and highlights that the craton destruction, especially the loss of its ancient refractory mantle root, should take place in a diachronous manner related to the craton-girded subduction episodes. Our study illustrates the potential of enriched basalts to recover the nature and evolution of mantle lithosphere beneath craton margins and associated

关键词： Enriched basalts Lithospheric mantle Northwest North China Craton Tectonic histories Early Cretaceous

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The Origin of Mesozoic A-type Granitoids,Fujian Province,Southeast China:Insights from Geochronology,Mineralogy and geochemistry

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Acta Geologica Sinica(English Edition) 2024年第3期98卷 630-640页

作者： XIE Qifeng DONG Yunpeng CAI Yuanfeng ZHAI Mingguo XIAO Aifang ZHANG Hong Zijin School of Geology and Mining Fuzhou UniversityFuzhou 350108China State key laboratory of Continental Dynamics Northwest UniversityXi’an 710069China State key laboratory for Mineral Deposits Research Nanjing UniversityNanjing 210023China State key laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China

The magma sources,origins and precise forming ages of the miarolite from Qishan and Kuiqi intrusions are still *** results reveal that,miarolites from the Qishan and Kuiqi intrusions yield crystallization ages of~101 and~98 Ma,and they have a high formation temperature(~910℃)and low oxygen fugacity value,indicating crystallization condition at low pressure in the upper crust with temperature of 678℃.The Qishan and Kuiqi miarolites are characterized by enrichment in SiO_(2) and high-K alkali,depletion in Ca and Mg,and belong to the high-K weak peraluminous rock *** samples are enriched in HFSEs(i.e.,Ta,Zr and Hf)and LILEs(i.e.,Ba,P and Sr),depleted in Ba and Sr with the negative anomaly of *** the primitive mantle normalized trace element spider diagram,the samples show a right-inclined‘seagull-type’pattern,combined the ratios of(La/Yb)_(N),10000×Al/Ga,Rb/Nb and Nb/Ta etc.,they were proved to be alkaline A-type *** the characterize of the trace elements,they were derived from clay-rich source accompanied pelite melting,and subjected to K-feldspar crystallization *** values of ε_(Hf)(t)and tDM2 are distributed in the range of-2.8 to 3.3 with~1.2 Ga,and-6.0 to 4.0 with~1.2 Ga,revealing that they were generated from the Mesoproterozoic Cathaysia basement *** comprehensive research reveals the Kuiqi and Qishan intrusions derived from crust-mantle mixing and partial melting of the crust,respectively,resulting from lithospheric extension generated by the Paleo-Pacific Plate subducted into the European-Asian Plate.

关键词： A-type granitoid geochronology extension subduction Mesozoic Southeast China

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elemental Compositions of Clinopyroxenes from Southern Okinawa Trough Basalt:Implications for Magmatism and Structural Environment in an Initial Back-Arc Basin

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Journal of Ocean University of China 2024年第3期23卷 643-653页

作者： GUO Kun ZHAI Shikui FAN Di ZHANG Xia ZHANG Yu ZHU Zhimin Laoshan laboratory Qingdao 266237China key laboratory of Submarine Geosciences and Prospecting Techniques Ministry of EducationCollege of Marine GeosciencesOcean University of ChinaQingdao 266100China key laboratory of Submarine Geosciences&Second Institute of Oceanography Ministry of Natural ResourcesHangzhou 310012China

The major and trace elemental compositions of clinopyroxene from basalt were used to characterize the nature of the primitive magma and structural environment beneath the southern Okinawa Trough(SOT),which is an initial back-arc basin at a continental *** clinopyroxenes in the basalt were augite with variable Mg^(#)contents(73.37-78.22).The regular variations in major oxide contents(i.e.,CaO,FeO,TiO_(2),and Cr)with decreasing Mg#implied that the clinopyroxenes evolved from being enriched in Mg,Ca,and Cr to being enriched in Fe and *** clinopyroxenes had relatively low rare earth element concentrations(7.51×10^(-6) to 12.68×10^(-6))and negative Eu anomalies(δEu=0.67-0.95).The Kd_(cpx) values of clinopyroxenes(0.2-0.26),which were used to examine whether the clinopyroxene was equilibrated with its host basalt,demonstrate that these clinopyroxene phenocrysts were not captured crystals but were instead produced by crystallization differentiation of the *** calculated clinopyroxene crystallization temperatures showed a narrow range of 990-1061℃,and their crystallization pressures ranged from 2.0 to 3.2 *** geochemistry features of these clinopyroxenes indicated that the parent magma belonged to the subalkaline tholeiitic magma series and suggested that the magma experienced crystallization differentiation of olivine,plagioclase,and clinopyroxene,where the crystallization of plagioclase occurred earlier than that of *** with geophysical data,this research on primitive magma and its crystallization differentiation from clinopyroxene indicates that the SOT is in the stage of‘seafloor spreading’and that basaltic rocks produced from tholeiitic magma represent the generation of oceanic crust.

关键词： trace elements clinopyroxenes southern Okinawa Trough seafloor spreading back-arc basin

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The Weixi High-silica Granitoids in the Central Sanjiang Orogenic Belt,Southwest China:Implications for Growth of the Continental Crust

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Acta Geologica Sinica(English Edition) 2024年第3期98卷 641-656页

作者： WANG Qiuyu CHEN Shouming ZHANG Hongrui LI Saisai SinoProbe laboratory Institute of GeologyChinese Academy of Geological SciencesBeijing 100037China Guangxi key laboratory of Hidden Metallic Ore Deposit Exploration GuilinGuangxi 541004China

High-silica granitoids record the formation and evolution of the continental crust.A new intrusive complex has been recognized among silicic volcanic rocks of the Weixi arc,Southwest *** intrusions consist of granites,granitic porphyries,and *** U-Pb age data indicate that the Weixi granitoids formed at 248-240 Ma and were coeval with silicic volcanic rocks of the Weixi *** Weixi granitoids are enriched in Rb,Th,and U,depleted in Ba,Sr,Nb,Ta,and Ti,and have high light/heavy rare earth element ratios and slightly negative Eu *** Weixi granitoids have negative ε_(Nd)(t)values(-9.8 to-7.8)and negative zircon ε_(Hf)(t)values(-12.02 to-5.11).The geochemical and isotopic features suggest the Weixi granitoids were derived by partial melting of ancient crustal *** Weixi granitoids and silicic volcanic rocks were derived from the same magma by crystal accumulation and melt extraction,respectively,and they record the formation of a continental arc in the central Sanjiang orogenic belt.

关键词： granitoids geochemistry crystal accumulation continental crust Sanjiang orogen

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Effects of melt percolation on the Re-Os systematics of continental mantle lithosphere: A case study of spinel peridotite xenoliths from Heilongjiang, NE China

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Science China Earth Sciences 2012年第6期55卷 949-965页

作者： YU SongYue SONG XieYan XU YiGang CHEN LieMeng LI Jie State key laboratory of Ore Deposit geochemistry Institute of Geochemistry Chinese Academy of Seiences Guiyang 550002 China key laboratory of lsotope Geochronology and geochemistry Guangzhou Institute ~Geochemistry Chinese Academy of Sciences Guangzhou 510640 China

Os isotope ratios of mantle peridotites have been considered to be largely immune to recent melt-rock interaction. However, Os isotope ratios and PGE (Platinum group elements) concentrations of the Yong'an xenoliths have been significantly modified by melt percolation, and are not suitable for determining the formation age of lithosphere mantle in Yong'an. In this study, the Yong'an spinel peridotite xenoliths are divided into two groups: N-Type and E-Type. The N-Type group including cpx (clinopyroxene)-poor lherzolite and harzburgite, shows a large variation of Cr#(sp) (13.2-48) and sulfur contents (from 171 ppm to below detection limit), whereas the E-Type peridotites are mainly refractory harzburgites and are characterized by high Cr#(sp) (35.3-42.2) and overall low sulfur contents (below 51 ppm). Both types show similar major and REE (rare earth element) patterns. Furthermore, the N-Type peridotites display a restricted range of iridium-group PGE (IPGE), Os/Ir and Ru/Ir ratios (Os/Ir = 0.64-1.12, Ru/Ir = 1.52-1.79) and variable palladium-group PGE (PPGE) contents (3.4-14.9 ppb), whereas the E-Type peridotites show a large variation of Os/Ir and Ru/Ir ratios (Os/Ir = 0.33-0.84, Ru/Ir = 0.94-1.6), and a restricted range of PPGE (4.3-6.9 ppb). 187Os/188Os ratios of E-Type peridotites are higher than those of N-Type peridotites at comparable fertility levels. These results suggest that N-Type peridotites may have been overprinted by metasomatism via small melt fractions, in which the percolation of the volatile-rich, small melt fractions only resulted in LILE (large ion lithophile element) enrichment of clinopyroxene, and their whole rock PGE contents and Re-Os isotope values were little changed. Moreover, E-Type peridotites may have been modified by melt-rock reaction involving relatively large melt fractions, which may result in the formation of secondary cpx and olivine and the removal of IPGE-bearing minerals such as Ru-Os-(Ir) alloys or laurite, followed by pre

关键词： peridotites highly siderophile element melt percolation sulfides NE China

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