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Enhanced High-Temperature Energy Storage Performance of All-Organic Composite Dielectric via Constructing Fiber-Reinforced Structure

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Energy & Environmental Materials 2024年第2期7卷 303-311页

作者： Mengjia Feng Yu Feng Changhai Zhang Tiandong Zhang Xu Tong Qiang Gao Qingguo Chen Qingguo Chi key laboratory of Engineering Dielectrics and Its Application Ministry of Education Harbin University of Science and Technology School of Electrical and Electronic Engineering Harbin University of Science and Technology

Optimizing the high-temperature energy storage characteristics of energy storage dielectrics is of great significance for the development of pulsed power devices and power control *** a polymer with a higher glass transition temperature（Tg） as the matrix is one of the effective ways to increase the upper limit of the polymer operating ***,current high-Tgpolymers have limitations,and it is difficult to meet the demand for high-temperature energy storage dielectrics with only one *** example,polyetherimide has high-energy storage efficiency,but low breakdown strength at high *** has high corona resistance,but low high-temperature energy storage *** this work,combining the advantages of two polymer,a novel high-Tgpolymer fiberreinforced microstructure is *** is designed as extremely fine fibers distributed in the composite dielectric,which will facilitate the reduction of high-temperature conductivity loss for *** the same time,due to the high-temperature resistance and corona resistance of polyimide,the high-temperature breakdown strength of the composite dielectric is *** the polyimide content with the best hightemperature energy storage characteristics is determined,molecular semiconductors（ITIC） are blended into the polyimide fibers to further improve the high-temperature ***,excellent hightemperature energy storage properties are *** 0.25 vol% ITICpolyimide/polyetherimide composite exhibits high-energy density and high discharge efficiency at 150℃(2.9 J cm-3,90%) and 180℃(2.16 J cm-3,90%).This work provides a scalable design idea for high-performance allorganic high-temperature energy storage dielectrics.

关键词： all-organic energy storage density high-temperature high-temperature breakdown strength

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Toughening additive manufactured Zr-based bulk metallic glass composites by martensite phase transformation

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Journal of Materials science & technology 2024年第3期170卷 95-102页

作者： Pengcheng Zhang Cheng Zhang Jie Pan Di Ouyang Lin Liu State key laboratory of Materials Processing and Die&Mould technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Additive manufacturing technology based on laser powder bed fusion(LPBF)offers a novel approach for fabricating bulk metallic glass(BMG)products without restriction in size and ***,the BMGs prepared by LPBF usually suffered from less plasticity and poorer fracture toughness as compared to their cast counterparts due to partial crystallization in heat-affected zones(HAZs).Since crystallization in HAZs is hard to avoid completely in LPBF BMGs,it is desirable to design a suitable alloy system,in which only ductile crystalline phase,instead of brittle intermetallics,is formed in *** unique structure could effectively increase the toughness/plasticity of the LPBF *** achieve this goal,a quaternary BMG system with a composition of Zr_(47.5)Cu_(45.5)Al_(5)Co_(2)is adopted and subjected to *** is found that nearly a single phase of B_(2)-ZrCu is precipitated in HAZs,while a fully amorphous phase is formed in molten pools(MPs).This B_(2)phase reinforced BMG composite exhibits excellent mechanical properties with enhanced plasticity and ***,it is easy to modulate the mechanical properties by altering the amount of the B_(2)phase via adjusting the laser energy ***,the best combination of strength,plasticity,and notch toughness is obtained in the BMG composite containing 27.4%B_(2)phase and 72.6%amorphous phase,which exhibits yield strength(σ_(s))of 1423 MPa,plastic strain(ε_(p))of 4.65%,and notch toughness(K_(q))of 53.9 MPa m 1/***,a notable strain-hardening is also *** improvement of plasticity/toughness and appearance of strain-hardening behavior are mainly due to the martensite phase transformation from the B_(2)phase to the Cm phase during plastic deformation(i.e.,the phase transformation-induced plasticity effect).The current work provides a guide for making advanced BMGs and BMG composites by additive manufacturing.

关键词： Laser powder bed fusion Bulk metallic glass composites Phase transformation-induced plasticity Deformation mechanism

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Characteristics and Genesis of Acid Drainage Contamination from a Rock Tunneling Project Site

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Journal of Earth science 2024年第1期35卷 190-200页

作者： Yanyun Li Zejiao Luo Shihua Qi Hubei key laboratory of Yangtze River Basin Environmental aquatic science School of Environmental StudiesChina University of GeosciencesWuhan 430078China State key laboratory of Biogeology and Environmental Geology China University of GeosciencesWuhan 430078China

While acid mine drainage(AMD)issues have become a topic of global concern,few studies have focused on acid drainage problems of non-mining *** conducted field research and a series of laboratory experiments to investigate the characteristics,release processes and formation of acid drainage *** rock samples and adjacent surface water,groundwater,soil and sediment samples were collected at a railway tunnel construction site in central China,and various parameters,such as the p H,mineral ion concentrations,and heavy metal concentrations,were *** on the measured concentrations,surface water and sediments were seriously contaminated by acids,sulfate salts and heavy *** in surface water showed a decreasing tendency as the distance from the spoils increased,while that in sediments showed a greater influence of coprecipitation and adsorption processes of heavy metal *** eluviation experiments of three rock samples indicated that R2(silty fine sandstone)was the most likely major acid drainage *** ferrooxidans was cultured and isolated from contaminated water to study the oxidation conditions during the release *** significant release of acid drainage when air and bacteria were both in the culture container suggested that oxygen and bacteria were necessary to produce acid drainage from spoils.

关键词： acid mine drainage heavy metals leaching oxidation

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Design and Implementation of a Time Synchronization Method for UOWC Networks

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Journal of Communications and Information Networks 2024年第1期9卷 56-63页

作者： Weijie Liu Jingyi Zhang Nuo Huang Zhengyuan Xu CAS key laboratory of Wireless-Optical Communications School of Information Science and TechnologyUniversity of Science and Technology of ChinaHefei 230027China

Underwater optical wireless communication (UOWC) technology facilitates high-speed data transmission among multiple nodes in underwater networks. Nevertheless, the absence of a common clock poses a challenge to achieving systematic and reliable access for multiple nodes within these networks. This paper presents a time synchronization method for UOWC networks to ensure the successful execution of the media access control (MAC) protocol. In this method, the node obtains timestamps by exchanging messages with the optical access point (OAP). Subsequently, the node calculates the clock drift relative to the OAP and the propagation time,ensuring that transmitted data packets can arrive approximately at the time specified by the OAP. To validate the effect of the proposed method, an experimental UOWC prototype, including the OAP and nodes, is implemented using field programmable gate array (FPGA). The experimental results demonstrate that the maximum difference between the actual arrival times of two data packets that are expected to reach the OAP simultaneously according to the MAC protocol meets the requirements of the quasi-synchronous code division multiple access (QS-CDMA) system, thereby substantiating the effectiveness of this synchronization method.

关键词： UOWC time synchronization MAC FPGA QS-CDMA

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3D Foam-Based MXene Architectures:Structural and Electrolytic Engineering for Advanced Potassium-Ion Storage

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Energy & Environmental Materials 2024年第4期7卷 64-73页

作者： Peng Zhang Yanmeng Peng Qizhen Zhu Razium Ali Soomro Ning Sun Bin Xu State key laboratory of Organic-Inorganic Composites Beijing Key Laboratory of Electrochemical Process and Technology for Materials Beijing University of Chemical Technology Beijing Advanced Innovation Centre for Soft Matter science and Engineering Beijing University of Chemical Technology

MXenes are emerging rapidly as promising electrode materials for energy storage due to their high electronic conductivity and rich surface chemistry,but their potassium storage performance is unsatisfactory because of... 详细信息

关键词： 3D foam-like scaffold electrolyte chemistry electrostatic neutralization MXene potassium-ion batteries

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Polaron interfacial entropy as a route to high thermoelectric performance in DAE-doped PEDOT:PSS films

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National science Review 2024年第3期11卷 259-270页

作者： Jiajia Zhang Caichao Ye Genwang Wei Liang Guo Yuhang Cai Zhi Li Xinzhi Wu Fangyi Sun Qikai Li Yupeng Wang Huan Li Yuchen Li Shuaihua Wang Wei Xu Xuefeng Guo Wenqing Zhang Weishu Liu Department of Materials science and Engineering Southern University of Science and Technology Academy for Advanced Interdisciplinary Studies and Guangdong Provincial key laboratory of Computational science and Material Design Southern University of Science and Technology Department of Mechanical and Energy Engineering Southern University of Science and Technology Beijing National laboratory for Molecular sciences Key Laboratory of Organic Solids Institute of Chemistry Chinese Academy of Sciences College of Chemistry and Molecular Engineering National Biomedical Imaging Centre Peking University Guangdong Provincial key laboratory of Functional Oxide Materials and Devices Southern University of Science and Technology

Enhancing the thermoelectric transport properties of conductive polymer materials has been a long-term challenge, in spite of the success seen with molecular doping strategies. However, the strong coupling between the thermopower and the electrical conductivity limits thermoelectric performance. Here, we use polaron interfacial occupied entropy engineering to break through this intercoupling for a PEDOT:PSS(poly（3,4-ethylenedioxythiophene）-poly（4-styrenesulfonate）) thin film by using photochromic diarylethene（DAE） dopants coupled with UV-light modulation. With a 10-fold enhancement of the thermopower from 13.5 μV K-1to 135.4 μV K-1and almost unchanged electrical conductivity, the DAE-doped PEDOT:PSS thin film achieved an extremely high power factor of 521.28 μW m-1K-2from an original value of 6.78 μW m-1K-2. The thermopower was positively correlated with the UV-light intensity but decreased with increasing temperature, indicating resonant coupling between the planar closed DAE molecule and PEDOT. Both the experiments and theoretical calculations consistently confirmed the formation of an interface state due to this resonant coupling. Interfacial entropy engineering of polarons could play a critical role in enhancing the thermoelectric performance of the organic film.

关键词： thermoelectric PEDOT: PSS interfacial occupied entropy resonant coupling UV-light modulation

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Constructing arbitrary self-similar Bessel-like beams via transverse-longitudinal mapping

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Chinese Optics Letters 2024年第2期22卷 167-171页

作者：李岩珂邹昱郭兆金刘圣李鹏魏冰妍温丹丹赵建林 key laboratory of Light Field Manipulation and Information Acquisition Ministry of Industry and Information TechnologyShaanxi Key Laboratory of Optical Information TechnologySchool of Physical Science and TechnologyNorthwestern Polytechnical UniversityXi’an 710129China

Based on the transverse-longitudinal mapping of Bessel beams,we propose a simple method to construct a self-similar Bessel-like beam whose transverse profile maintains a stretched form during ***,the propagatingvariant width of this beam can be flexibly *** experimentally demonstrate three types of self-similar Bessellike beams whose width variations are linear,piecewise,and period functions of propagation distance,*** experimental results match well with the theoretical *** also demonstrate that our approach enables the generation of self-similar higher-order vortex Bessel-like beams.

关键词： Bessel beams self-similarity transverse-longitudinal mapping

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Engineering oxygen vacancies on Tb-doped ceria supported Pt catalyst for hydrogen production through steam reforming of long-chain hydrocarbon fuels

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Chinese Journal of Chemical Engineering 2024年第4期68卷 181-192页

作者： Zhourong Xiao Changxuan Zhang Peng Li Desong Wang Xiangwen Zhang Li Wang Jijun Zou Guozhu Li State key laboratory of Metastable Materials science and technology(MMST) Hebei Key Laboratory of Applied ChemistryCollege of Environmental and Chemical EngineeringYanshan UniversityQinhuangdao 066004China key laboratory for Green Chemical technology of Ministry of Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China

Steam reforming of long-chain hydrocarbon fuels for hydrogen production has received great attention for thermal management of the hypersonic vehicle and fuel-cell *** this work,Pt catalysts supported on CeO_(2)and Tb-doped CeO_(2)were prepared by a precipitation *** physical structure and chemical properties of the as-prepared catalysts were characterized by powder X-ray diffraction,scanning electron microscopy,transmission electron microscopy,Raman spectroscopy,H_(2)temperature programmed reduction,and X-ray photoelectron *** results show that Tb-doped CeO_(2)supported Pt possesses abundant surface oxygen vacancies,good inhibition of ceria sintering,and strong metal-support interaction compared with CeO_(2)supported *** catalytic performance of hydrogen production via steam reforming of long-chain hydrocarbon fuels(n-dodecane)was *** with 2Pt/CeO_(2),2Pt/Ce_(0.9)Tb_(0.1)O_(2),and 2Pt/Ce_(0.5)Tb_(0.5)O_(2),the 2Pt/Ce_(0.7)Tb_(0.3)O_(2)has higher activity and stability for hydrogen production,on which the conversion of n-dodecane was maintained at about 53.2%after 600 min reaction under 700℃at liquid space velocity of 9 ml·g^(-1)·h^(-1).2Pt/CeO_(2)rapidly deactivated,the conversion of n-dodecane was reduced to only 41.6%after 600 min.

关键词： Steam reforming n-Dodecane Hydrogen production Pt-based catalyst Oxygen vacancy CeO_(2)

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Recent progress in visualization and digitization of coherent transformation structures and application in high-strength steel

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International Journal of Minerals,Metallurgy and Materials 2024年第6期31卷 1298-1310页

作者： Xuelin Wang Zhenjia Xie Xiucheng Li Chengjia Shang Collaborative Innovation Center of Steel technology University of Science and Technology BeijingBeijing 100083China State key laboratory for Advanced Metals and Materials University of Science and Technology BeijingBeijing 100083China Yangjiang Branch Guangdong Laboratory for Materials Science and Technology(Yangjiang Advanced Alloys Laboratory)Yangjiang 529500China

High-strength steels are mainly composed of medium-or low-temperature microstructures,such as bainite or martensite,with coherent transformation *** type of microstructure has a high density of dislocations and fine crystallographic structural units,which ease the coordinated matching of high strength,toughness,and ***,given its excellent welding perform-ance,high-strength steel has been widely used in major engineering constructions,such as pipelines,ships,and ***,visual-ization and digitization of the effective units of these coherent transformation structures using traditional methods(optical microscopy and scanning electron microscopy)is difficult due to their complex ***,the establishment of quantitative relationships with macroscopic mechanical properties and key process parameters presents additional *** article reviews the latest progress in microstructural visualization and digitization of high-strength steel,with a focus on the application of crystallographic methods in the development of high-strength steel plates and *** obtained the crystallographic data(Euler angle)of the transformed microstruc-tures through electron back-scattering diffraction and combined them with the calculation of inverse transformation from bainite or martensite to austenite to determine the reconstruction of high-temperature parent austenite and orientation relationship(OR)during con-tinuous cooling ***,visualization of crystallographic packets,blocks,and variants based on actual OR and digit-ization of various grain boundaries can be effectively completed to establish quantitative relationships with alloy composition and key process parameters,thereby providing reverse design guidance for the development of high-strength steel.

关键词： high-strength steel microstructure visualization digitization quantification mechanical properties

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Cycling performance of layered oxide cathode materials for sodium-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1720-1744页

作者： Jinpin Wu Junhang Tian Xueyi Sun Weidong Zhuang School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing 100083China State key laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China Beijing key laboratory for Green Recovery and Extraction of Rare and Precious Metals University of Science and Technology BeijingBeijing 100083China

Layered oxide is a promising cathode material for sodium-ion batteries because of its high-capacity,high operating voltage,and simple *** performance is an important criterion for evaluating the application prospects of ***,facing challenges,including phase transitions,ambient stability,side reactions,and irreversible anionic oxygen activity,the cycling performance of layered oxide cathode materials still cannot meet the application ***,this review proposes several strategies to address these ***,bulk doping is introduced from three aspects:cationic single doping,anionic single doping,and multi-ion ***,homogeneous surface coating and concentration gradient modification are *** addition,methods such as mixed structure design,particle engineering,high-entropy material construction,and integrated modification are ***,a summary and outlook provide a new horizon for developing and modifying layered oxide cathode materials.

关键词： sodium-ion battery layered oxide materials cycling performance bulking doping surface coating concentration gradient mixed structure high-entropy

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