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Energy & Environmental materials 2024年第1期7卷 5-12页

作者： Yang Guo Zhaoqing Jin Jianhao Lu Zilong Wang Zihao Song Anbang Wang Weikun Wang Yaqin Huang Beijing key laboratory of Electrochemical Process and Technology for materials Key Laboratory of Biomedical Materials of Natural Macromolecules Ministry of Education Beijing University of Chemical Technology Research Institute of Chemical Defense Beijing Key Laboratory of Advanced Chemical Energy Storage Technology and Materials

The sluggish kinetics of complicated multiphase conversions and the severe shuttling effect of lithium polysulfides（LiPSs） significantly hinder the applications of Li-S battery,which is one of the most promising candidates for the next-generation energy storage ***,a bifunctional electrocatalyst,indium phthalocyanine self-assembled with carbon nanotubes（InPc@CNT） composite material,is proposed to promote the conversion kinetics of both reduction and oxidation processes,demonstrating a bidirectional catalytic effect on both nucleation and dissolution of Li2S species.

关键词： bidirectional catalyst indium phthalocyanine lithium−sulfur batteries pouch cells

The deteriorated degradation resistance of Mg alloy microtubes for vascular stent under the coupling effect of radial compressive stress and dynamic medium

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Journal of Magnesium and Alloys 2024年第2期12卷 573-585页

作者： Mengyao Liu Yabo Zhang Qingyuan Zhang Yan Wang Di Mei Yufeng Sun Liguo Wang Shijie Zhu Shaokang Guan School of materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China Henan key laboratory of advanced Magnesium Alloys Zhengzhou 450002China key laboratory of advanced materials Processing&Mold ministry of education Zhengzhou 450002China

The degradation of Mg alloys relates to the service performance of Mg alloy biodegradable *** order to investigate the degradation behavior of Mg alloys as vascular stent materials in the near service environment,the hot-extruded fine-grained Mg-Zn-Y-Nd alloy microtubes,which are employed to manufacture vascular stents,were tested under radial compressive stress in the dynamic Hanks'Balanced Salt Solution(HBSS).The results revealed that the high flow rate accelerates the degradation of Mg alloy microtubes and its degradation is sensitive to radial compressive *** results contribute to understanding the service performance of Mg alloys as vascular stent materials.

关键词： Mg alloy Microtubes Degradation behavior Radial compressive stress Dynamic conditions

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Recent progress in photocatalytic NAD(P)H regeneration for photocatalytic-enzymatic-coupling system

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Frontiers of Chemical Science and Engineering 2024年第4期18卷 1-24页

作者： Wei Lan Maodi Wang Huicong Dai Qihua Yang key laboratory of the ministry of education for advanced Catalysis materials Zhejiang Key Laboratory for Reactive Chemistry on Solid SurfacesInstitute of Physical ChemistryZhejiang Normal UniversityJinhua 321004China

The enzymatic redox reactions in natural photosynthesis rely much on the participation of cofactors,with reduced nicotinamide adenine dinucleotide/nicotinamide adenine dinucleotide phosphate(NADH/NADPH)or their oxidized form(NAD+/NADP+)as an important redox *** photocatalytic regeneration of expensive and unstable NADH/NADPH in vitro is an important process in enzymatic reduction and has attracted much research *** different types of photocatalysts have been developed for photocatalytic NADH/NADPH regeneration,the efficiency is still relatively *** elucidate the key factors affecting the performance of photocatalytic NADH/NADPH regeneration is helpful to rationally design the photocatalyst and improve the photocatalytic *** this paper,we overview the recent progress in photocatalytic NADH/NADPH regeneration with the focus on the strategies to improve the visible light adsorption,the charge separation and migration efficiency,as well as the surface reaction,which jointly determine the overall photocatalytic regeneration *** potential development of photocatalytic NADH/NADPH regeneration and photocatalyticenzymatic-coupling system is prospected finally.

关键词： photocatalytic-enzymatic coupling NAD(P)H regeneration photocatalysis efficiency

Precipitating thermally reinforcement phase in aluminum alloys for enhanced strength at 400℃

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Journal of materials Science & Technology 2024年第5期172卷 71-82页

作者： Xiang Su Yuan Lei Yang Chen Hongjie Qu Zhixiang Qi Gong Zheng Xu Liu Henggao Xiang Guang Chen National key laboratory of advanced Casting technologies MIIT Key Laboratory of Advanced Metallic and Intermetallic Materials TechnologyEngineering Research Center of Materials Behavior and DesignMinistry of EducationNanjing University of Science and TechnologyNanjing 210094China School of Aviation and Mechanical Engineering Changzhou Institute of TechnologyChangzhou 213032China

Heat-resistant aluminum alloys are widely used in aerospace and automotive fields for manufacturing hot components due to their advantages in lightweight design and energy ***,the high-temperature strength of existing cast aluminum alloys is always limited to about 100 MPa at 350℃due to coarsening and transformation of strengthening ***,we reveal that the yield strength and ultimate tensile strength of the T6 state Al-8.4Cu-2.3Ce-1.0Mn-0.5Ni-0.2Zr alloy at 400◦C increase by 34%and 44%after re-aging at 300℃for 100 h,and its thermal strength exhibits distinguished ad-vantage over traditional heat-resistant aluminum *** enhanced elevated-temperature strength is attributed to the reprecipitation of the Ni-bearing T-Al_(20)Cu_(2)Mn_(3)phase,whose number density increases over one *** significant segregation of Ni,Ce,and Zr elements at the interfaces helps improve the thermal stability of the T *** thermostable T phase effectively strengthens the matrix by in-hibiting dislocation ***,a highly interconnected 3D intermetallic network along the grain boundaries can still remain after long-term re-aging at 300℃,which is conducive to imposing a drag on the grain boundaries at high *** finding offers a viable route for enhancing the elevated-temperature strength of heat-resistant aluminum alloys,which could provide expanded opportunities for higher-temperature applications.

关键词： Aluminum alloys Precipitation Thermally reinforcement phase Re-aging treatment High-temperature strength

Emerging probing perspective of two-dimensional materials physics:terahertz emission spectroscopy

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Light(Science & Applications) 2024年第7期13卷 1278-1298页

作者： Yifei Wu Yuqi Wang Di Bao Xiaonan Deng Simian Zhang Lin Yu-chun Shengxian Ke Jianing Liu Yingjie Liu Zeli Wang Pingren Ham Andrew Hanna Jiaming Pan Xinyue Hu Zhengcao Li Ji Zhou Chen Wang State key laboratory of New Ceramics and Fine Processing Key Laboratory of Advanced Materials of Ministry of EducationSchool of Materials Science and EngineeringTsinghua University100084 BeijingChina Beijing advanced Innovation Center for Integrated Circuits 100084 BeijingChina

Terahertz(THz)emission spectroscopy(TES)has emerged as a highly effective and versatile technique for investigating the photoelectric properties of diverse materials and nonlinear physical processes in the past few ***,research on two-dimensional(2D)materials has experienced substantial growth due to their atomically thin structures,exceptional mechanical and optoelectronic properties,and the potential for applications in flexible electronics,sensing,and ***,these materials offer advantages such as tunable bandgap,high carrier mobility,wideband optical absorption,and relatively short carrier *** applying TES to investigate the 2D materials,their interfaces and heterostructures,rich information about the interplay among photons,charges,phonons and spins can be unfolded,which provides fundamental understanding for future *** it is timely to review the nonlinear processes underlying THz emission in 2D materials including optical rectification,photon-drag,high-order harmonic generation and spin-to-charge conversion,showcasing the rich diversity of the TES employed to unravel the complex nature of these *** applications based on THz emissions,such as THz lasers,ultrafast imaging and biosensors,are also *** further,we analyzed the unique advantages of spintronic terahertz emitters and the future technological advancements in the development of new THz generation mechanisms leading to advanced THz sources characterized by wide bandwidth,high power and integration,suitable for industrial and commercial *** continuous advancement and integration of TES with the study of 2D materials and heterostructures promise to revolutionize research in different areas,including basic materials physics,novel optoelectronic devices,and chips for post-Moore’s era.

关键词： optoelectronic versatile exceptional

High performance and stable pure-blue quasi-2D perovskite light-emitting diodes by multifunctional zwitterionic passivation engineering

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advanced Photonics 2024年第2期6卷 32-40页

作者： Chao Shen Shuyan Fang Jibin Zhang Xiangfei Liang Chenhui Su Jian Qing Wanzhu Cai Yunhan Luo Renqiang Yang Lintao Hou Jinan University College of Physics and Optical Engineering Guangdong Provincial Engineering Technology Research Center of Vacuum Coating Technologies and New Energy Materials Guangzhou Key Laboratory of Vacuum Coating Technologies and New Energy Materials Jinan University College of Physics and Optical Engineering Guangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications Zhengzhou University School of Physics and Microelectronics Key Laboratory of Materials Physics of Ministry of Education Jinan University Key Laboratory of Optoelectronic Information and Sensing Technologies of Guangdong Higher Education Institutes Jianghan University School of Optoelectronic Materials and Technology Key Laboratory of Optoelectronic Chemical Materials and Devices of Ministry of Education

Despite the rapid advances of red and green perovskite light-emitting diodes（Pe LEDs）, achieving high brightness with high external quantum efficiency（EQE） remains a challenge for the pure-blue Pe LEDs,which greatly hinders their practical applications, such as white-light illumination and in optical communication as a high-speed and low-loss light source. Herein, we report a high-performance pure-blue Pe LED based on mixed-halide quasi-2D perovskites incorporated with a zwitterionic molecule of 3-（benzyldimethylammonio）propanesulfonate（3-BAS）. Experimental and density functional theory analysis reveals that 3-BAS can simultaneously eliminate non-radiative recombination loss, suppress halide migration, and regulate phase distribution for smoothing energy transfer in the mixed-halide quasi-2D perovskites, leading to the final perovskites with high photoluminescence quantum yield and robust spectrum stability. Thus, the highperformance pure-blue Pe LED with a recorded brightness with 1806 cd m;-2;and a relative higher EQE of 9.25% is achieved, which is successfully demonstrated in a visible light communication system for voice signal transmission. We pave the way for achieving highly efficient pure-blue Pe LEDs with great application potential in future optical communication networks.

关键词： pure-blue PeLEDs quasi-2D perovskite zwitterionic additive visible light communication

Construction of ternary PEG200-based DESs lubrication systems via tailoring tribo-chemistry

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Friction 2024年第4期12卷 655-669页

作者： Yuting LI Songyu LAN Yazhou LIU Cheng CAO Zicheng TANG Deyin DENG Fuyuan LIU Hao LI Xiaoqiang FAN Minhao ZHU key laboratory of advanced technologies of materials(ministry of education) School of Materials Science and EngineeringSouthwest Jiaotong UniversityChengdu 610031China Tribology Research Institute School of Mechanical EngineeringSouthwest Jiaotong UniversityChengdu 610031China

Designing novel lubricants with easily customized structures,devisable compositions,and simple and economic synthesis over traditional lubricants is critical to fulfilling complex applications,prolonging machine lifetime,and saving *** eutectic solvents(DESs),which show tunable composition,adjustable structure,easy fabrication,and environmental friendliness,are promising candidates for variable and complicated lubricants *** promote the use of DESs as lubricants,a series of PEG200-based DESs with active heteroatoms were fabricated to tailor the tribological performance via ***,PEG200/boric acid(BA)DES shows optimal lubrication performance by forming tribo-chemical reaction film composited of B2O3,iron oxides,and FeOOH,and PEG200/thiourea(TU)DES displays abrasive wear-reducing property by producing FeS tribo-chemical *** the excellent abrasive wear-resistance of PEG200/TU DES and friction reduction of PEG200/BA DES,ternary PEG200/BA/TU DESs,composited of PEG200/TU DES and PEG200/BA DES,are first *** ternary DESs possess superior wettability and thermal stability,which render them potential *** tests of the ternary DESs demonstrate that synergistic lubrication is achieved by forming a transfer film consisting of FexBy,BN,B2O3,and *** FexBy,BN,and B2O3 increase load bearing of the film,and FeS mitigates severe abrasive *** proposed design philosophy of novel DESs as lubricants opens up a unique realm that is unattainable by traditional DESs lubrication mechanisms and provides a platform to design next-generation DESs lubrication systems.

关键词： deep eutectic solvents(DESs) PEG200/boric acid DES PEG200/thiourea DES ternary DESs synergistic lubrication tribo-chemistry

Solvent-free carbon sphere nanofluids towards intelligent lubrication regulation

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Friction 2024年第1期12卷 95-109页

作者： Sheng ZHANG Wen LI Xiaoliang MA Xiaoqiang FAN Minhao ZHU Tribology Research Institute School of Mechanical EngineeringSouthwest Jiaotong UniversityChengdu 610031China key laboratory of advanced technologies of materials Ministry of EducationSchool of Materials Science and EngineeringSouthwest Jiaotong UniversityChengdu 610031China

By simply switching the electrical circuit installed on steel/steel contact,the tribological behaviors of nanofluids(NFs)can be regulated in real time,thereby achieving the desired performance of friction reduction and wear ***,solvent-free carbon spherical nanofluids(C-NFs)were successfully prepared for intelligent lubrication regulation.C-NFs with excellent lubrication performance can immediately reduce the coefficient of friction(COF)despite applying a weak electric potential(1.5 V).Moreover,polyethylene glycol 400(PEG400)containing 5.0 wt%C-NFs remained responsive to electrical stimulation under the intermittent voltage application with an average coefficient of friction(ACOF)reduction of 20.8%over *** intelligent lubrication regulation of C-NFs under an external electric field(EEF)mainly depends on the orderly arranged double-electric adsorption film of ion canopy-adsorbed carbon spheres(CSs).The intermittent electrical application can continuously reinforce the adsorption film and its durability for real-time controlling the sliding ***-stimulation-responsive intelligent lubricants provide a new technical support for realizing intelligent stepless control of devices.

关键词： solvent-free carbon spherical nanofluids(C-NFs) intelligent lubrication regulation lubrication performance adsorption film

Vibration-assisted material damage mechanism:From indentation cracks to scratch cracks

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Chinese Journal of Aeronautics 2024年第8期37卷 527-546页

作者： Bingrui LV Bin LIN Tianyi SUI Chunyan LIU Jinshuo ZHANG Longfei WANG Xuhui CHEN Jingguo ZHOU key laboratory of advanced Ceramics and Machining Technology Ministry of EducationTianjin UniversityTianjin 300072China key laboratory of Mechanism Theory and Equipment Design of ministry of education Tianjin UniversityTianjin 300072China Science and Technology of advanced Functional Composite laboratory Aerospace Research Institute of Materials and Processing TechnologyBeijing 100076China

Vibration-assisted grinding is one of the most promising technologies for manufacturing optical components due to its efficiency and quality ***,the damage and crack propagation mechanisms of materials in vibration-assisted grinding are not well *** order to elucidate the mechanism of abrasive scratching during vibration-assisted grinding,a kinematic model of vibration scratching was *** influence of process parameters on the evolution of vibration scratches to indentation or straight scratches is revealed by displacement metrics and velocity ***,scratch and vibration scratch experiments were performed on quartz glass,and the results showed that the vibration scratch cracks are a combination of indentation cracks and scratch *** scratch cracks change from indentation cracks to scratch cracks as the indenter moves from the entrance to the exit of the workpiece or as the vibration frequency changes from high to low.A vertical vibration scratch stress field model is established for the first time,which reveals that the maximum principal stress and tensile stress distribution is the fundamental cause for inducing the transformation of the vibration scratch cracking *** model provides a theoretical basis for understanding of the mechanism of material damage and crack propagation during vibration-assisted grinding.

关键词： Vibration assisted grinding Indentation Vibration scratch Material removal mechanism Stress field model Crack propagation mechanism

Spontaneous anchoring Cl intoα-Co(OH)_(2) as efficient and stable oxygen reduction electrocatalysts for seawater battery

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Rare Metals 2024年第7期43卷 3074-3083页

作者： Wang Zheng Xue-Rong Zheng Qi Lu Yan-Hui Cao Yang Wang Hai-Peng Fu Jin-Feng Zhang Yi-Da Deng Wen-Bin Hu School of materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin UniversityTianjin 300072China State key laboratory of Marine Resource Utilization in South China Sea School of Materials Science and EngineeringHainan UniversityHaikou 570228China key laboratory of Electromagnetic Processing of materials Ministry of EducationNortheastern UniversityShenyang 110819China

Seawater battery is an advanced energy storage system that enables conversion of chemical energy to electricity by consuming metals,dissolved oxygen and seawater in anode,cathode and electrolyte,***,the oxygen reduction reaction(ORR)activity and stability of electrocatalysts can be easily deactivated due to the severe Cl~-permeation and corrosion in seawater ***,we developed a structural buffer engineering strategy by spontaneously anchoring Cl~-intoα-Co(OH)_(2) as efficient and stable ORR electrocatalysts,in which the ultrathinα-Co(OH)_(2) nanosheets were synthesized using an ultrafast solution high-temperature shock(SHTS)*** large lattice space(~0.8 nm)of layeredα-Co(OH)_(2) ensured the spontaneously penetration of Cl~-into the lattice structure and replaced part of OH~-to formα-Co(OH)_(2-x)Cl_*** continuous leaching and compensating of saturated Cl inα-Co(OH)_(2-x)Cl_x could enhance the Cl~-corrosion resistance and modulate electronic structure of Co metallic sites,thus improving the ORR electrocatalytic activity and stability in seawater ***α-Co(OH)_(2-x)Cl_x seawater batteries display superior onset and half-wave potentials of 0.71 and 0.66 V,respectively,which are much better than the counterparts ofα-Co(OH)_(2) and ofβ-Co(OH)_(2) with no Cl~-penetrating and no buffer ***α-Co(OH)_(2-x)Cl_x-based seawater batteries display stable open-circuit potential of 1.69 V and outstanding specific capacity of 1345 mAh·g^(-1).

关键词： Seawater battery Oxygen reduction electrocatalyst Solution high-temperature shock Structural buffer engineering

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