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global and regional soil organic carbon estimates:Magnitudes and uncertainties

Pedosphere 2024年第4期34卷 685-698页

作者： Ziqi LIN Yongjiu DAI Umakant MISHRA Guocheng WANG Wei SHANGGUAN Wen ZHANG Zhangcai QIN School of atmospheric Sciences Guangdong Province Key Laboratory for Climate Change and Natural Disaster StudiesSun Yat-sen UniversityZhuhai 519082China Southern marine Science and Engineering Guangdong laboratory(Zhuhai) Zhuhai 519082China Computational Biology&Biophysics Sandia National LaboratoriesLivermore CA 94550USA Faculty of Geographical Science Beijing Normal UniversityBeijing 100875China State key laboratory of atmospheric Boundary Layer Physics and atmospheric chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China

globally,soil is the largest terrestrial carbon(C)*** quantification of soil organic C(SOC)stocks in existing global observation-based estimates avails accurate predictions in carbon-climate feedbacks and future climate *** investigated the magnitudes and distributions of global and regional SOC estimates(i.e.,density and stocks)based on five widely used global gridded SOC datasets,a regional permafrost dataset developed in 2021(UM2021),and a global-scale soil profile database(World Soil Information Service)reporting measurements of a series of physical and chemical edaphic *** five global gridded SOC datasets were the Harmonized World Soil Database(HWSD),World Inventory of Soil Emission Potentials at 30 arc-second resolution(WISE30sec),global Soil Dataset for Earth System Models(GSDE),global Gridded Soil Information at 250-m resolution(SoilGrids250m),and global Soil Organic Carbon Map(GSOCmap).Our analyses showed that the magnitude and distribution of SOC varied widely among datasets,with certain datasets showing region-specific *** the global scale,SOC stocks at the top 30 and 100 cm were estimated to be 828(range:577–1171)and 1873(range:1086–2678)Pg C,*** estimates from GSDE,GSOCmap,and WISE30sec were comparable,and those of SoilGrids250m and HWSD were at the upper and lower *** spatial SOC distribution varied greatly among datasets,especially in the northern circumpolar and Tibetan Plateau permafrost ***,UM2021 and WISE30sec performed well in the northern circumpolar permafrost regions,and GSDE performed well in *** estimates of SOC by different datasets also showed large variabilities across different soil layers and *** discrepancies were generally smaller for the 0–30 cm soil than the 0–100 cm *** datasets demonstrated relatively higher agreement in grasslands,croplands,and shrublands/savannas than in other biomes(e.g.,wetlands).The users should be mindful of the gaps b

关键词： biome carbon cycle Earth System Models permafrost region soil dataset soil map

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CAS-ESM2.0 Successfully Reproduces Historical atmospheric CO_(2) in a Coupled Carbon−Climate Simulation

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Advances in atmospheric Sciences 2024年第4期41卷 572-580页

作者： Jiawen ZHU Juanxiong HE Duoying JI Yangchun LI He ZHANG Minghua ZHANG Xiaodong ZENG Kece FEI Jiangbo JIN International Center for Climate and Environment Sciences Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters(CIC-FEMD) Nanjing University of Information Science&TechnologyNanjing 210044China College of global change and Earth System Science Beijing Normal UniversityBeijing 100875China State key laboratory of atmospheric Boundary Layer Physics and atmospheric chemistry Institute of atmospheric Physics Chinese Academy of SciencesBeijing 100029China School of marine and atmospheric Sciences Stony Brook UniversityNY 11790USA University of Chinese Academy of Sciences Beijing 100049China

The atmospheric carbon dioxide(CO_(2))concentration has been increasing rapidly since the Industrial Revolution,which has led to unequivocal global warming and crucial environmental *** is extremely important to investigate the interactions among atmospheric CO_(2),the physical climate system,and the carbon cycle of the underlying surface for a better understanding of the Earth *** system models are widely used to investigate these interactions via coupled carbon-climate *** Chinese Academy of Sciences Earth System Model version 2(CAS-ESM2.0)has successfully fixed a two-way coupling of atmospheric CO_(2)with the climate and carbon cycle on land and in the *** CAS-ESM2.0,we conducted a coupled carbon-climate simulation by following the CMIP6 proposal of a historical emissions-driven *** paper examines the modeled CO_(2)by comparison with observed CO_(2)at the sites of Mauna Loa and Barrow,and the Greenhouse Gases Observing Satellite(GOSAT)CO_(2)*** results showed that CAS-ESM2.0 agrees very well with observations in reproducing the increasing trend of annual CO_(2)during the period 1850-2014,and in capturing the seasonal cycle of CO_(2)at the two baseline sites,as well as over northern high *** agreements illustrate a good ability of CAS-ESM2.0 in simulating carbon-climate interactions,even though uncertainties remain in the processes *** paper reports an important stage of the development of CAS-ESM with the coupling of carbon and climate,which will provide significant scientific support for climate research and China’s goal of carbon neutrality.

关键词： CAS-ESM atmospheric CO_(2) coupled carbon-climate simulation emissions-driven CMIP6 experiment

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Sustainable all-weather CO2 utilization by mimicking natural photosynthesis in a single material

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National Science Review 2024年第2期11卷 177-187页

作者： Xianjin Shi Yu Huang Ran Long Zhenyu Wang Liqin Wang Junji Cao Gangqiang Zhu Yujie Xiong State key laboratory of Loess and Quaternary Geology(SKLLQG) Key Laboratory of Aerosol Chemistry and Physics Institute of Earth EnvironmentChinese Academy of Sciences Center of Excellence in Quaternary Science and global change Chinese Academy of Sciences University of Chinese Academy of Sciences Hefei National Research Center for Physical Sciences at the Microscale School of Chemistry and Materials Science and National Synchrotron Radiation Laboratory University of Science and Technology of China Institute of atmospheric Physics Chinese Academy of Sciences School of Physics and Information Technology Shaanxi Normal University

Solar-driven CO2conversion into hydrocarbon fuels is a sustainable approach to synchronously alleviating the energy crisis and achieving net ***,the dependence of the conversion process on solar illumination hinders its practical application due to the intermittent availability of sunlight at night and on cloudy or rainy ***,we report a model material of Pt-loaded hexagonal tungsten trioxide（Pt/h-WO3） for decoupling light and dark reaction processes,demonstrating the sustainable CO2conversion under dark conditions for the first *** such a material system,hydrogen atoms can be produced by photocatalytic water splitting under solar illumination,stored together with electrons in the h-WO3through the transition of W6+to W5+and spontaneously released to trigger catalytic CO2reduction under dark ***,we demonstrate using natural light that CH4production can persist at night and on rainy days,proving the accomplishment of all-weather CO2conversion via a sustainable way.

关键词： sustainable CO2 utilization artificial photosynthesis all-weather application charge storage

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Simulation of the Ecosystem Productivity Responses to Aerosol Diffuse Radiation Fertilization Effects over the Pan-Arctic during 2001–19

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Advances in atmospheric Sciences 2024年第1期41卷 84-96页

作者： Zhiding ZHANG Xu YUE Hao ZHOU Jun ZHU Yadong LEI Chenguang TIAN Jiangsu key laboratory of atmospheric Environment Monitoring and Pollution Control Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science&Technology(NUIST)Nanjing 210044China Climate change Research Center Institute of Atmospheric Physics(IAP)Chinese Academy of Sciences(CAS)Beijing 100029China University of Chinese Academy of Sciences Beijing 100049China State key laboratory of Severe Weather&key laboratory of atmospheric chemistry of CMA Chinese Academy of Meteorological SciencesBeijing 100081China

The pan-Arctic is confronted with air pollution transported from lower *** have shown that aerosols help increase plant photosynthesis through the diffuse radiation fertilization effects(DRFEs).While such DRFEs have been explored at low to middle latitudes,the aerosol impacts on pan-Arctic ecosystems and the contributions by anthropogenic and natural emission sources remain less ***,we perform regional simulations at 0.2o×0.2ousing a well-validated vegetation model(Yale Interactive terrestrial Biosphere,YIBs)in combination with multi-source of observations to quantify the impacts of aerosol DRFEs on the net primary productivity(NPP)in the pan-Arctic during *** show that aerosol DRFEs increase pan-Arctic NPP by 2.19 Pg C(12.8%)yr^(-1)under clear-sky conditions,in which natural and anthropogenic sources contribute to 8.9% and 3.9%,*** all-sky conditions,such DRFEs are largely dampened by cloud to only 0.26 Pg C(1.24%)yr^(-1),with contributions of 0.65% by natural and 0.59% by anthropogenic *** aerosols cause a positive NPP trend of 0.022% yr^(-1)following the increased fire activities in the *** contrast,anthropogenic aerosols induce a negative trend of-0.01% yr^(-1)due to reduced emissions from the middle *** trends in aerosol DRFEs show a turning point in the year of 2007 with more positive NPP trends by natural aerosols but negative NPP trends by anthropogenic aerosols *** affected by modeling uncertainties,this study suggests a likely increasing impact of aerosols on terrestrial ecosystems in the pan-Arctic under global warming.

关键词： diffuse radiation fertilization effects anthropogenic aerosols natural aerosols pan-Arctic net primary productivity

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Leading Pattern of Spring Drought Variability over East Asia and Associated Drivers

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Journal of Tropical Meteorology 2024年第1期30卷 1-10页

作者：赵庆红杨崧田红瑛邓开强 School of atmospheric Sciences Sun Yat-sen Universityand Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai)ZhuhaiGuangdong 519082 China Guangdong Province key laboratory for Climate change and Natural Disaster Studies Sun Yat-sen UniversityZhuhaiGuangdong 519082 China College of atmospheric Sciences Lanzhou UniversityLanzhou 730000 China

Drought events have become more frequent and intense over East Asia in recent decades,leading to huge socioeconomic *** the droughts have been studied extensively by cases or for individual regions,their leading variability and associated causes remain *** on the Standardized Precipitation Evapotranspiration Index(SPEI)and ERA5 reanalysis product from 1979 to 2020,this study evealuates the severity of spring droughts in East Asia and investigates their variations and associated *** results indicate that North China and Mongolia have experienced remarkable trends toward dryness during spring in recent decades,while southwestern China has witnessed an opposite trend toward *** first Empirical Orthogonal Function mode of SPEI variability reveals a similar seesawing pattern,with more severe dryness in northwestern China,Mongolia,North China,South Korea,and Japan but increased wetness in Southwestern China and southeast *** investigation reveals that the anomalously dry(wet)surface in North(Southwestern)China is significantly associated with anomalously high(low)temperature,less(more)precipitation,and reduced(increased)soil moisture during the previous winter and early spring,regulated by an anomalous anticyclone(cyclone)and thus reduced(increased)water vapor *** spring dry-wet pattern in East Asia is also linked to cold sea surface temperature anomalies in the central-eastern *** findings of this study have important implications for improving the prediction of spring drought events in East Asia.

关键词： drought leading pattern East Asia spring drivers

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Representation of the Stratospheric Circulation in CRA-40 Reanalysis:The Arctic Polar Vortex and the Quasi-Biennial Oscillation

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Advances in atmospheric Sciences 2024年第5期41卷 894-914页

作者： Zixu WANG Shirui YAN Jinggao HU Jiechun DENG Rongcai REN Jian RAO key laboratory of Meteorological Disaster Ministry of Education(KLME)Joint International Research Laboratory of Climate and Environment Change(ILCEC)Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters(CIC-FEMD)Nanjing University of Information Science&TechnologyNanjing 210044China key laboratory for Semi-Arid Climate change of the Ministry of Education College of Atmospheric SciencesLanzhou UniversityLanzhou 730000China State key laboratory of Numerical Modeling for atmospheric Sciences and Geophysical Fluid Dynamics Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China

The representation of the Arctic stratospheric circulation and the quasi-biennial oscillation(QBO)during the period 1981–2019 in a 40-yr Chinese global reanalysis dataset(CRA-40)is evaluated by comparing two widely used reanalysis datasets,ERA-5 and ***-40 demonstrates a comparable performance with ERA-5 and MERRA-2 in characterizing the winter and spring circulation in the lower and middle Arctic ***,differences in the climatological polar-mean temperature and polar night jet among the three reanalyses are within±0.5 K and±0.5 m s^(–1),*** onset dates of the stratospheric sudden warming and stratospheric final warming events at 10 hPa in CRA-40,together with the dynamics and circulation anomalies during the onset process of warming events,are nearly identical to the other two reanalyses with slight *** contrast,the CRA-40 dataset demonstrates a deteriorated performance in describing the QBO below 10 hPa compared to the other two reanalysis products,manifested by the larger easterly biases of the QBO index,the remarkably weaker amplitude of the QBO,and the weaker wavelet power of the QBO *** pronounced biases are mainly concentrated in the period 1981–98 and largely reduced by at least 39%in 1999–***,particular caution is needed in studying the QBO based on *** three reanalyses exhibit greater disagreement in the upper stratosphere compared to the lower and middle stratosphere for both the polar region and the tropics.

关键词： CRA-40 ERA-5 MERRA-2 Arctic stratosphere the QBO

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CAS-ESM2.0 Dataset for the Carbon Dioxide Removal Model Intercomparison Project(CDRMIP)

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Advances in atmospheric Sciences 2024年第5期41卷 989-1000页

作者： Jiangbo JIN Duoying JI Xiao DONG Kece FEI Run GUO Juanxiong HE Yi YU Zhaoyang CHAI He ZHANG Dongling ZHANG Kangjun CHEN Qingcun ZENG International Center for Climate and Environment Sciences Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China State key laboratory of Satellite Ocean Environment Dynamics Second Institute of OceanographyMinistry of Natural ResourcesHangzhou 310012China State key laboratory of Earth Surface Processes and Resource Ecology College of Global Change and Earth System ScienceBeijing Normal UniversityBeijing 100875China State key laboratory of Numerical Modeling for atmospheric Sciences and Geophysical Fluid Dynamics Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China

Understanding the response of the Earth system to varying concentrations of carbon dioxide(CO_(2))is critical for projecting possible future climate change and for providing insight into mitigation and adaptation strategies in the near *** this study,we generate a dataset by conducting an experiment involving carbon dioxide removal(CDR)—a potential way to suppress global warming—using the Chinese Academy of Sciences Earth System Model version 2.0(CASESM2.0).A preliminary evaluation is *** model is integrated from 200–340 years as a 1%yr^(−1) CO_(2) concentration increase experiment,and then to~478 years as a carbon dioxide removal experiment until CO_(2) returns to its original ***,another 80 years is integrated in which CO_(2) is kept *** in the 2-m temperature,precipitation,sea surface temperature,ocean temperature,Atlantic meridional overturning circulation(AMOC),and sea surface height are all *** the ramp-up period,the global mean 2-m temperature and precipitation both increase while the AMOC *** of all the above variables change in the opposite direction in the ramp-down period,with a delayed peak relative to the CO_(2) *** CO_(2) returns to its original value,the global mean 2-m temperature is still~1 K higher than in the original state,and precipitation is~0.07 mm d^(–1) *** the end of the simulation,there is a~0.5°C increase in ocean temperature and a 1 Sv weakening of the *** model simulation produces similar results to those of comparable experiments previously reported in the literature.

关键词： CAS-ESM2.0 CDRMIP carbon dioxide removal AMOC temperature precipitation sea surface height

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Short-term Association of Meteorological Elements on COVID-19 Pandemic in a Semi-arid City of Northwest China,2021-2022

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Biomedical and Environmental Sciences 2024年第5期37卷 537-542页

作者： FENG Feng Liu MA Yu Xia CHENG Bo Wen LIU Zong Rui ZHAO Yu Han YANG Jie College of atmospheric Sciences Key Laboratory of Semi-Arid Climate ChangeMinistry of EducationLanzhou UniversityLanzhou 730000GansuChina Minhe Meteorological Bureau Minhe 810800QinghaiChina

The coronavirus disease 2019(COVID-19)outbreak in late 2019 significantly impacted global *** virus’s rapid spread,with its long incubation period and high infection level,caused substantial disruption to regular social frameworks,production,and lifestyles^([1]).COVID-19 is primarily transmitted through close contact,long-range contaminants,and airborne routes.

关键词： Northwest COV primarily

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Elaborations of the influencing factors on the formation of secondary inorganic aerosols in a heavily polluted urban area of China

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Journal of Environmental Sciences 2024年第4期138卷 406-417页

作者： Shuang Wang Qiyuan Wang Ting Zhang Suixin Liu Steven Sai Hang Ho Jie Tian Hui Su Yong Zhang Luyao Wang Tingting Wu Junji Cao School of Human Settlements and Civil Engineering Xi’an Jiaotong UniversityXi’an 710049China key laboratory of Aerosol chemistry and Physics State Key Laboratory of Loess and Quaternary GeologyInstitute of Earth EnvironmentChinese Academy of SciencesXi’an 710061China CAS Center for Excellence in Quaternary Science and global change Xi’an 710061China National Observation and Research Station of Regional Ecological Environment change and Comprehensive Management in the Guanzhong Plain Xi’an 710061China Division of atmospheric Sciences Desert Research InstituteRenoNevada89512United States Hong Kong Premium Services and Research laboratory KowloonHong Kong SARChina Xi’an Institute for Innovative Earth Environment Research Xi’an 710061China Institute of atmospheric Physics Chinese Academy of SciencesBeijing 100029China

In this study,online water-soluble inorganic ions were detected to deduce the formation mechanism of secondary inorganic aerosol in Xianyang,China during *** dominant inorganic ions of sulfate(SO_(4)^(2-)),nitrate(NO_(3)^(-)),and ammonium(NH_(4)^(+))(the sum of those is abbreviated as SNA)accounted for 17%,21%,and 12% of PM_(2.5)mass,*** the air quality deteriorated from excellent to poor grades,the precursor gas sulfur dioxide(SO_(2))of SO_(4)^(2-)increased and then decreased with a fluctuation,while nitrogen dioxide(NO_(2))and ammonia(NH_(3)),precursors of NO_(3)^(-)and NH_(4)^(+),and SNA show increasing *** factors including boundary layer height(BLH),temperature,and wind speed also show decline trends,except relative humidity(RH).Meanwhile,the secondary conversion ratio shows a remarkable increasing trend,indicating that there was a strong secondary *** the perspective of chemical mechanisms,RH is positively correlated with sulfur oxidation ratios(SOR),nitrogen oxidation ratios(NOR),and ammonia conversion ratios,representing that the increase of humidity could promote the generation of ***,SOR and NOR were also positively related to the *** the one hand,the low wind speed and BLH led to the accumulation of *** the other hand,the increases of RH and ammonia promoted more formations of SNA and PM_(2.5).The results advance our identification of the contributors to the haze episodes and assist to establish more efficient emission controls in Xianyang,in addition to other cities with similar emission and geographical characteristics.

关键词： Haze episodes Secondary inorganic aerosol Secondary conversion ratio Meteorological factors

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Uncertainties of ENSO-related Regional Hadley Circulation Anomalies within Eight Reanalysis Datasets

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Advances in atmospheric Sciences 2024年第1期41卷 115-140页

作者： Yadi LI Xichen LI Juan FENG Yi ZHOU Wenzhu WANG Yurong HOU International Center for Climate and Environment Sciences(ICCES) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China University of Chinese Academy of Sciences Beijing 101408China College of global change and Earth System Science(GCESS) Beijing Normal UniversityBeijing 100875China

El Nino-Southern Oscillation(ENSO),the leading mode of global interannual variability,usually intensifies the Hadley Circulation(HC),and meanwhile constrains its meridional extension,leading to an equatorward movement of the jet *** studies have investigated the response of HC to ENSO events using different reanalysis datasets and evaluated their capability in capturing the main features of ENSO-associated HC ***,these studies mainly focused on the global HC,represented by a zonal-mean mass stream function(MSF).Comparatively fewer studies have evaluated HC responses from a regional perspective,partly due to the prerequisite of the Stokes MSF,which prevents us from integrating a regional *** this study,we adopt a recently developed technique to construct the three-dimensional structure of HC and evaluate the capability of eight state-of-the-art reanalyses in reproducing the regional HC response to ENSO *** show that all eight reanalyses reproduce the spatial structure of HC responses well,with an intensified HC around the central-eastern Pacific but weakened circulations around the Indo-Pacific warm pool and tropical *** spatial correlation coefficient of the three-dimensional HC anomalies among the different datasets is always larger than ***,these datasets may not capture the amplitudes of the HC responses *** uncertainty is especially large for ENSO-associated equatorially asymmetric HC anomalies,with the maximum amplitude in Climate Forecast System Reanalysis(CFSR)being about 2.7 times the minimum value in the Twentieth Century Reanalysis(20CR).One should be careful when using reanalysis data to evaluate the intensity of ENSO-associated HC anomalies.

关键词： regional Hadley circulation ENSO atmosphere-ocean interaction reanalysis data

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