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ZirconfO2: An Excel VBA program for magmatic and hydrothermal oxygen fugacity calculation using zircon trace elements

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Journal of Earth Science 2024年

作者： Jing Lei Yilin Xiao Chinese Academy of Sciences Center of Excellence in Comparative Planetology CAS key laboratory of crust-mantle materials and environments， School of Earth and Space Sciences， University of Science and Technology of China

Oxygen fugacity of magmas and hydrothermal fluids is an important factor affecting element migration and mineralization. Zircon is an excellent monitor for oxygen fugacity of melts and fluids due to its exceptionally stable nature. However， zircon oxybarometers involve many complex algorithms leading to difficulties in use. Therefore， there is an urgent need to realize automatic calculation of various zircon oxybarometers. This study developed a Visual Basic for Applications (VBA) program， ZirconfO2， built in an ExcelTMworkbook， for calculating the oxygen fugacity of magmatic and hydrothermal fluids through the trace element characteristics of zircons. The program covers almost all the algorithms of zircon oxybarometers commonly-used so far. Through the user-friendly interface， users may input data expediently， obtain multiple results of various algorithms and find the most reliable oxygen fugacity range， effectively avoiding the possible misdirection of a single algorithm.

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Trace Element Mobility in Subducted Marble and Associated Eclogite:Constraints from UHP Rocks in the Shuanghe Area,Central-East China

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Journal of Earth Science 2024年第1期35卷 1-15页

作者： Xingao Hou Zhiqiang Yu Shefa Chen Lei Liu Yilin Xiao key laboratory of Metallogenic Prediction of Nonferrous Metals and Geological Environment Monitoring Ministry of EducationSchool of Geosciences and Info-PhysicsCentral South UniversityChangsha 410083China key laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China CAS key laboratory of crust-mantle materials and environments School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China

In order to decipher element mobility in UHP meta-sedimentary rocks in the continental subduction zone,major and trace element compositions are investigated for a continuous profile from a representative UHP region in the Dabie *** the lithologic contact zone,contents of K,Ca,LREE,and LILE exhibit varying degrees of downward trends in both marble and eclogite toward the contact zone,indicating that marble and their associated eclogite can release a large amount of K,Ca,and a small number of LILEs and *** is the main Ti phase in both marble and *** rims around rutile can occasionally be seen in *** of Ti and HFSE exhibit a well-coupled relation among marble and eclogite,indicating that substantial Ti and HFSEs were migrated from eclogite to marble,in accord with the capacity of a melt *** and titanites in marble exhibit a relatively limited variation in Nb/Ta ratios(12.9-16.2),similar to those of titanites in eclogite(14.2-16.7),which demonstrates that rutiles and titanites in marble were sourced from eclogite because of short-distance migrations of Ti and *** to the P-T path and the temperature and pressure conditions of the peak metamorphism reported by previous studies,the eclogite associated with marble may not form supercritical fluids in the subduction zone because of the addition of carbonate minerals.

关键词： UHP metamorphism eclogite marble element migration fluid actions geochemistry

Plate tectonics in the Archean:Observations versus interpretations

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Science China Earth Sciences 2024年第1期67卷 1-30页

作者： YongFei ZHENG School of Earth and Space Sciences University of Science and Technology of ChinaHefei 230026China key laboratory of crust-mantle materials and Environment Chinese Academy of SciencesHefei 230026China Center of Excellence for Comparative Planetology Chinese Academy of SciencesHefei 230026China

Plate tectonics theory,established in the 1960s,has been successful in explaining many geological phenomena,processes and events that occurred in the ***,the theory has often struggled to provide a coherent framework in interpreting geological records in continental interior and Precambrian *** dealing with the relationship between plate tectonics and continental geology,continental interior tectonics was often separated from continental margin tectonics in the inheritance and development of their structure and *** separation led to the illusion that the plate tectonics theory is not applicable to Precambrian geology,particularly in explaining the fundamental geological characteristics of Archean *** this illusion does not mean that the Archean continental crust did not originate from a regime of plate tectonics,it led to the development of alternative tectonic models,often involving vertical movements under a regime of stagnant lid tectonics,including not only endogenous processes such as gravitational sagduction,mantle plumes and heat pipes but also exogenous processes such as bolide *** vertical processes were not unique to the Archean but persisted into the *** result from mantle poloidal convection at different depths,not specific to any particular *** the plate tectonics theory from the traditional kinematic model in the 20th century to a holistic kinematic-dynamic model in the 21st century and systematically examining the vertical transport of matter and energy at plate margins,it is evident that plate tectonics can explain the common geological characteristics of Archean cratons,such as lithological associations,structural patterns and metamorphic *** deciphering the structure and composition of convergent plate margins as well as their dynamics,the formation and evolution of continental crust since the Archean can be divided into ancient plate tectonics in the Preca

关键词： Plate tectonics Archean geology Continental origin crustal reworking Plate interior Plate margin

Distribution, bioaccumulation, trophic transfer and risk assessment of trace elements in fish from a typical shallow outflow lake basin, China

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Frontiers of Environmental Science & Engineering 2024年第7期18卷 141-156页

作者： Miao He Guijian Liu Xiaodan Shi Lei Wu Qiang Chen CAS key laboratory of crust-mantle materials and Environment School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China Anhui Academy of Environmental Sciences Hefei 230022China School of Resources and Environmental Engineering Hefei University of TechnologyHefei 230009China

Fish are important food sources for humans,and the availability of appropriate amount of trace elements(TEs)plays a crucial role in fish ***,due to large volumes of sewage discharge,high levels of certain elements are present in aquatic environments,and these elements accumulate in fish and potentially affect human *** this study,the distribution and bioaccumulation capacity of trace elements in six dominant fish species from Chaohu Lake(China)were *** results showed that the bioaccumulation capacity of fish for Zn was greater than other *** the source of the TEs in the fish were explored along with the concentration of the TEs in the aquatic environment,which indicated that TEs in fish were mainly obtained through ingestion and indirectly affected by the industrial activities in the ***,stable carbon and nitrogen isotopes were used to classify the trophic levels and explore the biological magnification of TEs of the *** was found that Sb and Sr showed biomagnification with the increase of trophic level of *** on the above analyses,the environmental biogeochemical cycle model of TEs in the lake was distinguished and established,which can offer valuable insights for sustainable fishery management in the downstream Yangtze River Delta ecosystem.

关键词： Trophic level Bioaccumulation Risk assessment Trace elements

Lithium Isotope Analytical Methods and Implications for Rare-Metal Mineralization in Granite-Pegmatite Systems: An Overview

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Journal of Earth Science 2024年

作者： Xiang-Ying Ye Bin Li Dong-Bo Tan Ke-Cheng Liu Zhi-Yong Zhu Hafiz Muhammad Siddique Yi-Lin Xiao key laboratory of Metallogenic Prediction of Nonferrous Metals and Geological Environment Monitoring (Ministry of Education)， School of Geosciences and Info-physics， Central South University CAS key laboratory of Geospace Environment and Department of Plasma Physics and Fusion Engineering， University of Science and Technology of China Institute of Geology， Chinese Academy of Geological Sciences CAS key laboratory of crust-mantle materials and environments， School of Earth and Space Sciences， University of Science and Technology of China Chinese Academy of Sciences Center of Excellence in Comparative Planetology

The origin of highly-fractionated granite-pegmatite systems and their associated rare metal mineralization has been widely studied， but there is still ongoing debate. Prevailing hypotheses suggest that pegmatite formation and the associated rare metal mineralization are closely related to aqueous fluid processes. Lithium (Li) isotope analysis has been widely applied to trace granite-pegmatite evolution. This is because lithium is widely present in various minerals (e.g.， mica， tourmaline) that record the melt and fluid compositions， and lithium isotopes are sensitive to magmatic-hydrothermal processes. We briefly review the methodology of Li isotope analyses， the mechanisms of Li isotopic fractionation， and， in particular， Li isotope fractionation in granite-pegmatite system based on Li isotope data we have collected and the latest developments in Li isotope geochemistry. With the development of analytical technology， high-precision measurement of the Li content and isotopic compositions have facilitated a series of scientific breakthroughs in understanding the magmatic-hydrothermal evolution of rare-element ore deposits. Li isotope analysis on bulk mineral separates show ability to trace various hydrothermal processes (e.g. exotic or exsolved fluids). In situ Li isotope analysis methods has been enhanced by the development of new， homogeneous mineral reference materials. In situ SIMS and LA-MC-ICP-MS Li isotope measurements on minerals (e.g.， tourmaline) will likely become more important in studying the fluid–rock interactions in magmatic， metamorphic， and hydrothermal processes， as well as on pegmatite petrogenesis and rare-metal mineralization.

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Return to the Moon:New perspectives on lunar exploration

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Science Bulletin 2024年第13期69卷 2136-2148页

作者： Yangting Lin Wei Yang Hui Zhang Hejiu Hui Sen Hu Long Xiao Jianzhong Liu Zhiyong Xiao Zongyu Yue Jinhai Zhang Yang Liu Jing Yang Honglei Lin Aicheng Zhang Dijun Guo Sheng Gou Lin Xu Yuyang He Xianguo Zhang Liping Qin Zongcheng Ling Xiongyao Li Aimin Du Huaiyu He Peng Zhang Jinbin Cao Xianhua Li key laboratory of Earth and Planetary Physics Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China State key laboratory for Mineral Deposits Research and School of Earth Sciences and Engineering Nanjing UniversityNanjing 210023China State key laboratory of Geological Processes and Mineral Resources School of Earth SciencesChina University of GeosciencesWuhan 430074China Institute of Geochemistry Chinese Academy of SciencesGuiyang 550002China Planetary Environmental and Astrobiological Research laboratory School of Atmospheric SciencesSun Yat-sen UniversityZhuhai 519082China National Space Science Center Chinese Academy of SciencesBeijing 100190China Deep Space Exploration laboratory/CAS key laboratory of crust-mantle materials and environments University of Science and Technology of ChinaHefei 230026China Shandong key laboratory of Optical Astronomy and Solar-Terrestrial Environment Institute of Space SciencesShandong UniversityWeihai 264209China Technology and Engineering Center for Space Utilization Chinese Academy of SciencesBeijing 100094China School of Space and Environment Beihang UniversityBeijing 100191China

Lunar exploration is deemed crucial for uncovering the origins of the Earth-Moon system and is the first step for advancing humanity’s exploration of deep *** the past decade,the Chinese Lunar Exploration Program(CLEP),also known as the Chang’e(CE)Project,has achieved remarkable *** has successfully developed and demonstrated the engineering capability required to reach and return from the lunar ***,the CE Project has made historic firsts with the landing and on-site exploration of the far side of the Moon,along with the collection of the youngest volcanic samples from the Procellarum KREEP *** achievements have significantly enhanced our understanding of lunar *** on this success,China has proposed an ambitious crewed lunar exploration strategy,aiming to return to the Moon for scientific exploration and *** plan encompasses two primary phases:the first crewed lunar landing and exploration,followed by a thousand-kilometer scale scientific expedition to construct a geological cross-section across the lunar *** the limitations of current lunar exploration efforts and China’s engineering and technical capabilities,this paper explores the benefits of crewed lunar exploration while leveraging synergies with robotic *** study refines fundamental lunar scientific questions that could lead to significant breakthroughs,considering the respective engineering and technological *** research lays a crucial foundation for defining the objectives of future lunar exploration,emphasizing the importance of crewed missions and offering insights into potential advancements in lunar science.

关键词： Crewed lunar exploration Water and volatiles Composition and structure of lunar interior Volcanic activity and evolution of lunar mantle Space weathering and radiation environments Exploration technology

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海水对下寒武统黑色页岩V矿化/富集的贡献

Science Bulletin 2024年第8期69卷 1006-1010页

作者：董琳慧卫炜徐林刚吝祎勃刘泽瑞潘松圻荆振华黄方 CAS key laboratory of crust–mantle materials and environments School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China CAS Center for Excellence in Comparative Planetology University of Science and Technology of ChinaHefei 230026China School of Earth Sciences and Resources China University of GeosciencesBeijing 100083China State key laboratory for Mineral Deposits Research School of Earth Sciences and EngineeringNanjing UniversityNanjing 210023China Frontiers Science Center for Critical Earth materials Cycling Nanjing UniversityNanjing 210023China School of Earth Resources China University of GeosciencesWuhan 430074China Research Institute of Petroleum Exploration and Development China National Petroleum CorporationBeijing 100083China

Early Cambrian black shales along the southern margin of the Yangtze Block are characterized by polymetallic mineralization in the lower part,including Ni-Mo sulfide ore,V ore,barite ore,phosphate ore,and"stone coal"(Fig.1a)[1,2],which were likely related to or at least coincident with the global ocean oxygenation event[3]and the radiation of early animals[4].The source of oreforming elements and the metallogenic mechanism of these polymetallic mineralization layers are highly *** models proposed include hydrothermal venting,seawater scavenging,and a combination of key mineralization factors such as terrigenous input,hydrothermal supply,seawater contribution,and impacts of clay mineral and organic matter(Fig.S1 online)[1].

关键词： mineralization hydrothermal shale

Methodological progress in trace amounts of structural water in nominally anhydrous minerals

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Science China Earth Sciences 2016年第5期59卷 901-909页

作者： SHENG YingMing GONG Bing LI WanCai XIA Mei CAS key laboratory of crust-mantle materials and environments School of Earth and Space Sciences University of Science and Technology of China

In the deep Earth, hydrogen mainly occurs as structural hydroxyl and molecular water in minerals and melts, constituting mobile and immobile aqueous components. Hydrous minerals contain hydrogen which occupies a specific structural position and constitutes an indispensable component of chemical formulae. On the other hand, nominally anhydrous minerals do not contain hydrogen in their chemical formulae, but can host trace amounts of water in structural position and lattice defect. The molecular water may occur in the lattice defect as fluid/melt inclusions in minerals. Even though the water content of nominally anhydrous minerals is very limited generally in the order of ppm(parts per million), they may play a significant role in influencing the physicochemical properties of mineral and rock systems. With the continuous improvement of modern instrumentations, the analytical methodology exhibits trends for higher spatial resolution, lower detection limit and integral multiple methods on the water amount and its isotopic ratio. Among these methods, Fourier transform infrared spectrometry remains the most widely used, while secondary ion mass spectrometry, continuous flow mass spectrometry, elastic recoil detection analysis and Raman spectrometry are promising. This paper provides a brief review on the methodological progress and their applications to the analysis of structural water in nominally anhydrous minerals.

关键词： Nominally anhydrous minerals Water content Structural hydroxyl Molecular water Fourier transform infrared spectrometry

Mesozoic mafic magmatism in North China:Implications for thinning and destruction of cratonic lithosphere

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Science China Earth Sciences 2018年第4期61卷 353-385页

作者： Yongfei ZHENG Zheng XU Zifu ZHAO Liqun DAI CAS key laboratory of crust-mantle materials and environments School of Earth and Space ScienceUniversity of Science and Technology of China

The North China Craton(NCC) has been thinned from >200 km to <100 km in its eastern part. The ancient subcontinental lithospheric mantle(SCLM) has been replaced by the juvenile SCLM in the Meoszoic. During this period... 详细信息

The North China Craton(NCC) has been thinned from >200 km to mantle(SCLM) has been replaced by the juvenile SCLM in the Meoszoic. During this period, the NCC was destructed as indicated by extensive magmatism in the Early Cretaceous. While there is a consensus on the thinning and destruction of cratonic lithosphere in North China, it has been hotly debated about the mechanism of cartonic *** study attempts to provide a resolution to current debates in the view of Mesozoic mafic magmatism in North China. We made a compilation of geochemical data available for Mesozoic mafic igneous rocks in the NCC. The results indicate that these mafic igneous rocks can be categorized into two series,manifesting a dramatic change in the nature of mantle sources at ~121 Ma. Mafic igneous rocks emplaced at this age start to show both oceanic island basalts(OIB)-like trace element distribution patterns and depleted to weakly enriched Sr-Nd isotope compositions. In contrast,mafic igneous rocks emplaced before and after this age exhibit both island arc basalts(IAB)-like trace element distribution patterrs and enriched Sr-Nd isotope *** difference indicates a geochemical mutation in the SCLM of North China at^121 Ma. Although mafic magmatism also took place in the Late Triassic, it was related to exhumation of the deeply subducted South China continental crust because the subduction of Paleo-Pacific slab was not operated at that time. Paleo-Pacific slab started to subduct beneath the eastern margin of Eruasian continent since the Jurrasic. The subducting slab and its overlying SCLM wedge were coupled in the Jurassic, and slab dehydration resulted in hydration and weakening of the cratonic mantle. The mantle sources of ancient IAB-like mafic igneous rocks are a kind of ultramafic metasomatites that were generated by reaction of the cratonic mantle wedge peridotite notonly with aqueous solutions

关键词： Cratonic destruction Mafic magmas IAB-like series OIB-like series Lithospheric thinning Slab subduction