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Electrocatalytic performance of CNTs/graphene co.posited rare earth phthalocyanines(M=La,Y,Yb,Sc)

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Journal of Rare Earths 2024年第2期42卷 323-333,I0004页

作者： Tingting Jiang Caixia Ou Luyi Wang Jun Chen Sydorov Dmytro Qian Zhang Jintian Luo Hua Wang jiangxi Key Laboratory of Power Batteries and Materials Faculty of Materials Metallurgy and ChemistryJiangxi University of Science and TechnologyGanzhou341000China Joint Department of Electrochemical Energy Systems Institute of Bioorganic Chemistry and PetrochemistryNational Academy of Sciences of Ukraine38A VernadskyAveKiev03142Ukraine Guangdong Jiana Energy technology co. Ltd.Qingyuan511500China

In this study,a class of rare earth co.posite sandwich phthalocyanines(MPcs,M=La,Y,Yb,Sc) were prepared and co.pounded with graphene and carbon nanotubes to obtain MPc/Gr and MPc/CNTs *** electrocatalytic behaviors of MPc/Gr and MPc/CNTs electrodes were further *** results show that the central rare earth metal has a large influence on the electrocatalytic *** the MPcs/Gr samples,ScPc with the smallest ionic radius and molecular size can be more uniformly dispersed in graphene,and the hydrogen precipitation overpotential of ScPc/Gr electrode is514 mV,co.responding to a Tafel slope of 148 mV/dec,with better electrocatalytic performance than other rare earth metal *** for the MPc/CNTs co.posites,LaPc,which has the largest ionic radius and molecular size,is more uniformly dispersed on the surface of CNTs,so that the LaPc/CNT electrode exhibits the best LSV performance with the smallest co.responding Tafel slope(176 mV/dec).The main reason is the different binding modes of MPcs molecules in Gr and *** rare earth phthalocyanine is co.bined with layered graphene,the smallest size of rare earth phthalocyanine(ScPc)is more easily embedded in the graphene layer,resulting in better homogeneity of the co.posite,larger effective co.tact area and better electrocatalytic *** co.trast,when rare earth phthalocyanine is bound to carbon nanotubes in a tubular structure,it is mainly bound by attaching to the surface or being entangled by the carbon *** this case,the rare-earth phthalocyanine molecules(LaPc)with larger layer spacing can provide more co.tact area with CNTs,forming a more uniform and effective co.posite,which eventually provides more active sites and better electrocatalytic performance.

关键词： Electrocatalysis Rare earth phthalocyanines Graphene(Gr) Carbon nanotubes(CNTs) co.posite

Identifying the geographical origin and processing technology of Moyao(Myrrh)on the basis of near-infrared spectrosco.y co.bined with chemometrics

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Journal of Traditional Chinese Medicine 2024年第3期44卷 505-514页

作者： XU Ningning YAN Ganming XU Fengjie DENG Linfeng QIAO Xinjiang LU Changzheng CHENG Shaomin TCM Diagnosis Institute College of Traditional Chinese MedicineJiangxi University of Chinese MedicineNanchang 330004China TCM Processing Institute Pharmaceutical CollegeJiangxi University of Chinese medicineNanchang 330004China School of Electronic Information and Artificial Intelligence Shaanxi University of Science and TechnologyXi'an 710021China Jiangzhong Pharmaceutical co. Ltd.Nanchang 330096China jiangxi Guhan Refined Chinese Herbal Pieces co. Ltd.Nanchang330041.China

OBJECTIVE:To evaluate the quality of Moyao(Myrrh)in the identification of the geographical origin and processing of the ***:Raw Moyao(Myrrh)and two kinds of Moyao(Myrrh)processed with vinegar from three co.ntries were identified using near-infrared(NIR)spectrosco.y co.bined with chemometric *** co.ponent analysis(PCA)was used to reduce the dimensionality of the data and visualize the clustering of samples from different categories.A classical chemometric algorithm(PLS-DA)and two machine learning algorithms[K-nearest neighbor(KNN)and support vector machine]were used to co.duct a classification analysis of the near-infrared spectra of the Moyao(Myrrh)samples,and their discriminative performance was ***:Based on the accuracy,precision,recall rate,and F1 value in each model,the results showed that the classical chemometric algorithm and the machine learning algorithm obtained positive *** all of the chemometric analyses,the NIR spectrum of Moyao(Myrrh)preprocessed by standard normal variation or Multivariate scattering co.rection co.bined with KNN achieved the highest accuracy in identifying the geographical origins,and the accuracy of identifying the processing technology established by the KNN method after first-order derivative pretreatment was the *** best accuracy of geographical origin discrimination and processing technology discrimination were 0.9853 and 0.9706 ***:NIR spectrosco.y co.bined with chemometric technology can be an important tool for tracking the origin and processing technology of Moyao(Myrrh)and can also provide a reference for evaluations of its quality and the clinical use.

关键词： Moyao(Myrrh) near-infrared spectrosco.y geographical origin processing technology

Current status and development of CMOS SiPM for scintillator-based radiation detectors toward all-digital sensors[Invited]

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Chinese Optics Letters 2024年第2期22卷 17-27页

作者： Nico.a D'Ascenzo 胡文韬劳慧华越轩张博房磊奚道明郑睿邱奥 Emanuele Antonecchia 凌怡清刘雨晴李琰俞航肖鹏谢庆国 Wuhan National Laboratory for Optoelectronics Wuhan 430074China Biomedical Engineering Department Huazhong University of Science and TechnologyWuhan 430074China RAYQUANT technology co. Ltd.Ezhou 436044China RAYSOLUTION Healthcare co. Ltd.Hefei 230000China RAYMEASURE technology co. Ltd.Suzhou 215000China RAYCAN technology co. Ltd.Suzhou 215000China co.lege of co.puter Science and Software Engineering Shenzhen UniversityShenzhen 518060China

Modern scintillator-based radiation detectors require silico. photomultipliers(Si PMs)with photon detection efficiency higher than 40%at 420 nm,possibly extended to the vacuum ultraviolet(VUV)region,single-photon time resolution(SPTR)co.nt rate(DCR)co.centrations at low CMOS scales,deep-level carrier generation in shallow trench isolation fabrication,and power co.sumption,among *** advances at 350 and 110 nm CMOS nodes are benchmarked against available Si PMs obtained in CMOS and co.mercial customized *** co.cept of digital multithreshold Si PMs with a single microcell readout is finally reported,proposing a possible direction toward fully digital scintillator-based radiation detectors.

关键词： silico. photomultiplier co.plementary metal-oxide semico.ductor digital SiPM

A Blockchain-Based Proxy Re-Encryption Scheme with co.ditional Privacy Protection and Auditability

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China co.munications 2024年第7期21卷 267-277页

作者： Chen Guo PengWeijun Wu Jing Fang Youxuan Ye Keke Xin Yanshuang China Mobile Information technology co. LtdBeijing 100037China China Mobile Information technology co. LtdShenzhen 518048China

With the development of Internet of Things technology,intelligent door lock devices are widely used in the field of house *** the traditional housing leasing scenario,problems of door lock information disclosure,tenant privacy disclosure and rental co.tract disputes frequently occur,and the security,fairness and auditability of the housing leasing transaction cannot be *** solve the above problems,a blockchain-based proxy re-encryption scheme with co.ditional privacy protection and auditability is *** scheme implements fine-grained access co.trol of door lock data based on attribute encryption technology with policy hiding,and uses proxy re-encryption technology to achieve auditable supervision of door lock information *** encryption technology and zero-knowledge proof technology are introduced to ensure the co.fidentiality of housing rent information and the fairness of rent *** co.struct a decentralized housing lease transaction architecture,the scheme realizes the efficient co.laboration between the door lock data ciphertext stored under the chain and the key information ciphertext on the chain based on the blockchain and InterPlanetary File ***,the security proof and co.puting performance analysis of the proposed scheme are carried *** results show that the scheme can resist the chosen plaintext attack and has low co.putational co.t.

关键词： attribute encryption blockchain homomorphic encryption house leasing proxy re-encryption zero-knowledge proof

An Image Fingerprint and Attention Mechanism Based Load Estimation Algorithm for Electric Power System

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co.puter Modeling in Engineering & Sciences 2024年第7期140卷 577-591页

作者： Qing Zhu Linlin Gu Huijie Lin Electricity technology Branch Nari Technology Co.Ltd.Nanjing211106China NARI-TECH Nanjing co.trol Systems co. Ltd.Nanjing211106China

With the rapid development of electric power systems,load estimation plays an important role in system operation and ***,load estimation techniques co.tain traditional,time series,regression analysis-based,and machine learning-based *** the machine learning-based method can lead to better performance,in this paper,a deep learning-based load estimation algorithm using image fingerprint and attention mechanism is ***,an image fingerprint co.struction is proposed for training *** the data preprocessing,the training data matrix is co.structed by the cyclic shift and cubic spline ***,the linear mapping and the gray-co.or transformation method are proposed to form the co.or image ***,a co.volutional neural network(CNN)co.bined with an attentionmechanism is proposed for training performance *** last,an experiment is carried out to evaluate the estimation *** with the support vector machine method,CNN method and long short-term memory method,the proposed algorithm has the best load estimation performance.

关键词： Load estimation deep learning attention mechanism image fingerprint co.struction

Fabrication and application prospects of Pr-Fe-B/Alnico.nanoco.posite alloys

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Journal of Rare Earths 2024年第9期42卷 1717-1723,I0003页

作者： Hui Liang Sajjad Ur Rehman Ruibiao Zhang Yongqiang Deng Haihua Liu Munan Yang National Rare Earth Functional Materials Innovation Center College of Rare EarthsJiangxi University of Science and TechnologyGanzhou341000China Zhejiang Tiantong Electronic Information Materials Research Institute co. Ltd.Haining314400China

The potentials of rare earth-based nanoco.posite alloys have never been realized due to strict microstructural *** to the easy demagnetization it is challenging to increase the soft magnetic phase *** avoid the easy demagnetization,Pr-Fe-B/Alnico.magnets were fabricated and reported in this *** co.tent of the Alnico.phase is increased from 0 to 25 wt%,while the co.tent of Pr element is reduced to below the sub-stoichiometry of the 2:14:1 main *** maximum magnetic energy product,which is the figure-of-merit for permanent magnets,is increased from 122 kJ/m^(3) for the standard alloy to 146 kJ/m^(3) for the alloy with 15 wt% Alnico.which shows a significant improvement co.sidering the fact that the Curie point of the magnet is also increased by~66 *** special microstructure co.tains distinctly and heterogeneously distributed 2:14:1 and Alnico.*** dimensions of neither the 2:14:1 nor the Alnico.phases meet the dimensional requirements of the nanoco.posite magnets,but still the smooth demagnetization curves are noted for the *** behavior of effective anisotropy,the performance of the magnets in applied magnetic field and the magnetic interactions among the various co.stituent grains were quantitatively studied by reversible susceptibility,irreversible susceptibility and re co.l loop *** study may provide some guiding principles for the development of nanoco.posite magnetic alloys with excellent magnetic properties by using much less RE elements.

关键词： co.posite alloys High performance magnets Magnetic properties Alnico.alloys Rare earth magnets

Performance Study of the MPC based on BPNN Prediction Model in Thermal Management System of Battery Electric Vehicles

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Journal of Thermal Science 2024年第6期33卷 2318-2335页

作者： HE Lian'ge JING Haodong ZHANG Yan LI Pengpai GU Zihan Key Laboratory of Advanced Manufacture technology for Automobile Parts(Chongqing University of technology) Ministry of Education Ningbo Shenglong Group co. Ltd. Chongqing Tsingshan Industrial co. Ltd.

In this paper,a model predictive co.trol(MPC) based on back propagation neural network(BPNN)prediction model was proposed for co.pressor speed co.trol of air co.ditioning system(ACS) and battery thermal management system(BTMS) co.pling system of battery electric vehicle(BEV).In order to solve the problem of high co.ling energy co.sumption and inferior thermal co.fort in the cabin of the battery electric vehicle thermal management system(BEVTMS) during summer time,this paper co.bines the respective superiorities of artificial neural network(ANN) predictive modeling and MPC,and creatively co.bines the two methods and uses them in the co.trol of ***,based on ANN and heat transfer theory,BPNN prediction model,ACS and BTMS co.pling system were established and ***,a mathematical method of MPC was established to co.trol the speed of the ***,the state parameters of the co.pled system were predicted using a BPNN prediction model,and the predicted values were passed to the MPC,thus achieving accurate co.trol of the co.pressor speed using the ***,the effects of PID co.trol and MPC based on BPNN prediction model on thermal co.fort of cabin and co.pressor energy co.sumption at different ambient temperatures were co.pared in simulation under New European Driving Cycle(NEDC) *** results showed for the co.structed BPNN prediction model predicted and tested values of the selected parameters the mean squared error(MSE) ranged from 2.498% to 8.969%,mean absolute percentage error(MAPE) ranged from 4.197% to 8.986%,and mean absolute error(MAE) ranged from 3.202% to 8.476%.At ambient temperatures of 25℃,35℃ and 45℃,the MPC based on the BPNN prediction model reduced the cumulative disco.fort time in the cabin by 100 s,39 s and 19 s,respectively,co.pared with the PID *** three NEDC co.ditions,the energy co.sumption is reduced by 1.82%,2.35% and 3.48%,*** the ambient temperature was 35℃,the MPC based on BPNN pre

关键词： air co.ditioning system back propagation neural network battery electric vehicle battery thermal management system model predictive co.trol

High cerium co.tent(Nd-Pr-Ce)_(2)Fe_(14)B melt-spun ribbons with high co.rcivity

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Journal of Rare Earths 2024年第4期42卷 690-695页

作者： Yujiang Zhong Junming Wang Zikai Yuan Ruijin Liu Minggang Zhu Zhe Liu Xin Chen Wei Li Zhaohui Guo Division of Functional Materials Central Iron and Steel Research InstituteBeijing100081China Ningbo Jinji Strong Magnetic Material co. Ltd.Ningbo315172China jiangxi Jiangwu Rare Metal New Material co. Ltd.Nanchang330013China

The effects of wheel speeds on the magnetic properties and microstructures of[(Nd,Pr)_(1-x)Ce_(x)]-Fe-B meltspun ribbons were *** to melt-spun ribbons with low cerium(Ce)co.tent(x=0.2),amorphous formation can be suppressed at high wheel speed in the ribbons with a relatively high Ce co.tent(x=0.8),and with the increase of the wheel speed,the magnetic properties of the ribbons with high Ce co.tent raise *** high wheel speed,the co.rcivity mechanism of melt-spun ribbons is mainly pinning field,and the high wheel speed introduces a large number of defects into the matrix as pinning ***,ribbons with high Ce co.tent form a fine and uniform grain structure,so the grain boundary area enlarges,which further hinders the movement of domain *** co.bined effects of the above factors enable ribbons with high Ce co.tent to have excellent magnetic properties(Hcj=0.977 T,Mr=64 m^(2) A/kg)at the wheel speed of 35 m/s.

关键词： Wheel speed Ceco.tent Microstructure Magnetic properties Rare earths

Molybdenum and cadmium co.induce necroptosis through Th1/Th2 imbalance-mediated endoplasmic reticulum stress in duck ovaries

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Journal of Environmental Sciences 2024年第8期142卷 92-102页

作者： Ting Cui Xueyan Dai Huiling Guo Dianyun Wang Bingyan Huang Wenjing Pu Xuesheng Chu Caiying Zhang jiangxi Provincial Key Laboratory for Animal Health Institute of Animal Population HealthCollege of Animal Science and TechnologyJiangxi Agricultural UniversityNanchang 330045China

Cadmium(Cd)and excess molybdenum(Mo)pose serious threats to animal *** previous study has determined that Cd and/or Mo exposure can cause ovarian damage of ducks,while the specific mechanism is still *** further investigate the toxic mechanism of Cd and Mo co.exposure in the ovary,forty 8-day-old female ducks were randomly allocated into four groups for 16 weeks,and the doses of Cd and Mo in basic diet per kg were as follows:co.trol group,Mo group(100 mg Mo),Cd group(4 mg Cd),and Mo+Cd group(100 mg Mo+4 mg Cd).Cadmium sulfate 8/3-hydrate(CdSO_(4)·8/3H_(2)O)and hexaammonium molybdate((NH_(4))_(6)Mo_(7)O_(24)·4H_(2)O)were the origins of Cd and Mo,*** the 16th week of the experiment,all ovary tissues were co.lected for the detection of related *** data indicated that Mo and/or Cd induced trace element disorders and Th1/Th2 balance to divert toward Th1 in the ovary,which activated endoplasmic reticulum(ER)stress and then provoked necroptosis through triggering RIPK1/RIPK3/MLKL signaling pathway,and eventually caused ovarian pathological injuries and necroptosis *** alterations of above indicators were most apparent in the joint *** all,this research illustrates that Mo and/or Cd exposure can initiate necroptosis through Th1/Th2 imbalance-modulated ER stress in duck ovaries,and Mo and Cd co.bined exposure aggravates ovarian *** research explores the molecular mechanism of necroptosis caused by Mo and/or Cd,which reveals that ER stress attenuation may be a therapeutic target to alleviate necroptosis.

关键词： Molybdenum Cadmium Th1/Th2 imbalance Endoplasmic reticulum stress Necroptosis Ovary