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高性能、光冲击稳定的钙钛矿室内光伏器件

Science Bulletin 2024年第3期69卷 334-344页

作者：李宸孙浩轩王旻甘山豆达李亮 School of Physical Science and Technology Jiangsu Key Laboratory of Thin FilmsCenter for Energy Conversion Materials&Physics(CECMP)Soochow UniversitySuzhou 215006China

Perovskite solar cells offer great potential as a sustainable power source for distributed electronic devices that operate indoors.However,the impact of advanced lighting technology,especially the widely used pulse width modulation(PWM)technology,on perovskite photovoltaics has been ignored.Herein,for the first time in photovoltaics,we find that the light impact emitted by the PWM lighting system caused dynamic strain in perovskite thin films,induced phase separation,and accelerated the generation of metallic lead(Pb^(0))defects,leading to irreversible degradation of the cell performance after 27 h(T_(80)).To address this issue,formamidinium triiodide(FAI_(3))is chosen to treat the surface of the perovskite and release residual stress,resulting in reduced lattice deformation during dynamic strain processes.Meanwhile,it suppresses harmful Pb0 defects and reduces Voc loss at low light intensity.The champion device achieves impressive power conversion efficiency(PCE)of 35.14%and retains 99.5%of the initial PCE after continuous strobe light soaking for 2160 h.

关键词： Perovskite solar cells Indoor photovoltaics Interface engineering Micro-strain releasing

Low Loss and Low EMI Noise Trench IGBT with Shallow Emitter Trench Controlled P-Type Dummy Region

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Chinese Journal of Electronics 2024年第2期33卷 326-335页

作者： Jinping ZHANG Xiaofeng LI Rongrong ZHU Kang WANG Bo ZHANG State key laboratory of Electronic thin films and Integrated Devices University of Electronic Science and Technology of China (UESTC) Institute of Electronic and Information Engineering of UESTC in Guangdong

A novel trench insulated gate bipolar transistor（TIGBT） with a shallow emitter trench controlled P-type dummy region（STCP-TIGBT） is proposed.Compared with the conventional TIGBT with floating P-type dummy region（CFP-TIGBT） and TIGBT with floating P-type dummy region and normally on hole path（HFPTIGBT）,the proposed STCP structure not only speeds up the extraction of excessive holes in the turn-off process but also reduces the Miller plateau charge(Qgc).Therefore,both the power loss and electromagnetic interference（EMI） noise are significantly reduced.Simulation results show that the Qgcof the proposed device is only 501 nC/cm2,which is reduced by 58.5% and 26.4% when compared to the CFP-TIGBT and HFP-TIGBT,respectively.At same on-state voltage drop(Vceon) of 1.02 V,the turn-off loss(Eoff) of the proposed device is 13.49 mJ/cm2,which is 64.6%and 67.6% less than those of the CFP-TIGBT and HFP-TIGBT,respectively.Moreover,the reverse recovery dVak/dt of the freewheeling diode at same turn-on loss(Eon) of 31.8 mJ/cm2for the proposed STCP-TIGBT is only 2.15 kV/μs,which is reduced by 91.3% and 57.2% when compared to 24.69 kV/μs and 5.02 kV/μs for the CFP-TIGBT and HFPTIGBT,respectively.The reduced dV/dt significantly suppresses the electromagnetic interference noise generated by the proposed device.

关键词： Trench insulated gate bipolar transistor On-state voltage drop Turn-off loss Turn-on loss Electromagnetic interference noise Shallow emitter trench P-type dummy region

A highoutput PDMS-MXene/gelatin triboelectric nanogenerator with the petal surface-microstructure

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Nano Research 2024年第5期17卷 4151-4162页

作者： Zekun Wang Congcong Hao Mingzhe Cai Juan Cui Yongqiu Zheng Chenyang Xue key laboratory of Instrumentation Science&Dynamic Measurement Ministry of Education North University of ChinaTaiyuan 030051China State key laboratory of Electronic thin films and Integrated Devices University of Electronic Science and Technology of ChinaChengdu 611731China

Triboelectric nanogenerator(TENG)has a promising future in the field of energy harvesting and self-powered sensing due to their simplicity in structure,low cost,and efficient energy harvesting from the surrounding environment.The output electrical performance of TENG can be improved by doping the friction material with functional materials and modifying the surface of the friction material.However,the current method of adding functional materials to friction materials is costly and wasteful,and the method of modifying the surface structure of friction materials is cumbersome and not easy to operate.In this work,we present a polydimethylsiloxane(PDMS)-MXene/gelatin triboelectric nanogenerator(PMMG-TENG)based on petal surface-microstructures,which has the advantages of low cost,simple preparation,high output performance,and ecological friendliness.By doping 0.03 wt.%of MXene in PDMS,the output electrical performance of TENG can be significantly improved,with an output current increase of up to 139.7%.Four different petals are used as natural molds to prepare PMMG-TENG.The results show that PMMG-TENG with peony petal surface microstructure has the best electrical performance,and the output current increase of up to 228.17%compared with PMMG-TENG without structure.The PMMG-TENG with peony petal surface-microstructure exhibits excellent electrical performance,demonstrating a maximum open-circuit voltage of 417.39 V and a maximum short-circuit current of 12.01μA at a size of 3 cm×3 cm,and a maximum power density of 170μW/cm^(2) at a load resistance of 107Ω.The PMMG-TENG’s output performance after 10,000 cycles is consistent with the initial state,highlighting excellent output stability.The PMMG-TENG can easily light up at least 100 light emitting diodes(LEDs).(operating voltage 3V.)Gelatin film exhibits excellent degradation performance,with complete degradation time of only 150 s in water at a constant temperature of 75℃.PMMG-TENG not only shows excellent performance in the field of energy harvesting,but also has a br

关键词： triboelectric nanogenerator(TENG) petal surface-microstructure gelatin MXene energy harvesting

Vortex localization and OAM selective conversion via cylindrical metagratings

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Chinese Optics Letters 2024年第3期22卷 137-141页

作者：郝占磊朱杉仇成伟徐亚东陈焕阳 Institute of Electromagnetics and Acoustics and Department of Physics College of Physical Science and TechnologyXiamen UniversityXiamen 361005China Department of Electrical and Computer Engineering National University of SingaporeSingapore 117583Singapore School of Physical Science and Technology and jiangsu key laboratory of thin films Soochow UniversitySuzhou 215006China

Vortex waves with orbital angular momentum(OAM)are a highly active research topic in various fields.In this paper,we design and investigate cylindrical metagratings(CMs)with an even number of unit cells that can efficiently achieve vortex localization and specific OAM selective conversion.The multifunctional manipulation of vortex waves and the new OAM conservation law have further been confirmed through analytical calculations and numerical simulations.In addition,we qualitatively and quantitatively determine the OAM range for vortex localization and the OAM value of vortex selective conversion and also explore the stability for performance and potential applications of the designed structure.This work holds potential applications in particle manipulation and optical communication.

关键词： vortex waves cylindrical metagratings vortex localization high-efficiency transmission vortex selective conversion

Nonstoichiometric In-S group yielding efficient carrier transfer pathway in In_(2)S_(3) photoanode for solar water oxidation

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SusMat 2024年第1期4卷 154-165页

作者： Runyu Chen Linxing Meng Changda Wang Weiwei Xu Yulong Huang Li Song Liang Li School of Physical Science and Technology Jiangsu Key Laboratory of Thin FilmsCenter for Energy Conversion Materials&PhysicsSoochow UniversitySuzhouJiangsuP.R.China jiangsu key laboratory of Advanced Negative Carbon Technologies Soochow UniversitySuzhouJiangsuP.R.China National Synchrotron Radiation laboratory CAS Center for Excellence in NanoscienceUniversity of Science and Technology of ChinaHefeiAnhuiP.R.China School of Electronic and Information Engineering Changshu Institute of TechnologyChangshuJiangsuP.R.China

The construction of high-efficiency photoanodes is essential for developing outstanding photoelectrochemical(PEC)water splitting cells.Furthermore,insufficient carrier transport capabilities and sluggish surface water oxidation kinetics limit its application.Using a solvothermal annealing strategy,we prepared a nonstoichiometric In-S(NS)group on the surface of an In_(2)S_(3) photoanode in situ and unexpectedly formed a type II transfer path of carrier,thereby reducing the interfacial recombination and promoting the bulk separation.Firstprinciples calculations and comprehensive characterizations demonstrated NS group as an excellent oxygen evolution cocatalyst(OEC)that effectively facilitated carrier transport,lowered the surface overpotential,increased the surface active site,and accelerated the surface oxygen evolution reaction kinetics by precisely altering the rate-determining steps of*to*OH and*O to*OOH.These synergistic effects remarkably enhanced the PEC performance,with a high photocurrent density of 5.02 mA cm^(−2)at 1.23 V versus reversible hydrogen electrode and a negative shift in the onset potential by 310 mV.This work provides a new strategy for the in situ preparation of high-efficiency OECs and provides ideas for constructing excellent carrier transfer and transport channels.

关键词： In_(2)S_(3) photoanode water splitting

Spin transport characteristics modulated by the GeBi interlayer in Y_(3)Fe_(5)O_(12)/GeBi/Pt heterostructures

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Chinese Physics B 2024年第2期33卷 471-475页

作者：李明明张磊金立川郭海中 key laboratory of Materials Physics Ministry of EducationSchool of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450052China State key laboratory of Electronic thin films&Integrated Devices University of Electronic Science and Technology of ChinaChengdu 610054China Institute of Quantum Materials and Physics Henan Academy of SciencesZhengzhou 450046China

For the past few years,germanium-based semiconductor spintronics has attracted considerable interest due to its potential for integration into mainstream semiconductor technology.The main challenges in the development of modern semiconductor spintronics are the generation,detection,and manipulation of spin currents.Here,the transport characteristics of a spin current generated by spin pumping through a GeBi semiconductor barrier in Y_(3)Fe_(5)O_(12)/GeBi/Pt heterostructures were investigated systematically.The effective spin-mixing conductance and inverse spin Hall voltage to quantitatively describe the spin transport characteristics were extracted.The spin-injection efficiency in the Y_(3)Fe_(5)O_(12)/GeBi/Pt heterostructures is comparable to that of the Y_(3)Fe_(5)O_(12)/Pt bilayer,and the inverse spin Hall voltage exponential decays with the increase in the barrier thickness.Furthermore,the band gap of the GeBi layer was tuned by changing the Bi content.The spin-injection efficiency at the YIG/semiconductor interface and the spin transportation within the semiconductor barrier are related to the band gap of the GeBi layer.Our results may be used as guidelines for the fabrication of efficient spin transmission structures and may lead to further studies on the impacts of different kinds of barrier materials.

关键词： spin current Y_(3)Fe_(5)O_(12)/GeBi/Pt heterostructures spin pumping inverse spin Hall effect

Texture and Se vacancy optimization induces high thermoelectric performance in Bi2Se3 flexible thin films

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Rare Metals 2024年第6期43卷 2796-2804页

作者： Dong-Wei Ao Wei-Di Liu Yue-Xing Chen Fan Ma Yi-Jie Gu Zhuang-Hao Zheng School of Machinery and Automation Weifang University Australian Institute for Bioengineering and Nanotechnology The University of Queensland Shenzhen key laboratory of Advanced thin films and Applications Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong ProvinceCollege of Physics and Optoelectronic EngineeringShenzhen University School of Materials Science and Engineering Inner Mongolia University of Technology

Bi2Se3-based flexible thin film with high thermoelectric performance is promising for the waste heat recovery technology.In this work,a novel post-selenization method is employed to prepare n-type Bi2Se3flexible thin films with highly textured structure.The strengthened texture and Se vacancy optimization can be simultaneously achieved by optimizing the selenization temperature.The highly oriented texture leads to the increased carrier mobility and results in a high electric conductivity of ～290.47 S·cm-1at 623 K.Correspondingly,a high Seebeck coefficient(> 110 μW·K-1) is obtained due to the reduced carrier concentration,induced by optimizing vacancy engineering.Consequently,a high power factor of 3.49 μW·cm-1·K-2at 623 K has been achieved in asprepared highly-bendable Bi2Se3flexible thin films selenized at 783 K.This study introduces an effective post-selenization method to tune the texture structure and vacancies of Bi2Se3flexible thin films,and correspondingly achieves high thermoelectric performance.

关键词： Thermoelectric Bi 2 Se 3 Flexible thin film Post-selenization

Elucidating the structure-activity relationship of Cu-Ag bimetallic catalysts for electrochemical CO_(2) reduction

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Journal of Energy Chemistry 2024年第6期93卷 345-351,I0009页

作者： Qining Huang Lili Wan Qingxuan Ren Jingshan Luo Institute of Photoelectronic thin Film Devices and Technology State Key Laboratory of Photovoltaic Materials and CellsKey Laboratory of Photoelectronic Thin Film Devices and Technology of TianjinMinistry of Education Engineering Research Center of Thin Film Photoelectronic TechnologyNankai UniversityTianjin 300350China Frontiers Science Center for New Organic Matter Nankai UniversityTianjin 300071China Haihe laboratory of Sustainable Chemical Transformations Tianjin 300192China

Developing bimetallic catalysts is an effective strategy for enhancing the activity and selectivity of electrochemical CO_(2) reduction reactions,where understanding the structure-activity relationship is essential for catalyst design.Herein,we prepared two Cu-Ag bimetallic catalysts with Ag nanoparticles attached to the top or the bottom of Cu nanowires.When tested in a flow cell,the Cu-Ag catalyst with Ag nanoparticles on the bottom achieved a faradaic efficiency of 54%for ethylene production,much higher than the catalyst with Ag nanoparticles on the top.The catalysts were further studied in the H-cell and zero-gap MEA cell.It was found that placing the two metals in the intensified reaction zone is crucial to triggering the tandem reaction of bimetallic catalysts.Our work elucidates the structure-activity relationship of bimetallic catalysts for CO_(2) reduction and demonstrates the importance of considering both catalyst structures and cell characteristics to achieve high activity and selectivity.

关键词： Electrochemical CO_(2)reduction Bimetallic catalyst Cu-Ag Structure-activity relationship

Rapid and controllable in-situ self-assembly of main-group metal nanofilms for highly efficient CO_(2)electroreduction to liquid fuel in flow cells

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Nano Research 2024年第6期17卷 5718-5725页

作者： Miao Wang Huaizhu Wang Yaoda Wang Junchuan Liang Mengfei Zhu Jiarui Li Zuoxiu Tie Zhong Jin State key laboratory of Coordination Chemistry MOE Key Laboratory of Mesoscopic ChemistryMOE Key Laboratory of High Performance Polymer Materials and TechnologyJiangsu Key Laboratory of Advanced Organic MaterialsTianchang New Materials and Energy Technology Researc

The electrocatalytic reduction of CO_(2)is a promising pathway to generate renewable fuels and chemicals.However,its advancement is impeded by the absence of electrocatalysts with both high selectivity and stability.Here,we present a scalable in-situ thermal evaporation technique for synthesizing series of Bi,In,and Sn nanofilms on carbon felt(CF)substrates with a high-aspect-ratio structure.The resulting main-group metal nanofilms exhibit a homogeneously distributed and highly exposed catalyst surface with ample active sites,thereby promoting mass transport and ad-/desorption of reaction intermediates.Benefiting from the unique fractal morphology,the Bi nanofilms deposited on CF exhibit optimal catalytic activities for CO_(2)electroreduction among the designed metal nanofilms electrodes,with the highest Faradaic efficiency of 96.9%for formate production at−1.3 V vs.reversible hydrogen electrode(RHE)in H-cell.Under an industrially relevant current density of 221.4 mA·cm−2 in flow cells,the Bi nanofilms retain a high Faradaic efficiency of 81.7%at−1.1 V(vs.RHE)and a good long-term stability for formate production.Furthermore,a techno-economic analysis(TEA)model shows the potential commercial viability of electrocatalytic CO_(2)conversion into formate using the Bi nanofilms catalyst.Our results offer a green and convenient approach for in-situ fabrication of stable and inexpensive thin-film catalysts with a fractal structure applicable to various industrial settings.

关键词： CO_(2)electroreduction non-noble metal nanofilms flow cells efficiency and selectivity techno-economic analysis