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Photo-responsive functional materials based on light-driven molecular motors

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Light(Science & Applications) 2024年第3期13卷 407-420页

作者： Yanping Deng Guiying Long Yang Zhang Wei Zhao Guofu Zhou Ben L.Feringa Jiawen Chen SCNU-UG international Joint Laboratory of Molecular Science and Displays National Center for International Research on Green OptoelectronicsSouth China Normal UniversityGuangzhou 510006China Stratingh institute for Chemistry University of GroningenNijenborgh 49747AG GroningenThe Netherlands

In the past two decades,the research and development of light-triggered molecular machines have mainly focused on developing molecular devices at the nanoscale.A key scientific issue in the field is how to amplify the controlled motion of molecules at the nanoscale along multiple length scales,such as the mesoscopic or the macroscopic scale,or in a more practical perspective,how to convert molecular motion into changes of properties of a macroscopic ***-driven molecular motors are able to perform repetitive unidirectional rotation upon irradiation,which offers unique opportunities for responsive macroscopic *** several reviews that focus on the design,synthesis and operation of the motors at the nanoscale,photo-responsive macroscopic materials based on light-driven molecular motors have not been comprehensively *** the present review,we first discuss the strategy of confining absolute molecular rotation into relative rotation by grafting motors on ***,examples of self-assemble motors in supramolecular polymers with high internal order are ***,we will focus on building of motors in a covalently linked system such as polymeric gels and polymeric liquid crystals to generate complex responsive ***,a perspective toward future developments and opportunities is *** review helps us getting a more and more clear picture and understanding on how complex movement can be programmed in light-responsive systems and how man-made adaptive materials can be invented,which can serve as an important guideline for further design of complex and advanced responsive materials.

关键词： functions materials material

GraphSTGAN:Situation understanding network of slow-fast high maneuvering targets for maritime monitor services of IoT data

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Digital Communications and Networks 2024年第3期10卷 620-630页

作者： Guanlin Wu Haipeng Wang Yu Liu You He Shenzhen international Graduate School Tsinghua UniversityShenzhen518071China institute of Space Science and Applied Technology Harbin Institute of TechnologyShenzhen518055China Department of Electronic Engineering Tsinghua UniversityBeijing100084China

With the rapid growth of the maritime Internet of Things(IoT)devices for Maritime Monitor Services(MMS),maritime traffic controllers could not handle a massive amount of data in *** unmanned MMS,one of the key technologies is situation ***,the presence of slow-fast high maneuvering targets and track breakages due to radar blind zones make modeling the dynamics of marine multi-agents difficult,and pose significant challenges to maritime situation *** order to comprehend the situation accurately and thus offer unmanned MMS,it is crucial to model the complex dynamics of multi-agents using IoT big ***,previous methods typically rely on complex assumptions,are plagued by unstructured data,and disregard the interactions between multiple agents and the spatial-temporal correlations.A deep learning model,Graph Spatial-Temporal Generative Adversarial Network(GraphSTGAN),is proposed in this paper,which uses graph neural network to model unstructured data and uses STGAN to learn the spatial-temporal dependencies and *** experiments show the effectiveness and robustness of the proposed method.

关键词： Internet of things Multi-agents Graph neural network Maritime monitoring services

Engineering of oxygen vacancy and bismuth cluster assisted ultrathin Bi_(12)O_(17)Cl_(2)nanosheets with efficient and selective photoreduction of CO_(2)to CO

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Carbon Energy 2024年第4期6卷 1-11页

作者： Meili Guan Ni Lu Xuan Zhang Qiuwan Wang Jian Bao Guiye Chen Hao Yu Huaming Li Jiexiang Xia Xuezhong Gong College of Chemical and Biological Engineering Shandong University of Science and TechnologyQingdaoShandongChina institute for Energy Research Jiangsu UniversityZhenjiangJiangsuChina National Center of international Joint Research for Hybrid Materials Technology Institute of Hybrid MaterialsCollege of Materials Science andEngineeringNational Base of International Science and Technology Cooperation on Hybrid MaterialsQingdao UniversityQingdaoShandongChina

The photocatalytic conversion of CO_(2)into solar‐powered fuels is viewed as a forward‐looking strategy to address energy scarcity and global *** work demonstrated the selective photoreduction of CO_(2)to CO using ultrathin Bi_(12)O_(17)Cl_(2)nanosheets decorated with hydrothermally synthesized bismuth clusters and oxygen vacancies(OVs).The characterizations revealed that the coexistences of OVs and Bi clusters generated in situ contributed to the high efficiency of CO_(2)–CO conversion(64.3μmol g^(−1)h^(−1))and perfect *** OVs on the facet(001)of the ultrathin Bi_(12)O_(17)Cl_(2)nanosheets serve as sites for CO_(2)adsorption and activation sites,capturing photoexcited electrons and prolonging light absorption due to defect *** addition,the Bi‐cluster generated in situ offers the ability to trap holes and the surface plasmonic resonance *** study offers great potential for the construction of semiconductor hybrids as multiphotocatalysts,capable of being used for the elimination and conversion of CO_(2)in terms of energy and environment.

关键词： Bi cluster Bi_(12)O_(17)Cl_(2)nanosheet oxygen vacancy photocatalytic CO_(2)reduction

A high precision two-axis GMR angular sensor manufactured by post-annealing

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Science China(Information Sciences) 2024年第6期67卷 465-466页

作者： Zitong ZHOU Zhiqiang CAO Shaohua YAN Xiaolong WANG Libo XIE Shiyang LU Dapeng ZHU Qunwen LENG Weisheng ZHAO School of Integrated Circuit Science and Engineering Beihang University Beihang Qingdao Microelectronics Research institute Beihang University National Key Lab of Spintronics Institute of International InnovationBeihang University

Angle sensors are widely used in numerous fields such as industry,military,medical care,and the Internet of Things(IoT)[1].Magnetoresistance angle sensors have become a mainstream approach for angle measurement becaus... 详细信息

关键词： Annealing

A Dual-Task Learning Approach for Bearing Anomaly Detection and State Evaluation of Safe Region

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Chinese Journal of Mechanical Engineering 2024年第1期37卷 229-241页

作者： Yuhua Yin Zhiliang Liu Bin Guo Mingjian Zuo School of Mechanical and Electrical Engineering University of Electronic Science and Technology of ChinaChengdu 611731China Qingdao international Academician Park Research institute Qingdao 266041China

Predictive maintenance has emerged as an effective tool for curbing maintenance costs,yet prevailing research predominantly concentrates on the abnormal *** the ostensibly stable healthy phase,the reliance on anomaly detection to preempt equipment malfunctions faces the challenge of sudden anomaly *** address this challenge,this paper proposes a dual-task learning approach for bearing anomaly detection and state evaluation of safe *** proposed method transforms the execution of the two tasks into an optimization issue of the hypersphere *** leveraging the monotonicity and distinguishability pertinent to the tasks as the foundation for optimization,it reconstructs the SVDD model to ensure equilibrium in the model’s performance across the two *** experiments verify the proposed method’s effectiveness,which is interpreted from the perspectives of parameter adjustment and enveloping *** the meantime,experimental results also show two deficiencies in anomaly detection accuracy and state evaluation *** theoretical analysis inspires us to focus on feature extraction and data collection to achieve *** proposed method lays the foundation for realizing predictive maintenance in a healthy stage by improving condition awareness in safe regions.

关键词： Bearing condition monitoring Anomaly detection Safe region Support vector data description

Scenario of solar energy and policies in India

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Clean Energy 2024年第5期8卷 117-128页

作者： Sathish Kumar M Prity Kumari Y.A.Lad Sherin Maria Teaching Assistant Symbiosis Institute of Business ManagementSymbiosis International(Deemed)UniversityNagpur440008MaharashtraIndia Assistant Professor and Head Department of Basic ScienceCollege of HorticultureAnand Agricultural UniversityAnand388110GujaratIndia Associate Professor&Head Department of HRD&PMInternational Agribusiness Management InstituteAnand Agricultural UniversityAnand388110GujaratIndia Research Assistant International Maize and Wheat Improvement Center(CIMMYT)HyderabadTelanganaIndia

Solar power is energy from the Sun that is converted into thermal or electrical ***,the USA,and India have the world’s richest solar energy *** receives solar radiation with an average intensity of 200 MW/km^(2) and 250–300 sunny days a *** solar radiation in India varies from 4 to 7 kWh/m^(2)/day,with 2300–3200 sunshine hours yearly,depending on the *** Solar Park,Jodhpur,India,is the world’s largest solar plant,with 2.25 GW of installed *** energy is the best alternative elec-tricity source used explicitly in the agricultural *** the farming sector,the consumption of solar energy has been *** major issues were the installation costs,low availability of technicians,and poor quality of *** focus on skill development equips the workforce to drive innovation,efficiency,and sustained growth in the renewable-energy *** the support of inter-national collaboration and a skilled workforce,India’s progress in solar energy development is a boon for the industry.

关键词： solar energy benefits policies challenges achievements

Simultaneously quantifying hundreds of acylcarnitines in multiple biological matrices within ten minutes using ultrahigh-performance liquid-chromatography and tandem mass spectrometry

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Journal of Pharmaceutical Analysis 2024年第1期14卷 140-148页

作者： Jingxian Zhang Qinsheng Chen Lianglong Zhang Biru Shi Men Yu Qingxia Huang Huiru Tang State Key Laboratory of Genetic Engineering School of Life SciencesHuman Phenome InstituteZhangjiang Fudan International Innovation CenterMetabonomics and Systems Biology Laboratory at Shanghai International Centre for Molecular PhenomicsZhongshan HospitalFudan UniversityShanghai200032China Wuhan Laboratory for Shanghai Metabolome institute(SMI)Ltd. Wuhan430000China

Acylcarnitines are metabolic intermediates of fatty acids and branched-chain amino acids having vital biofunctions and pathophysiological significances. Here, we developed a high-throughput method for quantifying hundreds of acylcarnitines in one run using ultrahigh performance liquid chromatography and tandem mass spectrometry (UPLC-MS/MS). This enabled simultaneous quantification of 1136 acylcarnitines (C0–C26) within 10-min with good sensitivity (limit of detection 0.992), accuracy (relative error 0.998) for predicting retention time (tR) of acylcarnitines with no standards and built a database of their multiple reaction monitoring parameters (tR, ion-pairs, and collision energy). Furthermore, we quantified 514 acylcarnitines in human plasma and urine, mouse kidney, liver, heart, lung, and muscle. This provides a rapid method for quantifying acylcarnitines in multiple biological matrices.

关键词： Acylcarnitine UPLC-MS/MS Quantitative structure-retention relationship Molecular phenotype

Joint Planning of Active Distribution Network and EV Charging Stations Considering Vehicle-to-Grid Functionality and Reactive Power Support

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CSEE Journal of Power and Energy Systems 2024年第5期10卷 2100-2113页

作者： Yongheng Wang Xinwei Shen Yan Xu institute for Tsinghua Shenzhen international Graduate School Tsinghua UniversityShenzhen 518055China School of Electrical and Electronic Engineering Nanyang Technological UniversitySingapore

This paper proposes a collaborative planning model for active distribution network(ADN)and electric vehicle(EV)charging stations that fully considers vehicle-to-grid(V2G)function and reactive power support of EVs in different *** paper employs a sequential decomposition method based on physical characteristics of the problem,breaking down the holistic problem into two sub-problems for *** I optimizes the charging and discharging behavior of autopilot electric vehicles(AEVs)using a mixed-integer linear programming(MILP)*** II uses a mixed-integer secondorder cone programming(MISOCP)model to plan ADN and retrofit or construct V2G charging stations(V2GCS),as well as multiple distributed generation resources(DGRs).The paper also analyzes the impact of bi-directional active-reactive power interaction of V2GCS on ADN *** presented model is tested in the 47-node ADN in Longgang District,Shenzhen,China,and the IEEE 33-node ADN,demonstrating that decomposition can significantly improve the speed of solving large-scale problems while maintaining accuracy with low AEV penetration.

关键词： Active distribution network large-scale problem reactive power support sequential decomposition V2G charging station

Multiple-dimensioned defect engineering for graphite felt electrode of vanadium redox flow battery

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Carbon Energy 2024年第2期6卷 143-153页

作者： Yingqiao Jiang Yinhui Wang Gang Cheng Yuehua Li Lei Dai Jing Zhu Wei Meng Jingyu Xi Ling Wang Zhangxing He School of Chemical Engineering North China University of Science and TechnologyTangshanChina Tsinghua Shenzhen international Graduate School Institute of Materials ResearchTsinghua UniversityShenzhenChina

The scarcity of wettability,insufficient active sites,and low surface area of graphite felt(GF)have long been suppressing the performance of vanadium redox flow batteries(VRFBs).Herein,an ultra-homogeneous multipledimensioned defect,including nano-scale etching and atomic-scale N,O codoping,was used to modify GF by the molten salt ***_(4)Cl and KClO_(3) were added simultaneously to the system to obtain porous N/O co-doped electrode(GF/ON),where KClO_(3) was used to ultra-homogeneously etch,and O-functionalize electrode,and NH4Cl was used as N dopant,***/ON presents better electrochemical catalysis for VO_(2)+/VO_(2)+ and V3+/V2+ reactions than only O-functionalized electrodes(GF/O)and *** enhanced electrochemical properties are attributed to an increase in active sites,surface area,and wettability,as well as the synergistic effect of N and O,which is also supported by the density functional theory ***,the cell using GF/ON shows higher discharge capacity,energy efficiency,and stability for cycling performance than the pristine cell at 140 mA cm^(−2) for 200 ***,the energy efficiency of the modified cell is increased by 9.7% from 55.2% for the pristine cell at 260 mA cm^(−2).Such an ultra-homogeneous etching with N and O co-doping through“boiling”molten salt medium provides an effective and practical application potential way to prepare superior electrodes for VRFB.

关键词： graphite felt molten salt N O co-doping ultra-homogeneous etching vanadium redox flow battery