检索结果-南通市图书馆

Interlayer exciton dynamics of transition metal dichalcogenide heterostructures under electric fields

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nano Research 2024年第5期17卷 4555-4572页

作者： Jian Tang Yue Zheng Ke Jiang Qi You Zhentian Yin Zihao Xie Henan Li Cheng Han Xiaoxian Zhang Yumeng Shi international collaborative laboratory of 2d materials for optoelectronics science and technology of ministry of education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060China College of Electronics and Information Engineering Shenzhen UniversityShenzhen 518060China Key laboratory of Luminescence and Optical Information Ministry of EducationInstitute of Optoelectronic TechnologyBeijing Jiaotong UniversityBeijing 100044China

Stacking single layers of atoms on top of each other provides a fundamental way to achieve novel material systems and engineer their physical properties,which offers opportunities for exploring fundamental physics and realizing next-generation optoelectronic *** the two-dimensional(2d)-stacked systems,transition metal dichalcogenide(TMdC)heterostructures are particularly attractive because they host tightly-bonded interlayer excitons which possess various novel and appealing *** interlayer excitons have drawn significant research attention and hold high potential for the application in unique optoelectronic devices,such as polarization-and wavelength-tunable single photon emitters,valley Hall transistors,and possible high-temperature *** development of these devices requires a comprehensive understanding of the fundamental properties of these interlayer excitons and the impact of electric fields on their *** this review,we summarize the recent advances on the understanding of interlayer exciton dynamics under electric fields in TMdC *** put emphasis on the electrical modulation of interlayer excitons’emission,the valley Hall transport of charge carriers after the separation of interlayer excitons by an electric field,and the correlation physics of interlayer excitons and charges under electrical doping and *** and perspectives are finally discussed for the application of TMdC heterostructures in future optoelectronics.

关键词： interlayer exciton transition metal dichalcogenide(TMdC)heterostructures circular polarization valley Hall effect strong coupling

durable hierarchical phosphorus‐doped biphase MoS_(2)electrocatalysts with enhanced H^(*)adsorption

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Carbon Energy 2024年第4期6卷 104-114页

作者： Yongteng Qian Jianmin Yu Zhiyi Lyu Qianwen Zhang Tae Hyeong Lee Huan Pang dae Joon Kang College of Pharmacy Jinhua PolytechnicJinhuaZhejiangChina department of Physics Sungkyunkwan UniversitySuwonGyeonggi‐doRepublic of Korea international collaborative laboratory of 2d materials for optoelectronic science and technology of ministry of education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhenGuangdongChina School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhouJiangsuChina

Phase engineering is an efficient strategy for enhancing the kinetics of electrocatalytic ***,phase engineering was employed to prepare high‐performance phosphorous‐doped biphase(1T/2H)MoS_(2)(P‐BMS)nanoflakes for hydrogen evolution reaction(HER).The doping of MoS_(2)with P atoms modifies its electronic structure and optimizes its electrocatalytic reaction kinetics,which significantly enhances its electrical conductivity and structural stability,which are verified by various characterization tools,including X‐ray photoelectron spectroscopy,high‐resolution transmission electron microscopy,X‐ray absorption near‐edge spectroscopy,and extended X‐ray absorption fine ***,the hierarchically formed flakes of P‐BMS provide numerous catalytic surface‐active sites,which remarkably enhance its HER *** optimized P‐BMS electrocatalysts exhibit low overpotentials(60 and 72 mV at 10 mA cm^(−2))in H_(2)SO_(4)(0.5 M)and KOH(1.0 M),*** mechanism of improving the HER activity of the material was systematically studied using density functional theory calculations and various electrochemical characterization *** study has shown that phase engineering is a promising strategy for enhancing the H*adsorption of metal sulfides.

关键词： 1T/2H MoS_(2) density functional theory electrocatalysts phase engineering phosphorous doping

Pure-high-even-order dispersion bound solitons complexes in ultra-fast fiber lasers

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Light(science & Applications) 2024年第5期13卷 957-972页

作者： Ying Han Bo Gao Honglin Wen Chunyang Ma Jiayu Huo Yingying Li Luyao Zhou Qi Li Ge Wu Lie Liu College of Communication Engineering Jilin UniversityChangchun 130012China. Research Center of Circuits and Systems Peng Cheng LaboratoryShenzhen 518055China. international collaborative laboratory of 2d materials for optoelectronics science and technology of ministry of education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060China. College of Electronic science and Engineering Jilin UniversityChangchun 130012China

Temporal solitons have been the focus of much research due to their fascinating physical *** solitons can form bound states,which are fundamentally crucial modes in fiber laser and present striking analogies with their matter molecules counterparts,which means they have potential applications in large-capacity transmission and alloptical information *** traditionally,second-order dispersion has been the dominant dispersion for conventional solitons,recent experimental and theoretical research has shown that pure-high-even-order dispersion(PHEOd)solitons with energy-width scaling can arise from the interaction of arbitrary negative-even-order dispersion and Kerr *** these advancements,research on the bound states of PHEOd solitons is currently *** this study,we obtained PHEOd bound solitons in a fiber laser using an intra-cavity spectral pulse shaper for high-order dispersion ***,we experimentally demonstrate the existence of PHEOd solitons and PHEOd bound solitons with pure-quartic,-sextic,-octic,and-decic *** simulations corroborate these experimental ***,vibrating phase PHEOd bound soliton pairs,sliding phase PHEOd bound soliton pairs,and hybrid phase PHEOd bound tri-soliton are discovered and *** results broaden the fundamental understanding of solitons and show the universality of multi-soliton patterns.

关键词： dispersion solitons soliton

Polymer: Non-fullerene acceptor heterojunction-based phototransistor for short-wave infrared photodetection

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nano Research 2024年第4期17卷 3087-3095页

作者： Jing Li Weigang Zhu Yang Han Yanhou Geng Wenping Hu Key laboratory of Organic Integrated Circuits of ministry of education&Key laboratory of Molecular optoelectronic sciences School of Science&Collaborative Innovation Center of Chemical Science and Engineering(Tianjin)Tianjin UniversityTianjin 300072China Key laboratory of Organic Integrated Circuits of ministry of education&Key laboratory of Molecular optoelectronic sciences School of Materials Science and EngineeringTianjin UniversityTianjin 300072China

It remains full of challenge for extending short-wave infrared(SWIR)spectral response and weak-light detection in the context of broad spectral responses for *** this work,a novel poly(2,5-bis(4-hexyldodecyl)-2,5-dihydro-3,6-di-2-thienyl-pyrrolo[3,4-c]pyrrole-1,4-dione-alt-thiophene)(PdPPT3-HdO):COTIC-4F organic bulk-heterojunction is prepared as active layer for bulk heterojunction ***3-HdO serves as a hole transport material,while COTIC-4F enhances the absorption of SWIR light to 1020 *** a result,smooth and connected PdPPT3-HdO film is fabricated by blade coating method and exhibits high hole mobility up to 2.34 cm^(2)·V^(-1)·s^(-1) with a current on/off ratio of 4.72×10^(5) in organic thin film ***3-HdO:COTIC-4F heterojunction phototransistors exhibit high responsivity of 2680 A·W^(-1) to 900 nm and 815 A·W^(-1) to 1020 nm,with fast response time(rise time~20 ms and fall time~100 ms).The photosensitivity of the heterojunction phototransistor improves as the mass ratio of non-fullerene acceptors increases,resulting in an approximately two orders of magnitude enhancement compared to the bare polymer ***,the phototransistor exhibits decent responsivity even under ultra-weak light power of 43μW·cm^(-2) to 1020 *** work represents a highly effective and general strategy for fabricating efficient and sensitive SWIR light photodetectors.

关键词： photodetection phototransistor organic semiconductor heterojunction non-fullerene acceptor

digital generation of super-Gaussian perfect vortex beams via wavefront shaping with globally adaptive feedback

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

High Power Laser science and Engineering 2024年第1期12卷 42-51页

作者： Rui Ma Ke Hai Luo Jing Song He Wei Li Zhang dian Yuan Fan Anderson S.L.Gomes Jun Liu international collaborative laboratory of 2d materials for optoelectronics science and technology of ministry of education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhenChina Institute for Advanced Study Shenzhen UniversityShenzhenChina Fiber Optics Research Centre School of Information and Communication EngineeringUniversity of Electronic Science and Technology of ChinaChengduChina departamento de Física Universidade Federal de PernambucoRecife-PEBrazil

High-intensity vortex beams with tunable topological charges and low coherence are highly demanded in applications such as inertial confinement fusion(ICF) and optical communication. However, traditional optical vortices featuring nonuniform intensity distributions are dramatically restricted in application scenarios that require a high-intensity vortex beam owing to their ineffective amplification resulting from the intensity-dependent nonlinear effect. Here, a low-coherence perfect vortex beam(PVB) with a topological charge as high as 140 is realized based on the super-pixel wavefront-shaping technique. More importantly, a globally adaptive feedback algorithm(GAFA) is proposed to efficiently suppress the original intensity fluctuation and achieve a flat-top PVB with dramatically reduced beam speckle contrast. The GAFA-based flat-top PVB generation method can pave the way for high-intensity vortex beam generation,which is crucial for potential applications in ICF, laser processing, optical communication and optical trapping.

关键词： digital micromirror device flat-top beam orbital angular momentum perfect vortex beam random fiber laser

Exploring the Roles of Single Atom in Hydrogen Peroxide Photosynthesis

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Nano-Micro Letters 2024年第2期16卷 32-67页

作者： Kelin He Zimo Huang Chao Chen Chuntian Qiu Yu Lin Zhong Qitao Zhang international collaborative laboratory of 2d materials for optoelectronics science and technology of ministry of education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518000China Queensland Micro‑and Nanotechnology Centre School of Environment and ScienceGriffith UniversityNathanQLD 4222Australia Institute for Sustainable Transformation School of Chemical Engineering and Light IndustryGuangdong University of TechnologyGuangzhou 51006China ZJU‑Hangzhou Global Scientific and Technological Innovation Center Zhejiang UniversityHangzhou 311215China

This comprehensive review provides a deep exploration of the unique roles of single atom catalysts(SACs)in photocatalytic hydrogen peroxide(H_(2)O_(2))*** offer multiple benefits over traditional catalysts such as improved efficiency,selectivity,and flexibility due to their distinct electronic structure and unique *** review discusses the critical elements in the design of SACs,including the choice of metal atom,host material,and coordination environment,and how these elements impact the catalytic *** role of single atoms in photocatalytic H_(2)O_(2)production is also analysed,focusing on enhancing light absorption and charge generation,improving the migration and separation of charge carriers,and lowering the energy barrier of adsorption and activation of *** these advantages,several challenges,including H_(2)O_(2)decomposition,stability of SACs,unclear mechanism,and low selectivity,need to be *** towards the future,the review suggests promising research directions such as direct utilization of H_(2)O_(2),high-throughput synthesis and screening,the creation of dual active sites,and employing density functional theory for investigating the mechanisms of SACs in H_(2)O_(2)*** review provides valuable insights into the potential of single atom catalysts for advancing the field of photocatalytic H_(2)O_(2)production.

关键词： Single atom catalysts H_(2)O_(2)photosynthesis Catalyst design and optimization

Graphene binding on black phosphorus enables high on/off ratios and mobility

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

National science Review 2024年第2期11卷 188-195页

作者： Fanrong Lin Zhonghan Cao Feiping Xiao Jiawei Liu Jiabin Qiao Minmin Xue Zhili Hu Ying Liu Huan Lu Zhuhua Zhang Jens Martin Qingjun Tong Wanlin Guo Yanpeng Liu Key laboratory for Intelligent Nano materials and devices of ministry of education State Key Laboratory of Mechanics and Control of Mechanical Structures and Institute for Frontier Science Nanjing University of Aeronautics and Astronautics Centre for Advanced 2d materials National University of Singapore School of Physics and Electronics Hunan University Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and MeasurementSchool of PhysicsBeijing Institute of Technology Leibniz Institute für Kristallzüchtung

Graphene is one of the most promising candidates for integrated circuits due to its robustness against short-channel effects, inherent high carrier mobility and desired gapless nature for Ohmic contact, but it is difficult to achieve satisfactory on/off ratios even at the expense of its carrier mobility, limiting its device applications. Here, we present a strategy to realize high back-gate switching ratios in a graphene monolayer with well-maintained high mobility by forming a vertical heterostructure with a black phosphorus multi-layer. By local current annealing, strain is introduced within an established area of the graphene, which forms a reflective interface with the rest of the strain-free area and thus generates a robust off-state via local current depletion. Applying a positive back-gate voltage to the heterostructure can keep the black phosphorus insulating, while a negative back-gate voltage changes the black phosphorus to be conductive because of hole accumulation. Then, a parallel channel is activated within the strain-free graphene area by edge-contacted electrodes, thereby largely inheriting the intrinsic carrier mobility of graphene in the on-state. As a result, the device can provide an on/off voltage ratio of >10～3 as well as a mobility of ～8000 cm2V-1s-1at room temperature, meeting the low-power criterion suggested by the international Roadmap for devices and Systems.

关键词： graphene on/off ratio mobility black phosphorus reflective interface

High-resolution recognition of FOAM modes via an improved EfficientNet V2 based convolutional neural network

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Frontiers of physics 2024年第3期19卷 175-183页

作者： Youzhi Shi Zuhai Ma Hongyu Chen Yougang Ke Yu Chen Xinxing Zhou international collaborative laboratory of 2d materials for optoelectronics science and technology Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060China Key laboratory of Low-dimensional Quantum Structures and Quantum Control of ministry of education Synergetic Innovation Center for Quantum Effects and ApplicationsSchool of Physics and ElectronicsHunan Normal UniversityChangsha 410081China Key laboratory of Hunan Province on Information Photonics and Freespace Optical Communications School of Information Science and EngineeringHunan Institute of Science and TechnologyYueyang 414006China

Vortex beam with fractional orbital angular momentum (FOAM) is the excellent candidate for improving the capacity of free-space optical (FSO) communication system due to its infinite modes. Therefore, the recognition of FOAM modes with higher resolution is always of great concern. In this work, through an improved EfficientNetV2 based convolutional neural network (CNN), we experimentally achieve the implementation of the recognition of FOAM modes with a resolution as high as 0.001. To the best of our knowledge, it is the first time this high resolution has been achieved. Under the strong atmospheric turbulence (AT) (C_(n)^(2)=10^(-15)m^(-2/3)), the recognition accuracy of FOAM modes at 0.1 and 0.01 resolution with our model is up to 99.12% and 92.24% for a long transmission distance of 2000 m. Even for the resolution at 0.001, the recognition accuracy can still remain at 78.77%. This work provides an effective method for the recognition of FOAM modes, which may largely improve the channel capacity of the free-space optical communication.

关键词： OAM free-space optical communication deep learning convolutional neural network

Combined effects of sea urchin-like structure and mixed Cu^(+)/Cu^(0)states on promoting C_(2)formation in electrocatalytic CO_(2)reduction

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Frontiers of Chemical science and Engineering 2024年第3期18卷 63-73页

作者： Mengqing Shan dongsheng Lu Jiatong dong Shen Yan Jinyu Han Hua Wang collaborative Innovation Center of Chemical science and Engineering Key Laboratory for Green Chemical Technology of the Ministry of EducationSchool of Chemical Engineering and TechnologyTianjin UniversityTianjin300354China

Surface engineering and Cu valence regulation are essential factors in improving the C_(2)selectivity during the electrochemical reduction of CO_(2).Herein,we present a sea urchin-like CuO/Cu_(2)O catalyst derived from rhombic dodecahedra Cu_(2)O through one-step oxidation/etching method where the mixed Cu^(+)/Cu^(0)states are formed via in situ reduction during *** combined effects of the morphology and the mixed Cu^(+)/Cu^(0)states on C–C coupling are evaluated by the Faradaic efficiency of C_(2)and the C_(2)/C1 ratio obtained in an H-cell.R-Cu^(O)/Cu_(2)O exhibited 49.5%Faradaic efficiency of C_(2)with a C_(2)/C1 ratio of 3.1 at−1.4 V *** hydrogen electrode,which are 1.5 and 3.2 times higher than those of R-Cu_(2)O,*** a flow-cell,68.0%Faradaic efficiency of C_(2)is achieved at a current density of 500 mA·cm^(−2).The formation of the mixed Cu^(+)/Cu^(0)states was confirmed by in situ Raman ***,the sea urchin-like structure provides more active sites and enables faster electron *** a result,the excellent C_(2)production on R-CuO/Cu_(2)O is primarily attributed to the synergistic effects of the sea urchin-like structure and the stable mixed Cu^(+)/Cu^(0)***,this work presents an integrated strategy for developing Cu-based electrocatalysts for C_(2)production through electrochemical CO_(2)reduction.

关键词： CO_(2)electrolysis sea urchin-like structure Cu^(+)/Cu^(0) C_(2)products