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Co-production of hydrogen, oxygen, and electricity via an integrated solar-driven system with decoupled water electrolyzer and Na-Zn ion battery

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Journal of Energy Chemistry 2025年第1期100卷 621-627页

作者： Fei Lv Longjie Liu Jiazhe Wu Pengfei Wang Lixia Pan Dengwei Jing Yubin Chen international Research center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049ShaanxiChina

Combining water electrolysis and rechargeable battery technologies into a single system holds great promise for the co-production of hydrogen (H_(2)) and ***,the design and development of such systems is still in its ***,an integrated hydrogen-oxygen (O_(2))-electricity co-production system featuring a bipolar membrane-assisted decoupled electrolyzer and a Na-Zn ion battery was established with sodium nickelhexacyanoferrate (NaNiHCF) and Zn^(2+)/Zn as dual redox *** decoupled electrolyzer enables to produce H_(2)and O_(2)in different time and space with almost 100%Faradaic efficiency at 100 mA cm^(-2).Then,the charged NaNiHCF and Zn electrodes after the electrolysis processes formed a Na-Zn ion battery,which can generate electricity with an average cell voltage of 1.75 V at 10 m A cm^(-2).By connecting Si photovoltaics with the modular electrochemical device,a well-matched solar driven system was built to convert the intermittent solar energy into hydrogen and electric energy with a solar to hydrogen-electricity efficiency of 16.7%,demonstrating the flexible storage and conversion of renewables.

关键词： Hydrogen Electricity Decoupled water electrolyzer Na-Zn ion battery Solar energy

Two paths, one goal: mechanism of calcium homeostasis to balance plant growth and immunity

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Science China(Life Sciences) 2025年第1期68卷 306-308页

作者： Aziz Ul Ikram Yanping Jing Huan Chen Jian Chen international Genome center Jiangsu UniversityZhenjiang 212013China Joint center for Single Cell Biology School of Agriculture and BiologyShanghai Jiao Tong UniversityShanghai 200240China

Calcium(Ca^(2+))is an essential nutrient and a cellular signal in *** level of free Ca^(2+)in the apoplast is~10,000-fold higher than that in the cytoplasm at the resting *** large Ca^(2+)level gradient across the membrane between the interior and exterior can cause Ca^(2+)overload and *** have evolved mechanisms to export Ca^(2+)out of the cytoplasm or store it in intracellular organelles,such as endoplasmic reticulum(ER),mitochondria,and ***,Ca^(2+)-binding proteins,including those containing the most common Ca^(2+)-binding EF-hand domains,maintain the cytosolic Ca^(2+)level by directly binding them,thus participating in Ca^(2+)***^(2+)/H+exchangers(CAXs,antiporter)and Ca^(2+)-ATPases(ACAs)are responsible for transferring Ca^(2+)from the cytosol to either the external space or intracellular stores(Bose et al.,2011).However,it is still unknown how these Ca^(2+)-scavenging transporters are activated when the cytosolic Ca^(2+)level is elevated to threshold ***“auto-regulatory”mechanism to scavenge excess cytosolic Ca^(2+),providing a guarding system to maintain cytosolic Ca^(2+)homeostasis in plants.

关键词： maintain mechanism immunity

Worldwide spread of the Ponseti method for clubfoot

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World Journal of Orthopedics 2014年第5期5卷 585-590页

作者： Lior Shabtai Stacy C Specht John E Herzenberg international center for limb lengthening Rubin Institute for Advanced Orthopedics Sinai Hospital

The Ponseti method has become the gold standard for the treatment of idiopathic clubfoot. Its safety and efficacy has been demonstrated extensively in the literature, leading to increased use around the world over the last two decades. This has been demonstrated by the increase in Ponseti related Pub Med publications from many countries. We found evidence of Ponseti activity in 113 of 193 United Nations members. The contribution of many organizations which provide resources to healthcare practitioners in low and middle income countries, as well as Ponseti champions and modern communication technology, have helped to spread the Ponseti method around the world. Despite this, there are many countries where the Ponseti method is not being used, as well as many large countries in which the extent of activity is unknown. With its low rate of complication, low cost, and high effectiveness,this method has unlimited potential to treat clubfoot in both developed and undeveloped countries. Our listing of countries who have not yet shown presence of Ponseti activity will help non-governmental organizations to target those countries which still need the most help.

关键词： Ponseti Clubfoot World Organization Children

Brassinosteroids alleviate wheat floret degeneration under low nitrogen stress by promoting the redistribution of sucrose from stems to spikes

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Journal of Integrative Agriculture 2025年第2期24卷 497-516页

作者： Zimeng Liang Xidan Cao Rong Gao Nian Guo Yangyang Tang Vinay Nangia Yang Liu College of Agronomy Northwest A&F University international center for Agricultural Research in the Dry Areas

The trade-off between yield and environmental effects caused by nitrogen fertilizer application is an important issue in wheat production. A reduction in fertile florets is one of the main reasons for the lower yields under low nitrogen application rates. Brassinosteroids(BRs) have been found to play a role in nitrogen-induced rice spikelet degeneration. However, whether BRs play a role in wheat floret development and the mechanisms involved are not clear. Therefore, a nitrogen gradient experiment and exogenous spraying experiment were conducted to investigate the role and mechanism of BRs in wheat floret development under low nitrogen stress. The results showed that as the nitrogen application decreased, the endogenous BRs content of the spikes decreased, photosynthesis weakened, and total carbon, soluble sugar and starch in the spikes decreased, leading to a reduction in the number of fertile florets. Under low nitrogen stress, exogenous spraying of 24-epibrassinolide promoted photosynthesis,and stimulated stem fructan hydrolysis and the utilization and storage of sucrose in spikes, which directed more carbohydrates to the spikes and increased the number of fertile florets. In conclusion, BRs mediate the effects of nitrogen fertilizer on wheat floret development, and under low nitrogen stress, foliar spraying of 24-epibrassinolide promotes the flow of carbohydrates from the stem to the spikes, alleviating wheat floret degeneration.

关键词： brassinosteroids fertile florets nitrogen application rate sucrose metabolism wheat

Efficient photocatalytic H2 evolution over tubular mesoporous carbon nitride with N-vacancy by microwave-assisted synthesis

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Science China Chemistry 2025年第3期 866-873页

作者： Yuanlong Pan Qiang Zhang Guangzheng Huang Yannan Luo Honglin Gao School of Materials and Energy National Center for International Research on Photoelectric and Energy MaterialsYunnan University

Modifying the microstructure of photocatalysts while simultaneously introducing vacancies has shown significant potential in enhancing their performance for hydrogen ***,a novel tubular mesoporous carbon nitride（TMCN） with nitrogen vacancies was fabricated using a microwave-assisted synthesis strategy,employing melamine-cyanuric acid supramolecular（MC-S） as the *** optimized TMCN exhibited an outstanding H2production rate,approximately 29 times higher than that of pristine *** N-vacancies serve as sites for reactant adsorption and activation,leading to enhanced delocalization of ***,the porous structures of TMCN facilitate the reactant diffusion,while its tubular architectures promote the oriented transfer of charge ***,the markedly improved photocatalytic performance of TMCN can be predominantly attributed to the synergistic effects arising from its superior structure and N-vacancy *** work opens new possibilities for the simultaneous formation of surface defect states as photocatalytic reaction sites and distinctive structures conducive to charge carrier transport.

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Constructing Pr-doped CoOOH catalytic sites for efficient electrooxidation of 5-hydroxymethylfurfural

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Journal of Energy Chemistry 2025年第1期100卷 234-244页

作者： Botao Fan Hao Zhang Bang Gu Feng Qiu Qiue Cao Wenhao Fang School of Chemical Science and Technology Yunnan UniversityKunming 650091YunnanChina National center for international Research on Photoelectric and Energy Materials School of Materials and EnergyYunnan UniversityKunming 650091YunnanChina

Electrocatalytic conversion of renewable biomass is emerging as a promising route for sustainable chemical production;hence it urgently calls for developing efficient electrocatalysts with low potentials and high current ***,a Pr-doped Co(OH)_(2)hexagonal sheet(Pr/Co=1/9,in mole)is synthesized by electrodeposition as highly performant catalyst for 5-hydroxymethylfurfural(HMF)oxidation reaction(HMFOR)to produce 2,5-furandicarboxylic acid(FDCA).This novel and low-cost catalyst possesses a rather low onset potential of 1.05 V(***)and requires only 1.10 V(***)to reach a current density of 10 mA cm^(-2)for HMFOR,significantly outperforming Co(OH)_(2)benchmark(i.e.,210 mV higher to reach10 m A cm^(-2)).The origin of Pr promotion effect as well as the evolution of CoOOH catalytic sites and HMFOR process has been deeply elucidated by physical characterizations,kinetic experiments,in situ electrochemical techniques,and theoretical *** unique Pr-ameliorated CoOOH active centers enable 100%conversion of HMF,99.6%selectivity of FDCA,and 99.7%Faraday efficiency,with a superior cycling durability toward *** can be one of the most outstanding results for Co-based HMFOR catalysts to date in the *** this work can help open up new horizons for constructing novel and efficient Co-based electrocatalysts by the utilization of lanthanide elements.

关键词： Biomass conversion Electrocatalysis 2,5-Furandicarboxylic acid Doped Co catalyst Co3+active sites Charge transfer rate

Research progress of lignin-derived materials in lithium/sodium ion batteries

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Green Energy & Environment 2025年第2期10卷 322-344页

作者： Jingke Zhang Hengxue Xiang Zhiwei Cao Shichao Wang Meifang Zhu Institute of Hybrid Materials National Center of International Research for Hybrid Materials TechnologyNational Base of International Science&Technology CooperationCollege of Materials Science and EngineeringQingdao UniversityQingdao266071China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai201620China

With the increase of energy consumption,the shortage of fossil resource,and the aggravation of environmental pollution,the development of cost-effective and environmental friendly bio-based energy storage devices has become an urgent *** the second most abundant natural polymer found in nature,lignin is mainly produced as the by-product of paper pulping and bio-refining *** possesses several inherent advantages,such as low-cost,high carbon content,abundant functional groups,and bio-renewable,making it an attractive candidate for the rechargeable battery ***,there has been a surge of research interest in utilizing lignin or lignin-based carbon materials as the components of lithium-ion(LIBs)or sodium-ion batteries(SIBs),including the electrode,binder,separator,and *** review provides a comprehensive overview on the research progress of lignin-derived materials used in LIBs/SIBs,especially the application of lignin-based carbons as the anodes of LIBs/*** preparation methods and properties of lignin-derived materials with different dimensions are systemically discussed,which emphasizes on the relationship between the chemical/physical structures of lignin-derived materials and the performances of LIBs/*** current challenges and future prospects of lignin-derived materials in energy storage devices are also proposed.

关键词： Lignin-based carbons Lithium battery Sodium battery Chemical structure evolution

New insight into the origin and evolution of the flora and fauna of Hainan Island,China

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Science China Earth Sciences 2025年第1期68卷 52-61页

作者： Hua ZHU center for Integrative Conservation Xishuangbanna Tropical Botanical GardenChinese Academy of SciencesYunnan International Joint Laboratory of Southeast Asia Biodiversity ConservationYunnan Key Laboratory for the Conservation of Tropical Rainforests and Asian ElephantsMengla666303China

The origin of the biota of Hainan Island,China,remains a fundamental scientific *** studies on the biota,geological tectonics,and paleomagnetism proposed that during the Eocene,Hainan Island connected Vietnam and Guangxi,and then moved to the southeast to reach its present *** review mainly discusses its biota origin from molecular phylogeny and palaeobotanical *** formation and evolution of the biological groups of Hainan Island were identified via research on their genomes,phylogeny,and molecular *** research showed that the genera and species that appeared and diverged early in their evolution(i.e.,before the Miocene)can be explained by the land connection between Hainan Island,Vietnam,and Guangxi during the *** to Southeast Asian tectonic theory,in the Middle Miocene(at about 15 million years ago),Hainan Island had moved to its present *** population and genetic divergence of species with late divergence times(after 15 Ma)can be reasonably explained by the close proximity(or land connection)between Hainan Island and the Leizhou Peninsula,enabling genetic communication between Hainan Island and the Chinese mainland,but have exceptional *** have been obtained through palaeobotanical studies,showing that in the Eocene-Oligocene period,southwest China and Hainan Island had subtropical vegetation and ***,the fossil group in southeast China(in Maoming,near present-day Hainan Island)in the Late Eocene indicated a tropical rainforest vegetation and *** suggests that in the Paleogene,Hainan Island may have been located near or on the southwest border of Guangxi and northern Vietnam,rather than in its present *** floristic division of the flora of Hainan Island basically presents a northeast-southwest inclined distribution *** pattern can be explained by the counterclockwise rotation of Hainan Island during its movement to the southeast as prop

关键词： Molecular phylogeny Biogeography Paleobotany Origin of flora and fauna Hainan Island of China

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Improving performance of perovskite solar cells enabled by defects passivation and carrier transport dynamics regulation via organic additive

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Chinese Chemical Letters 2025年第2期36卷 551-556页

作者： Rongjun Zhao Tai Wu Yong Hua Yude Wang Department of Physics Center for Optoelectronics Engineering ResearchYunnan University Yunnan Key Laboratory for Micro/Nano Materials&Technology International Joint Research Center for Optoelectronic and Energy MaterialsSchool of Materials and EnergyYunnan University Yunnan Key Laboratory of Carbon Neutrality and Green Low-carbon Technologies Yunnan University

Defects at the grain boundaries(GBs) of perovskite film highly restrict both the efficiency and stability of perovskite solar cells(PSCs). Herein, organic small molecules of butanedioic acid(BA) and acetylenedicarboxylic acid(AA), containing two carbonyl(C=O) groups and different core-units, were incorporated into perovskite as additives for PSCs application. Thanks to the strong coordination interaction between C=O group and under-coordinated Pb2+, the additives can effectively passivate film defects and regulate the perovskite crystallization, yielding high-quality perovskite films with lower defect densities. More importantly, the additives can efficiently regulate the charge transport behaviors in PSCs. Benefiting from the defects passivation and the regulation of charge carrier dynamics, the BA and AA-treaded PSCs show the power conversion efficiencies of 21.52% and 20.50%, which are higher than that of the control device(19.41%). Besides, the optimal devices exhibit a remarkable enhanced long-term stability and moisture tolerance compared to the pristine devices. Furthermore, the transient absorption spectrum reveals the mechanism of enhanced photovoltaic performances, attributing to the improvement of charge transport capability at the perovskite/Spiro-OMeTAD interfaces. This work affords a promising strategy to improve the efficiency and stability of PSCs through regulating the charge-carrier dynamic process in perovskite film.

关键词： Additives Carrier dynamics Defects passivation Perovskite solar cells Stability