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Recent progress of in-situ characterization of LiNi_(1−x−y)Co_(x)Mn_(y)O_(2) cathodes for lithium metal batteries: A mini review

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Nano Research 2024年第3期17卷 1384-1401页

作者： Huanzhu Lv Xiaoqi Zhu Jun Mei Yuanhua Xia Bin Wang Institute of Fundamental and Frontier science University of Electronic Science and Technology of ChinaChengdu 611731China Chengdu Development Center of science and Technology China Academy of Engineering PhysicsChengdu 610200China Key Laboratory of Neutron Physics and Institute of Nuclear Physics and Chemistry China Academy of Engineering Physics(CAEP)Mianyang 621999China

In the context of the gradual popularity of electric vehicles(EVs),the development of lithium battery systems with high energy density and power density is regarded as the foremost way to improve the range of ***_(1-x-y)Co_(x)Mn_(y)O_(2)(NCM)cathodes have been the focus of researchers due to their high energy density,excellent power performance,and low-temperature ***,the elaboration of the decay mechanism of NCM cathode based on lithium metal batteries(LMBs)is still being restricted to the primary *** the past decades,the development and application of advanced in-situ characterization tools have facilitated researchers'understanding of the internal operation mechanism of batteries during charging and *** this minireview,the latest progress of in-situ observation of the NCM cathode by X-ray diffraction(XRD),fourier transform infrared(FT-IR)spectroscopy,Raman spectroscopy,atomic force microscopy(AFM),transmission electron microscope(TEM),optical microscope,and other characterization tools is *** mechanisms of structural degradation,cathode-electrolyte interfaces(CEIs)composition,and dynamic changes of NCM,electrolyte breakdown,and gas production are ***,based on the existing research progress,the opportunities and challenges for future in-situ characterization technology in the study of the mechanism of LMBs are discussed in ***,the purpose of this minireview is to summarize recent work that focuses on the outstanding application of in-situ characterization techniques in the mechanistic study of LMBs,and pointing the way to the future development of high energy density and power density LMBs systems.

关键词： lithium metal batteries(LMBs) In-situ characterization LiNi_(1-x-y)Co_(x)Mn_(y)O_(2)(NCM)

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Numerical simulation of the dynamic migration mechanism and prediction of saturation of tight sandstone oil

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science China Earth sciences 2024年第1期67卷 179-195页

作者： Gaohui CAO Mian LIN Likuan ZHANG Lili JI Wenbin JIANG Institute of Mechanics Chinese Academy of SciencesBeijing 100190China School of engineering science University of Chinese Academy of SciencesBeijing 100049China Institute of Geology and Geophysics Chinese Academy of SciencesBeijing 100029China

Quantitative characterization of tight sandstone oil migration and accumulation is an emerging research frontier in the field of oil and gas *** this study,a conceptual model containing multiple basic geological elements is developed,and a nonlinear seepage numerical model for tight sandstone oil migration and accumulation is *** effects of the slip effect,overpressure driving force,buoyancy,and capillary force on the migration and accumulation of tight oil are *** results showed that(1)the differences in oil migration and accumulation between tight and conventional reservoirs are reflected in the growth mode of oil saturation,distribution characteristics of oil and water,and extent of the effect of the formation dip angle;(2)the slip effect has a significant impact when the average pore throat radius is less than 150 nm and the overpressure driving force and capillary force are the main mechanical mechanisms controlling oil migration and accumulation in tight sandstone,while the coupling effect of buoyancy,capillary force,and overpressure driving force controls the upper and lower limits of oil ***,a dimensional and dimensionless identification chart for rapidly predicting the oil saturation of tight sandstone is proposed and verified using the measured *** study provides a basis for analyzing the migration and accumulation mechanisms of tight sandstone oil and a new approach for predicting oil ***,we developed digital and visual analysis methods for the migration results,enriching the expression of the dynamics of hydrocarbon accumulation.

关键词： Tight sandstone Migration and accumulation Dynamics Oil saturation Numerical simulation

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A Deep Learning Method for Computing Eigenvalues of the Fractional Schrödinger Operator

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Journal of Systems science & Complexity 2024年第2期37卷 391-412页

作者： GUO Yixiao MING Pingbing LSEC Institute of Computational Mathematics and Scientific/Engineering ComputingAcademy of Mathematics and Systems ScienceChinese Academy of SciencesBeijing 100190China School of Mathematical sciences University of Chinese Academy of SciencesBeijing 100049China

The authors present a novel deep learning method for computing eigenvalues of the fractional Schrödinger *** proposed approach combines a newly developed loss function with an innovative neural network architecture that incorporates prior knowledge of the *** improvements enable the proposed method to handle both high-dimensional problems and problems posed on irregular bounded *** authors successfully compute up to the first 30 eigenvalues for various fractional Schrödinger *** an application,the authors share a conjecture to the fractional order isospectral problem that has not yet been studied.

关键词： Eigenvalue problem deep learning fractional Schrödinger operator isospectral problem

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Body-force modeling considering induced upstream effects for a transonic compressor with total temperature distortion

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Chinese Journal of Aeronautics 2024年第6期37卷 7-19页

作者： Jiahui QIU Chen YANG Wenqiang ZHANG Min ZHANG Juan DU Digital Twin Research Center Institute of Engineering ThermophysicsChinese Academy of SciencesBeijing 100190China School of engineering and science University of Chinese Academy of SciencesBeijing 100190China National Key Laboratory of science and Technology on Advanced Light-duty Gas-turbine Chinese Academy of SciencesBeijing 100190China School of Mechatronical engineering Beijing Institute of TechnologyBeijing 100081China

To numerically study the impact of total temperature distortion on a transonic compressor with reduced computational costs,a Body-Force Model(BFM)is ***,the interactions between the distorted flow and the compressor are analyzed using full-annulus Unsteady Reynolds-Averaged Navier-Stokes(URANS)results and the orbit *** is found that the induced swirl distortion and the mass flux nonuniformity are intensified in the compressor upstream flow field.A correction factor is thus added to the BFM to account for the effect of the induced swirl,which is crucial for the accurate representation of distortion transfer in the ***,steady simulations with large-amplitude 180circumferential total temperature distortion are performed using the developed *** is shown that the distorted compressor map simulated with the BFM matches well with URANS *** circumferential phase shift of total temperature and the generation of the additional total pressure distortion across the rotor are in line with the time-averaged URANS flow *** compressor upstream effects on the distorted inflow can also be exactly *** above-mentioned results demonstrate the BFM developed in this paper can effectively capture the distorted flow features inside the compressor,and significantly reduce the computational costs by five orders of magnitude compared with URANS.

关键词： Upstream effect Orbit method Induced swirl distortion Body force model Correction factor Time-averaged URANS

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New Hybrid CHP System Integrating Solar Energy and Exhaust Heat Thermochemical Synergistic Conversion with Dual-Source Energy Storage

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Journal of Thermal science 2024年第3期33卷 970-984页

作者： QIN Yuanlong LIU Taixiu LI Peijing ZHAO Kai JIAO Fan PEI Gang LIU Qibin Department of Thermal science and Energy engineering University of Science and Technology of ChinaHefei230027China Institute of engineering Thermophysics Chinese Academy of SciencesBeijing100190China University of Chinese academy of sciences Beijing100049China School of Energy Power and Mechanical EngineeringNorth China Electric Power UniversityBeijing102206China

For the efficient use of solar and fuels and to improve the supply-demand matching performance in combined heat and power(CHP)systems,this paper proposes a hybrid solar/methanol energy system integrating solar/exhaust thermochemical and thermal energy *** proposed system includes parabolic trough solar collectors(PTSC),a thermochemical reactor,an internal combustion engine(ICE),and hybrid storage of thermal and chemical energy,which uses solar energy and methanol fuel as input and outputs power and *** methanol thermochemical decomposition reaction,mid-and-low temperature solar heat and exhaust heat are upgraded to chemical energy for efficient power *** thermal energy storage(TES)stores surplus thermal energy,acting as a backup source to produce heat without emitting CO_(2).Due to the energy storage,time-varying solar energy can be used steadily and efficiently;considerable supply-demand mismatches can be avoided,and the operational flexibility is *** the design condition,the overall energy efficiency,exergy efficiency,and net solar-to-electric efficiency achieve 72.09%,37.65%,and 24.63%,*** fuel saving rate(FSR)and the CO_(2) emission reduction(ER_(CO_(2)))achieve 32.97%and 25.33%,*** research findings provide a promising approach for the efficient and flexible use of solar energy and fuels for combined heat and power.

关键词： hybrid energy system solar thermochemical exhaust heat energy storage operational flexibility

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Design and performance investigation of modified dual reflector parabolic trough collector with double planar mirrors

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science China(Technological sciences) 2024年第3期67卷 902-918页

作者： LI Peijing LIU TaiXiu QIN YuanLong LI JiChao LIU QiBin School of Energy Powerand Mechanical EngineeringNorth China Electric Power University Beijing 226China Institute of engineering Thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese academy of sciences Beijing 100049China Department of Thermal science and Energy engineering University of Science and Technology of ChinaHefei 230027China

In a typical parabolic trough collector(PTC), sunlight is concentrated at the bottom of the absorber tube. This concentrated solar flux leads to uneven heat distribution, resulting in high local temperatures and significant thermal stress on the absorber *** limitations have restricted the application of PTCs in solar thermochemistry and other fields and have impacted their safe operation. In this study, a new PTC with dual planar mirrors(DPMS) is proposed to homogenize the circumferential solar flux distribution of the absorber tube. A design method and single-objective optimization of the new PTC with a DPMS are proposed,and an uncertainty analysis of the operational and structural parameters is performed. A coupled light-heat-structure numerical model was developed to study the heat transfer performance and structural mechanical properties. The thermodynamic properties of the PTC with DPMS under different boundary conditions were analyzed. The results show that the circumferential temperature difference of the new PTC is within 2.6 K, and the circumferential thermal deformation is within 0.9 mm under typical working conditions(the inlet velocity of the heat transfer fluid is 3 m/s, inlet temperature is 573.15 K, and the direct normal irradiance is 1000 W/m^(2)). Compared with conventional PTCs, the circumferential temperature difference is reduced by 74%–90%, and the maximum thermal deformation along the y-axis is reduced by more than 95% under all working conditions(1–5 m/s, 373.5–675.15 K, 200–1000 W/m^(2)). The new PTC maintains the uniformity of the circumferential solar flux distribution for different operating parameters(sun incident angle of 0°–3°) and installation errors(±3 mm), is suitable for solar energy applications in various fields, and has the potential for large-scale applications.

关键词： solar thermal energy parabolic trough collector secondary reflector solar flux distribution optical optimization

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Preparation and Photostriction Properties of BiFeO_(3)-BaTiO_(3)Ceramics

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Journal of Wuhan University of Technology(Materials science) 2024年第5期39卷 1079-1086页

作者： ZHENG Zewei ZHANG Liqiang CHEN Chen CAO Minghe YI Zhiguo LIU Hanxing School of Materials science and engineering Wuhan University of TechnologyWuhan 430070China State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China School of Microelectronics Shanghai UniversityShanghai 200444China international School of Materials science and engineering Wuhan University of TechnologyWuhan 430070China

Under illumination by 405,520 and 655 nm monochromatic visible light(light intensity of 30 kW/m^(2)),large photostriction(ΔL/L)of 0.19%,0.13%and 0.26%for 67BiFeO_(3)-33BaTiO_(3)(67BF-33BT)lead-free ferroelectric ceramics are obtained,*** studying the ferroelectric and photoelectric properties in conjunction with in situ Raman spectroscopy,it is found that the photostrictive effect of 67BF-33BT is not caused by the electrical strain induced by abnormal photovoltaic voltage,but related to the optical induced oxygen octahedral *** 67BF-33BT lead-free ferroelectric material with excellent photostrictive response in the visible light region is expected to play an important role in the field of optical drive electromechanical devices.

关键词： ferroelectric ceramics photostrictive effect visible light response

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Experimental realization of fractal fretwork metasurface for sound anomalous modulation

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Chinese Physics B 2024年第5期33卷 473-478页

作者：何佳杰于书萌江雪他得安 Department of Biomedical engineering School of Information Science and TechnologyFudan UniversityShanghai 200433China academy for engineering and Technology Fudan UniversityShanghai 200433China

Natural creatures and ancient cultures are full of potential sources to provide inspiration for applied *** by the fractal geometry in nature and the fretwork frame in ancient culture,here we design the acoustic metasurface to realize sound anomalous modulation,which manifests itself as an incident-dependent propagation behavior:sound wave propagating in the forward direction is allowed to transmit with high efficiency while in the backward direction is obviously *** quantitatively investigate the dependences of asymmetric transmission on the propagation direction,incident angle and operating frequency by calculating sound transmittance and energy *** compact fractal fretwork metasurface for acoustic anomalous modulation would promote the development of integrated acoustic devices and expand versatile applications in acoustic communication and information encryption.

关键词： acoustic metasurface fractal geometry sound anomalous modulation

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Remote heteroepitaxy of transition metal dichalcogenides through monolayer hexagonal boron nitride

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Nano Research 2024年第4期17卷 3224-3231页

作者： Jidong Huang Jingren Chen Junhua Meng Siyu Zhang Ji Jiang Jingzhen Li Libin Zeng Zhigang Yin Jinliang Wu Xingwang Zhang Key Lab of Semiconductor Materials science Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China Center of Materials science and Optoelectronics engineering University of Chinese Academy of SciencesBeijing 100049China Faculty of science Beijing University of TechnologyBeijing 100124China

As a very promising epitaxy technology,the remote epitaxy has attracted extensive attention in recent years,in which graphene is the most used interlayer *** an isomorphic of graphene,two-dimensional(2D)hexagonal boron nitride(h-BN),is another promising interlayer for the remote ***,there is a current debate on the feasibility of using h-BN as interlayer in the remote ***,we demonstrate that the potential field of sapphire can completely penetrate monolayer h-BN,and hence the remote epitaxy of ZrS_(2) layers can be realized on sapphire substrates through monolayer *** field of sapphire can only partially penetrate the bilayer h-BN and result in the mixing of remote epitaxy and van der Waals(vdWs)*** to the weak interfacial scattering and high crystalline quality of ZrS_(2) epilayer,the ZrS_(2) photodetector with monolayer h-BN shows the best performance,with an on/off ratio of more than 2×10^(5) and a responsivity up to 379 mA·W^(-1).This work provides an efficient approach to prepare single-crystal transition metal dichalcogenides and their heterojunctions with h-BN,which have great potential in developing large-area 2D electronic devices.

关键词： remote epitaxy hexagonal boron nitride transition metal dichalcogenides chemical vapor deposition photodetectors

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Stacking order modulated anomalous valley Hall effect in antiferromagnetic MXene

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Journal of Materiomics 2024年第1期10卷 269-276页

作者： Tong Zhao Shucheng Xing Jian Zhou Naihua Miao Zhimei Sun School of Materials science and engineering Beihang UniversityBeijing100191China Center for Integrated Computational Materials engineering International Research Institute for Multidisciplinary ScienceBeihang UniversityBeijing100191China

The valley index is a promising degree of freedom for information processing in electronic ***,the researches on valley polarization are mainly focused on ferromagnetic order,which breaks the time reversal symmetry ***,a novel paradigm for achieving stacking order modulated anomalous valley Hall(AVH)effect is proposed in antiferromagnetic *** paradigm involves the introduction and reversal of nonuniform potentials by modulating the position of substrate,to break the combined symmetry of spatial inversion and time reversal(PT symmetry)and achieve stacking-dependent valley spin *** on first-principles calculations,we discover spontaneous valley polarization in antiferromagnetic Cr_(2)CH_(2) MXene and stacking-dependent valley spin splitting in Cr_(2)CH_(2)/Sc_(2)CO_(2) ***,switching the ferroelectric polarization of monolayer Sc_(2)CO_(2) results in a semiconductor-metal transition in Cr_(2)CH_(2)/Sc_(2)CO_(2),accompanied by the disappearance of valley *** findings provide an alternative way to develop controllable valleytronics devices based on antiferromagnetic monolayers.

关键词： Stacking order Antiferromagnetism AVH effect Electrical control

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