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Yb:Sc_(2)O_(3) Transparent Ceramics Fabricated from Co-precipitated Nano-powders:Microstructure and Optical Property

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无机材料学报 2025年第2期40卷 215-224页

作者： YE Junhao ZHOU Zhenzhen HU Chen WANG Yanbin JING Yanqiu LI Tingsong CHENG Ziqiu WU Junlin IVANOV Maxim HRENIAK Dariusz LI Jiang Transparent Ceramics Research Center Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 201899China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Center of Excellence for Photoconversion Vinča Institute of Nuclear SciencesNational Institute of the Republic of SerbiaUniversity of Belgrade11001 BelgradeSerbia institute of Electrophysics ural branch Russian Academy of SciencesEkaterinburg 620016Russia institute of Low Temperature and Structure Research Polish Academy of SciencesWroclaw 326109Poland

Sc_(2)O_(3),as a host for solid-state laser gain materials,has advantage of high thermal conductivity and easy matching with activating ions,which is promising in high-power laser ***,Yb-doped Sc_(2)O_(3) ceramics have been fabricated at very high sintering temperatures,but their optical quality and sintering process still need further *** this work,5%Yb:Sc_(2)O_(3)(in mass)nano-powders were obtained by co-precipitation,and then transparent ceramics were fabricated by vacuum pre-sintering and hot isostatic pressing(HIP)*** cubic Yb:Sc_(2)O_(3) nano-powders with good dispersity and an average crystallite of 29 nm were *** of pre-sintering temperatures(1500-1700℃)on densification process,microstructure changes,and optical transmittance of Yb:Sc_(2)O_(3) ceramics was *** data revealed that all samples have a uniform microstructure,while the average grain sizes increase with the increase of the sintering ***,the optimum in-line transmittance of Yb:Sc_(2)O_(3) ceramics,pre-sintered at 1550℃after HIP post-treatment,reaches 78.1%(theoretical value of 80%)at 1100 *** properties of the Yb:Sc_(2)O_(3) ceramics reveal that the minimum population inversion parameterβ2 and the luminescence decay time of 5%Yb:Sc_(2)O_(3) ceramics are 0.041 and 0.49 ms,respectively,which demonstrate that the optical quality of the Yb:Sc_(2)O_(3) has been ***,their best vacuum sintering temperature can be controlled down to a lower temperature(1550℃).In conclusion,Yb:Sc_(2)O_(3) nano-powders are successfully synthesized by co-precipitation method,and good optical quality transparent ceramics are fabricated by vacuum pre-sintering at 1550℃and HIP post-treatment.

关键词： nano-powder Yb:Sc_(2)O_(3) transparent ceramic hot isostatic pressing optical property

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A special core-shell material(Mxene@Ag@Phytate)to improve EVA composite fire safety,radiation cross-linking effect,and electromagnetic shielding

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Nuclear Science and Techniques 2025年第2期36卷 27-39页

作者： Si-Yi Xu Dan-Yi Li Wen-Rui Wang Lin Lin Ying Sun Ji-Hao Li Lin-Fan Li Shanghai institute of Applied physics Chinese Academy of SciencesShanghai 201800China University of Chinese academy of sciences Beijing 100049China

High-performance MXene-based polymer nanocomposites are well-suited for various industrial applications owing to their excellent mechanical,thermal,and other ***,the fabrication of flame-retardant polymer/MXene nanocom-posites remains challenging owing to the limited flame-retardant properties of MXene *** study prepared a novel MXene@Ag@PA hybrid material via radiation modification and complexation *** material was used to further enhance the key properties of ethylene-vinyl acetate(EVA),such as its mechanical properties,thermal conductivity,flame retardancy,and electromagnetic *** addition of two parts of this hybrid material increased the thermal conduc-tivity of EVA by 44.2%and reduced its peak exothermic rate during combustion by 30.1%compared with pure *** material also significantly reduced smoke production and increased the residue *** the X-band,the electromagnetic shielding effectiveness of the EVA composites reached 20 ***,the MXene@Ag@PA hybrid material could be used to further enhance the mechanical properties of EVA composites under electron-beam ***,this study contributes to the development of MXene-based EVA advanced materials that are fire-safe,have high strength,and exhibit good electromagnetic shielding performance for various applications.

关键词： MXene@Ag@PA Ethylene-vinyl acetate(EVA) Flame retardancy Electromagnetic shielding performance

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Great influence of demagnetization history on internal interaction and magnetization process of mischmetal-based magnets

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Science China(physics,Mechanics & Astronomy) 2025年第2期68卷 183-192页

作者： Dan Liu Jiefu Xiong Lichen Wang Xinqi Zheng Xin Ming Jiaying Jin Jiazheng Hao He Bai Zhenxing Li Tongyun Zhao Fengxia Hu Jirong Sun Jun Shen Baogen Shen Department of physics Beijing Technology and Business UniversityBeijing 10048China Ningbo institute of Materials Technology&Engineering Chinese Academy of SciencesNingbo 31521China School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083China School of Materials Science and Engineering Zhejiang UniversityHangzhou 310027China Spallation Neutron Source Science Center Dongguan 523803China School of Mechanical Engineering Beijing Institute of Technology Beijing 100081China Beijing National Laboratory for Condensed Matter physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical sciences University of Chinese Academy of SciencesBeijing 101408China Ganjiang Innovation academy Chinese Academy of SciencesGanzhou 341000China

The magnetization process and corresponding magnetization curve are usually used to analyze the coercivity mechanism of NdFe-B based sintered ***,different demagnetization histories will seriously influence the magnetization curve,leading to an inaccurate understanding and analysis of magnetization *** this work,we investigated the magnetization behavior of multi-main phase(MMP)magnets with thermal demagnetized and alternating current demagnetized *** curves of initial magnetization process and demagnetization process of thermal demagnetized magnets reflect the movement of domain walls inside the grains and the magnetization interaction between the grains,*** is noted that the former process cannot represent the magnetization reversal of the entire magnet,which is not appropriate to analyze coercivity mechanism *** the recoil curves of both two processes of AC demagnetized magnets can illustrate the magnetization reversal of the entire grains and the interaction between ***-optical Kerr microscope shows that the grains of thermal demagnetized magnets are in multi-domain states,and the grains of AC demagnetized magnets are almost in singledomain *** walls of thermal demagnetized magnets move easily within the grains,which is more conducive to magnetization saturation in industrial *** addition,the minorloops of thermal demagnetized magnets can independently represent the transition of grains from multi-domain to single-domain and the demagnetization of single-domain grains,which is equivalent to characterizing the internal interactions by recoil *** investigation of magnetization characteristics of MMP sintered magnets starting from different demagnetized states is helpful to further understand the internal interaction and magnetic hardening mechanism.

关键词： permanent magnet demagnetization history magnetization reversal misch-metal rare earth

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New Insights on Gamma-Ray Burst Radiation Mechanisms from Multiwavelength Observations

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Research in Astronomy and Astrophysics 2025年第2期25卷 3-12页

作者： Yu-Hua Yao Fang-Sheng Min Shi Chen Yi-Qing Guo College of physics Chongqing University Key Laboratory of Particle Astrophysics Institute of High Energy Physics Chinese Academy of Sciences Wisconsin Ice Cube Particle Astrophysics Center University of Wisconsin–Madison University of Chinese academy of sciences School of physics and Astronomy Yunnan University Tianfu Cosmic Ray Research Center

The study of high-energy gamma-ray emission from gamma-ray bursts(GRBs) involves complex synchrotron radiation and synchrotron self-Compton(SSC) scattering mechanisms with multiple parameters exhibiting a wide distribution. Recent advancements in GRB research, particularly the observation of very high energy(VHE,>100 Ge V) radiation, have ushered in a new era of multiwavelength exploration, offering fresh perspectives and limitations for understanding GRB radiation mechanisms. This study aimed to leverage VHE observations to refine constraints on synchrotron + SSC radiation from electrons accelerated by forward shocks. By analyzing two external environments—the uniform interstellar medium and stratified stellar wind medium, we conducted spectral and variability fitting for five specific bursts(GRB 180720B, GRB 190114C, GRB 190829A, GRB 201216C, and GRB 221009A) to identify the optimal parameters characterizing these events. A comparative analysis of model parameter distributions with and without VHE radiation observations reveals that the magnetic energy equipartition factor εBis more concentrated with VHE emissions. This suggests that VHE emissions may offer greater constraints on this microphysical parameter. Additionally, we found that the energy budget between VHE and ke V–Me V γ-ray emissions under the SSC radiation exhibits an almost linear relationship, which may serve as a tool to differentiate radiation mechanisms. We anticipate future statistical analyses of additional VHE bursts to validate our findings.

关键词： (transients:) gamma-ray bursts gamma-rays: ISM radiation mechanisms: non-thermal

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Low‑Temperature Fabrication of Stable Black‑Phase CsPbI_(3) Perovskite Flexible Photodetectors Toward Wearable Health Monitoring

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Nano-Micro Letters 2025年第3期17卷 232-245页

作者： Yingjie Zhao Yicheng Sun Chaoxin Pei Xing Yin Xinyi Li Yi Hao Mengru Zhang Meng Yuan Jinglin Zhou Yu Chen Yanlin Song College of Chemistry and Pingyuan Laboratory Zhengzhou UniversityZhengzhou 450001People’s Republic of China Key Laboratory of Green Printing Institute of ChemistryChinese Academy of SciencesBeijing 100190People’s Republic of China Key Laboratory of Bio‑Inspired Materials and Interfacial Science Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190People’s Republic of China institute of High Energy physics Chinese Academy of SciencesBeijing 100049People’s Republic of China

Flexible wearable optoelectronic devices fabricated fromorganic–inorganic hybrid perovskites significantly accelerate the developmentof portable energy,biomedicine,and sensing fields,but their poor thermal stabilityhinders further ***,all-inorganic perovskites possessexcellent thermal stability,but black-phase all-inorganic perovskite filmusually requires high-temperature annealing steps,which increases energy consumptionand is not conducive to the fabrication of flexible wearable *** this work,an unprecedented low-temperature fabrication of stable blackphaseCsPbI3perovskite films is demonstrated by the in situ hydrolysis reactionof diphenylphosphinic chloride *** released diphenyl phosphateand chloride ions during the hydrolysis reaction significantly lower the phasetransition temperature and effectively passivate the defects in the perovskitefilms,yielding high-performance photodetectors with a responsivity of 42.1 AW−1 and a detectivity of 1.3×10^(14)***,high-fidelity imageand photoplethysmography sensors are demonstrated based on the fabricated flexible wearable *** work provides a newperspective for the low-temperature fabrication of large-area all-inorganic perovskite flexible optoelectronic devices.

关键词： In situ hydrolyzation Low-temperature processing All-inorganic perovskite Flexible photodetectors Health monitoring

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Failure mechanisms of AlGaN/GaN HEMTs irradiated by high-energy heavy ions with and without bias

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Nuclear Science and Techniques 2025年第1期36卷 49-58页

作者： Pei-Pei Hu Li-Jun Xu Sheng-Xia Zhang Peng-Fei Zhai Ling Lv Xiao-Yu Yan Zong-Zhen Li Yan-Rong Cao Xue-Feng Zheng Jian Zeng Yuan He Jie Liu institute of Modern physics Chinese Academy of Sciences(CAS)Lanzhou 730000China Key Laboratory of Wide Band‑gap Semiconductor Materials Ministry of EducationXidian UniversityXi’an 710071China University of Chinese academy of sciences(UCAS) Beijing 100049China

Gallium nitride(GaN)-based devices have significant potential for space ***,the mechanisms of radiation damage to the device,particularly from strong ionizing radiation,remains *** study investigates the effects of radiation on p-gate AlGaN/GaN high-electron-mobility transistors(HEMTs).Under a high voltage,the HEMT leakage current increased sharply and was accompanied by a rapid increase in power density that caused"thermal burnout"of the *** addition,a burnout signature appeared on the surface of the burned devices,proving that a single-event burnout effect ***,degradation,including an increase in the on-resistance and a decrease in the breakdown voltage,was observed in devices irradiated with high-energy heavy ions and without *** latent tracks induced by heavy ions penetrated the heterojunction interface and extended into the GaN ***,a new type of N_(2)bubble defect was discovered inside the tracks using Fresnel *** accumulation of N_(2)bubbles in the heterojunction and buffer layers is more likely to cause leakage and *** study indicates that electrical stress accelerates the failure rate and that improving heat dissipation is an effective reinforcement method for GaN-based devices.

关键词： GaN HEMTs Heavy ions Single-event burnout Latent tracks Degradation

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Four-wave mixing in a laser diode gain medium induced by the feedback from a high-Q microring resonator

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Photonics Research 2025年第1期13卷 59-68页

作者： DARIA M.SOKOL NIKITA YU DMITRIEV DMITRY A.CHERMOSHENTSEV SERGEY N.KOPTYAEV ANATOLY V.MASALOV VALERY E.LOBANOV IGOR A.BILENKO ARTEM E.SHITIKOV russian Quantum Center Moscow institute of physics and Technology (MIPT) Skolkovo institute of Science and Technology Lebedev Physical institute Russian Academy of Sciences Faculty of physics M.V.Lomonosov Moscow State University

Laser diodes are widely used and play a crucial role in myriad modern applications including nonlinear optics and ***,we explore the four-wave mixing effect in a laser diode gain medium induced by the feedback from the high-Q microring *** phenomenon can be observed at a laser frequency scan close to the microresonator eigenfrequency,prior to the transition of the laser diode from a free-running to a self-injection locking *** effect opens up the possibility for generation of remarkably low-noise,stable,and adjustable microwave *** provide a detailed numerical study of this phenomenon proven with experimental results and demonstrate the generation of the signals in the GHz *** obtained results reveal the stability of such regime and disclose the parameter ranges enabling to achieve ***,our findings uncover,to our knowledge,a novel laser diode operation regime and pave the way for the creation of new types of chip-scale,low-noise microwave sources,which are highly demanded for diverse applications,including telecommunication,metrology,and sensing.

关键词： Four wave mixing

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Preface to the Special Topic on Solar Energy Meteorology

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Advances in Atmospheric sciences 2025年第2期42卷 249-251页

作者： Dazhi YANG Xiang’ao XIA School of Electrical Engineering and Automation Harbin Institute of TechnologyHarbin 150001China Chongqing Research institute of Harbin institute of Technology Chongqing 401151China institute of Atmospheric physics Chinese Academy of SciencesBeijing 100029China University of Chinese academy of sciences Beijing 100049China

Advances in Atmospheric sciences has long been a natural home for atmospheric scientists,but as the scope of the atmospheric sciences rapidly expands,it is logical and attractive to also broaden the scope of the *** this point,we are pleased to present this special topic on solar energy meteorology,a collection of five invited articles,addressing several important aspects including satellite remote sensing,solar system modeling,photovoltaic power forecasting,thermal balance of solar panels,and decarbonization *** articles are contributed by established scientists,and readers can expect to enjoy the content of this special topic.

关键词： Solar meteorology attractive

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Perovskite LiBaH3 for photo-assisted dinitrogen fixation

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Science China Chemistry 2025年第3期 1169-1174页

作者： Kaixun Cui Yeqin Guan Yongli Cai Runze Wang Qianru Wang Wenbo Gao Jianping Guo Ping Chen Department of Chemical physics University of Science and Technology of China Dalian institute of Chemical physics Chinese Academy of Sciences Center of Materials and Optoelectronics Engineering University of Chinese Academy of Sciences

Establishing supply chains for future ammonia energy systems requires the development of efficient materials and processes for ammonia production under mild *** researches disclose unique functionalities of binary alkali and alkaline earth metal hydrides in mediating ammonia *** to the rich compositional and structural properties of the metalhydrogen system,we herein report that LiBaH3,as a narrow band gap perovskite hydride,exhibits a strong response to visible light ***,hydridic hydrogen undergoes reductive elimination of producing H2and creates an electron-rich *** an environment favors dinitrogen fixation to form N–H *** on this chemical property,a chemical looping ammonia synthesis process mediated by LiBaH3and driven by both photo and thermal energies was proposed and *** work demonstrates that hydride perovskites are promising candidates for mediating photo-assisted nitrogen fixation reactions.

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Mechanisms behind the surprising observation of supra-thermal ions in NIF’s fusion burning plasmas

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Science Bulletin 2025年第3期70卷 359-364页

作者： Yuhan Xue Dong Wu Jie Zhang Key Laboratory for Laser Plasmas and Department of physics and Astronomy Collaborative Innovation Center of IFSA(CICIFSA)Shanghai Jiao Tong UniversityShanghai 200240China institute of physics Chinese Academy of SciencesBeijing 100190China

Although ignition had been achieved at the National Ignition Facility(NIF),recent observations of the experiments indicate novel physics that beyond theoretical predictions emerge,e.g.,the neutron analysis of experiments has revealed deviations from the Maxwellian distributions in ion relative kinetic energies of burning plasmas,with the surprising emergence of supra-thermal deuterium and tritium(DT)ions that fall outside the predictions of macroscopic statistical hydrodynamic *** our newly developed hybrid-particle-in-cell code,incorporating the newly-proposed model of large-angle collisions,we infer that that this could be attributed to the increased significance of large-angle collisions among DT ions andα-particles in the burning *** and unprecedented kinetic investigations into the implications of large-angle collisions in the burning plasma have yielded several key findings,including an ignition moment promotion by~10 ps,the presence of supra-thermal ions below an energy threshold,and approximately twice the expected deposition ofα-particles *** rationality of our findings is confirmed through the congruency between the neutron spectral moment analyses conducted by the NIF and our kinetic simulations,both highlighting progressively widening disparities between neutron spectral moment analyses and hydrodynamics predictions,which becomes more pronounced as the yield *** kinetic simulations with large-angle collisions not only provide novel insights for experiment interpretation but also open new research opportunities for the largely unexplored regime of the nuclear burning plasmas,which are distinguished by their exceptionally high energy densities and hold immense potential for illuminating the intricate physics that underpins the evolution of the early universe.

关键词： lon kinetics Supra-thermal ions Large-angle collisions Non-equilibrium ignition Inertial confinement fusion Burning plasmas

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