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Low-temperature replacement construction of three-dimensional corrosion-resistant interface for deeply rechargeable Zn metal batteries

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Nano Materials Science 2024年第3期6卷 329-336页

作者： Jinze Li Daniel Rohrens Gianluca Dalfollo Xiaochao Wu Ziheng Lu Qiang Gao Bo Han Ruimin Sun Chenggang Zhou Jindi Wang Zhao Cai Faculty of Materials Science and Chemistry China University of GeosciencesWuhan430074China institute of Inorganic Chemistry RWTH Aachen UniversityAachen52074Germany Microsoft Research AI4Science Beijing10080China institute of New Energy on Chemical Storage and Power Sources College of Applied Chemistry and Environmental EngineeringYancheng Teachers UniversityYancheng224000China

Aqueous Zn batteries are promising candidates for grid-scale renewable energy *** electrodes have been widely investigated and applied as anode materials for aqueous Zn batteries,however,they suffer from limited surface area and severe interfacial issues including metallic dendrites and corrosion side reactions,limiting the depth of discharge(DOD)of the foil electrode ***,a low-temperature replacement reaction is utilized to in-situ construct a three-dimensional(3D)corrosion-resistant interface for deeply rechargeable Zn foil ***,the deliberate low-temperature environment controlled the replacement rate between polycrystalline Zn metal and oxalic acid,producing a Zn foil electrode with distinct 3D corrosion-resistant interface(3DCI-Zn),which differed from conventional two-dimensional(2D)protective structure and showed an order of magnitude higher surface ***,the 3DCI-Zn electrode exhibited dendrite-free and anticorrosion properties,and achieved stable plating/stripping performance for 1000 h at 10 mA cm^(-2)and 10 mAh cm^(-2)with a remarkable DOD of 79%.After pairing with a MnO2cathode with a high areal capacity of 4.2 mAh cm^(-2),the pouch cells delivered 168 Wh L^(-1)and a capacity retention of 89.7%after 100 cycles with a low negative/positive(N/P)ratio of 3:1.

关键词： Aqueous batteries Foil electrodes Depth of discharge Dendrites Corrosion side reactions

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Location Prediction from Social Media Contents using Location Aware Attention LSTM Network

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Journal of Harbin institute of Technology(New series) 2024年

作者： Madhur Arora Sanjay Agrawal Ravindra Patel Department of Computer Application， National institute of Technical teachers Training and Research Department of Computer Application， University institute of Technology， Rajiv Gandhi Proudyogiki Vishwavidyalaya

Location prediction in social media， a growing research field， employs machine learning to identify users’ locations from their online activities. This technology， useful in targeted advertising and urban planning， relies on natural language processing to analyze social media content and understand the temporal dynamics and structures of social networks. A key application is predicting a Twitter user’s location from their tweets， which can be challenging due to the short and unstructured nature of tweet text. To address this challenge， the research introduces a novel machine learning model called the location-aware attention LSTM (LAA-LSTM). This hybrid model combines a Long Short-Term Memory (LSTM) network with an attention mechanism. The LSTM is trained on a dataset of tweets， and the attention network focuses on extracting features related to latitude and longitude， which are crucial for pinpointing the location of a user’s tweet. The result analysis shows approx. 10% improvement in accuracy over other existing machine learning approaches.

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An aqueous rechargeable Fe//LiMn_(2)O_()hybrid battery with superior electrochemical performance beyond mainstream Fe-based batteries

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Nano Research 2024年第6期17卷 5168-5178页

作者： Yu Liu Dehui Xie Yuxin Shi Rongguan Lv Yingna Chang Yuzhen Sun Zhiyuan Zhao Jindi Wang Kefan Song Huayu Wu Tuan K.A.Hoang Rong Xing Huan Pang institute of New Energy on Chemical Storage and Power Sources School of Chemical and Environmental EngineeringYancheng Teachers UniversityYancheng 224000China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225009China Department of Chemical Engineering University of Waterloo200 University Avenue WestWaterlooOntario N2L 3G1Canada

Aqueous rechargeable batteries(ARBs)are generally safer than non-aqueous analogues,they are also less-expensive,and more friendly to the ***,the inherent disadvantage of the narrow electrochemical window of H2O seriously restricts the energy density and output voltage of ARBs,especially aqueous rechargeable Fe-based ***,we introduce a new battery system:the anode contains C@Fe/Fe_(2)O_(3)composite,which is interfaced with an alkaline electrolyte;the cathode contains LiMn_(2)O_()in contact with a neutral electrolyte.A Li^(+)-conducting membrane is carefully selected to decouple the electrode-electrolyte,which effectively widens the electrochemical window to above 2.65 V,thereby enables an aqueous rechargeable iron *** average output voltage is 1.83 V and its energy density is 235.3 Wh/kg at 549 W/*** this work,we propose the energy storage mechanism with the aid of density functional theory(DFT).The calculated reduction potential of the anode agrees with the experimental ***,this battery system demonstrates long cycle lifespan of approximately 2500 cycles at 2 A/g,corresponding to a capacity retention of 82.1%.These results are very far superior than those of mainstream aqueous rechargeable Fe-based batteries,which guarantee future investigation for storing electricity energy.

关键词： aqueous battery high voltage high energy iron oxide theoretical calculation

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Magnetocaloric effect and phase transition critical behavior of La0.75Sr0.25Mn0.9Co0.1O3 compound synthesized under the high pressure

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Tungsten 2024年第3期6卷 621-632页

作者： Jing Zhao Lei Gao Jian-Jun Zhao Wei Wei Hui-Qin Yun Ru Xing Huai-Jin Ma Xiang Jin Luo-Meng Chao School of Physical Science and Technology Key Laboratory of Magnetism and Magnetic Materials for Higher Education in Inner Mongolia Autonomous Region Baotou Teachers' College National Key Laboratory of Baiyunobo Rare Earth Resource Research and Comprehensive Utilization Baotou Research Institute of Rare Earths School of Physics and Electronic Information Inner Mongolia Normal University College of Science Inner Mongolia University of Science and Technology

In this study,a novel method is proposed for producing perovskite rare-earth manganese oxide magnetic refrigeration materials that exhibit superior properties compared to similar *** maximum magnetic entropy change values for this sample are 1.44 and 3.75 J·kg-1·K-1for magnetic fields of 2 and 7 T,***,its relative cooling power has been calculated to be 101.96 and 404.78 J·kg-1,indicating good *** results were obtained using the sample synthesized under a pressure of 4 GPa,and the sample has undergone a second phase *** critical behavior of the sample fits well with the mean field *** different magnetic fields,there is a significant overlap between the values of the maximum magnetic entropy change and the temperature-averaged entropy change,indicating that the refrigeration performance of the sample after high pressure can approach its maximum capability.

关键词： High-pressure synthesis Magnetocaloric effect Relative cooling power Magnetic phase transition

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Warming and increased precipitation alter soil carbon cycling in a temperate desert steppe of Inner Mongolia

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Journal of Plant Ecology 2024年第2期17卷 161-172页

作者： Mu Lan Xiao Qiu Wei La Huimin Wang Yahong Liu Liqing Zhao Hailian Sun Inner Mongolia Key Laboratory of Grassland Ecology and School of Ecology and Environment Inner Mongolia UniversityHohhot 010021China Inner Mongolia Academy of Agricultural and Animal Husbandry Sciences Hohhot 010031China State Key Laboratory of Vegetation and Environmental Change Institute of Botanythe Chinese Academy of SciencesBeijing 100093China College of Resources and Environment Baotou Teachers’CollegeBaotou 014030China

Warming and precipitation are key global change factors driving soil carbon(C)dynamics in terrestrial ***,the effects of warming and altered precipitation on soil microbial diversity and functional genes involved in soil C cycling remain largely *** investigated the effects of warming and increased precipitation on soil C cycling in a temperate desert steppe of Inner Mongolia using metagenomic *** found that warming reduced plant richness,Shannon-Wiener and Simpson *** contrast,increased precipitation signifcantly infuenced Shannon-Wiener and Simpson *** reduced soil microbial species by 5.4%while increased precipitation and warming combined with increased precipitation led to increases in soil microbial species by 23.3%and 2.7%,*** relative abundance of Proteobacteria,which involve C cycling genes,was signifcantly increased by warming and increased *** signifcantly reduced the abundance of GAPDH(Calvin cycle)and celF(cellulose degradation)while it enhanced the abundance of glxR(lignin degradation).Increased precipitation signifcantly enhanced the abundance of pgk(Calvin cycle),coxL(carbon monoxide oxidation),malZ(starch degradation),and mttB(methane production).Moreover,a wide range of correlations among soil properties and C cycling functional genes was detected,suggesting the synergistic and/or antagonistic relationships under scenario of global *** results may suggest that warming is benefcial to soil C storage while increased precipitation negatively affects soil C *** fndings provide a new perspective for understanding the response of microbial communities to warming and increased precipitation in the temperate desert steppe.

关键词： carbon cycling desert steppe functional genes global change soil microbes precipitation warming

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Influence of high-pressure heat treatment on magnetocaloric effects and magnetic phase transition in single crystal Gd3Ga5O12

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Journal of Rare Earths 2024年第11期42卷 2112-2118页

作者： Xiang Jin Jing Zhao Lei Gao Huaijin Ma Haschuluu Oimod Hongwei Zhu Qi Li Taichao Su Hongyu Zhu Tegus O Jianjun Zhao Inner Mongolia Key Laboratory for Physics and Chemistry of Functional Materials Inner Mongolia Normal University School of Physical Science and Technology Baotou Teachers' CollegeKey Laboratory of Magnetism and Magnetic Materials for Higher Education in Inner Mongolia Autonomous Region National Key Laboratory of Baiyunobo Rare Earth Resource Researches and Comprehensive Utilization Baotou Research Institute of Rare Earths College of Science Guilin University of Technology

The magnetic properties and magnetic phase transition critical behavior of Gd3Ga5O12single crystals subjected to high-pressure heat treatment were *** results show that high-pressure heat treatment reduces the Curie temperature and magnetization of the *** a magnetic field change of 5 T,the maximum isothermal magnetic entropy of the sample is approximately 19.73 J/（kg·K）.High-pressure heat treatment increases the phase transition temperature range and leads to an increase in the magnetic refrigeration *** Gd3Ga5O12single crystals and the high-pressure heat-treated sample undergo a second-order phase *** critical behavior of the samples aligns with the mean field model acquired via critical model *** indicates that the samples exhibit long-range exchange interactions in the system near the Curie ***,this material can be used as a magnetic refrigerant for low-temperature applications.

关键词： High-pressure heat treatment Magnetic phase transition Magnetic refrigeration Magnetocaloric effect Rare earths

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Comparative Study of the Reliability and Complexity of Symmetrical and Asymmetrical Cryptosystems for the Protection of Academic Data in the Democratic Republic of Congo

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Journal of Information Security 2024年第3期15卷 299-307页

作者： Mugaruka Buduge Gulain Jeremie Ndikumagenge Buhendwa Nyenyezi Justin Bulonza Masumbuko Alexis Katho Seba Jacques Department of Management Computing for Companies Section of Commercial and Computing Sciences Teachers Training College of Bukavu Bukavu The Democratic Republic of the Congo Center of Research in Infracture Environment and Technology (CRIET) Doctoral School University of Burundi Bujumbura Burundi Department of Maths-Physics Section of Exact Sciences Teachers Training College of Bukavu Bukavu The Democratic Republic of the Congo Higher institute of Medical Techniques of Bukavu Bukavu The Democratic Republic of the Congo Department of Maths-Physics Section of Exact Sciences Teachers Training College of Bunia Bunia The Democratic Republic of the Congo

In the digital age, the data exchanged within a company is a wealth of knowledge. The survival, growth and influence of a company in the short, medium and long term depend on it. Indeed, it is the lifeblood of any modern company. A companys operational and historical data contains strategic and operational knowledge of ever-increasing added value. The emergence of a new paradigm: big data. Today, the value of the data scattered throughout this mother of knowledge is calculated in billions of dollars, depending on its size, scope and area of intervention. With the rise of computer networks and distributed systems, the threats to these sensitive resources have steadily increased, jeopardizing the existence of the company itself by drying up production and losing the interest of customers and suppliers. These threats range from sabotage to bankruptcy. For several decades now, most companies have been using encryption algorithms to protect and secure their information systems against the threats and dangers posed by the inherent vulnerabilities of their infrastructure and the current economic climate. This vulnerability requires companies to make the right choice of algorithms to implement in their management systems. For this reason, the present work aims to carry out a comparative study of the reliability and effectiveness of symmetrical and asymmetrical cryptosystems, in order to identify one or more suitable for securing academic data in the DRC. The analysis of the robustness of commonly used symmetric and asymmetric cryptosystems will be the subject of simulations in this article.

关键词： Comparative Study Cryptosystems Symmetric Encryption Asymmetric Encryption

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Loss of the accessory chromosome converts a pathogenic tree-root fungus into a mutualistic endophyte

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Plant Communications 2024年第1期5卷 164-180页

作者： Huanshen Wei Zhenhui Zhong Zhongfeng Li Yuwei Zhang Eva H.Stukenbrock Boping Tang Ningning Yang Riccardo Baroncelli Long Peng Zhuo Liu Xinghua He Yuzhan Yang Zhilin Yuan State Key Laboratory of Tree Genetics and Breeding Chinese Academy of ForestryBeijing 100091China Research institute of Subtropical Forestry Chinese Academy of ForestryHangzhou 311400China State Key Laboratory of Ecological Pest Control for Fujian and Taiwan Crops Fujian Agriculture and Forestry UniversityFuzhou 350002China Environmental Genomics Christian-Albrechts University24118 KielGermany Max Planck Fellow Group Environmental Genomics Max Planck Institute for Evolutionary Biology24306 PlonGermany Jiangsu Key Laboratory for Bioresources of Saline Soils School of WetlandsYancheng Teachers UniversityYancheng 224002China Department of Agricultural and Food Sciences(DISTAL) University of Bologna40127 BolognaItaly

Some fungal accessory chromosomes(ACs)may contribute to virulence in ***,the mecha-nisms by which ACs determine specific traits associated with lifestyle transitions along a symbiotic contin-uum are not *** we delineated the genetic divergence in two sympatric but considerably variable isolates(16B and 16W)of the poplar-associated fungus Stagonosporopsis *** identified a-0.6-Mb horizontally acquired AC in 16W that resulted in a mildly parasitic lifestyle in *** deletion of the AC(D16W)significantly altered the fungal ***,D16W was morphologically more similar to 16B,showed enhanced melanization,and established beneficial interactions with poplar plants,thereby acting as a dark septate *** sequencing(RNA-seq)analysis showed that AC loss induced the upregulation of genes related to root colonization and biosynthesis of indole acetic acid and *** observed that the AC maintained a more open status of chromatin across the genome,indicating an impressive remodeling of cis-regulatory elements upon AC loss,which potentially enhanced symbiotic *** demonstrated that the symbiotic capacities were non-host-specific through comparable experiments on Triticum–and Arabidopsis–fungus ***,the three isolates generated symbiotic interactions with a nonvascular *** summary,our study suggests that the AC is a suppressor of symbiosis and provides insights into the underlying mechanisms of mutualism with vascular plants in the absence of traits encoded by the *** speculate that AC-situ-ated effectors and other potential secreted molecules may have evolved to specifically target vascular plants and promote mild virulence.

关键词： dark septate endophytes effectors lifestyle transition root–fungus symbioses

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Geometries, Electronic Structures, and Electron Detachment Energies of Small Boron Sulfide Anions: A Density Functional Theory Investigation

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Chinese Journal of Structural Chemistry 2008年第6期27卷 651-658页

作者：郭巧灵郭谨昌李思殿 Department of Chemistry Taiyuan Teachers' College institute of Materials Science and Department of Chemistry Xinzhou Teachers' University institute of Materials Science and Department of Chemistry Xinzhou Teachers’ University

A density functional theory investigation on the geometries, electronic structures, and electron detachment energies of BS, BS2, B（BS）2 and B（BS）3 has been performed in this work. The linear ground-state structures of BS （C∞v, ^1∑^＋） and BS2^- （O∞h, ^1∑g^＋） prove to be similar to the previously reported BO and BO2 with systematically lower electron detachment energies. Small boron sulfide clusters are found to favor the formation of -B=S groups which function basically as a-radicals and dominate the ground-state structures of the systems. The perfect linear B（BS）2^-（D∞h, ^3∑g） and beautiful equilateral triangle B（BS）3^- （D3h,^2A1”） turn out to be analogous to the well-known C2v BH2 and O3h BH3, respectively. The electron affinities of BS, BS2, B（BS）2 and B（BS）3 are predicted to be 2.3, 3.69, 3.00 and 3.45 eV, respectively. The electron detachment energies calculated for BS^-, BS2^-, B（BS）2^-, and B（BS）3^- may facilitate future photoelectron spectroscopy measurements to characterize the geometrical and electronic structures of these anions.

关键词： boron sulfides density functional theory geometries electronic structures electron detachment energies photoelectron spectroscopy

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Development of in situ characterization techniques in molecular beam epitaxy

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Journal of Semiconductors 2024年第3期45卷 9-32页

作者： Chao Shen Wenkang Zhan Manyang Li Zhenyu Sun Jian Tang Zhaofeng Wu Chi Xu Bo Xu Chao Zhao Zhanguo Wang Laboratory of Solid State Optoelectronics Information Technology Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China College of Materials Science and Opto-Electronic Technology University of Chinese Academy of SciencesBeijing 101804China School of Physics Science and Technology Xinjiang UniversityUrumqi 830046China School of New Energy and Electronics Yancheng Teachers UniversityYancheng 224002China Key Laboratory of Optoelectronic Materials and Devices Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China

Ex situ characterization techniques in molecular beam epitaxy(MBE)have inherent limitations,such as being prone to sample contamination and unstable surfaces during sample transfer from the MBE *** recent years,the need for improved accuracy and reliability in measurement has driven the increasing adoption of in situ characterization *** techniques,such as reflection high-energy electron diffraction,scanning tunneling microscopy,and X-ray photoelectron spectroscopy,allow direct observation of film growth processes in real time without exposing the sample to air,hence offering insights into the growth mechanisms of epitaxial films with controlled *** combining multiple in situ characterization techniques with MBE,researchers can better understand film growth processes,realizing novel materials with customized properties and extensive *** review aims to overview the benefits and achievements of in situ characterization techniques in MBE and their applications for material science *** addition,through further analysis of these techniques regarding their challenges and potential solutions,particularly highlighting the assistance of machine learning to correlate in situ characterization with other material information,we hope to provide a guideline for future efforts in the development of novel monitoring and control schemes for MBE growth processes with improved material properties.

关键词： epitaxial growth thin film in situ characterization molecular beam epitaxy(MBE)

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