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Mixing states and secondary formation processes of organic nitrogen-containing single particles in Guangzhou,China

Journal of environmental Sciences 2024年第4期138卷 62-73页

作者： Lijun Yun Chunlei Cheng Suxia Yang Zaihua Wang Mei Li Qi En Zhong LiyuanMao Sulin Liu Xiaoya Cheng Duanying Chen Fan Yang Zhen Zhou institute of Mass Spectrometry and Atmospheric environment Guangdong Provincial Engineering Research Center for on-line source apportionment system of air pollutionJinan UniversityGuangzhou 510632China Guangdong-Hongkong-Macao Joint Laboratory of Collaborative Innovation for environmental Quality Guangzhou 510632China State Key Laboratory of Loess and Quaternary Geology Institute of Earth EnvironmentChinese Academy ScienceXi’an 710061China institute for environment and Climate Research Jinan UniversityGuangzhou 510632China Guangdong Academy of Sciences Institute of Resources Utilization and Rare Earth DevelopmentGuangzhou 510650China environmental Monitoring Station of Pudong New District Shanghai 201200China

Organic nitrogen(ON)compounds play a significant role in the light absorption of brown carbon and the formation of organic aerosols,however,the mixing state,secondary formation processes,and influencing factors of ON compounds are still *** paper reports on the mixing state of ON-containing particles based on measurements obtained using a highperformance single particle aerosol mass spectrometer in January 2020 in *** ON-containing particles accounted for 21% of the total detected single particles,and the particle count and number fraction of the ON-containing particles were two times higher at night than during the *** prominent increase in the content of ON-containing particles with the enhancement of NO_xmainly occurred at night,and accompanied by high relative humidity and nitrate,which were associated with heterogeneous reactions between organics and gaseous NO_(x)and/or NO_(3)*** synchronous decreases in ON-containing particles and the mass absorption coefficient of water-soluble extracts at 365 nm in the afternoon may be associated with photo-bleaching of the ON species in the *** addition,the positive matrix factorization analysis found five factors dominated the formation processes of ON particles,and the nitrate factor(33%)mainly contributed to the production of ON particles at *** results of this study provide unique insights into the mixing states and secondary formation processes of the ON-containing particles.

关键词： Organic nitrogen compounds Single particles Mixing state Secondary formation Nighttime chemistry

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Effects of operating conditions on iron(hydr)oxides evolution and ciprofloxacin degradation in potassium ferrate-ozone stepwise oxidation system

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Journal of environmental Sciences 2024年第1期135卷 367-378页

作者： Xiaochen Li Yifan Wang Ning Wang Mei Li Maomao Bai Jingtao Xu Hongbo Wang School of Municipal and environmental Engineering Shandong Jianzhu UniversityJinan 250101China Resources and environment Innovation institute Shandong Jianzhu UniversityJinan 250101China

In this study,a stepwise oxidation system of potassium ferrate(K_(2)FeO_(4))combined with ozone(O+3)was used to degrade ciprofloxacin(CIP).The effects of pH and pre-oxidation time of K_(2)FeO_(4) on the evolution of K_(2)FeO_(4) reduction products(iron(hydr)oxides)and CIP degradation were *** was found that in addition to its own oxidation capacity,K_(2)FeO_(4) can also influence the treatment effect of CIP by changing the catalyst *** presence of iron(hydr)oxides effectively enhanced the mineralization rate of CIP by catalyzing *** pH value can influence the content and types of the components with catalytic ozonation effect in iron(hydr)*** K_(2)FeO_(4) pre-oxidation stage can produce more iron(hydr)oxides with catalytic components for subsequent ozonation,but the evolution of iron(hydr)oxides components was influenced by O_(3) *** can also avoid the waste of oxidation capacity owing to the oxidation of iron(hydr)oxides by O_(3) and free *** intermediate degradation products were identified by Fourier transform ion cyclotron resonance mass spectrometry(FT-ICR-MS).Besides,the degradation pathways were *** the degradation products of CIP,the product with broken quinolone ring structure only appeared in the stepwise oxidation system.

关键词： Potassium ferrate reduction products Catalytic ozonation Ciprofloxacin Potassium ferrate pre-oxidation time

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Precipitation and anthropogenic activities regulate the changes of NDVI in Zhegucuo Valley on the southern Tibetan Plateau

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Journal of Mountain Science 2024年第2期21卷 607-618页

作者： ZHAO Wanglin WANG Hengying ZHANG Huifang ZHANG Lin School of Ecology and environment Tibet UniversityLhasa 850000China institute of Tibetan Plateau Research Chinese Academy of SciencesBeijing 100101China Southwest Survey and Planning institute of National Forestry and Grassland Administration Kunming 650000China Monitoring Center for Ecological environment of Xizang Autonomous Region Lhasa 850000China

Whether climate change or anthropogenic activities play a more pivotal role in regulating vegetation growth on the Tibetan Plateau is still controversial.A better understanding on grassland changes at a fine scale may provide important guidance for local government policy and grassland *** two of the most reliable satellite NDVI products(MODIS NDVI and SPOT NDVI),we evaluated the dynamic of grasslands in the Zhegucuo valley on the southern Tibetan Plateau from 2000 to 2020,and analyzed its driving factors and relative influences of climate change and anthropogenic ***,the key indicators of climate change were assumed to be precipitation and *** main results were:(1)the grassland NDVI in Zhegucuo valley did not reflect a significant temporal change during the last 21 *** variation of precipitation during the early growing season(GSP)resembled that of NDVI,and the GSP was positively correlated with *** the pixel level,the partial correlation analysis showed that 37.79%of the pixels depicted a positive relationship between GSP and NDVI,while 11.32%of the pixels showed a negative relationship between temperature during the early growing season(GST)and NDVI.(2)In view of the spatial distribution,the areas mainly controlled by GSP were generally distributed in the southern part,while those affected by GST stood in the eastern part,mainly around the Zhegucuo lake where most population in Cuomei County settled down.(3)Decreasing NDVI trends were mainly occurred in alpine steppe at lower elevations rather than alpine meadow at higher elevations.(4)The residual trend(RESTREND)analysis further indicated that the anthropogenic activities played a more pivotal role in regulating the annual changes of NDVI rather than climate factors in this *** studies should pay more attention on climate extremes rather than the simple temporal ***,the influence of human activities on alpine grassland needs to be accessed and fully

关键词： Anthropogenic activities Climate change Precipitation Fencing Vegetation degradation

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Regulating solid electrolyte interphase film on fluorinedoped hard carbon anode for sodium-ion battery

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Carbon Energy 2024年第6期6卷 200-215页

作者： Cuiyun Yang Wentao Zhong Yuqiao Liu Qiang Deng Qian Cheng Xiaozhao Liu Chenghao Yang Guangzhou Key Laboratory for Surface Chemistry of Energy Materials New Energy Research InstituteSchool of Environment and EnergySouth China University of TechnologyGuangzhouChina

For the performance optimization strategies of hard carbon,heteroatom doping is an effective way to enhance the intrinsic transfer properties of sodium ions and electrons for accelerating the reaction ***,the previous work focuses mainly on the intrinsic physicochemical property changes of the material,but little attention has been paid to the resulting interfacial regulation of the electrode surface,namely the formation of solid electrolyte interphase(SEI)*** this work,element F,which has the highest electronegativity,was chosen as the doping source to,more effectively,tune the electronic structure of the hard *** effect of F-doping on the physicochemical properties of hard carbon was not only systematically analyzed but also investigated with spectroscopy,optics,and in situ characterization techniques to further verify that appropriate F-doping plays a positive role in constructing a homogenous and inorganic-rich SEI *** experimentally demonstrated link between the electronic structure of the electrode and the SEI film properties can reframe the doping optimization strategy as well as provide a new idea for the design of electrode materials with low reduction kinetics to the *** a result,the optimized sample with the appropriate F-doping content exhibits the best electrochemical performance with high capacity(434.53 mA h g^(-1)at 20mA g^(-1))and excellent rate capability(141 mAh g^(-1)at 400 mA g^(-1)).

关键词： F-doping hard carbon reduction kinetics sodium-ion batteries solid electrolyte interphase film

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Peroxidase-like active Cu-ZIF-8 with rich copper(I)-nitrogen sites for excellent antibacterial performances toward drug-resistant bacteria

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Nano Research 2024年第8期17卷 7427-7435页

作者： Xiaoze Wang Hui Wang Jingkun Zhang Ning Han Wenjun Ma Donghai Zhang Mingshui Yao Xianliang Wang Yunfa Chen State Key Laboratory of Mesoscience and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of the Chinese Academy of Sciences Beijing 100049China Laboratory of Theoretical and Computational Nanoscience CAS Key Laboratory of Nanosystem and Hierarchial FabricationCAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China China CDC Key Laboratory of environment and Population health National Institute of Environmental HealthChinese Center for Disease Control and PreventionBeijing 100021China

Bacterial pathogens pose a serious threat to human health,and there is an urgent need to develop highly effective antibacterial materials to eliminate the increasingly serious contamination of drug-resistant ***,a Cu-doped ZIF-8 particle with unsaturated copper exhibits high peroxidase-like activity.99.998%antibacterial efficiency against *** can be achieved for 30 min at a low concentration of 50μg·mL^(−1),as well as complete sterilization against ***(up to 8 log).99.999%antibacterial efficiency against Methicillin-resistant Staphylococcus aureus can be achieved,performing orders of magnitude higher than *** mechanism shows that the unsaturated Cu-Nx sites are enzyme-like active centers,which could promote the consumption of bacteria reducing substances by H_(2)O_(2),and the generated*OH further aggravates bacterial oxidative stress and membrane *** importantly,the oxidation activity of adsorbed oxygen species on Cu-ZIF-8 is enhanced by charge transfer and structural changes between the ligand and copper center like natural ***-doped ZIF-8 with peroxidase-like activity shows great potential in antibacterial application and the revealed catalytic mechanism is helpful for understanding the high antibacterial activity of nanoparticles with Cu-Nx sites.

关键词： Cu-doped ZIF-8 peroxidase-like reactive oxygen species(ROS) catalytic mechanism antibacterial activity

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Hard carbon for sodium storage:Mechanism and performance optimization

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Nano Research 2024年第7期17卷 6038-6057页

作者： Yongxin Wang Meng Li Yu Zhang Naiqing Zhang State Key Laboratory of Urban Water Resource and environment School of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001China School of Energy Science and Engineering Harbin Institute of TechnologyHarbin 150001China

Due to the shortage of lithium resource reserves and the pressure of rising prices,sodium-ion batteries have regained the attention of the public,and shown great potential for application in the fields of grid energy storage and low-speed vehicles to achieve the purpose of complementing lithium-ion batteries,so it is imperative to promote the commercial application of sodiumion *** sodium-ion battery anode materials,hard carbon is the material most likely to be used ***,there is still much work to be done before its *** review provides a comprehensive overview of the current research status from the following three ***,the microstructure and sodium storage active sites of hard carbon are ***,the mechanism of sodium storage in hard carbon is investigated,which can be broadly categorized into four model,“insertion–filling”,“adsorption–insertion”,“adsorption–filling”,and“multistage”.Finally,from the perspective of improving the electrochemical performance of hard carbon,the performance improvement strategies proposed in recent years are *** with the performance of hard carbon commercial products of some enterprises,the future development goal of hard carbon is prospected,hoping that all sectors of society can work hard for this common goal.

关键词： sodium-ion battery hard carbon mechanism performance optimization

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Exploring the blindspot:The soil plastisphere

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Soil Ecology Letters 2024年第2期6卷 1-4页

作者： Xiaoxuan Su Kai Yang Interdisciplinary Research Center for Agriculture Green Development in Yangtze River Basin Southwest UniversityChongqing400715China Key Laboratory of Urban environment and health Institute of Urban EnvironmentChinese Academy of SciencesXiamen361021China

Plastic pollution is a growing concern in soil ecosystems *** accumulation of(micro)plastic debris leads to a unique microenvironment,termed the“plastisphere.”Notably,the dynamics and behaviors of the soil plastisphere diverge from its marine counterpart,where it is initially defined,thereby likely exhibiting an uncharacterized feature in ecological effects and *** understanding of the soil plastisphere holds significant implications for environmental science and practical applications in pollution management and agricultural *** with the oceanic plastisphere,research on the soil plastisphere is still in its infancy with limited but significant studies contributing to current knowledge.A recent seminal work by Rillig et al.(Rillig et al.,*** Reviews ***:10.1038/s41579-023-00967-2)has inspired us and provided comprehensive insights into the characteristics and function of the soil *** this commentary,we present core aspects of the soil plastisphere,encompassing its microbial communities,biogeochemical processes,and ecological implications,as well as highlight current methodologies probing this domain.

关键词： soil pollution thereby

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Straw mulching alters the composition and loss of dissolved organic matter in farmland surface runoff by inhibiting the fragmentation of soil small macroaggregates

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Journal of Integrative Agriculture 2024年第5期23卷 1703-1717页

作者： Shanshan Cai Lei Sun Wei Wang Yan Li Jianli Ding Liang Jin Yumei Li Jiuming Zhang Jingkuan Wang Dan Wei College of Land and environment Shenyang Agricultural UniversityShenyang 110866China Heilongjiang Academy of Black Soil Conservation and Utilization Harbin 150086China institute of Plant Nutrition Resources and EnvironmentBeijing Academy of Agricultural and Forestry SciencesBeijing 100097China

Straw mulching is a widespread practice for reducing the soil carbon loss caused by ***,the effects of straw mulching on dissolved organic matter(DOM)runoff loss from black soil are not well *** straw mulching affects the composition and loss of runoff DOM by changing soil aggregates remains largely ***,a straw mulching treatment was compared to a no mulching treatment(as a control)on sloping farmland with black soil erosion in Northeast *** divided the soil into large macroaggregates(>2 mm),small macroaggregates(0.25-2 mm),and microaggregates(<0.25 mm).After five rain events,the effects of straw mulching on the concentration(characterized by dissolved organic carbon(DoC)and composition(analyzed by fluorescence spectroscopy)of runoff and soil aggregate DOM were *** results showed that straw mulching reduced the runoff amount by 54.7%.Therefore,although straw mulching increased the average DOc concentration in runoff,it reduced the total runoff DOM loss by 48.3%.The composition of runoff DOM is similar to that of soil,as both contain humic-like acid and protein-like *** straw mulching treatment,the protein-like components in small macroaggregates accumulated and the protein-like components in runoff declined with rain *** spectroscopy technology may help in understanding the hydrological paths of rain events by capturing the dynamic changes of runoff and soil DOM characteristics.A variation partitioning analysis(VPA)indicated that the DOM concentration and composition of microaggregates explained 68.2%of the change in runoff DOM from no mulching plots,while the change in runoff DOM from straw mulching plots was dominated by small macroaggregates at a rate of 55.1%.Taken together,our results demonstrated that straw mulching reduces the fragmentation of small macroaggregates and the loss of microaggregates,thus effecting DOM compositions in soil and reducing the DOM loss in *** results provi

关键词： dissolved organic matter black soil surface runoff aggregates fluorescence spectrum

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Spatiotemporal dynamics of city-level WEEE generation from different sources in China

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Frontiers of Engineering Management 2024年第2期11卷 181-193页

作者： Wanjun WANG Yupeng LIU Kuishuang FENG Wei-Qiang CHEN Key Research institute of Yellow River Civilization and Sustainable Development&Collaborative Innovation Center of Yellow River Civilization Henan UniversityKaifeng 475001China Key Laboratory of Urban environment and health Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China Department of Geographical Sciences University of MarylandCollege ParkUSA

China stands as one of the leading producers of waste electrical and electronic equipment(WEEE),facing significant challenges in managing the substantial volumes *** existing regulations,the informal treatment of WEEE persists in some areas due to inadequate recycling networks at the city ***,there is a critical need for a detailed geographical mapping of WEEE generation to address improper disposal practices *** study introduces the cMAC–EEEs(city Material Cycles and Manufactured Capital–EEEs)database,providing estimates of WEEE generation across approximately 300 prefecture-level cities from 1978 to *** focuses on five commonly used types of electrical and electronic equipment(refrigerators,air conditioners,washing machines,computers,TVs)originating from three key sources(urban residents,rural residents,enterprises).The findings reveal(1)significant spatial variation in WEEE generation within China,with eastern and central city clusters identified as hotspots,particularly for urban residents and enterprises,while the western region exhibits the highest growth rate in WEEE generation,notably among rural residents.(2)The growth in obsolete computers and air conditioners is prominent,especially in rural areas and among enterprises,whereas the generation of obsolete TVs,washing machines,and refrigerators is leveling off and expected to decrease in some urban areas.(3)Enterprises account for a substantial portion of WEEE generation,though uncertainties exist,necessitating further *** study highlights that less developed regions lack adequate recycling facilities,with specific limitations in refrigerators and air conditioners recycling *** enhance WEEE management,it advocates for increased interregional collaboration and capacity building in less developed ***,the regulation of WEEE from private enterprises requires *** the product level,a greater focus on recycling practices

关键词： WEEE obsolete electrical and electronic equipment urban mining waste management industrial ecology

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Unlocking the potential of thin-film composite reverse osmosis membrane performance:Insights from mass transfer modeling

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Chinese Chemical Letters 2024年第5期35卷 66-76页

作者： Kexin Yuan Yulei Liu Haoran Feng Yi Liu Jun Cheng Beiyang Luo Qinglian Wu Xinyu Zhang Ying Wang Xian Bao Wanqian Guo Jun Ma State Key Laboratory of Urban Water Resource and environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China College of Architecture and environment Sichuan UniversityChengdu 610065China School of Municipal and environmental Engineering Shandong Jianzhu UniversityJi’nan 250101China College of Water Conservancy and Hydropower Engineering Sichuan Agricultural UniversityYaan 625014China

Thin-film composite(TFC)reverse osmosis(RO)membranes have attracted considerable attention in water treatment and desalination processes due to their specific separation ***,the trade-off effect between water flux and salt rejection poses huge challenges to further improvement in TFC RO membrane *** research works have been dedicated to optimizing membrane fabrication and modification for addressing this *** the meantime,several reviews summarized these ***,the existing reviews seldom analyzed these methods from a theoretical perspective and thus failed to offer effective optimization directions for the RO process from the root *** this review,we first propose a mass transfer model to facilitate a better understanding of the entire process of how water and solute permeate through RO membranes in detail,namely the migration process outside the membrane,the dissolution process on the membrane surface,and the diffusion process within the ***,the water and salt mass transfer behaviors obtained from model deduction are comprehensively analyzed to provide potential guidelines for alleviating the trade-off effect between water flux and salt rejection in the RO ***,inspired by the theoretical analysis and the accurate identification of existing bottlenecks,several promising strategies for both regulating RO membranes and optimizing operational conditions are proposed to further exploit the potential of RO membrane *** review is expected to guide the development of high-performance RO membranes from a mass transfer theory standpoint.

关键词： Reverse osmosis Mass transfer model Trade-off effect Membrane performance Optimization strategies

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