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Relative Impacts of Sea Ice Loss and Atmospheric Internal Variability on the Winter Arctic to East Asian Surface Air Temperature Based on Large-Ensemble Simulations with NorESM2

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Advances in Atmospheric Sciences 2024年第8期41卷 1511-1526页

作者： Shengping HE Helge DRANGE Tore FUREVIK Huijun WANG Ke FAN Lise Seland GRAFF Yvan J.ORSOLINI Geophysical institute University of Bergen and Bjerknes Centre for Climate ResearchBergen 5020Norway Nansen environmental and remote sensing Center Bergen 5007Norway Key Laboratory of Meteorological Disaster Ministry of Education/Joint International Research Laboratory of Climate and Environment Change(ILCEC)/Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters(CIC-FEMD)Nanjing University of Information Science&TechnologyNanjing 211544China Nansen-Zhu International Research Center Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai) Zhuhai 511458China School of Atmospheric Science Sun Yat-Sen Universityand Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai)Zhuhai 519082China Norwegian Meteorological institute Oslo 0313Norway Norwegian institute for Air Research Kjeller 2007Norway

To quantify the relative contributions of Arctic sea ice and unforced atmospheric internal variability to the “warm Arctic, cold East Asia”(WACE) teleconnection, this study analyses three sets of large-ensemble simulations carried out by the Norwegian Earth System Model with a coupled atmosphere–land surface model, forced by seasonal sea ice conditions from preindustrial, present-day, and future periods. Each ensemble member within the same set uses the same forcing but with small perturbations to the atmospheric initial state. Hence, the difference between the present-day(or future) ensemble mean and the preindustrial ensemble mean provides the ice-loss-induced response, while the difference of the individual members within the present-day(or future) set is the effect of atmospheric internal variability. Results indicate that both present-day and future sea ice loss can force a negative phase of the Arctic Oscillation with a WACE pattern in winter. The magnitude of ice-induced Arctic warming is over four(ten) times larger than the ice-induced East Asian cooling in the present-day(future) experiment;the latter having a magnitude that is about 30% of the observed cooling. Sea ice loss contributes about 60%(80%) to the Arctic winter warming in the present-day(future) experiment. Atmospheric internal variability can also induce a WACE pattern with comparable magnitudes between the Arctic and East Asia. Ice-lossinduced East Asian cooling can easily be masked by atmospheric internal variability effects because random atmospheric internal variability may induce a larger magnitude warming. The observed WACE pattern occurs as a result of both Arctic sea ice loss and atmospheric internal variability, with the former dominating Arctic warming and the latter dominating East Asian cooling.

关键词： Arctic sea ice loss warm Arctic–cold East Asia atmospheric internal variability large-ensemble simulation NorESM2 PAMIP

功能-要素-流视角下的乡村活力空间识别与评价——以中国杭州市临安区为例

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Journal of Geographical Sciences 2024年第6期34卷 1228-1250页

作者：张晶管晨悦章琳虞舟鲁叶成煊朱从谋李思楠王珂干牧野 institute of Applied remote sensing and Information Technology College of Environmental and Resource SciencesZhejiang UniversityHangzhou 310058China Zhejiang Key Research Laboratory of Agricultural remote sensing and Information Technology Hangzhou 310058China Shandong(Linyi)institute of Modern Agriculture Linyi 276000ShandongChina Huzhou Spatial Planning Preparation and Research Center Huzhou 313000ZhejiangChina Zhejiang Digital Governance Space Planning and Design Co. Ltd.Hangzhou 310000China Department of Land Resources Management Zhejiang Gongshang UniversityHangzhou 310018China

Rural vitality is the life force expressed by a combination of endogenous dynamics and external influences. Exploring the complex relationship between rural functions, elements and flows could achieve sustainable rural development. This study constructed a theoretical framework guided by the four functions of production, living, ecology and culture with the support of mobile big data. Furthermore, the network centrality of villages was estimated to reflect the intensity of urban-rural social mobility ties. The results indicated marked spatial disparities in rural vitality, and the coupling of ecological-cultural vitality has a high degree of coherence. Four rural vitality grades were identified: high level(38, 14.08%), medium-high level(66, 24.44%), medium-low level(110, 40.74%) and low level(56, 20.74%), covering 270 administrative village units. The flow intensity of social linkage elements is consistent with rural vitality and the socioeconomic spillover effect of urban centers on neighboring villages was noticeable. Topographic complexity negatively affected the living function, mainly in the T1 and T2 terrain gradients;the rural ecological function was not fully correlated with urban adjacency, and proximity could lead to adverse effects such as urban sprawl and resource destruction. The application of this study is to explore the importance of “flow” by utilizing mobile big data to refine the evaluation unit to the village scale. Accelerating the construction of network coverage and information interconnection and promoting the elemental flow of people, transportation and information between urban and rural areas are important ways to enhance rural vitality.

关键词： rural vitality rural multifunction elements urban-rural flows mobile big data

Application of Optical Hydrogels in environmental sensing

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Energy & environmental Materials 2024年第3期7卷 315-340页

作者： Shuo Yang Shruti Sarkar Xing Xie Dan Li Jianmin Chen Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3) Department of Environmental Science and EngineeringFudan University School of Civil and environmental Engineering Georgia Institute of Technology

The ever-increasing complexity of environmental pollutants urgently warrants the development of new detection *** based on the optical properties of hydrogels enabling fast and easy in situ detection are attracting increasing *** this paper,the data from 138 papers about different optical hydrogels (OHs) are extracted for statistical *** detection performance and potential of various types of OHs in different environmental pollutant detection scenarios were evaluated and compared to those obtained using the standard detection *** on this analysis,the target recognition and sensing mechanisms of two main types of OHs are reviewed and discussed:photonic crystal hydrogels (PCHs) and fluorescent hydrogels (FHs).For PCHs,the environmental stimulus response,target receptors,inverse opal structures,and molecular imprinting techniques related to PCHs are reviewed and ***,the different types of fluorophores (i.e.,compound probes,biomacromolecules,quantum dots,and luminescent microbes) of FHs are ***,the potential academic research directions to address the challenges of applying and developing OHs in environmental sensing are proposed,including the fusion of various OHs,introduction of the latest technologies in various fields to the construction of OHs,and development of multifunctional sensor arrays.

关键词： environmental sensors fluorescent hydrogel optical hydrogel photonic crystal hydrogel pollution detection

Turbulent Image Restoration in Atmosphere with Cyclopean Processing via Binocular Fusion

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Chinese physics Letters 2024年第8期41卷 33-38页

作者： Han Yao Jin-Yan Lin Li-Bang Chen Yi-Kun Liu Jian-Ying Zhou State Key Laboratory of Optoelectronic Materials and Technologies School of PhysicsSun Yat-Sen UniversityGuangzhou 510275China Guangdong Provincial Key Laboratory of Quantum Metrology and sensing School of Physics and AstronomySun Yat-Sen University(Zhuhai Campus)Zhuhai 519082China

The outstanding issue to overcoming atmospheric turbulence on distant imaging is a fundamental interest and technological *** propose a novel scenario and technique to restore the optical image in turbulent environmental by referring to Cyclopean image with binocular *** human visual intelligence,image distortion resulting from the turbulence is shown to be substantially *** simulation results taking into account of the atmospheric turbulence,optical image system,image sensors,display and binocular vision perception are presented to demonstrate the robustness of the image restoration,which is compared with a single channel planar optical imaging and *** involving binocular telescope,image recording and the stereo-image display is conducted and good agreement is obtained between the simulation with perceptive experience.A natural extension of the scenario is to enhance the capability of anti-vibration or anti-shaking for general optical imaging with Cyclopean image.

关键词： image turbulence shaking

Surface-modified Ag@Ru-P25 for photocatalytic CO_(2) conversion with high selectivity over CH_(4) formation at the solid–gas interface

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Carbon Energy 2024年第1期6卷 182-196页

作者： Chaitanya B.Hiragond Sohag Biswas Niket SPowar Junho Lee Eunhee Gong Hwapyong Kim Hong Soo Kim Jin-Woo Jung Chang-Hee Cho Bryan M.Wong Su-Il In Department of Energy Science&Engineering Daegu Gyeongbuk Institute of Science and Technology(DGIST)DaeguRepublic of Korea Department of Chemical&environmental Engineering Materials Science&Engineering ProgramDepartment of ChemistryDepartment of Physics&AstronomyUniversity of California-RiversideRiversideCaliforniaUSA Department of physics and Chemistry Daegu Gyeongbuk Institute of Science and Technology(DGIST)DaeguRepublic of Korea NiceScience Corporation DaeguRepublic of Korea

Systematic optimization of the photocatalyst and investigation of the role of each component is important to maximizing catalytic activity and comprehending the photocatalytic conversion of CO_(2) reduction to solar fuels.A surface-modified Ag@Ru-P25 photocatalyst with H_(2)O_(2) treatment was designed in this study to convert CO_(2) and H_(2)O vapor into highly selective *** doping followed by Ag nanoparticles(NPs)cocatalyst deposition on P25(TiO_(2))enhances visible light absorption and charge separation,whereas H_(2)O_(2) treatment modifies the surface of the photocatalyst with hydroxyl(–OH)groups and promotes CO_(2) ***-resonance transmission electron microscopy,X-ray photoelectron spectroscopy,X-ray absorption near-edge structure,and extended X-ray absorption fine structure techniques were used to analyze the surface and chemical composition of the photocatalyst,while thermogravimetric analysis,CO_(2) adsorption isotherm,and temperature programmed desorption study were performed to examine the significance of H_(2)O_(2) treatment in increasing CO_(2) reduction *** optimized Ag1.0@Ru1.0-P25 photocatalyst performed excellent CO_(2) reduction activity into CO,CH4,and C2H6 with a~95%selectivity of CH4,where the activity was~135 times higher than that of pristine TiO_(2)(P25).For the first time,this work explored the effect of H_(2)O_(2) treatment on the photocatalyst that dramatically increases CO_(2) reduction activity.

关键词： gas-phase CO_(2) reduction H_(2)O_(2) treatment plasmonic nanoparticles solar fuel photocatalyst surface modification

Data error propagation in stacked bioclimatic envelope models

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Integrative Zoology 2024年第2期19卷 262-276页

作者： Xueyan LI Babak NAIMI Peng GONG Miguel B.ARAÚJO Guangdong Provincial Key Laboratory of remote sensing and Geographical Information System Guangdong Open Laboratory of Geospatial Information Technology and ApplicationGuangzhou Institute of GeographyGuangdong Academy of ScienceGuangzhouChina ‘Rui Nabeiro’Biodiversity Chair CHANGE-MED InstituteUniversity ofÉvoraÉvoraPortugal Department of Geography and Department of Earth Sciences University of Hong KongHong KongChina Department of Biogeography and Global Change National Museum of Natural SciencesCSICMadridSpain

Stacking is the process of overlaying inferred species potential distributions for multiple species based on outputs of bioclimatic envelope models(BEMs).The approach can be used to investigate patterns and processes of species *** data limitations on individual species distributions are inevitable,but how do they affect inferences of patterns and processes of species richness?We investigate the influence of different data sources on estimated species richness gradients in *** fitted BEMs using species distributions data for 334 bird species obtained from(1)global range maps,(2)regional checklists,(3)museum records and surveys,and(4)citizen science data using presence-only(Mahalanobis distance),presence-background(MAXENT),and presence–absence(GAM and BRT)*** species predictions were stacked to generate species richness ***,we show that different data sources and BEMs can generate spatially varying gradients of species *** environmental predictors that best explained species distributions also differed between data *** using citizen-based data had the highest accuracy,whereas those using range data had the lowest *** richness patterns estimated by GAM and BRT models were robust to data *** multiple data sets exist for the same region and taxa,we advise that explicit treatments of uncertainty,such as sensitivity analyses of the input data,should be conducted during the process of modeling.

关键词： richness patterns species distribution stacked bioclimatic envelope models uncertainty

Characteristics and source apportionment of ambient volatile organic compounds and ozone generation sensitivity in urban Jiaozuo,China

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Journal of environmental Sciences 2024年第4期138卷 607-625页

作者： Pengzhao Li Chun Chen Dan Liu Jie Lian Wei Li Chuanyi Fan Liangyu Yan Yue Gao Miao Wang Hang Liu Xiaole Pan Jing Mao State Centre for International Cooperation on Designer Low-Carbon and environmental Materials School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China Henan Key Laboratory of environmental Monitoring Technology Henan Ecological Environment Monitoring and Safety CenterZhengzhou 450046China Jiaozuo Ecological Environment Monitoring Center of Henan Province Jiaozuo 454003China State Key Laboratory of Atmospheric Boundary Layer physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China

In recent years,many cities have taken measures to reduce volatile organic compounds(VOCs),an important precursor of ozone(O_(3)),to alleviate O_(3) pollution in China.116 VOC species were measured by online and offline methods in the urban area of Jiaozuo from May to October in 2021 to analyze the compositional *** sources were analyzed by a positive matrix factorization(PMF)model,and the sensitivity of ozone generation was determined by ozone isopleth plotting research(OZIPR)*** results showed that the average volume concentration of total VOCs was 30.54 ppbv and showed a bimodal feature due to the rush-hour traffic in the morning and at *** most dominant VOC groups were oxygenated VOCs(OVOCs,29.3%)and alkanes(26.7%),and the most abundant VOC species were acetone and ***,based on the maximum incremental reactivity(MIR)method,the major VOC groups in terms of ozone formation potential(OFP)contribution were OVOCs(68.09μg/m^(3),31.5%),aromatics(62.90μg/m^(3),29.1%)and alkene/alkynes(54.90μg/m^(3),25.4%).This indicates that the control of OVOCs,aromatics and alkene/alkynes should take *** sources of VOCs were quantified by PMF,including fixed sources of fossil fuel combustion(27.8%),industrial processes(25.9%),vehicle exhaust(19.7%),natural and secondary formation(13.9%)and solvent usage(12.7%).The empirical kinetic modeling approach(EKMA)curve obtained by OZIPR on O_(3) exceedance days indicated that the O_(3) sensitivity varied in different *** results provide theoretical support for O_(3) pollution prevention and control in Jiaozuo.

关键词： Volatile organic compounds(VOCs) Online and offline measurement Ozone formation potential(OFP) Positive matrix factorization(PMF) Ozone isopleth plotting research(OZIPR) Jiaozuo

A sponge-based iron-tannic-acid hydrogel interface evaporator designed for clean water production

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Science China(Technological Sciences) 2024年第5期67卷 1579-1591页

作者： ZHANG ZeKun LI ChengLong TAO HuaYu GE Bo ZHANG YongLe ZHAO LiMin LIU JunChang REN GuiNa ZHANG ZhaoZhu School of Materials Science and Engineering Liaocheng UniversityLiaocheng252059China School of environmental and Material Engineering Yantai UniversityYantai264405China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou730000China

Due to the rapid advancement of technologies,there has been a significant increase in the discharge of industrial wastewater,and freshwater is becoming a scarce ***,research on solar evaporators is mainly focused on the efficient production of clean water,with less emphasis on the removal of residual pollutants remaining in the original *** this study,problems,including the difficult recovery of catalyst powder and the difficult removal of floating organic matter are solved by co-depositing low-surface-tension zirconia particles and bismuth tungstate onto the floating *** and melamine sponges were combined to solve the problem that traditional hydrogels lack mechanical *** excellent water-repellent effect can be seen from the contact angle between the liquid globule and canvas/felt,which is greater than 155°.The steam generation rate of the assembled evaporation system is 1.78 kg m^(-2)h^(-1),and its purification efficiency for methyl orange and rhodamine B exceeds 99%.This study presents a novel strategy for treating wastewater contaminated with organic dyes,aiming to solve problems including environmental damage,water pollution,and water scarcity.

关键词： oil removal non-wetting interface

Surface tension of single suspended aerosol microdroplets

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Chinese Chemical Letters 2024年第4期35卷 520-524页

作者： Yukai Tong Zhijun Wu Bo Zhou Min Hu Anpei Ye Key Laboratory for the physics and Chemistry of Nanodevices School of ElectronicsPeking UniversityBeijing 100871China State Key Joint Laboratory of environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China Aerospace Information Research institute Chinese Academy of SciencesBeijing 100094China

The surface tension of troposphere aerosols can significantly influence their atmospheric processes and key properties, particularly on the morphology, the phase transition, the activation as cloud condensation nuclei, and the gas-particle partitioning. However, directly measuring the surface tension of single ambient aerosol is quite challenging, due to the limitations of their picolitre volumes and thermal motion. Here, we developed a dual laser tweezers Raman spectroscopy(DLT-RS) system to directly sense the surface tension of single airborne microdroplets(PM10particles). A pair of aerosol droplets were trapped and driven to coalesce by the laser tweezers. Meanwhile, the backscattering light intensity and brightfield images during the coalescence process were recorded to characterize the aerosol surface tension. A remarkable advantage of directly sensing aerosol surface tension is that the solutes in aerosols are often supersaturated, which is common in atmospheric aerosols but almost unavailable in bulk *** experimentally measured the surface tension of aerosols composed of nitrates or oxalic acid/nitrate mixture. Besides, the variation of surface tension during aerosol aging process was also explored, which brings possible implications on the surface evolution of actual ambient aerosol during their atmospheric lifetime.

关键词： Surface tension Droplet coalescence Single aerosol Laser tweezers Aerosol aging