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In Situ Coupling of Highly Dispersed Ni/Fe Metal-NC Sites and N-Doped 3D Carbon Fibers Toward Free-Standing Bifunctional Cathode for Flexible Zinc-Air Battery

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Energy & environmental Materials 2024年第1期7卷 121-130页

作者： Chenglong Lai Mengjun Li Yi Shen Min Zhou Wei Wang Kai Jiang Haomiao Li Kangli Wang State Key Laboratory of Advanced Electromagnetic engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China School of Materials Science and engineering Huazhong University of Science and TechnologyWuhanHubei 430074China engineering Research Center of Power Safety and Efficiency Ministry of EducationWuhanHubei 430074China

Designing flexible free-standing air-electrode with efficient OER/ORR performance is of vital importance for the application of Zinc-air batteries in flexible ***,a flexible free-standing electrode(Ni/Fe-NC/NCF/CC)is synthesized by in-situ coupling of binary Ni/Fe-NC nanocubes and N-doped carbon nanofibers(NCF)rooted on carbon *** highly dispersed binary Ni/Fe-NC sites ensure excellent ORR activity and create efficient OER active sites relative to Ni-NC and *** in-situ coupling of Ni/Fe-NC and NCF constructs a 3D interconnected network structure that not only provides abundant and stabilized reactive sites but also guarantees fast electron transfer and gas transportation,thus achieving efficient and fast operation of ORR/***,Ni/Fe-NC/NCF/CC displays a much positive potential(0.952 V)at 4.0 mA cm^(-2)for ORR and a low OER overpotential(310 mV)at 50 mA cm^(-2).The Zinc-air battery with Ni/Fe-NC/NCF/CC air-electrode exhibits excellent battery performance with outstanding discharge/charge durability for 2150 *** flexible Zn-air batteries with foldable mechanical properties display a high power density of 105.0 mW cm^(-2).This work widened the way to prepare flexible bifunctional air-electrode by designing composition/structure and in-situ coupling.

关键词： binary Ni/Fe-NC sites in-situ coupling synergistic catalytic effect Zn-air battery

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Application of carbon-supported single-atom catalysts for electrochemical reactions

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新型炭材料(中英文) 2024年

作者： WANG Yi-cheng MA Xiao-bo Ayeza WANG Chen-xu LI Yang YANG Cheng-long WANG Zhe-fan WANG Chao HU Chao ZHANG Ya-ting Xi'an Thermal Power Research institute Co. Ltd. College of Chemistry and Chemical engineering Xi'an University of Science and Technology Tsinghua Shenzhen International Graduate School Tsinghua University School of Chemical engineering and Technology Xi'an Jiaotong University

The recent advances in carbon-supported single-atom catalysts (SACs) for electrochemical reactions are comprehensively reviewed. The development and advantages of carbon-supported SACs are briefly introduced, followed by a detailed summary of the synthesis strategies employed for various carbon-supported SACs, including vapor phase transport, high temperature pyrolysis,and wet chemical methods. Subsequently, the advanced characterization techniques for carbon-supported SACs are reviewed. The applications of carbon-supported SACs in diverse fields, such as oxygen reduction reaction, carbon dioxide reduction reaction, nitrogen reduction reaction, hydrogen evolution reaction, and oxygen evolution reaction are summarized. Special emphasis is given to the modification strategies enabling carbon-supported SACs to exhibit excellent electrocatalytic performance. Finally, the prospects and challenges associated with utilizing carbon-supported SACs for electrochemical reactions are discussed.

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A Practical Study of Knowledge Mapping Empowering the Construction of engineering Costing Software Application Courses in Undergraduate Colleges and Universities

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Journal of Contemporary Educational Research 2024年第9期8卷 129-133页

作者： Hongmei Wang Ying Lin Xiaolin Gan Chongqing institute of engineering Chongqing 400056China

Relying on the talent cultivation program of Chongqing institute of engineering,this paper combines the characteristics of the engineering Costing Software Application course with its current status quo,analyzes the existing problems and teaching pain points,and introduces knowledge *** course construction is carried out in terms of the combing of knowledge points,the optimization of the course structure,the innovation of the teaching method,and the evaluation and feedback of the teaching in order to improve the systematicity and structural nature of the teaching content,enhance students’learning experience,and enhance their learning *** is conducive to the formation of students’knowledge systems and provides a basis for discussion and reference for improving the quality of teaching and cultivating application-oriented talents who meet the market demand.

关键词： Knowledge mapping Curriculum construction Structure optimization

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晶体石墨炔的最新研究进展与挑战

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Science China Materials 2024年第3期67卷 729-751页

作者：刘心康赵亚松杜江王丹 Henan Province Industrial Technology Research institute of Resources and Materials Zhengzhou UniversityZhengzhou 450001China School of Materials Science and engineering Zhengzhou UniversityZhengzhou 450001China State Key Laboratory of Biochemical engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

石墨炔(GYs)是一种新型碳同素异形体,由sp和sp^(2)杂化碳原子组成.其中,石墨双炔(GDY)是目前研究和关注度最广泛的材料.其独特的sp杂化、均匀的孔隙和高度共轭的结构带来了优良的电子、光学和力学特性,其被广泛应用于电子器件、储能和... 详细信息

石墨炔(GYs)是一种新型碳同素异形体,由sp和sp^(2)杂化碳原子组成.其中,石墨双炔(GDY)是目前研究和关注度最广泛的材料.其独特的sp杂化、均匀的孔隙和高度共轭的结构带来了优良的电子、光学和力学特性,其被广泛应用于电子器件、储能和转换、催化、气体分离、海水淡化等领域.然而,GDY材料仍然面临着诸多挑战,包括高结晶GDY的合成和快速无损的表征方法.本文就高结晶度GDY的设计、合成和结构表征进行了综述.本文还描述了GDY在各个领域的应用,为高度均匀的单晶GDY材料带来新的机遇.

关键词： crystalline graphdiyne controlled synthesis energy conversion energy storage

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MXene Enhanced 3D Needled Waste Denim Felt for High‑Performance Flexible Supercapacitors

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Nano-Micro Letters 2024年第2期16卷 383-394页

作者： Wei Fan Qi Wang Kai Rong Yang Shi Wanxi Peng Handong Li Zhanhu Guo Ben Bin Xu Hua Hou Hassan Algadi Shengbo Ge Key Laboratory of Functional Textile Material and Product of the Ministry of Education School of Textile Science and EngineeringInstitute of Flexible electronics and Intelligent TextileXi’an Polytechnic UniversityXi’an 710048People’s Republic of China Co‑Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and EngineeringNanjing Forestry UniversityNanjing 210037People’s Republic of China Henan Province International Collaboration Lab of Forest Resources Utilization School of ForestryHenan Agricultural UniversityZhengzhou 450002People’s Republic of China Integrated Composites Lab Department of Mechanical and Construction EngineeringNorthumbria UniversityNewcastle Upon Tyne NE18STUK College of Materials Science and engineering Taiyuan University of Science and TechnologyTaiyuan 030024People’s Republic of China Department of Electrical engineering Faculty of EngineeringNajran University11001 NajranSaudi Arabia

MXene,a transition metal carbide/nitride,has been prominent as an ideal electrochemical active material for ***,the low MXene load limits its practical *** environmental concerns and sustainable development become more widely recognized,it is necessary to explore a greener and cleaner technology to recycle textile by-products such as *** present study proposes an effective 3D fabrication method that uses MXene to fabricate waste denim felt into ultralight and flexible supercapacitors through needling and *** 3D structure provided more sites for loading MXene onto Z-directional fiber bundles,resulting in more efficient ion exchange between the electrolyte and ***,the carbonization process removed the specific adverse groups in MXenes,further improving the specific capacitance,energy density,power density and electrical conductivity of *** electrodes achieve a maximum specific capacitance of 1748.5 mF cm-2 and demonstrate remarkable cycling stability maintaining more than 94%after 15,000 galvanostatic charge/discharge ***,the obtained supercapacitors present a maximum specific capacitance of 577.5 mF cm^(-2),energy density of 80.2μWh cm^(-2)and power density of 3 mW cm^(-2),*** resulting supercapacitors can be used to develop smart wearable power devices such as smartwatches,laying the foundation for a novel strategy of utilizing waste cotton in a high-quality manner.

关键词： MXene 3D needled waste denim felt Supercapacitors Carbonization

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The Forms and Overall Characteristics of Dong Brocade

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China Book International 2024年第1期 102-105页

作者： Chen Xiaoling Fashion Depar tment at Hunan institute of engineering

This book,through field surveys,literature review,and classification,explores the origins and heritage of Dong *** analyzes the cultural,artistic,and aesthetic features of Dong Brocade in Xiangxi Corridor,along with its weaving *** then proposes ideas for the innovative development and protective heritage of Dong Brocade and explains in detail how to apply Dong Brocade art in designing creative products.

关键词： Broca Forms apply

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Excellentπ-Bowl Semiconductors Based on C_(70)Subunit

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CCS Chemistry 2024年第2期6卷 353-364页

作者： Meng Chen Yuxiao Duan Xinyue Liu Qian Zhan Hironobu Hayashi Kyohei Matsuo Hiroko Yamada Guangpeng Gao Yonghao Zheng Lei Zhang Beijing Advanced Innovation Center for Soft Matter Science and engineering Beijing University of Chemical TechnologyBeijing 100029 School of Optoelectronic Science and engineering University of Electronic Science and Technology of China(UESTC)Chengdu 610054 Division of Materials Science Nara Institute of Science and Technology(NAIST)IkomaNara 630-0192 Key Laboratory of Cluster Science of Ministry of Education Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion MaterialsSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 100081

As open substructures of fullerenes,aromaticπ-bowls are promising candidates as new organic semiconductors,as well as attractive hosts for *** demonstrate herein the synthesis and characterization of a novel C_(2v)symmetricπ-bowl,pyracyleno[6,5,4,3,2,1-pqrstuv]pentaphene(3).Bowl 3 was equipped with two distinctive reactive sites,allowing for bromination and cross-coupling reactions to readily yield functionalized bowls with two 2,4,6-trimethylphenyl(5)and triethylsilyl(TES)-ethynyl(6)substituents,***-temperature 1H NMR analysis and density functional theory(DFT)calculations indicated bowl-to-bowl inversions of 3,5,and 6 at room *** alternating the substituents,the crystal structures of the threeπ-bowls 3,5,and 6 could be controlled from 1D linear to 1D slipped to 2D herringbone packing motifs,providing insight into the packing behavior ofπ-bowls.1H NMR titration study indicated that the TES-ethynyl substituent enhanced the ability ofπ-bowl to bind C_(70)with an association constant of 2485 M−*** C_(70)molecules withπ-bowls 3 and 6 formed 1:1 complexes,in which C_(70)molecules aggregated into zig-zag and 1D linear arrays,*** hole mobility of 2.3 cm^(2)V^(−1)^s(−1)and electron mobility of 0.16 cm^(2)V^(−1)^s(−1)ofπ-bowl 3 and its complex with C_(70)were demonstrated,respectively,which proved a great value for the development of aromaticπ-bowl semiconductors with tunable properties for organic electronic devices.

关键词： organic semiconductor π-bowl fullerene crystal engineering mobility

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A Review of Artificial Waterfalls in Gardens

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Journal of World Architecture 2024年第1期8卷 31-34页

作者： Ni Lan Tiantian Chen Qiushuang Fan Shiyu Mi Chongqing institute of engineering Chongqing 400056China

When artificial waterfalls are built in gardens,leaves from trees or vegetation often fall into the water storage pool and block the pipelines,requiring regular cleaning of *** not only increases the manpower needed for maintenance but also disrupts the use of the ***,it is necessary to design a new type of artificial waterfall that is suitable for *** waterfall should incorporate features that make cleaning easier,including filter plates and water funnels to prevent clogging caused by fallen leaves and debris.

关键词： Intelligence Efficiency improvement Transportation pipeline Technical artificial waterfall

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Spatiotemporal distribution,environmental risk and carbon emission reduction potential of livestock manure in Shaanxi Province,China

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Frontiers of Agricultural Science and engineering 2024年第3期11卷 381-396页

作者： Mengyuan QIAO Jianchun ZHU Ronghua LI Junting PAN Ran XIAO Hailong WANG Kuok Ho Daniel TANG Zengqiang ZHANG College of Humanities&Social Development Northwest A&F UniversityYangling 712100China College of Natural Resources and Environment Northwest A&F UniversityKey Laboratory of Low-carbon Green Agriculture in Northwestern ChinaMinistry of Agriculture and Rural AffairsYangling 712100China Key Laboratory of Non-point Source Pollution of Ministry of Agricultural and Rural Affairs Institute of Agricultural Resources and Regional PlanningChinese Academy of Agricultural SciencesBeijing 100081China Interdisciplinary Research Center for Agriculture Green Development in Yangtze River Basin College of Resources and EnvironmentSouthwest UniversityChongqing 400715China Biochar engineering Technology Research Center of Guangdong Province School of Environmental and Chemical EngineeringFoshan UniversityGuangdong 528000China Department of environmental Science University of ArizonaTucsonAZ 85721USA

Shaanxi is a leading province in animal husbandry(AH)in ***,the lack of provincial information on the characteristics and utilization potential of livestock manure(LM)hinders crucial management ***,we investigated the spatiotemporal distribution,availability and biogas potential of LM in Shaanxi,and examine the carbon emission reduction potential of *** has been a 1.26-fold increase in LM quantities in Shaanxi over the past 35 years,reaching 4635.6×10^(4)t by *** was mainly concentrated in northern Shaanxi and the eastern part of *** and pig manure were the primary sources of LM,with the average LM land-load of 14.57 t·ha^(−1)in *** the overall AH in Shaanxi has not exceeded the environmental capacity,the actual scales of AH in Ankang and Hanzhong have already surpassed the respective environmental capacities,posing a higher risk of N and P *** 2021,the estimated biogas energy potential of LM was 1.2×10^(11)*** 2012 to 2021,the average carbon emission reduction potential in Shaanxi was 22%,with an average potential scale of 10%.The results of this research provide valuable data and policy recommendations for promoting the intensive use of LM and reducing carbon emissions in Shaanxi.

关键词： Livestock manure emission estimation N and P loads biogas potential carbon emission reduction

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Recovery of cathode copper and ternary precursors from CuS slag derived by waste lithium-ion batteries:Process analysis and evaluation

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Chinese Chemical Letters 2024年第7期35卷 178-182页

作者： Yun Wei Lei Zhou Wenbin Hu Liming Yang Guang Yang Chaoqiang Wang Hui Shi Fei Han Yufa Feng Xuan Ding Penghui Shao Xubiao Luo National-Local Joint engineering Research Center of Heavy Metals Pollutants Control and Resource Utilization Nanchang Hangkong UniversityNanchang 330063China School of Life Science Jinggangshan UniversityJi’an 343009China CAS Key Laboratory of Green Process and engineering National Engineering Research Center of Green Recycling for Strategic Metal ResourcesInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China Biomass Molecular engineering Center and Anhui Provincial Key Laboratory of Microbial Pest Control Anhui Agricultural UniversityHefei 230036China Jiangxi Ganfeng Recycling Technology Co.LTD. Xinyu 338004China

The efficient and environmentally friendly recycling technology of waste residue that including abundant heavy metal produced during the recovery of lithium batteries has become a research ***,a novelty process of acid leaching-selective electrodeposition-deep impurity removal-regeneration was proposed to recovery of the CuS slag,which has been efficient transferred to high purity cathode copper and commercially available ternary *** cathode with a purity of 99.67%was prepared under electrochemical reaction conditions at-0.55 V for 2 h.A novel impurity remover-Mn powder,which was used to remove the residual impurities and as a feedstock for the ternary ***,NCM523 was regenerated by *** process is superior to the traditional process in economy,energy consumption,CO_(2)emissions,product purity and process *** study provides a new approach for solid waste recovery and precious metal enrichment.

关键词： CuS slag Electrodeposition Cathode copper Ternary precursor Solid waste recovery

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