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From waste to wealth:Coal tar residue derived carbon materials as low-cost anodes for potassium-ion batteries

International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 464-475页

作者： Zhonghua Lu Jun Shen Xin Zhang Lingcong Chao Liang Chen Ding Zhang Tao Wei Shoudong Xu College of Chemical engineering and Technology Taiyuan University of TechnologyTaiyuan 030024China College of Chemistry Taiyuan University of TechnologyTaiyuan 030024China School of Chemical engineering and Pharmacy Wuhan Institute of TechnologyWuhan 430205China School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212003China

Carbon materials are widely recognized as highly promising electrode materials for various energy storage system *** tar residues(CTR),as a type of carbon-rich solid waste with high value-added utilization,are crucially important for the development of a more sustainable *** this study,we employed a straightforward direct carbonization method within the temperature range of 700-1000℃to convert the worthless solid waste CTR into economically valuable carbon materials as anodes for potassium-ion batteries(PIBs).The effect of carbonization temperature on the microstructure and the potassium ions storage properties of CTR-derived carbons(CTRCs)were systematically explored by structural and morphological characterization,alongside electrochemical performances *** on the co-regulation between the turbine layers,crystal structure,pore structure,functional groups,and electrical conductivity of CTR-derived carbon carbonized at 900℃(CTRC-900H),the electrode material with high reversible capacity of 265.6m Ah·g^(-1)at 50 m A·g^(-1),a desirable cycling stability with 93.8%capacity retention even after 100 cycles,and the remarkable rate performance for PIBs were ***,cyclic voltammetry(CV)at different scan rates and galvanostatic intermittent titration technique(GITT)have been employed to explore the potassium ions storage mechanism and electrochemical kinetics of *** indicate that the electrode behavior is predominantly governed by surface-induced capacitive processes,particularly under high current densities,with the potassium storage mechanism characterized by an“adsorption-weak intercalation”*** work highlights the potential of CTR-based carbon as a promising electrode material category suitable for high-performance PIBs electrodes,while also provides valuable insights into the new avenues for the high value-added utilization of CTR.

关键词： coal tar residue carbon materials anode potassium-ion batteries high value-added

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Role of iron ore in enhancing gasification of iron coke:Structural evolution,influence mechanism and kinetic analysis

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 58-69页

作者： Jie Wang Wei Wang Xuheng Chen Junfang Bao Qiuyue Hao Heng Zheng Runsheng Xu School of Chemistry and Materials Science Hubei Engineering UniversityXiaogan 432000China Key Laboratory for Ferrous Metallurgy and Resources Utilization of Ministry of Education Wuhan University of Science and TechnologyWuhan 430081China Institue of Ironmaking Technology Baosteel Central Research InstituteShanghai 201999China State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China

The utilization of iron coke provides a green pathway for low-carbon *** uncover the influence mechanism of iron ore on the behavior and kinetics of iron coke gasification,the effect of iron ore on the microstructure of iron coke was ***,a comparative study of the gasification reactions between iron coke and coke was conducted through non-isothermal thermogravimetric *** findings indicate that compared to coke,iron coke exhibits an augmentation in micropores and specific surface area,and the micropores further extend and *** provides more adsorption sites for CO_(2) molecules during the gasification process,resulting in a reduction in the initial gasification temperature of iron *** the heating rate in non-isothermal gasification can enhance the reactivity of iron *** metallic iron reduced from iron ore is embedded in the carbon matrix,reducing the orderliness of the carbon structure,which is primarily responsible for the heightened reactivity of the carbon *** kinetic study indicates that the random pore model can effectively represent the gasification process of iron coke due to its rich pore ***,as the proportion of iron ore increases,the activation energy for the carbon gasification gradually decreases,from 246.2 kJ/mol for coke to 192.5 kJ/mol for iron coke 15wt%.

关键词： low-carbon ironmaking iron coke gasification structural evolution kinetic model

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Identifying the dynamic behaviors in complete reconstruction of Co-based complex precatalysts during electrocatalytic oxygen evolution

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Journal of Energy Chemistry 2025年第1期100卷 226-233页

作者： Jingfang Zhang Danyang Wu Linke Cai Youluan Lu Fanpeng Cheng Lijuan Shi Qun Yi Yao Liu Yi Huang Key Laboratory of Green Chemical engineering Process of Ministry of Education Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education Hubei Key Laboratory of Novel Reactor and Green Chemical Technology School of Chemical Engineering & Pharmacy Wuhan Institute of Technology Key Laboratory of Pesticide & Chemical Biology of Ministry of Education Engineering Research Center of Photoenergy Utilization for Pollution Control and Carbon Reduction of Ministry of Education College of Chemistry Central China Normal University College of Materials Science and engineering Fuzhou University

Transition metal-based nanomaterials have emerged as promising electrocatalysts for oxygen evolution reaction（OER）. Considerable research efforts have shown that self-reconstruction occurs on these nanomaterials under operating conditions of OER process. However, most of them undergo incomplete reconstruction with limited thickness of reconstruction layer, leading to low component utilization and arduous exploration of real catalytic mechanism. Herein, we identify the dynamic behaviors in complete reconstruction of Co-based complexes during OER. The hollow phytic acid（PA） cross-linked CoFe-based complex nanoboxes with porous nanowalls are designed because of their good electrolyte penetration and mass transport ability, in favor of the fast and complete reconstruction. A series of experiment characterizations demonstrate that the reconstruction process includes the fast substitution of PA by OH-to form Co（Fe）(OH)xand subsequent potential-driven oxidation to Co（Fe）OOH. The obtained CoFeOOH delivers a low overpotential of 290 mV at a current density of 10 mA cm-2and a long-term *** experiment results together with theory calculations reveal that the Fe incorporation can result in the electron rearrangement of reconstructed CoFeOOH and optimization of their electronic structure,accounting for the enhanced OER activity. The work provides new insights into complete reconstruction of metal-based complexes during OER and offers guidelines for rational design of high-performance electrocatalysts.

关键词： Complete reconstruction Co-based complex Precatalysts Oxygen evolution reaction

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Research on Global Clock Synchronization Mechanism in Software-Defined Control Architecture

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Chinese Journal of Electronics 2022年第5期31卷 915-929页

作者： LYU Shuyu DAI Xinfa MA Zhong GAO Yi HU Zhekun Harbin engineering University wuhan digital engineering institute

Adopt software-definition technology to decouple the functional components of the industrial control system(ICS) in a service-oriented and distributed form is an important way for the industrial Internet of things to integrate information technology, communication technology, and operation technology. Therefore, this paper presents the concept of software-defined control architecture and describes the time consistency requirements under the paradigm shift of ICS architecture. By analyzing the physical clock and virtual clock mechanism models, the global clock synchronization space is logically divided into the physical and virtual clock synchronization domains, and a formal description of the global clock synchronization space is proposed. According to the fundamental analysis of the clock state model, the physical clock linear filtering synchronization model is derived, and a distributed observation fusion filtering model is constructed by considering the two observation modes of the virtual clock to realize the time synchronization of the global clock space by way of timestamp layer-by-layer transfer and fusion estimation. Finally, the simulation results show that the proposed model can significantly improve the accuracy and stability of clock synchronization.

关键词： software-defined control architecture communication technology clock state model information technology global clock synchronization mechanism synchronisation global clock space global clock synchronization space distributed observation fusion filtering model adopt software-definition technology time synchronization industrial control operation technology industrial control system synchronization model virtual clock mechanism models physical clock clocks filtering theory ICS architecture

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Event-based Implicit Invocation Decentralized in Ada

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wuhan University Journal of Natural Sciences 2001年第Z1期6卷 239-246页

作者： Liang Xian zhong, Wang Zhen yu wuhan digital engineering institute, P. O. Box 74223, wuhan 430074, China wuhan digital engineering institute Wuhan China

Nowadays more and more attraction is drawn by the event based implicit invocation one of useful architectural patterns, because of its loose coupling between components in the architecture and reactive integration in software systems. Analyzing object oriented interaction with objects, this paper, based upon the principle of software architecture, presents an approach on event based object model with Ada exception handler. Consequently it is possible for us to improve, with adding specific architectural patterns, traditional programming languages into architectural description languages.

关键词： implicit invocation architectural pattern EBO (event based object) exception handler

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MORE ON ADDITIVE ENUMERATION PROBLEMS OVER TREES

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Acta Mathematica Scientia 1990年第4期10卷 396-401页

作者：王振宇孙潮义 wuhan digital engineering institute Wuhan China

The present paper discusses more about additive enumeration problems over some tree families, especially, the trees with nodes and leaves of given numbers. It establishes a uniform solving scheme for additive enumeration problems over V (ery) simple generated tree families. Based on the uniform scheme, a series of additive enumeration problems over tree families, including leaf path length counting and node path length counting, are solved. The tree families related include: binary tree, t-ary tree and ordered tree.

关键词：树可加枚举问题

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Remolding Diversified Objects in Ada95: Toward A Object Pattern

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wuhan University Journal of Natural Sciences 2001年第Z1期6卷 247-255页

作者： Liang Xian zhong, Wang Zhen yu wuhan digital engineering institute P. O. Box 74223, wuhan 430074, China wuhan digital engineering institute Wuhan China

Ada provides full capacities of supporting object orientation, but the diversified objects patterned in Ada are so intricate that Ada95's aim would be demolished. In order to complement the disfigurement that Ada does lack for a pristine notion of class, this paper presents a remolded object pattern known as A object, an Ada based class description language A ObjAda aiming at support for A object pattern and the related approach for key algorithms and implementation. In consequent, A ObjAda hereby promotes Ada with highlighted object orientation, which not only effectively exploits the capacities in Ada95, but also rationally hides befuddling concepts from Ada95.

关键词： ADT (abstract data type) ASM (abstract state machine) V object U object A object pattern

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Luminescence: a new perspective for investigating perovskite precursors

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Science China Materials 2025年第1期 312-313页

作者： Haofeng Zheng Shaocong Hou School of Electrical engineering and Automation Wuhan University wuhan University Shenzhen Research institute

In the past two decades, perovskite materials have made significant progress in optoelectronic semiconductors, emerging as formidable candidates for the next generation of commercial solar cells, light-emitting diodes (LEDs), and *** the fundamental solution chemistry and photophysics in solution-processed perovskite devices is crucial for comprehending to achieve highly efficient optoelectronic devices.

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Defense Against Software-Defined Network Topology Poisoning Attacks

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Tsinghua Science and Technology 2023年第1期28卷 39-46页

作者： Yang Gao Mingdi Xu Platform Research and Development Department Wuhan Institute of Digital EngineeringWuhan 430073China

Software-Defined Network(SDN)represents a new network *** conventional networks,SDNs separate control planes and data *** function of a data plane is enabled using switches,whereas that of a control plane is facilitated by a *** controller learns network topologies and makes traffic forwarding ***,some serious vulnerabilities are gradually exposed in the topology management services of current SDN controller *** vulnerabilities mainly exist in host tracking and link discovery *** can exploit these weak points to poison the network topology information in SDN *** this study,a novel solution is proposed to defend against topology poisoning *** analyzing the existing topology attack principles and threat models,this work constructs legal conditions for host migration to detect host hijacking *** checking of the Link Layer Discovery Protocol(LLDP)source and integrity is designed to defend against link fabrication attacks.A relay-type link fabrication attack detection method based on entropy is also *** show that the proposed solution can effectively detect existing topological attacks and provide complete and comprehensive topological security protection.

关键词： Software-Defined Network(SDN) topology discovery topology poisoning attacks

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ρ Graph: Rendezvous Ordering Graph forAda Concurrent Programs

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Journal of Computer Science & Technology 1998年第6期13卷 615-622页

作者：王振宇 wuhan digital engineering institute Wuhan P.R. China

In disciplined Ada software development and maintenance, an adequate and suitable graphical representation for concurrency is important. To describe rendezvous ordering, tasking andexecuting flow of tasks, p graph--Rendezvous Ordering Graph is presenced in this paper. pgraph is a kind of-hierarchical oriented graph with nodes representing rendezvouses and edgesshowing'ordering relations between rendezvouses as well as flow of tasks. It can be used insoftware understanding, design description and documentation.

关键词： Ada concurrent program rendezvous relation rendezvous ordering graph.

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